/ 3 1 / 3 / 3 1 /

8-18-29 3 291415 297 1-11-4 3/31/ 3/31/ 29 8 22 29 1 17 24

8-1 29 [1] PCB [2] HCB [3] [4] [5] DDT [6-1] p,p'-ddt [6-2] p,p'-dde pg/l ( ) nd 2,4 (46/47) 2.9 18 (47/47) 84 12 pg/g-dry ( ) nd 61, (61/62) 4,6 3 11, (62/62) 82 [6] [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7] [8] [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans- 2 21 (47/47) tr(2) 15 (47/47) nd 12 (19/47) tr(.6) 36 (47/47) tr(2) 12 (47/47) nd 6 (2/47) nd 83 (46/47) nd (/47) 19 15 nd 4.6 13 nd 4.7 nd nd 2,8 (61/62) tr(1) 3, (62/62) nd 78 (41/62) nd 1,5 (61/62) nd 2,6 (61/62) nd 4 (53/62) nd 15 (51/62) nd (/62) 47 53 tr(1) 31 47 1.2 1.9 nd [9-1] Parlar-26 [9] [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch [11] [11-3] γ-hch [11-4] δ-hch [12] 3.7 68 (47/47) 12 83 (47/47) 2.1 19 (47/47) tr(.4) 69 (47/47) 47 1 17 8.2 1. 1,9 (62/62) 5.7 3,4 (62/62) tr(.4) 1,9 (62/62) tr(.2) 1,7 (62/62) [13] 1 nd 1/2 2 3 tr(x)x 77 14 23 25 241

4 1 [14-1] [14-2] [14-3] [14] [14-4] [14-5] [14-6] [14-7] [15] PFOS [16] PFOA [17] [18-1] α- [18] [18-2] β- 1,2,5,6,9,1- [19-1] α-1,2,5,6,9,1- [19-2] β-1,2,5,6,9,1- [19] [19-3] γ-1,2,5,6,9,1- [19-4] δ-1,2,5,6,9,1- [19-5] ε-1,2,5,6,9,1- [2] [21] -1,3- [22] [22-1] [22-2] [23-1] [23-2] [23] [23-3] [23-4] ( ) nd 12 (44/47) nd 8 (24/47) nd tr(6) (1/47) nd 3 (1/47) nd 33 (22/47) nd 46 (37/47) nd 4,1 (46/47) 2. 14 (47/47) nd 3,5 (43/47) nd 1, (32/47) nd tr(1,6) (1/47) nd 3,1 (13/47) nd 1, (4/47) nd 1, (7/47) pg/l tr(4) nd nd nd tr(2) 17 15 8.8 86 tr(1) nd nd nd nd pg/g-dry ( ) nd 57 (44/62) nd 56 (37/62) nd 57 (44/62) nd 58 (36/62) nd 1,9 (48/62) nd 29, (61/62) tr(27) 58, (62/62) 1.3 2,8 (62/62) tr(16) 32, (62/62) 8 7,4 (62/62) nd 19 (61/62) nd 17, (12/62) nd 37, (19/62) nd 44, (19/62) nd 94, (18/62) 13 1 16 18 38 4 4,6 61 63 35 34 nd nd nd nd [24] 1 nd 1/2 2 3 tr(x)x 4 59 242

8-2 29 [1] PCB [2] HCB [3] [4] [5] DDT [6-1] p,p'-ddt [6-2] p,p'-dde pg/g-wet pg/m 3 ( ) ( ) ( ) ( ) 5 19, 86 16, 4, 38, 26 3,3 2,5 1, 39, (3/3) (19/19) (2/2) (37/37) 12 26 99 33 1,1 23 4,9 73 55 41 19 1,1 (3/3) (19/19) (2/2) (37/37) 13 [6] [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7] [7-2] trans- [7-3] [8] [9] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch [11] [11-3] γ-hch [11-4] δ-hch [12] [13] 6 32 (3/3) 21 6 (3/3) tr(2) 11 (3/3) tr(1) 3 (3/3) 15 39 4 tr(1.7) nd 13 (18/19) 4 29 (19/19) nd 3 (16/19) nd 23 (15/19) 2 54 5.9 7 93 (2/2) 3 3,5 (2/2) tr(1) 2 (2/2) nd tr(1) (1/2) 1 nd 1/2 2 3 tr(x)x 2.4 81 1, 4.5 nd 4.9 7 (37/37).67 59 (37/37).84 93 (37/37) nd 46 (36/37) 36 4.1 1.8 243

4 1 [14-1] 23 2 (3/3) [14-2] tr(6) 62 (3/3) [14-3] nd 36 (2/3) [14] [14-4] nd tr(9) (1/3) [14-5] nd tr(9) (1/3) [14-6] nd (/3) [14-7] nd tr(18) (1/3) [15] nd 16 PFOS (2/3) [16] nd 18 PFOA (2/3) 14 22 [17] (3/3) [18-1] α- [18] [18-2] β- 1,2,5,6,9,1- [19-1] α-1,2,5,6,9,1-86 43 (3/3) [19-2] β-1,2,5,6,9,1- nd 36 (1/3) [19] [19-3] γ-1,2,5,6,9,1- tr(2) 2 (3/3) [19-4] δ-1,2,5,6,9,1- [19-5] ε-1,2,5,6,9,1- nd 1,4 [2] (2/3) [21] -1,3- [22] [22-1] nd tr(35) (1/3) [22-2] tr(2) 36 (3/3) nd 1,8 [23-1] (2/3) [23-2] tr(3) 11, [23] (3/3) 1,3 4,7 [23-3] (3/3) tr(3) 3,1 [23-4] (3/3) [24] 1 2 3 4 5 pg/g-wet pg/m 3 ( ) ( ) ( ) ( ) 47 18 tr(14) nd nd nd nd 22 tr(6.3) 18 19 tr(9) 49 46 nd 6 67 2,2 2, 87 tr(7) 36 (19/19) nd 87 (18/19) nd 21 (18/19) nd 55 (1/19) nd 88 (9/19) nd 68 (1/19) nd 2,1 (1/19) tr(4) 11, (19/19) nd 79 (12/19) 4 17 (19/19) tr(9) 7,8 (19/19) nd tr(12) (2/19) nd 12 (12/19) nd 36 (17/19) nd 11 (14/19) tr(1) 12 (19/19) nd 2,1 (16/19) nd 24, (16/19) nd 19, (18/19) nd 4,1 (8/19) 8 23 49 tr(11) tr(9.7) nd nd 15 tr(6.4) 29 14 nd tr(16) 32 tr(15) 6.7 tr(41) 1,9 2,1 26 66 (2/2) 12 5 (2/2) 51 1, (2/2) tr(18) 44 (2/2) 25 72 (2/2) nd (/2) nd (/2) 3, 32, (2/2) 85 68 (2/2) 35 47 (2/2) 5 2,2 (2/2) nd (/2) nd tr(18) (1/2) tr(18) 46 (2/2) 3 11, (2/2) 11 47 (2/2) nd 1,6 (1/2) 8 31, (2/2) 1,2 25, (2/2) nd 8,1 (1/2) 13 77 23 89 13 nd nd 9,8 24 13 33 nd tr(9) 91 1,8 23 tr(4) 5, 5,5.6 4.1 (37/37) nd 3.4 (33/37) nd 2.1 (11/37) nd 3.2 (1/37) nd 5.7 (28/37) nd 4 (31/37) nd 14 (34/37) 1.1 8.9 (37/37) 2 15 (37/37) 32 2 (37/37) nd 3.3 (36/37) nd.8 (33/37) nd.8 (2/37) 7 92 (37/37) 1,1 23, (37/37).7 33 (37/37) 6 21 (37/37) 7 1,5 (37/37) 9 2,3 (37/37) 3 73 (37/37) nd 1,6 (35/37).39.11 nd nd tr(.19) nd 1/2 tr(x)x -1,3-3/ 5946 47 tr(29) 9.75 4.2 2.9 14 71.53 tr(.2) tr(.1) 11 4,2 4.6 34 37 5 19 15 244

9 29 [1] PCB [2] HCB pg/l pg/g-dry pg/g-wet pg/m 3 [3] [4] [5] DDT [6-1] p,p'-ddt [6-2] p,p'-dde 16 [5.5] 2.1 [.8] 14 [5.] 3 [1] 68 [23] 3.9 [1.3] 7. [2.3].5 [.2] [6] [6-3] p,p'-ddd [7] [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9] [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch [11] [11-3] γ-hch [11-4] δ-hch [12] 2 [1] 3 [1] 4 [2] 1.5 [.6] 3 [1] 3 [1] 1.6 [.6] 2.3 [.9].9 [.4] 1.8 [.7] 1.4 [.5] 1. [.4] 4.8 [1.6] 4 [1] 3 [1] 1.7 [.7] 6 [2].9 [.3] 1.2 [.5] 2. [.8].5 [.2] 1.5 [.6] 1. [.4].6 [.2] [13] 1 2[] 3 4 3[1] 3[1] 3[1] 2.3 [.9].8 [.3].11 [.4].1 [.4].8 [.3] 245

pg/l pg/g-dry pg/g-wet pg/m 3 4 1 [14-1] 9 [3] 9 [4] 16 [6].15 [.5] [14-2] 3 [1] 9 [4] 12 [5].1 [.4] [14-3] 7 6 17.3 [14] [3] [2] [7] [.1] [14-4] 14 [5] 15 [6] 22 [8].4 [.2] [14-5] 2 [1] 5 [2] 2 [8].21 [.7] [14-6] 7 [3] 15 [5] 5 [2].6 [.2] [14-7] [15] PFOS [16] PFOA [17] [18-1] α- [18] [18-2] β- 1,2,5,6,9,1- [19-1] α-1,2,5,6,9,1- [19-2] β-1,2,5,6,9,1- [19] [19-3] γ-1,2,5,6,9,1- [19-4] δ-1,2,5,6,9,1- [19-5] ε-1,2,5,6,9,1- [2] [21] -1,3- [22] [22-1] [22-2] [23-1] [23-2] [23] [23-3] [23-4] [24] 24 [8] 1.4 [.6] 3 [1] 14 [5] 3,3 [1,1] 1,5 [5] 3,3 [1,1] 3,6 [1,2] 3 [1] 1.2 [.5] 27 [9.1] 4 [2] 5 [2] 1, [4,] 1, [4,] 11, [4,] 12, [5,] 1 2[] 3 4 21 [8] 12 [4] 12 [4] 4 [1] 24 [9] 23 [9] 24 [9] 33 [12] 36 [12] 4 [1] 5 [2] 8 [3] 9 [3] 5 [2] 2.4 [.8].3 [.1] 3.3 [1.1].3 [.1].3 [.1].3 [.1].3 [.1].67 [.24] 6 [2].6 [.2] 1.2 [.5] 14 [5] 19 [6] 1 [3] 12 [4] 246

1-1 14 29 [1] PCB [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd 7 5 9 13 1 18 7 9 5 12 6 15 6 5 9 8 6 11 [7-1] cis- 7 5 1 [7-2] trans- [7-3] X X X [7-4] cis- [7-5] trans- 13 7 5 [8-1] X X X X [8-2] cis- [8-3] trans- X X X X X [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] [11] HCH [11-1] α-hch [11-2] β-hch [11-3] γ-hch 11 8 16 13 1 2 6 5 7 5 4 8 8 6 1 6 4 12 7 6 8 18 14 27 5 5 6 [11-4] δ-hch * * X 1 AIC 95 2 X 3 11 4 29 5 3 95 247

[14] [14-1] [14-2] [14-3] [14-4] [14-5] X X X X X X X X X X X X X X X X X X X X [14-6] * * X X [14-7] * * X X [17] 1 AIC 95 2 X 3 11 4 21 22 248

1-2 14 29 [1] PCB 17 12 3 11 9 17 [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans- 8 7 12 13 9 2 7 5 1 1 7 15 7 5 12 8 7 11 [7-3] X * X [7-4] cis- [7-5] trans- 12 9 19 1 8 15 1 7 15 15 13 2 12 9 17 [8-1] X X [8-2] cis- * X [8-3] trans- X X X X X [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] [11] HCH [11-1] α-hch [11-2] β-hch 11 8 18 [11-3] γ-hch [11-4] δ-hch 1 AIC 95 2 X 3 11 4 29 5 3 95 249

[14] [14-1] * [14-2] X [14-3] X [14-4] * X * [14-5] X [14-6] [14-7] [17] 1 AIC 95 2 X 3 11 4 21 22 25

1-3 14 29 [1] PCB [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] [11] HCH [11-1] α-hch 1 7 18 [11-2] β-hch [11-3] γ-hch [11-4] δ-hch X 1 AIC 95 2 X 3 29 4 3 95 251

[14] [15] [14-1] [14-2] [14-3] [14-4] [14-5] [14-6] [14-7] PFOS [16] PFOA X X X X X X X X [17] X * 1 AIC 95 2 X 3 2 PFOSPFOA 21 22 X X X X 252

1-4 14 29 [1] PCB 18 11 43 [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch 19 [11] 1 1 [11-3] γ-hch 23 18 33 [11-4] δ-hch 1 AIC 95 2 3 29 4 3 95 5 HCH 21 253

[14-1] [14-2] X [14] [14-3] X [14-4] X [14-5] X [14-6] X [14-7] X [15] PFOS [16] PFOA [17] 1 AIC 95 2 X 3 21 PFOSPFOA 22 19 254

11 14 29 茨 255

29 14 15 PCB HCB HCH 4 1 PFOSPFOA 1,2,5,6,9,1- α-1,2,5,6,9,1-β- 1,2,5,6,9,1- γ-1,2,5,6,9,1- -1,3- trans- 4 1 1,2,5,6,9,1- β-1,2,5,6,9,1-256

[1] PCB PCB 49 6 POPs 16 13 53 13 8 9 12 13 14 47 5.5 pg/l 47 46 2,4pg/L 14 29 14 29 PCB [] PCB (pg/l) H14 47 33 11, 6 7.4 [2.5] 114/114 38/38 H15 53 45 3,1 23 9.4 [2.5] 36/36 36/36 H16 63 54 4,4 14 14 [5.] 38/38 38/38 H17 52 37 7,8 14 1 [3.2] 47/47 47/47 H18 24 2 4,3 15 9 [3] 48/48 48/48 H19 18 14 2,7 12 7.6 [2.9] 48/48 48/48 H2 26 25 4,3 27 7.8 [3.] 48/48 48/48 H21 21 17 3,9 14 1 [4] 48/48 48/48 H22 12 99 2,2 nd 73 [24] 41/49 41/49 H23 15 13 2,1 16 4.5 [1.7] 49/49 49/49 H24 4 28 6,5 72 44 [15] 48/48 48/48 H25 14 11 2,6 tr(13) 25 [8] 48/48 48/48 H26 15 12 4,8 16 8.2 [2.9] 48/48 48/48 H27 2 16 4,2 34 21 [7.3] 48/48 48/48 H28 14 12 3,1 tr(7.2) 8.4 [2.8] 48/48 48/48 H29 84 79 2,4 nd 16 [5.5] 46/47 46/47 1 14 2[] [] 62 5. pg/g-dry 62 61 61,pg/g-dry 14 29 257

14 29 PCB [] PCB (pg/g-dry) H14 11, 11, 63, 39 1 [3.5] 189/189 63/63 H15 9,4 9,5 5,6, 39 1 [3.2] 186/186 62/62 H16 8,4 7,6 1,3, 38 7.9 [2.6] 189/189 63/63 H17 8,6 7,1 69, 42 6.3 [2.1] 189/189 63/63 H18 8,8 6,6 69, 36 4 [1] 192/192 64/64 H19 7,4 6,8 82, 19 4.7 [1.5] 192/192 64/64 H2 8,7 8,9 63, 22 3.3 [1.2] 192/192 64/64 H21 7,6 7,1 1,7, 17 5.1 [2.1] 192/192 64/64 H22 6,5 7,8 71, nd 66 [22] 56/64 56/64 H23 6,3 7,4 95, 24 12 [4.5] 64/64 64/64 H24 5,7 6,7 64, tr(32) 51 [18] 63/63 63/63 H25 6,2 8, 65, tr(43) 44 [13] 62/62 62/62 H26 4,9 5,5 44, tr(35) 61 [21] 63/63 63/63 H27 6,4 7,5 1,1, nd 62 [22] 61/62 61/62 H28 5,3 5,3 77, tr(21) 53 [18] 62/62 62/62 H29 4,6 6,2 61, nd 14 [5.] 61/62 61/62 1 14 21 2[] [] 3 23pg/g-wet 3 5 19,pg/g-wet 19 23pg/gwet 19 86 16,pg/g-wet 2 23pg/g-wet 2 4, 38,pg/gwet 14 29 14 29 PCB PCB [] H14 8,8 28, 16, 2 25 [8.4] 38/38 8/8 H15 11, 9,6 13, 1, 5 [17] 3/3 6/6 H16 11, 11, 15, 1,5 85 [29] 31/31 7/7 H17 11, 13, 85, 92 69 [23] 31/31 7/7 H18 8,5 8,6 77, 69 42 [14] 31/31 7/7 H19 9, 11, 66, 98 46 [18] 31/31 7/7 H2 8,6 8,6 69, 87 47 [17] 31/31 7/7 H21 8,7 11, 62, 78 32 [11] 31/31 7/7 H22 9,2 11, 46, 1,5 52 [2] 6/6 6/6 H23 8,9 17, 65, 82 22 [74] 4/4 4/4 H24 6,6 12, 34, 68 34 [11] 5/5 5/5 H25 5,2 7,8 44, 73 44 [14] 5/5 5/5 H26 2,9 2,6 15, 6 95 [31] 3/3 3/3 H27 2,4 2,5 9,6 58 52 [17] 3/3 3/3 H28 2,3 2,3 12, 42 6 [2] 3/3 3/3 H29 2,5 1,6 19, 5 68 [23] 3/3 3/3 258

PCB [] H14 17, 8,1 55, 1,5 25 [8.4] 7/7 14/14 H15 11, 9,6 15, 87 5 [17] 7/7 14/14 H16 15, 1, 54, 99 85 [29] 7/7 14/14 H17 14, 8,6 54, 8 69 [23] 8/8 16/16 H18 13, 9, 31, 99 42 [14] 8/8 16/16 H19 11, 6,2 53, 79 46 [18] 8/8 16/16 H2 12, 9,1 33, 1,2 47 [17] 85/85 17/17 H21 12, 12, 29, 84 32 [11] 9/9 18/18 H22 13, 1, 26, 88 52 [2] 18/18 18/18 H23 14, 12, 25, 9 22 [74] 18/18 18/18 H24 13, 14, 13, 92 34 [11] 19/19 19/19 H25 14, 13, 27, 1, 44 [14] 19/19 19/19 H26 13, 1, 23, 94 95 [31] 19/19 19/19 H27 11, 7,7 18, 1,3 52 [17] 19/19 19/19 H28 11, 8,4 15, 1,2 6 [2] 19/19 19/19 H29 1, 8,3 16, 86 68 [23] 19/19 19/19 H14 12, 14, 22, 4,8 25 [8.4] 1/1 2/2 H15 19, 22, 42, 6,8 5 [17] 1/1 2/2 H16 9, 9,4 13, 5,9 85 [29] 1/1 2/2 H17 1, 9,7 19, 5,6 69 [23] 1/1 2/2 H18 12, 9,8 48, 5,6 42 [14] 1/1 2/2 H19 7,6 7,8 15, 3,9 46 [18] 1/1 2/2 H2 9,7 7,4 56, 3, 47 [17] 1/1 2/2 H21 5,9 5,7 9,5 3,9 32 [11] 1/1 2/2 H22 7,7 --- 9,1 6,6 52 [2] 2/2 2/2 H23 --- --- 5,4 5,4 22 [74] 1/1 1/1 H24 5,9 --- 6,2 5,6 34 [11] 2/2 2/2 H25 36, --- 51, 25, 44 [14] 2/2 2/2 H26 46, --- 14, 15, 95 [31] 2/2 2/2 H27 --- --- 5, 5, 52 [17] 1/1 1/1 H28 31, --- 1, 9,8 6 [2] 2/2 2/2 H29 39, 19, 38, 4, 68 [23] 2/2 2/2 1 14 21 2[] [] 3 25 24 37 2.3pg/m 3 37 26 3,3pg/m 3 15 29 259

14 29 PCB [] PCB H14 1 1 88 16 99 [33] 12/12 34/34 H15 26 34 2,6 36 35/35 35/35 6.6 [2.2] H15 11 12 63 17 34/34 34/34 H16 24 25 3,3 25 2.9 [.98] H16 13 13 1,5 2 H17 19 21 1,5 23.38 [.14] H17 66 64 38 2 H18 17 18 1,5 21.8 [.3] H18 82 9 45 19 H19 25 29 98 37 24/24 24/24.37 [.13] H19 72 76 23 25 22/22 22/22 H2 2 17 96 52 22/22 22/22.8 [.3] H2 93 86 1,5 21 36/36 36/36 pg/m 3 H21 2 19 1,4 43 34/34 34/34.75 [.26] H21 85 78 38 2 34/34 34/34 H22 16 15 97 36 35/35 35/35 7.3 [2.5] H22 84 86 63 19 35/35 35/35 H23 15 16 66 32 35/35 35/35 18 [5.9] H23 76 66 32 tr(17) H24 13 13 84 27 35/35 35/35 26 [8.5] H24 54 62 28 tr(16) 35/35 35/35 H25 14 13 1,1 24 35/35 35/35 2 [6.5] H25 57 55 3 tr(19) 35/35 35/35 H26 14 15 1,3 28 4.1 [1.4] 36/36 36/36 H27 98 11 95 17 5.9 [2.] 35/35 35/35 H28 13 14 1,3 16 7.8 [2.7] H29 12 11 3,3 26 7. [2.3] 1[] [] 2 14 26

[1] PCB (pg/l) 7 6 5 4 3 2 1 [](pg/l) 14 7.4 [2.5] 15 9.4 [2.5] 16 14 [5.] 17 1 [3.2] 18 9 [3] 19 7.6 [2.9] 2 7.8 [3.] 21 1 [4] 22 73 [24] 23 4.5 [1.7] 24 44 [15] 25 25 [8] 26 8.2 [2.9] 27 21 [7.3] 28 7.8 [2.7] 29 16 [5.5] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 3-1-1 PCB [1] PCB (pg/g-dry) 12, 1, 8, 6, 4, 2, [] (pg/g-dry) 14 1 [3.5] 15 1 [3.2] 16 7.9 [2.6] 17 6.3 [2.1] 18 4 [1] 19 4.7 [1.5] 2 3.3 [1.2] 21 5.1 [2.1] 22 66 [22] 23 12 [4.5] 24 51 [18] 25 44 [13] 26 61 [21] 27 62 [22] 28 53 [18] 29 14 [5.] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 21 3-1-2 PCB 261

[1] PCB 2, 15, 1, 5, 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 [] 14 25 [8.4] 15 5 [17] 16 85 [29] 17 69 [23] 18 42 [14] 19 46 [18] 2 47 [17] 21 32 [11] 22 52 [2] 23 22 [74] 24 34 [11] 25 44 [14] 26 95 [31] 27 52 [17] 28 6 [2] 29 68 [23] 1 14 21 2 25 24 3-1-3 PCB [1] PCB 3 pg/m 3 25 2 15 1 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-1-4 PCB [] (pg/m 3 ) 14 99 [33] 15 6.6 [2.2] 16 2.9 [.98] 17.38 [.14] 18.8 [.3] 19.37 [.13] 2.8 [.3] 21.75 [.26] 22 7.3 [2.5] 23 18 [5.9] 24 26 [8.5] 25 2 [6.5] 26 4.1 [1.4] 27 5.9 [2.] 28 7.8 [2.7] 29 7. [2.3] 262

[2] HCB HCB 54 8 POPs 16 13 53 8 1 12 13 61 1 61 13 14 47.8 pg/l 47 2.9 18 pg/l 14 29 5 5 14 29 HCB HCB [] H14 37 28 1,4 9.8.6 [.2] 114/114 38/38 H15 29 24 34 11 5 [2] 36/36 36/36 H16 3 tr(29) 18 tr(11) 3 [8] 38/38 38/38 H17 21 17 21 tr(6) 15 [5] 47/47 47/47 H18 16 tr(12) 19 nd 16 [5] 46/48 46/48 H19 17 14 19 tr(4) 8 [3] 48/48 48/48 H2 16 13 48 4 3 [1] 48/48 48/48 H21 15 17 18 2.4.5 [.2] 49/49 49/49 (pg/l) H22 tr(1) tr(8) 12 nd 13 [4] 39/49 39/49 H23 13 12 14 tr(3) 5 [2] 49/49 49/49 H24 29 23 33 8.1 2.2 [.7] 48/48 48/48 H25 14 11 26 tr(4) 7 [2] 48/48 48/48 H26 12 9.7 2 2.7.9 [.4] 48/48 48/48 H27 15 13 14 4.2 1.8 [.6] 48/48 48/48 H28 13 11 13 4.2.9 [.3] 48/48 48/48 H29 12 1 18 2.9 2.1 [.8] 47/47 47/47 14 62 1 pg/g-dry 62 3 11, pg/g-dry 14 29 263

14 29 HCB HCB [] H14 24 2 19, 7.6.9 [.3] 189/189 63/63 H15 16 12 42, 5 4 [2] 186/186 62/62 H16 14 1 25, tr(6) 7 [3] 189/189 63/63 H17 17 13 22, 13 3 [1] 189/189 63/63 H18 18 12 19, 1 2.9 [1.] 192/192 64/64 H19 14 11 65, nd 5 [2] 191/192 64/64 H2 16 97 29, 4.4 2. [.8] 192/192 64/64 H21 15 12 34, nd 1.8 [.7] 19/192 64/64 (pg/g-dry) H22 13 96 21, 4 3 [1] 64/64 64/64 H23 15 11 35, 11 7 [3] 64/64 64/64 H24 1 11 12, 3 3 [1] 63/63 63/63 H25 12 91 6,6 7.2 5.3 [1.8] 63/63 63/63 H26 95 85 5,6 tr(4) 6 [2] 63/63 63/63 H27 1 9 17, 4 3 [1] 62/62 62/62 H28 84 74 6,4 4 3 [1] 62/62 62/62 H29 82 65 11, 3 3 [1] 62/62 62/62 14 21 3 1.3 pg/g-wet 3 26 99pg/g-wet 19 1.3 pg/g-wet 19 33 1,1pg/g-wet 2 1.3 pg/g-wet 2 23 4,9pg/g-wet 14 29 HCB HCB [] H14 21 22 33 2.4.18 [.6] 38/38 8/8 H15 44 27 66 tr(21) 23 [7.5] 3/3 6/6 H16 32 31 8 14 14 [4.6] 31/31 7/7 H17 51 28 45 19 11 [3.8] 31/31 7/7 H18 46 28 34 11 3 [1] 31/31 7/7 H19 37 22 4 11 7 [3] 31/31 7/7 H2 38 24 24 13 7 [3] 31/31 7/7 H21 34 32 2 12 4 [2] 31/31 7/7 H22 34 48 21 tr(4) 5 [2] 6/6 6/6 H23 45 34 92 4 4 [1] 4/4 4/4 H24 39 38 34 1 8.4 [2.8] 5/5 5/5 H25 32 39 25 nd 31 [1] 4/5 4/5 H26 34 26 1 15 1 [3] 3/3 3/3 H27 35 26 12 tr(14) 2 [6.5] 3/3 3/3 H28 38 22 15 17 8.1 [2.7] 3/3 3/3 H29 41 26 99 26 3.9 [1.3] 3/3 3/3 H14 14 18 91 19.18 [.6] 7/7 14/14 H15 18 17 1,5 28 23 [7.5] 7/7 14/14 H16 23 21 1,8 26 14 [4.6] 7/7 14/14 H17 18 16 1,7 29 11 [3.8] 8/8 16/16 H18 18 22 1,4 25 3 [1] 8/8 16/16 H19 16 14 1,5 17 7 [3] 8/8 16/16 H2 17 21 1,5 25 7 [3] 85/85 17/17 H21 21 18 3, 29 4 [2] 9/9 18/18 H22 24 28 1,7 36 5 [2] 18/18 18/18 H23 26 32 1,5 34 4 [1] 18/18 18/18 H24 2 3 1,1 33 8.4 [2.8] 19/19 19/19 H25 24 22 1,5 36 31 [1] 19/19 19/19 H26 28 34 1,9 37 1 [3] 19/19 19/19 H27 17 15 1,7 43 2 [6.5] 19/19 19/19 H28 15 15 1,3 24 8.1 [2.7] 19/19 19/19 H29 19 18 1,1 33 3.9 [1.3] 19/19 19/19 264

HCB [] H14 1, 1,2 1,6 56.18 [.6] 1/1 2/2 H15 1,8 2, 4,7 79 23 [7.5] 1/1 2/2 H16 98 1,3 2,2 41 14 [4.6] 1/1 2/2 H17 1, 1,1 2,5 4 11 [3.8] 1/1 2/2 H18 97 1,1 2,1 49 3 [1] 1/1 2/2 H19 96 1,1 2, 42 7 [3] 1/1 2/2 H2 88 1,1 2,5 24 7 [3] 1/1 2/2 H21 85 91 1,5 4 4 [2] 1/1 2/2 H22 97 --- 1,9 5 5 [2] 2/2 2/2 H23 --- --- 46 46 4 [1] 1/1 1/1 H24 84 --- 1,5 47 8.4 [2.8] 2/2 2/2 H25 3,9 --- 5,2 2,9 31 [1] 2/2 2/2 H26 42 --- 5,6 32 1 [3] 2/2 2/2 H27 --- --- 76 76 2 [6.5] 1/1 1/1 H28 1,7 --- 5,3 55 8.1 [2.7] 2/2 2/2 H29 1,1 2,6 4,9 23 3.9 [1.3] 2/2 2/2 1 14 21 2 25 24 37.2 pg/m 3 37 73 55pg/m 3 1429 HCB HCB [] H14 99 93 3, 57.9 [.3] 12/12 34/34 H15 15 13 43 81 35/35 35/35 2.3 [.78] H15 94 9 32 64 34/34 34/34 H16 13 13 43 47 1.1 [.37] H16 98 89 39 51 H17 88 9 25 27.14 [.34] H17 77 68 18 44 H18 83 89 21 23.21 [.7] H18 65 74 17 8.2 H19 11 1 23 72 24/24 24/24.9 [.3] H19 77 72 12 55 22/22 22/22 H2 12 11 26 78 22/22 22/22.22 [.8] H2 87 83 16 58 36/36 36/36 (pg/m 3 H21 11 11 21 78 34/34 34/34 ).6 [.2] H21 87 87 15 59 34/34 34/34 H22 12 12 16 73 1.8 [.7] H22 1 96 38 56 H23 12 11 18 87 35/35 35/35 2.3 [.75] H23 96 96 16 75 H24 12 11 15 84 36/36 36/36 4.3 [1.4] H24 97 95 15 68 36/36 36/36 H25 11 11 18 52 36/36 36/36 3.8 [1.3] H25 97 97 18 73 36/36 36/36 H26 15 16 24 84 1.4 [.5] 36/36 36/36 H27 12 13 17 74.5 [.2] 35/35 35/35 H28 13 13 22 79.8 [.3] H29 13 12 55 73.5 [.2] 265

[2] HCB (pg/l) 4 3 2 1 [](pg/l) 14.6 [.2] 15 5 [2] 16 3 [8] 17 15 [5] 18 16 [5] 19 8 [3] 2 3 [1] 21.5 [.2] 22 13 [4] 23 5 [2] 24 2.2 [.7] 25 7 [2] 26.9 [.4] 27 1.8 [.6] 28.9 [.3] 29 2.1 [.8] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 3-2-1 HCB [2] HCB (pg/g-dry) 3 25 2 15 1 5 [](pg/g-dry) 14.9 [.3] 15 4 [2] 16 7 [3] 17 3 [1] 18 2.9 [1.] 19 5 [2] 2 2. [.8] 21 1.8 [.7] 22 3 [1] 23 7 [3] 24 3 [1] 25 5.3[1.8] 26 6 [2] 27 3 [1] 28 3 [1] 29 3 [1] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 21 3-2-2 HCB 266

[2] HCB 3 25 2 15 1 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 [] 14.18 [.6] 15 23 [7.5] 16 14 [4.6] 17 11 [3.8] 18 3 [1] 19 7 [3] 2 7 [3] 21 4[2] 22 5 [2] 23 4 [1] 24 8.4 [2.8] 25 31 [1] 26 1 [3] 27 2 [6.5] 28 8.1 [2.7] 29 3.9 [1.3] 1 14 21 2 25 24 3-2-3 HCB [2] HCB pg/m 3 16 14 12 1 8 6 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-2-4 HCB [] (pg/m 3 ) 14.9 [.3] 15 2.3 [.78] 16 1.1 [.37] 17.14 [.34] 18.21 [.7] 19.9 [.3] 2.22 [.8] 21.6 [.2] 22 1.8 [.7] 23 2.3 [.75] 24 4.3 [1.4] 25 3.8 [1.3] 26 1.4 [.5] 27.5 [.2] 28.8 [.3] 29.5 [.2] 267

[3] 46 5 56 1 POPs 16 13 53 3 5 14 14 21 26 27 29 26 26 14 21 [] H14.8.9 18 nd.6 [.2] 93/114 37/38 H15.9.9 3.8 nd.6 [.2] 34/36 34/36 H16 tr(1.5) tr(1.8) 13 nd 2 [.4] 33/38 33/38 H17 tr(.6) tr(.7) 5.7 nd.9 [.3] 32/47 32/47 (pg/l) H18 nd nd 4.4 nd 1.7 [.6] 18/48 18/48 H19 tr(.6) tr(.6) 9.5 nd 1. [.3] 34/48 34/48 H2 tr(.8) tr(.7) 21 nd 1.4 [.6] 26/48 26/48 H21.7.9 22 nd.7 [.3] 32/49 32/49 14 14 21 [] (pg/g-dry) H14 14 12 57 nd 6 [2] 149/189 56/63 H15 19 18 1, nd 2 [.6] 178/186 6/62 H16 1 1 39 nd 2 [.6] 17/189 62/63 H17 8.4 7.1 5 nd 1.4 [.5] 173/189 62/63 H18 1 9.3 33 nd 1.9 [.6] 184/192 64/64 H19 7.5 6.7 33 nd 1.8 [.6] 172/192 6/64 H2 6 6 37 nd 3 [1] 153/192 56/64 H21 8.9 7.8 54 nd.5 [.2] 18/192 64/64 14 21 268

14 26 [] H14 tr(1.6) nd 34 nd 4.2 [1.4] 12/38 4/8 H15 tr(1.7) tr(.85) 51 nd 2.5 [.84] 15/3 3/6 H16 tr(2.5) tr(1.6) 46 nd 4. [1.3] 16/31 4/7 H17 tr(1.8) nd 84 nd 3.5 [1.2] 11/31 3/7 H18 tr(2) nd 19 nd 4 [2] 11/31 3/7 H19 tr(2) nd 26 nd 5 [2] 5/31 2/7 H2 tr(2) nd 2 nd 5 [2] 5/31 3/7 H21 tr(1.6) tr(.8) 89 nd 2.1 [.8] 16/31 6/7 H26 nd nd nd nd 1.8 [.7] /3 /3 H14 nd nd tr(2.) nd 4.2 [1.4] 1/7 1/14 H15 nd nd tr(1.9) nd 2.5 [.84] 16/7 7/14 H16 nd nd tr(2.4) nd 4. [1.3] 5/7 2/14 H17 nd nd 6.4 nd 3.5 [1.2] 11/8 5/16 H18 nd nd tr(2) nd 4 [2] 2/8 2/16 H19 nd nd tr(2) nd 5 [2] 2/8 2/16 H2 nd nd tr(2) nd 5 [2] 1/85 1/17 H21 nd nd 3.1 nd 2.1 [.8] 22/9 7/18 H26 nd nd 2.4 nd 1.8 [.7] 4/19 4/19 H14 nd nd nd nd 4.2 [1.4] /1 /2 H15 nd nd nd nd 2.5 [.84] /1 /2 H16 nd nd nd nd 4. [1.3] /1 /2 H17 nd nd nd nd 3.5 [1.2] /1 /2 H18 nd nd nd nd 4 [2] /1 /2 H19 nd nd nd nd 5 [2] /1 /2 H2 nd nd nd nd 5 [2] /1 /2 H21 nd nd nd nd 2.1 [.8] /1 /2 H26 nd --- nd nd 1.8 [.7] /2 /2 1 14 21 2 26 24 3 22 25 14 26 [] H14 tr(.3) nd 3.2 nd.6 [.2] 41/12 19/34 H15 1.5 1.9 28 nd 34/35 34/35.23 [.77] H15.55.44 6.9.3 34/34 34/34 H16 tr(.12) nd 14 nd 15/37 15/37.15 [.5] H16 tr(.8) nd 13 nd 14/37 14/37 H17.33.56 1 nd 29/37 29/37.8 [.3] H17 tr(.4) nd 1.8 nd 9/37 9/37 H18.3.35 8.5 nd 31/37 31/37 (pg/m 3.14 [.5] ) H18 tr(.5) nd 1.1 nd 16/37 16/37 H19.58.48 19 nd 35/36 35/36.5 [.2] H19.14.15 2.1 nd 34/36 34/36 H2.27.3 9.4 tr(.2) 25/25 25/25.4 [.2] H2.9.8 1.3 nd 22/25 22/25 H21.7 nd 1 nd 1/25 1/25.4 [.2] H21 tr(.3) nd 1.8 nd 8/24 8/24 H26 nd nd 17 nd 12 [4] 6/34 6/34 22 25 269

[3] 2 1.5 [](pg/l) 14.6 [.2] 15.6 [.2] 16 2 [.4] 17.9 [.3] 18 1.7 [.6] 19 1. [.3] 2 1.4 [.6] 21.7 [.3] (pg/l) 1.5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 22 29 3 18 1/2 3-3-1 [3] (pg/g-dry) 2 15 1 [](pg/g-dry) 14 6 [2] 15 2 [.6] 16 2 [.6] 17 1.4 [.5] 18 1.9 [.6] 19 1.8 [.6] 2 3 [1] 21.5 [.2] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 22 29 3-3-2 27

[3] 3 2.5 2 1.5 1 [](pg/gwet) 14 4.2 [1.4] 15 2.5 [.84] 16 4 [1.3] 17 3.5 [1.2] 18 4 [2] 19 5 [2] 2 5 [2] 21 2.1 [.8] 26 1.8 [.7].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 3 26 21 4 22 25 27 29 5 26 1/2 3-3-3 [3] 2.5 pg/m 3 2 1.5 1 [] (pg/m 3 ) 14.6 [.2] 15.23 [.77] 16.15 [.5] 17.8 [.3] 18.14 [.5] 19.5 [.2] 2.4 [.2] 21.4 [.2] 26 12 [4].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 22 25 27 29 2 26 1/2 3-3-4 271

[4] 3 46 5 56 1 POPs 16 13 53 8 1 12 13 61 1 61 13 14 14 21 23 26 27 29 26 26 14 26 [] (pg/l) H14 42 41 94 3.3 1.8 [.6] 114/114 38/38 H15 57 57 51 9.7.7 [.3] 36/36 36/36 H16 55 51 43 9 2 [.5] 38/38 38/38 H17 39 49 63 4.5 1. [.34] 47/47 47/47 H18 36 32 8 6 3 [1] 48/48 48/48 H19 38 36 75 3.1 2.1 [.7] 48/48 48/48 H2 36 37 45 3.6 1.5 [.6] 48/48 48/48 H21 36 32 65 2.7.6 [.2] 49/49 49/49 H23 33 38 3 2.1 1.6 [.6] 49/49 49/49 H26 28 27 2 2.7.5 [.2] 48/48 48/48 1 14 2 22 24 25 14 23 [] (pg/g-dry) H14 7 51 2,3 4 3 [1] 189/189 63/63 H15 66 56 9,1 nd 4 [2] 184/186 62/62 H16 65 62 3,7 tr(1.9) 3 [.9] 189/189 63/63 H17 61 55 4,2 tr(2) 3 [1] 189/189 63/63 H18 61 54 1,5 tr(1.7) 2.9 [1.] 192/192 64/64 H19 49 4 2,7 tr(1.2) 2.7 [.9] 192/192 64/64 H2 48 43 2,9 tr(.7) 1.2 [.5] 192/192 64/64 H21 51 47 3, 1.1.8 [.3] 192/192 64/64 H23 47 44 2,2 2 5 [2] 64/64 64/64 1 14 21 2 22 272

14 26 [] H14 44 39 19, tr(7) 12 [4] 38/38 8/8 H15 44 16 78, 46 4.8 [1.6] 3/3 6/6 H16 63 27 69, 42 31 [1] 31/31 7/7 H17 5 14 39, 34 9.4 [3.4] 31/31 7/7 H18 45 12 47, 3 7 [3] 31/31 7/7 H19 38 11 77, 37 9 [3] 31/31 7/7 H2 43 15 24, 47 9 [3] 31/31 7/7 H21 49 23 28, 48 7 [2] 31/31 7/7 H23 39 69 3,8 16 3 [1] 4/4 4/4 H26 18 3 49 41 3 [1] 3/3 3/3 H14 29 27 2,4 46 12 [4] 7/7 14/14 H15 22 2 1, 29 4.8 [1.6] 7/7 14/14 H16 25 23 2,8 tr(23) 31 [1] 7/7 14/14 H17 23 25 1,4 21 9.4 [3.4] 8/8 16/16 H18 23 22 1,4 19 7 [3] 8/8 16/16 H19 25 21 1,9 23 9 [3] 8/8 16/16 H2 24 24 1,3 15 9 [3] 85/85 17/17 H21 24 19 1,4 29 7 [2] 9/9 18/18 H23 27 34 1,1 17 3 [1] 18/18 18/18 H26 27 31 1, 27 3 [1] 19/19 19/19 H14 1,1 1,1 1,7 82 12 [4] 1/1 2/2 H15 1,3 1,4 2,2 79 4.8 [1.6] 1/1 2/2 H16 6 61 96 37 31 [1] 1/1 2/2 H17 83 74 1,8 5 9.4 [3.4] 1/1 2/2 H18 7 69 1,3 44 7 [3] 1/1 2/2 H19 71 71 91 56 9 [3] 1/1 2/2 H2 68 62 1,3 26 9 [3] 1/1 2/2 H21 47 42 89 33 7 [2] 1/1 2/2 H23 --- --- 77 77 3 [1] 1/1 1/1 H26 32 --- 53 19 3 [1] 2/2 2/2 1 14 21 2 26 23 3 22 24 25 14 26 [] H14 5.6 5.4 11.73.6 [.2] 12/12 34/34 H15 19 22 26 2.1 35/35 35/35 2.1 [.7] H15 5.7 5.2 11 tr(.82) 34/34 34/34 H16 17 22 28 1.1.33 [.11] H16 5.5 6.9 76.81 H17 14 12 2 1.5.54 [.24] H17 3.9 3.6 5.88 H18 15 14 29 1.5.3 [.1] H18 4.5 4.2 25.7 (pg/m 3 ) H19 19 22 31 1.3 36/36 36/36.18 [.7] H19 4.5 3.7 75.96 36/36 36/36 H2 14 16 22 1.6.24 [.9] H2 4.9 3.8 72.68 H21 13 13 15.91.6 [.2] H21 4.5 4. 8.52 H23 12 15 23.8 35/35 35/35.42 [.14] H23 4.3 4.9 96.52 H26 11 9.9 16.89.34 [.11] 36/36 36/36 22 24 25 273

[4] (pg/l) 6 5 4 3 2 [](pg/l) 14 1.8 [.6] 15.7 [.3] 16 2 [.5] 17 1. [.34] 18 3 [1] 19 2.1 [.7] 2 1.5 [.6] 21.6 [.2] 23 1.6 [.6] 26.5 [.2] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 22 24 25 27 29 3-4-1 [4] (pg/g-dry) 8 6 4 [](pg/g-dry) 14 3 [1] 15 4 [2] 16 3 [.9] 17 3 [1] 18 2.9 [1.] 19 2.7 [.9] 2 1.2 [.5] 21.8 [.3] 23 5 [2] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 22 24 29 3-4-2 274

[4] 8 6 4 [] 14 12 [4] 15 4.8 [1.6] 16 31 [1] 17 9.4 [3.4] 18 7 [3] 19 9 [3] 2 9 [3] 21 7[2] 23 3 [1] 26 3 [1] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 26 23 3 22 24 25 27 29 3-4-3 [4] 2 pg/m 3 15 1 [] (pg/m 3 ) 14.6 [.2] 15 2.1 [.7] 16.33 [.11] 17.54 [.24] 18.3 [.1] 19.18 [.7] 2.24 [.9] 21.6 [.2] 23.42 [.14] 26.34 [.11] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 22 24 25 27 29 3-4-4 275

[5] 5 56 1 POPs 16 13 53 3 5 14 14 21 23 26 27 29 26 26 14 26 [] (pg/l) H14 tr(4.8) tr(5.5) 31 nd 6. [2.] 11/114 36/38 H15 5.7 6. 78.7.7 [.3] 36/36 36/36 H16 7 7 1 tr(.7) 2 [.5] 38/38 38/38 H17 4. 4.5 12 nd 1.1 [.4] 45/47 45/47 H18 3.1 3.5 26 nd 1.3 [.4] 44/48 44/48 H19 3.5 3.4 25 nd 1.9 [.6] 46/48 46/48 H2 3 4 2 nd 3 [1] 45/48 45/48 H21 2. 2.3 67 nd.7 [.3] 39/49 39/49 H23 3.8 4.6 71 nd 1.6 [.6] 47/49 47/49 H26 2.5 2.2 25 tr(.4).5 [.2] 48/48 48/48 1 14 2 22 24 25 14 23 [] (pg/g-dry) H14 1 1 19, nd 6 [2] 141/189 54/63 H15 12 11 29, nd 5 [2] 15/186 53/62 H16 15 13 6,9 nd 3 [.9] 182/189 63/63 H17 12 11 19, nd 2.6 [.9] 17/189 61/63 H18 12 1 61, nd 4 [1] 178/192 63/64 H19 11 9 61, nd 5 [2] 151/192 55/64 H2 11 11 38, nd 1.9 [.7] 168/192 61/64 H21 9.6 8.4 11, nd 1.6 [.6] 168/192 63/64 H23 8.8 14 1,1 nd 1.1 [.4] 59/64 59/64 1 14 21 2 22 276

14 26 [] H14 42 27 12, nd 18 [6] 35/38 7/8 H15 38 21 5, 6.3 4.8 [1.6] 3/3 6/6 H16 65 25 4,6 tr(5.7) 12 [4.2] 31/31 7/7 H17 39 19 2,1 nd 17 [5.5] 27/31 7/7 H18 4 15 3,1 tr(5) 11 [4] 31/31 7/7 H19 28 12 3, tr(6) 9 [3] 31/31 7/7 H2 3 1 1,5 tr(6) 8 [3] 31/31 7/7 H21 38 19 1,4 tr(5) 7 [3] 31/31 7/7 H23 33 62 11 tr(3) 4 [2] 4/4 4/4 H26 23 17 84 8 3 [1] 3/3 3/3 H14 2 24 18 nd 18 [6] 54/7 13/14 H15 14 1 18 nd 4.8 [1.6] 67/7 14/14 H16 18 24 22 nd 12 [4.2] 57/7 13/14 H17 19 tr(16) 2,1 nd 17 [5.5] 58/8 12/16 H18 13 tr(1) 15 nd 11 [4] 66/8 16/16 H19 13 12 17 nd 9 [3] 69/8 15/16 H2 11 1 2 nd 8 [3] 63/85 14/17 H21 17 12 27 nd 7 [3] 86/9 18/18 H23 18 19 16 nd 4 [2] 16/18 16/18 H26 16 16 14 nd 3 [1] 18/19 18/19 H14 28 52 99 nd 18 [6] 7/1 2/2 H15 22 3 96 5.4 4.8 [1.6] 1/1 2/2 H16 tr(11) 25 62 nd 12 [4.2] 5/1 1/2 H17 18 28 64 nd 17 [5.5] 7/1 2/2 H18 16 23 57 tr(4) 11 [4] 1/1 2/2 H19 17 28 55 nd 9 [3] 9/1 2/2 H2 1 26 83 nd 8 [3] 5/1 1/2 H21 11 17 43 tr(3) 7 [3] 1/1 2/2 H23 --- --- tr(3) tr(3) 4 [2] 1/1 1/1 H26 4.5 --- 5 4 3 [1] 2/2 2/2 1 14 21 2 22 24 25 3 26 23 14 26 [] H14.22.28 2.5 nd.9 [.3] 9/12 32/34 H15.74.95 6.2.81 35/35 35/35.42 [.14] H15.23.2 2.1.42 34/34 34/34 H16.64.68 6.5 tr(.54).14 [.48] H16.23.26 1.9 nd 36/37 36/37 H17 tr(.4) tr(.3) 2.9 nd 27/37 27/37.5 [.2] H17 nd nd.7 nd 8/37 8/37 H18.31.32 5.4 nd 32/37 32/37.3 [.1] H18 nd nd 5. nd 7/37 7/37 (pg/m 3 ) H19.69.73 6.3 tr(.6) 36/36 36/36.9 [.4] H19.16.13 1.5 nd 33/36 33/36 H2.53.68 4.6 tr(.6).1 [.4] H2.18.18 1.8 nd 35/37 35/37 H21.49.51 3.4 nd 36/37 36/37.9 [.4] H21.17.15 1.8 nd 36/37 36/37 H23.46.62 5.1 nd 34/35 34/35.9 [.4] H23.16.16 1.8 nd 33/37 33/37 H26.39.48 2.9 nd.2 [.7] 32/36 32/36 22 24 25 277

[5] (pg/l) 8 6 4 [](pg/l) 14 6. [2.] 15.7 [.3] 16 2 [.5] 17 1.1 [.4] 18 1.3 [.4] 19 1.9 [.6] 2 3 [1] 21.7 [.3] 23 1.6 [.6] 26.5 [.2] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 22 24 25 27 29 3-5-1 [5] (pg/g-dry) 16 12 8 [](pg/g-dry) 14 6 [2] 15 5 [2] 16 3 [.9] 17 2.6 [.9] 18 4 [1] 19 5 [2] 2 1.9 [.7] 21 1.6 [.6] 23 1.1 [.4] 4 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 22 24 29 3-5-2 278

[5] 8 6 4 [] 14 18 [6] 15 4.8 [1.6] 16 12 [4.2] 17 17 [5.5] 18 11 [4] 19 9 [3] 2 8 [3] 21 7[3] 23 4 [2] 26 3 [1] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 22 24 25 27 29 3-5-3 [5].8 pg/m 3.6.4 [] (pg/m 3 ) 14.9 [.3] 15.42 [.14] 16.14 [.48] 17.5 [.2] 18.3 [.1] 19.9 [.4] 2.1 [.4] 21.9 [.4] 23.9 [.4] 26.2 [.7].2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 22 24 25 27 29 2 17 18 1/2 3-5-4 279

[6] DDT DDT HCH 46 56 1 p,p'-ddt POPs 16 DDT DDT p,p'-ddt o,p'-ddt DDT p,p'-dde o,p'-dde p,p'-ddd o,p'-ddd 53 13 p,p'-ddt p,p'-dde p,p'-ddd 53 13 61 1 61 13 o,p'-ddt o,p'-dde o,p'-ddd 53 8 1 12 13 14 p,p'-ddt p,p'-dde p,p'-ddd o,p'-ddt o,p'-dde o,p'-ddd 14 22 25 26 27 28 29 27 27 p,p'-ddt p,p'-dde p,p'-ddd 14 26 p,p'-ddt p,p'-dde p,p'-ddd p,p'-ddt [] H14 13 11 44.25.6 [.2] 114/114 38/38 H15 14 12 74 tr(2.8) 3 [.9] 36/36 36/36 H16 15 14 31 nd 6 [2] 36/38 36/38 H17 8 9 11 1 4 [1] 47/47 47/47 H18 9.1 9.2 17 tr(1.6) 1.9 [.6] 48/48 48/48 (pg/l) H19 7.3 9.1 67 nd 1.7 [.6] 46/48 46/48 H2 11 11 1,2 nd 1.2 [.5] 47/48 47/48 H21 9.2 8.4 44.81.15 [.6] 49/49 49/49 H22 8.5 7.6 7,5 tr(1.) 2.4 [.8] 49/49 49/49 H26 4.4 3.9 38 nd.4 [.1] 47/48 47/48 28

p,p'-dde [] H14 25 26 76 1.3.6 [.2] 114/114 38/38 H15 26 22 38 5 4 [2] 36/36 36/36 H16 36 34 68 tr(6) 8 [3] 38/38 38/38 H17 26 24 41 4 6 [2] 47/47 47/47 H18 24 24 17 tr(4) 7 [2] 48/48 48/48 (pg/l) H19 22 23 44 tr(2) 4 [2] 48/48 48/48 H2 27 28 35 2.5 1.1 [.4] 48/48 48/48 H21 23 23 24 3.4 1.1 [.4] 49/49 49/49 H22 14 12 1,6 2.4 2.3 [.8] 49/49 49/49 H26 16 17 61 1.9.5 [.2] 48/48 48/48 p,p'-ddd [] H14 16 18 19.57.24 [.8] 114/114 38/38 H15 19 18 41 4 2 [.5] 36/36 36/36 H16 19 18 74 tr(2.4) 3 [.8] 38/38 38/38 H17 17 16 13 tr(1.8) 1.9 [.64] 47/47 47/47 H18 16 17 99 2. 1.6 [.5] 48/48 48/48 (pg/l) H19 15 12 15 tr(1.5) 1.7 [.6] 48/48 48/48 H2 22 2 85 2..6 [.2] 48/48 48/48 H21 14 13 14 1.4.4 [.2] 49/49 49/49 H22 12 1 97 1.6.2 [.8] 49/49 49/49 H26 9. 8.7 87 1. 1. [.4] 48/48 48/48 1 14 2 23 25 14 26 p,p'-ddt p,p'-dde p,p'-ddd p,p'-ddt [] H14 38 24 97, tr(5) 6 [2] 189/189 63/63 H15 29 22 55, 3 2 [.4] 186/186 62/62 H16 46 23 98, 7 2 [.5] 189/189 63/63 H17 36 23 1,7, 5.1 1. [.34] 189/189 63/63 H18 31 24 13, 4.5 1.4 [.5] 192/192 64/64 (pg/g-dry) H19 21 15 13, 3 1.3 [.5] 192/192 64/64 H2 27 18 1,4, 4.8 1.2 [.5] 192/192 64/64 H21 25 17 2,1, 1.9 1. [.4] 192/192 64/64 H22 23 2 22, 9.3 2.8 [.9] 64/64 64/64 H26 14 14 12, tr(.2).4 [.2] 63/63 63/63 p,p'-dde [] (pg/g-dry) p,p'-ddd (pg/g-dry) H14 78 63 23, 8.4 2.7 [.9] 189/189 63/63 H15 79 78 8, 9.5.9 [.3] 186/186 62/62 H16 72 7 39, 8 3 [.8] 189/189 63/63 H17 71 73 64, 8.4 2.7 [.94] 189/189 63/63 H18 71 82 49, 5.8 1. [.3] 192/192 64/64 H19 67 9 61, 3.2 1.1 [.4] 192/192 64/64 H2 92 94 96, 9. 1.7 [.7] 192/192 64/64 H21 7 66 5, 6.7.8 [.3] 192/192 64/64 H22 68 79 4, 11 5 [2] 64/64 64/64 H26 53 61 64, 11 1.8 [.6] 63/63 63/63 [] H14 64 69 51, tr(2.2) 2.4 [.8] 189/189 63/63 H15 67 58 32, 3.7.9 [.3] 186/186 62/62 H16 65 55 75, 4 2 [.7] 189/189 63/63 H17 6 57 21, 5.2 1.7 [.64] 189/189 63/63 H18 56 54 53, 2.2.7 [.2] 192/192 64/64 H19 52 55 8, 3.5 1. [.4] 192/192 64/64 H2 74 66 3, 2.8 1. [.4] 192/192 64/64 H21 54 56 3, 3.9.4 [.2] 192/192 64/64 H22 51 51 78, 4.4 1.4 [.5] 64/64 64/64 H26 33 41 21, 4.9 4.2 [1.4] 63/63 63/63 1 14 21 2 23 25 281

14 25 p,p'-ddt p,p'-dde p,p'-ddd p,p'-ddt [] H14 2 2 1,2 38 4.2 [1.4] 38/38 8/8 H15 29 29 1,8 49 11 [3.5] 3/3 6/6 H16 36 34 2,6 48 3.2 [1.1] 31/31 7/7 H17 24 17 1,3 66 5.1 [1.7] 31/31 7/7 H18 25 22 1,1 56 6 [2] 31/31 7/7 H19 24 15 1,2 49 5 [2] 31/31 7/7 H2 16 1 1,4 12 5 [2] 31/31 7/7 H21 24 17 9,6 46 3 [1] 31/31 7/7 H22 18 28 47 43 3 [1] 6/6 6/6 H25 19 21 89 46 3.3 [1.1] 5/5 5/5 p,p'-dde H14 43 45 24, 6.8 4.2 [1.4] 7/7 14/14 H15 22 4 1,9 tr(3.7) 11 [3.5] 7/7 14/14 H16 41 33 53, 5.5 3.2 [1.1] 7/7 14/14 H17 28 33 8,4 tr(3.8) 5.1 [1.7] 8/8 16/16 H18 3 34 3, tr(5) 6 [2] 8/8 16/16 H19 26 32 1,8 9 5 [2] 8/8 16/16 H2 28 31 2,9 7 5 [2] 85/85 17/17 H21 25 3 2, 4 3 [1] 9/9 18/18 H22 24 28 2,1 7 3 [1] 18/18 18/18 H25 28 25 3,3 5.2 3.3 [1.1] 19/19 19/19 H14 44 51 1,3 76 4.2 [1.4] 1/1 2/2 H15 61 62 1,4 18 11 [3.5] 1/1 2/2 H16 34 32 7 16 3.2 [1.1] 1/1 2/2 H17 43 55 9 18 5.1 [1.7] 1/1 2/2 H18 58 49 1,8 11 6 [2] 1/1 2/2 H19 48 35 1,9 16 5 [2] 1/1 2/2 H2 16 17 27 56 5 [2] 1/1 2/2 H21 3 19 2,9 85 3 [1] 1/1 2/2 H22 3 --- 15 nd 3 [1] 1/2 1/2 H25 14 --- 46 4.3 3.3 [1.1] 2/2 2/2 [] H14 1, 1,7 6, 14 2.4 [.8] 38/38 8/8 H15 1,2 1, 6,5 19 5.7 [1.9] 3/3 6/6 H16 1,3 1,4 8,4 22 8.2 [2.7] 31/31 7/7 H17 1,2 1,6 6,6 23 8.5 [2.8] 31/31 7/7 H18 1, 1,2 6, 16 1.9 [.7] 31/31 7/7 H19 1,1 1,2 5,6 18 3 [1] 31/31 7/7 H2 9 1,1 5,8 12 3 [1] 31/31 7/7 H21 94 1,1 6,4 15 4 [1] 31/31 7/7 H22 1,1 1,3 6,3 23 3 [1] 6/6 6/6 H25 79 1,6 3, 17 4.3 [1.4] 5/5 5/5 H14 2,9 2,2 98, 51 2.4 [.8] 7/7 14/14 H15 2, 2,2 12, 18 5.7 [1.9] 7/7 14/14 H16 3, 2,1 52, 39 8.2 [2.7] 7/7 14/14 H17 2,4 2,4 73, 23 8.5 [2.8] 8/8 16/16 H18 2,2 2,6 28, 28 1.9 [.7] 8/8 16/16 H19 2,2 2, 22, 16 3 [1] 8/8 16/16 H2 2,5 2, 53, 32 3 [1] 85/85 17/17 H21 2,3 2,1 2, 26 4 [1] 9/9 18/18 H22 2,3 2,1 13, 26 3 [1] 18/18 18/18 H25 2,9 2,8 16, 43 4.3 [1.4] 19/19 19/19 H14 36, 6, 17, 8,1 2.4 [.8] 1/1 2/2 H15 66, 76, 24, 18, 5.7 [1.9] 1/1 2/2 H16 34, 65, 2, 6,8 8.2 [2.7] 1/1 2/2 H17 44, 86, 3, 7,1 8.5 [2.8] 1/1 2/2 H18 38, 57, 16, 5,9 1.9 [.7] 1/1 2/2 H19 4, 56, 32, 6,7 3 [1] 1/1 2/2 H2 51, 79, 16, 7,5 3 [1] 1/1 2/2 H21 3, 64, 22, 4,3 4 [1] 1/1 2/2 H22 32, --- 16, 6,3 3 [1] 2/2 2/2 H25 17, --- 17, 17, 4.3 [1.4] 2/2 2/2 282

p,p'-ddd [] H14 34 71 3,2 11 5.4 [1.8] 38/38 8/8 H15 39 64 2,6 tr(7.5) 9.9 [3.3] 3/3 6/6 H16 44 24 8,9 7.8 2.2 [.7] 31/31 7/7 H17 37 8 1,7 13 2.9 [.97] 31/31 7/7 H18 3 48 1,4 7.3 2.4 [.9] 31/31 7/7 H19 31 36 1,5 7 3 [1] 31/31 7/7 H2 28 28 1,3 6 3 [1] 31/31 7/7 H21 22 17 2,4 5.8 2.4 [.9] 31/31 7/7 H22 18 33 96 11 1.3 [.5] 6/6 6/6 H25 27 52 1,3 19 1.9 [.7] 5/5 5/5 H14 75 68 14, 8 5.4 [1.8] 7/7 14/14 H15 51 52 3,7 43 9.9 [3.3] 7/7 14/14 H16 77 51 9,7 56 2.2 [.7] 7/7 14/14 H17 51 65 6,7 29 2.9 [.97] 8/8 16/16 H18 52 58 4,3 6 2.4 [.9] 8/8 16/16 H19 47 49 4,1 36 3 [1] 8/8 16/16 H2 46 44 4,1 33 3 [1] 85/85 17/17 H21 44 46 2,5 57 2.4 [.9] 9/9 18/18 H22 56 61 2,9 57 1.3 [.5] 18/18 18/18 H25 5 5 4,7 68 1.9 [.7] 19/19 19/19 H14 58 74 3,9 14 5.4 [1.8] 1/1 2/2 H15 64 86 3,9 11 9.9 [3.3] 1/1 2/2 H16 33 52 1,4 52 2.2 [.7] 1/1 2/2 H17 31 54 1,4 45 2.9 [.97] 1/1 2/2 H18 41 74 1,8 55 2.4 [.9] 1/1 2/2 H19 44 78 2,3 7 3 [1] 1/1 2/2 H2 24 49 1,1 35 3 [1] 1/1 2/2 H21 28 43 3,4 31 2.4 [.9] 1/1 2/2 H22 44 --- 1,6 12 1.3 [.5] 2/2 2/2 H25 14 --- 27 7 1.9 [.7] 2/2 2/2 1 14 21 2 25 22 3 23 24 14 27 p,p'-ddt p,p'-dde p,p'-ddd [] p,p'-ddt H14 1.9 1.8 22.25.24 [.8] 12/12 34/34 H15 5.8 6.6 24.75 35/35 35/35.14 [.46] H15 1.7 1.6 11.31 34/34 34/34 H16 4.7 5.1 37.41.22 [.74] H16 1.8 1.7 13.29 H17 4.1 4.2 31.44.16 [.54] H17 1.1.99 4.8.25 H18 4.2 3.8 51.35.17 [.6] H18 1.4 1.2 7.3.29 H19 4.9 5.2 3.6 36/36 36/36 (pg/m 3.7 [.3] ) H19 1.2 1.2 8.8.23 36/36 36/36 H2 3.6 3. 27.76.7 [.3] H2 1.2 1. 15.22 H21 3.6 3.6 28.44.7 [.3] H21 1.1 1. 8..2 H22 3.5 3.1 56.28.1 [.3] H22 1.3.89 16.3 H25 2.8 3.6 17.2 36/36 36/36.11 [.4] H25.65.53 4.5.18 36/36 36/36 H27 1.5 1.8 13.18.15 [.5] 35/35 35/35 283

[] p,p'-dde H14 2.8 2.7 28.56.9 [.3] 12/12 34/34 H15 7.2 7. 51 1.2 35/35 35/35.4 [.13] H15 2.8 2.4 22 1.1 34/34 34/34 H16 6.1 6.3 95.62.12 [.39] H16 2.9 2.6 43.85 H17 5. 5.7 42 1.2.14 [.34] H17 1.7 1.5 9.9.76 H18 5. 4.7 49 1.7.1 [.3] H18 1.9 1.7 9.5.52 H19 6.4 6.1 12.54 36/36 36/36 (pg/m 3.4 [.2] ) H19 2.1 1.9 39.73 36/36 36/36 H2 4.8 4.4 96.98.4 [.2] H2 2.2 2. 22.89 H21 4.9 4.8 13.87.8 [.3] H21 2.1 1.9 1.6 H22 4.9 4.1 2 tr(.41).62 [.21] H22 2.2 1.8 28 tr(.47) H25 4.1 4.3 37.2 36/36 36/36.1 [.3] H25 1.6 1.5 11.6 36/36 36/36 H27 2.4 2.6 34.31.12 [.4] 35/35 35/35 [] p,p'-ddd H14.12.13.76 nd.18 [.6] 11/12 34/34 H15.3.35 1.4.63 35/35 35/35.54 [.18] H15.13.14.52 tr(.37) 34/34 34/34 H16.24.27 1.4 tr(.36).53 [.18] H16.12.12.91 tr(.25) H17.24.26 1.3 tr(.7).16 [.5] H17 tr(.6) tr(.7).29 nd 28/37 28/37 H18.28.32 1.3 nd 36/37 36/37.13 [.4] H18.14 tr(.12).99 nd 36/37 36/37 H19.26.27 1.4.46 36/36 36/36 (pg/m 3.11 [.4] ) H19.93.87.5.26 36/36 36/36 H2.17.17 1.1.37.25 [.9] H2.91.81.31.36 H21.17.18.82.3.3 [.1] H21.8.8.35 tr(.2) H22.2.17 1.7.4.2 [.1] H22.1.9.41.2 H25.16.18.8.27 36/36 36/36.18 [.7] H25.56.54.14 tr(.15) 36/36 36/36 H27 nd nd tr(.31) nd.33 [.11] 17/35 17/35 23 24 26 o,p'-ddt o,p'-dde o,p'-ddd 14 26 o,p'-ddt o,p'-dde o,p'-ddd o,p'-ddt [] H14 5.4 4.6 77.19 1.2 [.4] 114/114 38/38 H15 6 5 1 tr(1.5) 3 [.7] 36/36 36/36 H16 tr(4.5) 5 85 nd 5 [2] 29/38 29/38 H17 3 3 39 nd 3 [1] 42/47 42/47 H18 2.8 2.4 52.51 2.3 [.8] 48/48 48/48 (pg/l) H19 tr(2.1) tr(2.2) 86 nd 2.5 [.8] 38/48 38/48 H2 3.1 3. 23 nd 1.4 [.5] 44/48 44/48 H21 2.4 2.4 1.43.16 [.6] 49/49 49/49 H22 1.5 tr(1.2) 7 nd 1.5 [.5] 43/49 43/49 H26 1. 1. 63 nd.4 [.2] 42/48 42/48 284

o,p'-dde [] H14 2.4 2.1 68 nd.9 [.3] 113/114 38/38 H15 2.2 2. 17 tr(.42).8 [.3] 36/36 36/36 H16 3 2 17 tr(.6) 2 [.5] 38/38 38/38 H17 2.5 2.1 41.4 1.2 [.4] 47/47 47/47 H18 tr(1.6) tr(1.4) 21 nd 2.6 [.9] 28/48 28/48 (pg/l) H19 tr(1.5) tr(1.1) 21 nd 2.3 [.8] 29/48 29/48 H2 1.5 1.8 26 nd.7 [.3] 39/48 39/48 H21 1.3 1.1 14 nd.22 [.9] 47/49 47/49 H22.97.65 18 tr(.13).24 [.9] 49/49 49/49 H26.6.6 56 nd.3 [.1] 36/48 36/48 o,p'-ddd [] H14 5.6 6. 11 nd.6 [.2] 113/114 38/38 H15 7.1 5. 16 1.1.8 [.3] 36/36 36/36 H16 6 5 81 tr(.7) 2 [.5] 38/38 38/38 H17 5.2 5.4 51 tr(.5) 1.2 [.4] 47/47 47/47 H18 2.5 3.3 39 nd.8 [.3] 4/48 4/48 (pg/l) H19 4.6 3.9 41 tr(.3).8 [.3] 48/48 48/48 H2 6.7 7.2 17 nd.8 [.3] 47/48 47/48 H21 4.4 3.8 41.44.22 [.9] 49/49 49/49 H22 4.6 3.8 17 tr(.5).6 [.2] 49/49 49/49 H26 3.7 3.2 38.33.2 [.8] 48/48 48/48 1 14 2 23 25 14 26 o,p'-ddt o,p'-dde o,p'-ddd o,p'-ddt [] H14 76 47 27, nd 6 [2] 183/189 62/63 H15 5 43 3,2 nd.8 [.3] 185/186 62/62 H16 69 5 17, tr(1.1) 2 [.6] 189/189 63/63 H17 58 46 16,.8.8 [.3] 189/189 63/63 H18 57 52 18, tr(.8) 1.2 [.4] 192/192 64/64 (pg/g-dry) H19 38 31 27, nd 1.8 [.6] 186/192 63/64 H2 51 4 14, tr(.7) 1.5 [.6] 192/192 64/64 H21 44 3 1, nd 1.2 [.5] 19/192 64/64 H22 4 33 13, 1.4 1.1 [.4] 64/64 64/64 H26 26 24 2,4 nd.4 [.2] 62/63 62/63 o,p'-dde [] (pg/g-dry) o,p'-ddd (pg/g-dry) H14 54 37 16, nd 3 [1] 188/189 63/63 H15 48 39 24, tr(.5).6 [.2] 186/186 62/62 H16 4 34 28, nd 3 [.8] 184/189 63/63 H17 4 32 31, nd 2.6 [.9] 181/189 62/63 H18 42 4 27, tr(.4) 1.1 [.4] 192/192 64/64 H19 37 41 25, nd 1.2 [.4] 186/192 63/64 H2 5 48 37, nd 1.4 [.6] 186/192 63/64 H21 37 31 33, nd.6 [.2] 191/192 64/64 H22 37 32 25, tr(.7) 1.2 [.5] 64/64 64/64 H26 3 32 41, tr(.5).8 [.3] 63/63 63/63 [] H14 16 15 14, nd 6 [2] 184/189 62/63 H15 16 13 8,8 tr(1.) 2 [.5] 186/186 62/62 H16 14 12 16, tr(.7) 2 [.5] 189/189 63/63 H17 13 11 32, tr(.8) 1. [.3] 189/189 63/63 H18 12 11 13, tr(.3).5 [.2] 192/192 64/64 H19 11 13 21, tr(.5) 1. [.4] 192/192 64/64 H2 17 15 5,.5.3 [.1] 192/192 64/64 H21 12 12 24,.5.5 [.2] 192/192 64/64 H22 13 13 6,9 tr(.8).9 [.4] 64/64 64/64 H26 74 85 3,2 tr(.7) 1.2 [.5] 63/63 63/63 1 14 21 2 23 25 285

14 25 o,p'-ddt o,p'-dde o,p'-ddd o,p'-ddt [] H14 11 83 48 22 12 [4] 38/38 8/8 H15 13 12 48 35 2.9 [.97] 3/3 6/6 H16 16 14 91 2 1.8 [.61] 31/31 7/7 H17 98 57 44 29 2.6 [.86] 31/31 7/7 H18 92 79 38 24 3 [1] 31/31 7/7 H19 79 52 35 2 3 [1] 31/31 7/7 H2 58 37 33 5 3 [1] 31/31 7/7 H21 74 48 2,5 17 2.2 [.8] 31/31 7/7 H22 51 67 16 15 3 [1] 6/6 6/6 H25 49 51 18 12 3 [1] 5/5 5/5 o,p'-dde H14 13 13 2,3 tr(6) 12 [4] 7/7 14/14 H15 85 12 52 2.9 2.9 [.97] 7/7 14/14 H16 16 14 1,8 3.7 1.8 [.61] 7/7 14/14 H17 1 11 1,5 5.8 2.6 [.86] 8/8 16/16 H18 1 11 7 6 3 [1] 8/8 16/16 H19 69 9 43 3 3 [1] 8/8 16/16 H2 72 92 72 3 3 [1] 85/85 17/17 H21 61 73 47 2.4 2.2 [.8] 9/9 18/18 H22 58 71 55 5 3 [1] 18/18 18/18 H25 58 76 31 4 3 [1] 19/19 19/19 H14 12 tr(1) 58 nd 12 [4] 8/1 2/2 H15 24 16 66 8.3 2.9 [.97] 1/1 2/2 H16 8.5 13 43 tr(.87) 1.8 [.61] 1/1 2/2 H17 11 14 24 3.4 2.6 [.86] 1/1 2/2 H18 14 1 12 3 3 [1] 1/1 2/2 H19 9 9 26 tr(2) 3 [1] 1/1 2/2 H2 4 6 16 nd 3 [1] 8/1 2/2 H21 6.3 7.6 12 tr(1.4) 2.2 [.8] 1/1 2/2 H22 nd --- nd nd 3 [1] /2 /2 H25 nd --- tr(1) nd 3 [1] 1/2 1/2 [] H14 83 66 1,1 13 3.6 [1.2] 38/38 8/8 H15 85 1 46 17 3.6 [1.2] 3/3 6/6 H16 86 69 36 19 2.1 [.69] 31/31 7/7 H17 7 89 47 12 3.4 [1.1] 31/31 7/7 H18 62 81 34 12 3 [1] 31/31 7/7 H19 56 69 41 8.9 2.3 [.9] 31/31 7/7 H2 49 52 39 8 3 [1] 31/31 7/7 H21 46 58 31 8 3 [1] 31/31 7/7 H22 46 58 16 7.8 1.5 [.6] 6/6 6/6 H25 28 31 26 4 4 [1] 5/5 5/5 H14 91 5 13, 3.6 3.6 [1.2] 7/7 14/14 H15 51 54 2,5 nd 3.6 [1.2] 67/7 14/14 H16 76 48 5,8 tr(.89) 2.1 [.69] 7/7 14/14 H17 54 45 12, tr(1.4) 3.4 [1.1] 8/8 16/16 H18 56 43 4,8 tr(1) 3 [1] 8/8 16/16 H19 45 29 4,4 nd 2.3 [.9] 79/8 16/16 H2 5 37 13, tr(1) 3 [1] 85/85 17/17 H21 46 33 4,3 tr(1) 3 [1] 9/9 18/18 H22 47 37 2,8 tr(1.2) 1.5 [.6] 18/18 18/18 H25 51 4 3, tr(1) 4 [1] 19/19 19/19 H14 28 26 49 2 3.6 [1.2] 1/1 2/2 H15 tr(2.3) tr(2.) 4.2 nd 3.6 [1.2] 9/1 2/2 H16 tr(1.) tr(1.1) 3.7 nd 2.1 [.69] 5/1 1/2 H17 tr(1.2) tr(1.9) tr(2.9) nd 3.4 [1.1] 7/1 2/2 H18 tr(1) tr(2) 3 tr(1) 3 [1] 1/1 2/2 H19 tr(1.) tr(1.4) 2.8 nd 2.3 [.9] 6/1 2/2 H2 tr(1) nd 3 nd 3 [1] 5/1 1/2 H21 nd tr(1) tr(2) nd 3 [1] 6/1 2/2 H22 tr(1.1) --- 3.7 nd 1.5 [.6] 1/2 1/2 H25 nd --- tr(1) nd 4 [1] 1/2 1/2 286

o,p'-ddd [] H14 12 19 2,9 tr(9) 12 [4] 38/38 8/8 H15 2 22 1,9 6.5 6. [2.] 3/3 6/6 H16 22 13 2,8 6. 5.7 [1.9] 31/31 7/7 H17 17 28 1,8 1 3.3 [1.1] 31/31 7/7 H18 15 2 1, 7 4 [1] 31/31 7/7 H19 15 2 1,2 6 3 [1] 31/31 7/7 H2 13 14 1,1 5 4 [2] 31/31 7/7 H21 95 51 1, 5 3 [1] 31/31 7/7 H22 57 5 4 5.8.6 [.2] 6/6 6/6 H25 1 74 1,8 7.8 1.8 [.7] 5/5 5/5 H14 95 9 1,1 nd 12 [4] 66/7 14/14 H15 75 96 92 nd 6. [2.] 66/7 14/14 H16 12 96 1,7 nd 5.7 [1.9] 68/7 14/14 H17 83 81 1,4 nd 3.3 [1.1] 79/8 16/16 H18 8 86 1,1 tr(1) 4 [1] 8/8 16/16 H19 66 62 1,3 nd 3 [1] 78/8 16/16 H2 65 74 1, nd 4 [2] 8/85 16/17 H21 63 64 76 nd 3 [1] 87/9 18/18 H22 75 99 7 2.6.6 [.2] 18/18 18/18 H25 7 85 94 nd 1.8 [.7] 18/19 18/19 H14 15 15 23 tr(8) 12 [4] 1/1 2/2 H15 15 14 36 tr(5.) 6. [2.] 1/1 2/2 H16 6.1 5.7 25 nd 5.7 [1.9] 9/1 2/2 H17 7.3 7.5 9.7 4.7 3.3 [1.1] 1/1 2/2 H18 8 8 19 5 4 [1] 1/1 2/2 H19 7 7 1 5 3 [1] 1/1 2/2 H2 4 tr(3) 14 tr(2) 4 [2] 1/1 2/2 H21 6 5 13 3 3 [1] 1/1 2/2 H22 6.3 --- 11 3.6.6 [.2] 2/2 2/2 H25 5.4 --- 12 2.4 1.8 [.7] 2/2 2/2 1 14 21 2 25 22 3 23 24 14 27 o,p'-ddt o,p'-dde o,p'-ddd [] o,p'-ddt H14 2.2 2. 4.41.15 [.5] 12/12 34/34 H15 6.9 7.7 38.61 35/35 35/35.12 [.4] H15 1.6 1.4 6.4.43 34/34 34/34 H16 5.1 5.4 22.54.93 [.31] H16 1.5 1.4 9.4.35 H17 3. 3.1 14.67.1 [.34] H17.76.67 3..32 H18 2.5 2.4 2.55.9 [.3] H18.9.79 3.9.37 H19 2.9 2.6 19.24 36/36 36/36 (pg/m 3.3 [.1] ) H19.77.63 3.4.31 36/36 36/36 H2 2.3 2.1 18.33.3 [.1] H2.8.62 6.5.32 H21 2.3 2.2 14.33.19 [.8] H21.8.71 3.7.2 H22 2.2 1.9 26.19.14 [.5] H22.81.69 5.5.22 H25 1.7 1.7 12.15 36/36 36/36.54 [.18] H25.47.44 2.4.2 36/36 36/36 H27.99 1.2 6.8.14.12 [.4] 35/35 35/35 287

[] o,p'-dde H14.6.56 8.5.11.3 [.1] 12/12 34/34 H15 1.4 1.5 7.5.17 35/35 35/35.2 [.68] H15.5.47 1.7.18 34/34 34/34 H16 1.1 1.2 8.9.14.37 [.12] H16.53.49 3.9.14 H17 1.6 1.5 7.9.33.74 [.24] H17.62.59 2..24 H18 1.1 1.1 7.4 nd 36/37 36/37.9 [.3] H18.65.56 2.6.19 H19.66.67 7.96 36/36 36/36 (pg/m 3.17 [.7] ) H19.3.29 3.7.12 36/36 36/36 H2.48.52 5..11.25 [.9] H2.3.24 1.1.15 H21.51.46 6.7.98.16 [.6] H21.27.24 23.72 H22.49.41 9..9.4 [.1] H22.27.23 2.3.8 H25.38.35 3.3.51 36/36 36/36.23 [.9] H25.21.19.65.97 36/36 36/36 H27.25.24 1.1 nd.18 [.6] 34/35 34/35 [] o,p'-ddd H14.14.18.85 nd.21 [.7] 97/12 33/34 H15.37.42 1.3.59 35/35 35/35.42 [.14] H15.15.14.42.62 34/34 34/34 H16.31.33 2.6 tr(.52).14 [.48] H16.14 tr(.13).86 nd 35/37 35/37 H17.22.19.9 tr(.7).1 [.3] H17 tr(.7) tr(.7).21 nd 35/37 35/37 H18.28.28 1.4 tr(.5).1 [.3] H18.12.11.79 nd 34/37 34/37 H19.28.29 1.9.5 36/36 36/36 (pg/m 3.5 [.2] ) H19.95.9.33 tr(.3) 36/36 36/36 H2.19.16 1.6.5.4 [.1] H2.1.9.26.4 H21.2.19.9.4.3 [.1] H21.8.8.28 tr(.2) H22.21.19 1.8.4.3 [.1] H22.1.9.48 tr(.2) H25.17.18 1.2 tr(.3) 36/36 36/36.5 [.2] H25.6.6.17 nd 35/36 35/36 H27 tr(.9) tr(.1).37 nd.2 [.7] 25/35 25/35 23 24 26 288

[6-1] p,p'-ddt (pg/l) 16 12 8 [] (pg/l) 14.6 [.2] 15 3 [.9] 16 6 [2] 17 4 [1] 18 1.9 [.6] 19 1.7 [.6] 2 1.2 [.5] 21.15 [.6] 22 2.4 [.8] 26.4 [.1] 4 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 23 25 27 29 3-6-1-1 p,p'-ddt [6-1] p,p'-ddt (pg/g-dry) 5 4 3 2 [](pg/g-dry) 14 6 [2] 15 2 [.4] 16 2 [.5] 17 1. [.34] 18 1.4 [.5] 19 1.3 [.5] 2 1.2 [.5] 21 1. [.4] 22 2.8 [.9] 26.4 [.2] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 23 25 27 29 3-6-1-2 p,p'-ddt 289

[6-1] p,p'-ddt 5 4 3 2 [] 14 4.2 [1.4] 15 11 [3.5] 16 3.2 [1.1] 17 5.1 [1.7] 18 6 [2] 19 5 [2] 2 5 [2] 21 3[1] 22 3 [1] 25 3.3[1.1] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 22 3 23 24 26 29 3-6-1-3 p,p'-ddt [6-1] p,p'-ddt 6 pg/m 3 5 4 3 2 [] (pg/m 3 ) 14.24 [.8] 15.14 [.46] 16.22 [.74] 17.16 [.54] 18.17 [.6] 19.7 [.3] 2.7 [.3] 21.7 [.3] 22.1 [.3] 25.11 [.4] 27.15 [.5] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 23 24 26 28 29 3-6-1-4 p,p'-ddt 29

[6-2] p,p'-dde (pg/l) 4 3 2 [](pg/l) 14.6 [.2] 15 4 [2] 16 8 [3] 17 6 [2] 18 7 [2] 19 4 [2] 2 1.1 [.4] 21 1.1 [.4] 22 2.3 [.8] 26.5 [.2] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 23 25 27 29 3-6-2-1 p,p'-dde [6-2] p,p'-dde (pg/g-dry) 1, 8 6 4 [](pg/g-dry) 14 2.7 [.9] 15.9 [.3] 16 3 [.8] 17 2.7 [.94] 18 1. [.3] 19 1.1 [.4] 2 1.7 [.7] 21.8 [.3] 22 5 [2] 26 1.8 [.6] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 23 25 27 29 3-6-2-2 p,p'-dde 291

[6-2] p,p'-dde 3,5 3, 2,5 2, 1,5 1, [] 14 4.2 [1.4] 15 11 [3.5] 16 3.2 [1.1] 17 5.1 [1.7] 18 6 [2] 19 5 [2] 2 5 [2] 21 3[1] 22 3 [1] 25 4.3[1.4] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 22 3 23 24 26 29 3-6-2-3 p,p'-dde [6-2] p,p'-dde 8 pg/m 3 6 4 2 [] (pg/m 3 ) 14.9 [.3] 15.4 [.13] 16.12 [.39] 17.14 [.34] 18.1 [.3] 19.4 [.2] 2.4 [.2] 21.8 [.3] 22.62 [.21] 25.1 [.3] 27.12 [.4] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 23 24 26 28 29 3-6-2-4 p,p'-dde 292

[6-3] p,p'-ddd (pg/l) 25 2 15 1 [](pg/l) 14.24 [.8] 15 2 [.5] 16 3 [.8] 17 1.9 [.64] 18 1.6 [.5] 19 1.7 [.6] 2.6 [.2] 21.4 [.2] 22.2 [.8] 26 1. [.4] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 23 25 27 29 3-6-3-1 p,p'-ddd [6-3] p,p'-ddd (pg/g-dry) 8 6 4 [](pg/g-dry) 14 2.4 [.8] 15.9 [.3] 16 2 [.7] 17 1.7 [.64] 18.7 [.2] 19 1. [.4] 2 1. [.4] 21.4 [.2] 22 1.4 [.5] 26 4.2 [1.4] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 23 25 27 29 3-6-3-2 p,p'-ddd 293

[6-3] p,p'-ddd 8 6 4 [] 14 5.4 [1.8] 15 9.9 [3.3] 16 2.2 [.7] 17 2.9 [.97] 18 2.4 [.9] 19 3 [1] 2 3 [1] 21 2.4 [.9] 22 1.3 [.5] 25 1.9[.7] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 22 3 23 24 26 29 3-6-3-3 p,p'-ddd [6-3] p,p'-ddd pg/m 3.35.3.25.2.15.1 [] (pg/m 3 ) 14.18 [.6] 15.54 [.18] 16.53 [.18] 17.16 [.5] 18.13 [.4] 19.11 [.4] 2.25 [.9] 21.3 [.1] 22.2 [.1] 25.18 [.7] 27.33 [.11].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 23 24 26 28 29 2 27 1/2 3-6-3-4 p,p'-ddd 294

[6-4] o,p'-ddt (pg/l) 7 6 5 4 3 [](pg/l) 14 1.2 [.4] 15 3 [.7] 16 5 [2] 17 3 [1] 18 2.3 [.8] 19 2.5 [.8] 2 1.4 [.5] 21.16 [.6] 22 1.5 [.5] 26.4 [.2] 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 23 25 27 29 3-6-4-1 o,p'-ddt [6-4] o,p'-ddt (pg/g-dry) 8 6 4 [](pg/g-dry) 14 6 [2] 15.8 [.3] 16 2 [.6] 17.8 [.3] 18 1.2 [.4] 19 1.8 [.6] 2 1.5 [.6] 21 1.2 [.5] 22 1.1 [.4] 26.4 [.2] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 23 25 27 29 3-6-4-2 o,p'-ddt 295

[6-4] o,p'-ddt 2 15 1 [] 14 12 [4] 15 2.9 [.97] 16 1.8 [.61] 17 2.6 [.86] 18 3 [1] 19 3 [1] 2 3 [1] 21 2.2 [.8] 22 3 [1] 25 3 [1] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 22 3 23 24 26 29 3-6-4-3 o,p'-ddt [6-4] o,p'-ddt 8 pg/m 3 6 4 2 [] (pg/m 3 ) 14.15 [.5] 15.12 [.4] 16.93 [.31] 17.1 [.34] 18.9 [.3] 19.3 [.1] 2.3 [.1] 21.19 [.8] 22.14 [.5] 25.54 [.18] 27.12 [.4] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 23 24 26 28 29 3-6-4-4 o,p'-ddt 296

[6-5] o,p'-dde (pg/l) 3.5 3 2.5 2 1.5 [](pg/l) 14.9 [.3] 15.8 [.3] 16 2 [.5] 17 1.2 [.4] 18 2.6 [.9] 19 2.3 [.8] 2.7 [.3] 21.22 [.9] 22.24 [.9] 26.3 [.1] 1.5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 23 25 27 29 3-6-5-1 o,p'-dde [6-5] o,p'-dde (pg/g-dry) 6 5 4 3 2 [](pg/g-dry) 14 3 [1] 15.6 [.2] 16 3 [.8] 17 2.6 [.9] 18 1.1 [.4] 19 1.2 [.4] 2 1.4 [.6] 21.6 [.2] 22 1.2 [.5] 26.8 [.3] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 o,p'-ddt 13 2 14 21 3 23 25 27 29 3-6-5-2 o,p'-dde 297

[6-5] o,p'-dde 1 8 6 4 [] 13 [1,] 14 3.6 [1.2] 15 3.6 [1.2] 16 2.1 [.69] 17 3.4 [1.1] 18 3 [1] 19 2.3 [.9] 2 3 [1] 21 3[1] 22 1.5 [.6] 25 4 [1] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 22 3 23 24 26 29 3-6-5-3 o,p'-dde [6-5] o,p'-dde 2 pg/m 3 1.5 1.5 [] (pg/m 3 ) 14.3 [.1] 15.2 [.68] 16.37 [.12] 17.74 [.24] 18.9 [.3] 19.17 [.7] 2.25 [.9] 21.16 [.6] 22.4 [.1] 25.23 [.9] 27.18 [.6] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 23 24 26 28 29 3-6-5-4 o,p'-dde 298

[6-6] o,p'-ddd (pg/l) 1 8 6 4 [](pg/l) 14.6 [.2] 15.8 [.3] 16 2 [.5] 17 1.2 [.4] 18.8 [.3] 19.8 [.3] 2.8 [.3] 21.22 [.9] 22.6 [.2] 26.2 [.8] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 23 25 27 29 3-6-6-1 o,p'-ddd [6-6] o,p'-ddd (pg/g-dry) 2 15 1 [](pg/g-dry) 14 6 [2] 15 2 [.5] 16 2 [.5] 17 1. [.3] 18.5 [.2] 19 1. [.4] 2.3 [.1] 21.5 [.2] 22.9 [.4] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 o,p'-ddt 13 2 14 21 3 23 25 27 29 3-6-6-2 o,p'-ddd 299

[6-6] o,p'-ddd 25 2 15 1 [](pg/gwet) 14 12 [4] 15 6. [2.] 16 5.7 [1.9] 17 3.3 [1.1] 18 4 [1] 19 3 [1] 2 4 [2] 21 3[1] 22.6 [.2] 25 1.8 [.7] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 22 3 23 24 26 29 3-6-6-3 o,p'-ddd [6-6] o,p'-ddd.5 pg/m 3.4.3.2.1 [] (pg/m 3 ) 14.21 [.7] 15.42 [.14] 16.14 [.48] 17.1 [.3] 18.1 [.3] 19.5 [.2] 2.4 [.1] 21.3 [.1] 22.3 [.1] 25.5 [.2] 27.2 [.7] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 23 24 26 28 29 3-6-6-4 o,p'-ddd 3

[7] 43 61 9 POPs 16 cis- trans- γ- cis-trans- cis- trans- 8 58 57 5 cis-trans-cis- trans- 13 58 13 cis-trans-cis- trans- 61 1 61 13 14 cis-trans- cis- trans- 14 25 28 29 cis- trans- cis-47 1 pg/l 47 2 21 pg/l 14 29 trans-47 1 pg/l 47 tr(2) 15 pg/l 31

14 29 cis- trans- cis- [] H14 42 32 88 2.5.9 [.3] 114/114 38/38 H15 69 51 92 12 3 [.9] 36/36 36/36 H16 92 87 1,9 1 6 [2] 38/38 38/38 H17 53 54 51 6 4 [1] 47/47 47/47 H18 31 26 44 5 5 [2] 48/48 48/48 H19 23 22 68 nd 4 [2] 47/48 47/48 (pg/l) H2 29 29 48 2.9 1.6 [.6] 48/48 48/48 H21 29 26 71 4.4 1.1 [.4] 49/49 49/49 H22 19 14 17 nd 11 [4] 47/49 47/49 H23 2 16 5 3.8 1.4 [.6] 49/49 49/49 H24 43 37 35 1 1.6 [.6] 48/48 48/48 H25 18 16 26 2.9 2.7 [.9] 48/48 48/48 H29 19 19 21 2 2 [1] 47/47 47/47 trans- [] (pg/l) H14 33 24 78 3.1 1.5 [.5] 114/114 38/38 H15 34 3 41 6 5 [2] 36/36 36/36 H16 32 26 1,2 5 5 [2] 38/38 38/38 H17 25 21 2 3 4 [1] 47/47 47/47 H18 24 16 33 tr(4) 7 [2] 48/48 48/48 H19 16 2 58 nd 2.4 [.8] 47/48 47/48 H2 23 22 42 3 3 [1] 48/48 48/48 H21 23 18 69 3..8 [.3] 49/49 49/49 H22 15 tr(11) 31 nd 13 [4] 44/49 44/49 H23 16 13 47 3.2 1. [.4] 49/49 49/49 H24 41 33 3 12 2.5 [.8] 48/48 48/48 H25 15 13 2 3 3 [1] 48/48 48/48 H29 15 15 15 tr(2) 3 [1] 47/47 47/47 1 14 2 26 28 cis-62 1.6 pg/g-dry 62 61 2,8 pg/g-dry 14 29 trans-62 1 pg/g-dry 62 tr(1) 3, pg/g-dry 14 29 14 29 cis- trans- cis- [] H14 14 98 18, 1.8.9 [.3] 189/189 63/63 H15 19 14 19, tr(3.6) 4 [2] 186/186 62/62 H16 16 97 36, 4 4 [2] 189/189 63/63 H17 15 1 44, 3.3 1.9 [.64] 189/189 63/63 H18 1 7 13, tr(.9) 2.4 [.8] 192/192 64/64 H19 82 55 7,5 nd 5 [2] 191/192 64/64 H2 1 63 11, tr(2.3) 2.4 [.9] 192/192 64/64 (pg/g-dry) H21 84 61 8,6 2..7 [.3] 192/192 64/64 H22 82 62 7,2 tr(4) 6 [2] 64/64 64/64 H23 7 58 4,5 1.7 1.1 [.4] 64/64 64/64 H24 69 61 11, tr(2.6) 2.9 [1.] 63/63 63/63 H25 65 55 5,4 tr(1.9) 2. [.8] 63/63 63/63 H29 47 36 2,8 nd 4.8 [1.6] 61/62 61/62 32

trans- [] H14 15 11 16, 2.1 1.8 [.6] 189/189 63/63 H15 13 1 13, tr(2.4) 4 [2] 186/186 62/62 H16 11 8 26, 3 3 [.9] 189/189 63/63 H17 11 81 32, 3.4 2.3 [.84] 189/189 63/63 H18 11 76 12, 2.2 1.1 [.4] 192/192 64/64 H19 82 58 7,5 nd 2.2 [.8] 191/192 64/64 H2 11 66 1, 2.4 2. [.8] 192/192 64/64 (pg/g-dry) H21 91 68 8,3 2.1 1.7 [.7] 192/192 64/64 H22 95 69 8, tr(4) 11 [4] 64/64 64/64 H23 73 64 4,3 3.2 1.3 [.5] 64/64 64/64 H24 8 71 13, tr(2.9) 4. [1.3] 63/63 63/63 H25 74 65 5,6 2.5 1.8 [.7] 63/63 63/63 H29 53 41 3, tr(1) 4 [1] 62/62 62/62 1 14 21 2 26 28 cis- trans- 47 2 pg/l 47 19 12 pg/l cis-47.6 pg/l 47 tr(.6) 36 pg/l trans-47 1 pg/l 47 tr(2) 12 pg/l 14 29 14 29 cis- trans- [] H14 2.7 3.5 41 nd 1.2 [.4] 96/114 35/38 H15 3 2 39 tr(.6) 2 [.5] 36/36 36/36 H16 3.2 2.9 47 tr(.7) 2 [.5] 38/38 38/38 H17 2.6 2.1 19 nd 1.1 [.4] 46/47 46/47 H18 tr(2.5) tr(2.4) 18 nd 2.8 [.9] 43/48 43/48 H19 tr(2) nd 41 nd 6 [2] 25/48 25/48 H2 1.9 1.9 14 nd 1.9 [.7] 4/48 4/48 (pg/l) H21 2. 1.9 19 nd 1.1 [.4] 45/49 45/49 H22 1.5 1.3 45 nd.7 [.3] 47/49 47/49 H23 1.9 1.8 34 nd 1.3 [.5] 44/49 44/49 H24 2.2 2.3 17 nd.9 [.4] 44/48 44/48 H25 1.8 1.8 12 nd.9 [.4] 41/48 41/48 H29 nd nd 12 nd 4 [2] 19/47 19/47 cis- [] (pg/l) H14 7.9 6.7 25.23 1.8 [.6] 114/114 38/38 H15 8. 7. 13 1.3.3 [.1] 36/36 36/36 H16 7.5 6.3 34.8.6 [.2] 38/38 38/38 H17 6. 5.9 43.9.5 [.2] 47/47 47/47 H18 6.6 5.6 83 1..8 [.3] 48/48 48/48 H19 5.9 6.1 21 nd 2.4 [.8] 43/48 43/48 H2 6.5 5.9 13.9.9 [.3] 48/48 48/48 H21 7.1 5.5 21 1.4.3 [.1] 49/49 49/49 H22 5.4 3.9 4 tr(.9) 1.3 [.4] 49/49 49/49 H23 5. 4.3 13.8.6 [.2] 49/49 49/49 H24 6.4 5.9 58 1.1.8 [.3] 48/48 48/48 H25 5.1 4.6 74 tr(.7).8 [.3] 48/48 48/48 H29 4.6 4.6 36 tr(.6) 1.5 [.6] 47/47 47/47 33

trans- [] H14 3 24 78 1.8 1.2 [.4] 114/114 38/38 H15 26 2 45 4 2 [.5] 36/36 36/36 H16 25 19 1,1 tr(3) 4 [2] 38/38 38/38 H17 2 17 15 2.6 2.5 [.84] 47/47 47/47 H18 21 16 31 3.2 3. [1.] 48/48 48/48 H19 17 17 54 tr(2) 5 [2] 48/48 48/48 H2 18 17 34 1.9 1.6 [.6] 48/48 48/48 (pg/l) H21 2 17 53 2.7 1. [.4] 49/49 49/49 H22 12 11 93 nd 8 [3] 45/49 45/49 H23 15 12 48 2.6 1.3 [.5] 49/49 49/49 H24 3 26 21 7.9 1.5 [.6] 48/48 48/48 H25 14 11 17 2.3 1.5 [.6] 48/48 48/48 H29 13 14 12 tr(2) 3 [1] 47/47 47/47 1 14 2 26 28 62 1 pg/g-dry 62 41 78 pg/g-dry 14 29 5 5 cis-62.7 pg/g-dry 62 61 1,5 pg/g-dry 14 29 trans-62 2 pg/g-dry 62 61 2,6 pg/g-dry 14 29 14 29 cis- trans- [] H14 2.7 1.7 12 nd 1.5 [.5] 153/189 59/63 H15 2 2 85 nd 1 [.4] 158/186 57/62 H16 tr(2.1) tr(1.3) 14 nd 3 [.8] 129/189 54/63 H17 2.3 tr(1.9) 16 nd 2. [.7] 133/189 51/63 H18 tr(2.5) tr(1.7) 28 nd 2.9 [1.] 141/192 54/64 H19 tr(2.1) tr(1.5) 76 nd 2.5 [.9] 117/192 46/64 H2 tr(2) tr(1) 34 nd 3 [1] 11/192 48/64 (pg/g-dry) H21 2 tr(1) 15 nd 2 [1] 97/192 45/64 H22 1.7 1.2 6 nd 1. [.4] 56/64 56/64 H23 tr(1.6) tr(1.2) 83 nd 2.2 [.9] 36/64 36/64 H24 tr(1.4) tr(1.) 75 nd 1.7 [.7] 38/63 38/63 H25 1.5 1.3 54 nd 1.3 [.5] 5/63 5/63 H29 tr(1) tr(1) 78 nd 3 [1] 41/62 41/62 34

cis- [] H14 76 66 7,8 nd 2.1 [.7] 188/189 63/63 H15 66 5 6,5 nd 3 [.9] 184/186 62/62 H16 53 34 9,4 tr(.8) 2 [.6] 189/189 63/63 H17 56 42 9,9 tr(1.1) 1.9 [.64] 189/189 63/63 H18 58 48 5,8 tr(.6) 1.2 [.4] 192/192 64/64 H19 48 35 4,2 nd 1.6 [.6] 191/192 64/64 H2 57 42 5,1 1.1.6 [.2] 192/192 64/64 (pg/g-dry) H21 53 38 4,7 1.4 1. [.4] 192/192 64/64 H22 53 45 3,6 2.3.9 [.3] 64/64 64/64 H23 41 38 2,9 nd 1.1 [.4] 63/64 63/64 H24 44 35 4,9 tr(1) 3 [1] 63/63 63/63 H25 41 31 3,1 tr(.6).7 [.3] 63/63 63/63 H29 31 25 1,5 nd 1.7 [.7] 61/62 61/62 trans- [] H14 13 83 13, 3.1 1.5 [.5] 189/189 63/63 H15 11 78 11, 2 2 [.6] 186/186 62/62 H16 94 63 23, 3 2 [.6] 189/189 63/63 H17 99 72 24, 2.4 1.5 [.54] 189/189 63/63 H18 1 65 1, 3.4 1.2 [.4] 192/192 64/64 H19 78 55 8,4 tr(1.6) 1.7 [.6] 192/192 64/64 H2 91 53 8,4 tr(1.6) 2.2 [.8] 192/192 64/64 (pg/g-dry) H21 85 58 7,8 2..9 [.3] 192/192 64/64 H22 8 65 6,2 tr(3) 6 [2] 64/64 64/64 H23 68 52 4,5 1.7.8 [.3] 64/64 64/64 H24 69 62 1, 2.5 2.4 [.8] 63/63 63/63 H25 67 54 4,7 2.2 1.2 [.4] 63/63 63/63 H29 47 39 2,6 nd 6 [2] 61/62 61/62 1 14 21 2 26 28 35

28 cis- trans- 14 28 cis- trans- cis- [] H14 73 1,2 26, 24 2.4 [.8] 38/38 8/8 H15 1,1 1,4 14, 11 3.9 [1.3] 3/3 6/6 H16 1,3 1,6 14, 91 18 [5.8] 31/31 7/7 H17 1, 96 13, 78 12 [3.9] 31/31 7/7 H18 97 1,1 18, 67 4 [1] 31/31 7/7 H19 87 59 19, 59 5 [2] 31/31 7/7 H2 75 56 11, 85 5 [2] 31/31 7/7 H21 1,2 1,1 16, 83 4 [2] 31/31 7/7 H22 1,6 2,3 15, 67 4 [2] 6/6 6/6 H23 79 88 3,4 16 3 [1] 4/4 4/4 H24 71 5 3,5 18 5 [2] 5/5 5/5 H25 41 41 2, 75 13 [4] 5/5 5/5 H28 22 26 5 8 3 [1] 3/3 3/3 H14 61 55 6,9 57 2.4 [.8] 7/7 14/14 H15 51 4 4,4 43 3.9 [1.3] 7/7 14/14 H16 62 49 9,8 68 18 [5.8] 7/7 14/14 H17 52 6 8, 42 12 [3.9] 8/8 16/16 H18 52 42 4,9 56 4 [1] 8/8 16/16 H19 43 36 5,2 3 5 [2] 8/8 16/16 H2 43 34 3,5 36 5 [2] 85/85 17/17 H21 43 45 3,2 41 4 [2] 9/9 18/18 H22 45 63 3,4 51 4 [2] 18/18 18/18 H23 58 66 3,8 79 3 [1] 18/18 18/18 H24 58 55 3,1 98 5 [2] 19/19 19/19 H25 54 45 5,7 65 13 [4] 19/19 19/19 H28 34 44 2,2 67 3 [1] 19/19 19/19 H14 67 18 45 1 2.4 [.8] 1/1 2/2 H15 47 12 37 6.8 3.9 [1.3] 1/1 2/2 H16 39 11 24 tr(5.8) 18 [5.8] 1/1 2/2 H17 53 12 34 tr(5.8) 12 [3.9] 1/1 2/2 H18 32 83 25 5 4 [1] 1/1 2/2 H19 29 83 23 tr(4) 5 [2] 1/1 2/2 H2 24 87 28 tr(3) 5 [2] 1/1 2/2 H21 21 48 13 4 4 [2] 1/1 2/2 H22 27 --- 18 4 4 [2] 2/2 2/2 H23 --- --- 6 6 3 [1] 1/1 1/1 H24 23 --- 11 5 5 [2] 2/2 2/2 H25 37 --- 14 tr(1) 13 [4] 2/2 2/2 H28 38 --- 11 13 3 [1] 2/2 2/2 36

trans- [] H14 39 84 2,3 33 2.4 [.8] 38/38 8/8 H15 55 84 2,8 69 7.2 [2.4] 3/3 6/6 H16 56 77 2,8 53 48 [16] 31/31 7/7 H17 47 66 2,4 4 1 [3.5] 31/31 7/7 H18 47 58 2,8 41 4 [2] 31/31 7/7 H19 44 46 1,5 34 6 [2] 31/31 7/7 H2 36 41 1,3 52 7 [3] 31/31 7/7 H21 54 56 16, 48 4 [1] 31/31 7/7 H22 52 64 5,5 31 3 [1] 6/6 6/6 H23 49 47 2,9 15 4 [1] 4/4 4/4 H24 39 31 1,3 14 7 [2] 5/5 5/5 H25 28 23 1,7 58 16 [5.2] 5/5 5/5 H28 12 99 33 56 6 [2] 3/3 3/3 H14 19 16 2,7 2 2.4 [.8] 7/7 14/14 H15 16 12 1,8 9.6 7.2 [2.4] 7/7 14/14 H16 2 13 5,2 tr(17) 48 [16] 7/7 14/14 H17 16 18 3,1 tr(9.8) 1 [3.5] 76/8 16/16 H18 15 12 2, 14 4 [2] 8/8 16/16 H19 13 1 2,1 8 6 [2] 8/8 16/16 H2 12 71 1,3 14 7 [3] 85/85 17/17 H21 13 14 1,3 1 4 [1] 9/9 18/18 H22 12 17 1,1 9 3 [1] 18/18 18/18 H23 18 24 1,3 2 4 [1] 18/18 18/18 H24 17 14 1,1 19 7 [2] 19/19 19/19 H25 16 17 2,7 tr(14) 16 [5.2] 19/19 19/19 H28 1 11 8 12 6 [2] 19/19 19/19 trans- [] H14 14 14 26 8.9 2.4 [.8] 1/1 2/2 H15 11 12 27 tr(5.9) 7.2 [2.4] 1/1 2/2 H16 nd nd tr(26) nd 48 [16] 5/1 1/2 H17 11 12 3 tr(4.5) 1 [3.5] 1/1 2/2 H18 7 8 17 tr(3) 4 [2] 1/1 2/2 H19 7 8 19 tr(3) 6 [2] 1/1 2/2 H2 tr(5) 9 27 nd 7 [3] 7/1 2/2 H21 6 7 13 tr(3) 4 [1] 1/1 2/2 H22 4 --- 1 tr(2) 3 [1] 2/2 2/2 H23 --- --- 5 5 4 [1] 1/1 1/1 H24 tr(6) --- 1 tr(4) 7 [2] 2/2 2/2 H25 26 --- 68 tr(1) 16 [5.2] 2/2 2/2 H28 18 --- 46 7 6 [2] 2/2 2/2 1 14 21 2 25 24 3 26 27 37

14 28 cis- trans- [] cis- H14 31 4 67.86.6 [.2] 12/12 34/34 H15 11 12 1,6 6.4 35/35 35/35.51 [.17] H15 3 38 22 2.5 34/34 34/34 H16 92 16 1, 2.3.57 [.19] H16 29 49 29 1.2 H17 92 12 1, 3.4.16 [.54] H17 16 19 26 1.4 H18 82 11 76 2.9.13 [.4] H18 19 19 28 2. H19 9 12 1,1 3.3 36/36 36/36.1 [.4] H19 17 2 23 1.4 36/36 36/36 H2 75 12 79 1.9.14 [.5] (pg/m 3 ) H2 21 34 2 1.5 H21 67 11 79 2.7.16 [.6] H21 19 22 18.65 H22 68 1 7 1.8.17 [.6] H22 2 27 13.84 H23 66 95 7 1.5 35/35 35/35 1.3 [.42] H23 2 31 24 tr(.88) H24 61 98 65 2.9 36/36 36/36 1.5 [.51] H24 1 14 74 nd 35/36 35/36 H25 58 97 58 1.5 36/36 36/36.7 [.2] H25 11 15 86 tr(.5) 36/36 36/36 H28 53 86 81.9.9 [.3] [] trans- H14 36 48 82.62.6 [.2] 12/12 34/34 H15 13 15 2, 6.5 35/35 35/35.86 [.29] H15 37 44 29 2.5 34/34 34/34 H16 11 19 1,3 2.2.69 [.23] H16 35 6 36 1.5 H17 1 13 1,3 3.2.34 [.14] H17 19 23 31 1.9 H18 96 14 1,2 3.4.17 [.6] H18 22 21 35 2. H19 1 14 1,3 3.8 36/36 36/36.12 [.5] H19 2 24 3 1.5 36/36 36/36 H2 87 13 99 2.5.17 [.6] (pg/m 3 ) H2 25 41 25 1.8 H21 79 12 96 2.6.12 [.5] H21 23 3 21.68 H22 79 12 82 2. 1.2 [.4] H22 24 34 15 tr(1.) H23 76 11 81 tr(1.4) 35/35 35/35 1.6 [.53] H23 24 37 29 tr(.7) H24 7 12 78 2.8 36/36 36/36 2.1 [.7] H24 12 18 95 nd 35/36 35/36 H25 64 12 69 1.7 36/36 36/36.8 [.3] H25 13 18 11 tr(.4) 36/36 36/36 H28 61 95 1,1 tr(.7) 1. [.3] 26 27 38

cis- trans- 14 28 cis- trans- [] H14 71 83 5,6 nd 3.6 [1.2] 37/38 8/8 H15 93 62 1,9 11 8.4 [2.8] 3/3 6/6 H16 11 1 1,7 14 9.2 [3.1] 31/31 7/7 H17 99 79 1,4 12 9.3 [3.1] 31/31 7/7 H18 91 9 2,4 7 7 [3] 31/31 7/7 H19 7 43 2,2 8 6 [2] 31/31 7/7 H2 64 55 1,1 7 7 [2] 31/31 7/7 H21 1 89 82 1 4 [1] 31/31 7/7 H22 24 39 3,3 11 8 [3] 6/6 6/6 H23 68 1 26 8 3 [1] 4/4 4/4 H24 66 8 45 12 3 [1] 5/5 5/5 H25 42 44 21 8 3 [1] 5/5 5/5 H28 27 4 43 11 3 [1] 3/3 3/3 cis- H14 17 14 3,9 16 3.6 [1.2] 7/7 14/14 H15 15 16 82 3 8.4 [2.8] 7/7 14/14 H16 16 14 1,5 25 9.2 [3.1] 7/7 14/14 H17 15 15 1,9 2 9.3 [3.1] 8/8 16/16 H18 15 12 3, 28 7 [3] 8/8 16/16 H19 12 1 1,9 17 6 [2] 8/8 16/16 H2 13 13 2,2 15 7 [2] 85/85 17/17 H21 12 99 2,4 23 4 [1] 9/9 18/18 H22 12 14 1, 33 8 [3] 18/18 18/18 H23 14 13 2,3 33 3 [1] 18/18 18/18 H24 14 18 39 28 3 [1] 19/19 19/19 H25 13 13 56 31 3 [1] 19/19 19/19 H28 96 8 95 31 3 [1] 19/19 19/19 H14 64 63 89 47 3.6 [1.2] 1/1 2/2 H15 76 7 1,3 61 8.4 [2.8] 1/1 2/2 H16 46 45 73 32 9.2 [3.1] 1/1 2/2 H17 61 66 86 39 9.3 [3.1] 1/1 2/2 H18 51 56 72 27 7 [3] 1/1 2/2 H19 44 4 74 29 6 [2] 1/1 2/2 H2 56 53 96 29 7 [2] 1/1 2/2 H21 3 29 54 19 4 [1] 1/1 2/2 H22 4 --- 51 32 8 [3] 2/2 2/2 H23 --- --- 59 59 3 [1] 1/1 1/1 H24 25 --- 36 17 3 [1] 2/2 2/2 H25 2,5 --- 3,4 1,9 3 [1] 2/2 2/2 H28 58 --- 1,4 24 3 [1] 2/2 2/2 [] H14 17 3 87 8.6 1.2 [.4] 38/38 8/8 H15 29 26 1,8 48 4.8 [1.6] 3/3 6/6 H16 32 38 1,8 43 3.4 [1.1] 31/31 7/7 H17 27 22 1,3 27 4.5 [1.5] 31/31 7/7 H18 27 18 1,5 31 3 [1] 31/31 7/7 H19 25 25 1, 26 3 [1] 31/31 7/7 H2 21 21 78 33 4 [1] 31/31 7/7 H21 3 31 1, 31 3 [1] 31/31 7/7 H22 28 31 1,3 35 3 [1] 6/6 6/6 H23 25 28 1,3 77 1.8 [.7] 4/4 4/4 H24 2 19 67 52 2 [1] 5/5 5/5 H25 15 14 9 38 2.2 [.7] 5/5 5/5 H28 72 46 22 37 1.4 [.6] 3/3 3/3 H14 46 42 5,1 46 1.2 [.4] 7/7 14/14 H15 36 36 2,6 19 4.8 [1.6] 7/7 14/14 H16 43 31 1, 48 3.4 [1.1] 7/7 14/14 H17 38 36 6,2 27 4.5 [1.5] 8/8 16/16 H18 37 33 3,3 33 3 [1] 8/8 16/16 H19 32 28 3,7 16 3 [1] 8/8 16/16 H2 35 3 3,2 46 4 [1] 85/85 17/17 H21 34 34 2,6 27 3 [1] 9/9 18/18 H22 32 37 2,2 23 3 [1] 18/18 18/18 H23 44 45 2,9 45 1.8 [.7] 18/18 18/18 H24 42 45 2,2 33 2 [1] 19/19 19/19 H25 43 42 3, 34 2.2 [.7] 19/19 19/19 H28 3 17 1,9 53 1.4 [.6] 19/19 19/19 39

cis- trans- [] H14 2 24 45 68 1.2 [.4] 1/1 2/2 H15 2 26 66 68 4.8 [1.6] 1/1 2/2 H16 14 15 24 73 3.4 [1.1] 1/1 2/2 H17 16 18 37 86 4.5 [1.5] 1/1 2/2 H18 12 13 27 6 3 [1] 1/1 2/2 H19 13 14 3 42 3 [1] 1/1 2/2 H2 14 15 41 37 4 [1] 1/1 2/2 H21 81 85 16 44 3 [1] 1/1 2/2 H22 1 --- 19 57 3 [1] 2/2 2/2 H23 --- --- 76 76 1.8 [.7] 1/1 1/1 H24 75 --- 1 56 2 [1] 2/2 2/2 H25 27 --- 97 74 2.2 [.7] 2/2 2/2 H28 24 --- 77 74 1.4 [.6] 2/2 2/2 [] H14 45 1,1 1,8 21 2.4 [.8] 38/38 8/8 H15 8 7 3,8 14 3.6 [1.2] 3/3 6/6 H16 78 87 3,4 11 13 [4.2] 31/31 7/7 H17 7 65 3,4 72 6.2 [2.1] 31/31 7/7 H18 66 61 3,2 85 3 [1] 31/31 7/7 H19 64 61 2,4 71 7 [3] 31/31 7/7 H2 51 51 2, 94 6 [2] 31/31 7/7 H21 78 68 33, 79 3 [1] 31/31 7/7 H22 79 87 6, 84 4 [2] 6/6 6/6 H23 64 68 3, 2 3 [1] 4/4 4/4 H24 53 4 1,8 19 4 [1] 5/5 5/5 H25 38 37 2, 98 1 [3.4] 5/5 5/5 H28 2 15 52 97 3 [1] 3/3 3/3 H14 1, 9 8,3 98 2.4 [.8] 7/7 14/14 H15 92 84 5,8 85 3.6 [1.2] 7/7 14/14 H16 1,1 76 21, 14 13 [4.2] 7/7 14/14 H17 97 75 13, 8 6.2 [2.1] 8/8 16/16 H18 94 68 6,9 12 3 [1] 8/8 16/16 H19 8 68 7,9 71 7 [3] 8/8 16/16 H2 86 75 6,9 87 6 [2] 85/85 17/17 H21 81 72 7,4 68 3 [1] 9/9 18/18 H22 8 1, 4,7 11 4 [2] 18/18 18/18 H23 1,1 1, 5, 19 3 [1] 18/18 18/18 H24 1,1 1,3 4,2 14 4 [1] 19/19 19/19 H25 1,1 1,1 7,8 15 1 [3.4] 19/19 19/19 H28 69 41 3,4 17 3 [1] 19/19 19/19 H14 89 98 1,9 35 2.4 [.8] 1/1 2/2 H15 1,1 1,4 3,7 35 3.6 [1.2] 1/1 2/2 H16 69 78 1,2 39 13 [4.2] 1/1 2/2 H17 87 88 2, 44 6.2 [2.1] 1/1 2/2 H18 65 62 1,5 31 3 [1] 1/1 2/2 H19 59 68 1,4 2 7 [3] 1/1 2/2 H2 74 85 2,6 18 6 [2] 1/1 2/2 H21 4 43 73 22 3 [1] 1/1 2/2 H22 51 --- 88 29 4 [2] 2/2 2/2 H23 --- --- 4 4 3 [1] 1/1 1/1 H24 36 --- 48 27 4 [1] 2/2 2/2 H25 55 --- 17 18 1 [3.4] 2/2 2/2 H28 6 --- 13 28 3 [1] 2/2 2/2 1 14 21 2 25 24 3 26 27 31

14 28 cis- trans- [] H14.96.98 8.3 nd.24 [.8] 11/12 34/34 H15 2.5 2.7 12.41 35/35 35/35.45 [.15] H15.87.88 3.2.41 34/34 34/34 H16 1.9 2. 7.8.41.13 [.42] H16.8.76 3.9.27 H17 1.9 2. 8.8.65.16 [.54] H17.55.5 2.2.27 H18 1.8 1.9 5.7.47.23 [.8] H18.54.56 5.1 tr(.13) H19 1.9 1.8 8.6.56 36/36 36/36.5 [.2] H19.61.63 2.4.26 36/36 36/36 H2 1.7 1.7 7.1.5.4 [.1] (pg/m 3 ) H2.61.63 1.8.27 H21 1.7 1.8 6.5.38.4 [.2] H21.65.61 2.7.24 H22 1.5 1.5 6.2.44.3 [.1] H22.56.55 2.3.26 H23 1.5 1.5 5.2.28 35/35 35/35.7 [.3] H23.61.57 2.6.21 H24 1.4 1.6 6.7.34 36/36 36/36.8 [.3] H24.41.38 1..22 36/36 36/36 H25 1.4 1.5 4.7.36 36/36 36/36.3 [.1] H25.43.41 1..2 36/36 36/36 H28 1.4 1.4 8.9.19.16 [.6] [] cis- H14 3.1 4. 62.71.3 [.1] 12/12 34/34 H15 12 15 22.81 35/35 35/35.26 [.88] H15 2.7 3.5 23.18 34/34 34/34 H16 1 15 13.36.72 [.24] H16 2.7 4.4 28.87 H17 1 14 16.3.8 [.3] H17 1.6 1.6 34.8 H18 11 12 17.28.15 [.5] H18 2.4 2. 41 tr(.14) H19 1 14 15.31 36/36 36/36.3 [.1] H19 1.6 1.7 22.9 36/36 36/36 H2 7.9 12 87.18.3 [.1] (pg/m 3 ) H2 2. 2.7 19.16 H21 7.5 1 11.33.4 [.2] H21 1.9 2.1 18.7 H22 7.5 1 68.23.11 [.4] H22 1.8 2.1 13 tr(.6) H23 7.4 8.8 89.24 35/35 35/35.15 [.51] H23 1.9 2.9 28 nd 36/37 36/37 H24 6.9 11 89.29 36/36 36/36.12 [.5] H24.98 1.1 1 tr(.5) 36/36 36/36 H25 6.4 1 72.15 36/36 36/36.7 [.2] H25 1. 1.4 12 tr(.6) 36/36 36/36 H28 6.1 9.9 12 tr(.13).14 [.5] 311

[] trans- H14 24 3 55.64.3 [.1] 12/12 34/34 H15 87 1 1,2 5.1 35/35 35/35.35 [.12] H15 24 28 18 2.1 34/34 34/34 H16 72 12 87 1.9.48 [.16] H16 23 39 24.95 H17 75 95 87 3.1.13 [.44] H17 13 16 21 1.2 H18 68 91 8 3..1 [.3] H18 16 15 24 1.4 H19 72 96 94 2.5 36/36 36/36.9 [.3] H19 13 15 19 1.1 36/36 36/36 H2 59 91 65 1.5.9 [.3] (pg/m 3 ) H2 17 25 17 1.3 H21 54 81 63 2.2.7 [.3] H21 16 19 14.75 H22 52 78 52 1.7.8 [.3] H22 15 17 89 tr(.7) H23 53 72 55 1.2 35/35 35/35 1.1 [.35] H23 16 24 21 tr(.7) H24 49 79 51 2.5 36/36 36/36 1.2 [.41] H24 8.1 1 61 tr(.5) 36/36 36/36 H25 46 78 47 1.2 36/36 36/36.5 [.2] H25 8.5 12 75.5 36/36 36/36 H28 42 69 65.8.7 [.2] 26 27 312

[7-1] cis- (pg/l) 1 8 6 4 [](pg/l) 14.9 [.3] 15 3 [.9] 16 6 [2] 17 4 [1] 18 5 [2] 19 4 [2] 2 1.6 [.6] 21 1.1 [.4] 22 11 [4] 23 1.4 [.6] 24 1.6 [.6] 25 2.7 [.9] 29 2 [1] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 26 28 3-7-1-1 cis- [7-1] cis- (pg/g-dry) 2 15 1 [](pg/g-dry) 14.9 [.3] 15 4 [2] 16 4 [2] 17 1.9 [.64] 18 2.4 [.8] 19 5 [2] 2 2.4 [.9] 21.7 [.3] 22 6 [2] 23 1.1 [.4] 24 2.9 [1.] 25 2.[.8] 29 4.8[1.6] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 26 28 3-7-1-2 cis- 313

[7-2] trans- (pg/l) 5 4 3 2 [](pg/l) 14 1.5 [.5] 15 5 [2] 16 5 [2] 17 4 [1] 18 7 [2] 19 2.4 [.8] 2 3 [1] 21.8 [.3] 22 13 [4] 23 1. [.4] 24 2.5 [.8] 25 3 [1] 29 3 [1] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 26 28 3-7-2-1 trans- [7-2] trans- (pg/g-dry) 16 12 8 [](pg/g-dry) 14 1.8 [.6] 15 4 [2] 16 3 [.9] 17 2.3 [.84] 18 1.1 [.4] 19 2.2 [.8] 2 2. [.8] 21 1.7 [.7] 22 11 [4] 23 1.3 [.5] 24 4. [1.3] 25 1.8 [.7] 29 4 [1] 4 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 26 28 3-7-2-2 trans- 314

[7-3] (pg/l) 4 3 2 [](pg/l) 14 1.2 [.4] 15 2 [.5] 16 2 [.5] 17 1.1 [.4] 18 2.8 [.9] 19 6 [2] 2 1.9 [.7] 21 1.1 [.4] 22.7 [.3] 23 1.3 [.5] 24.9 [.4] 25.9 [.4] 29 4 [2] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 26 28 3 29 1/2 3-7-3-1 [7-3] (pg/g-dry) 3 2.5 2 1.5 1 [](pg/g-dry) 14 1.5 [.5] 15 1 [.4] 16 3 [.8] 17 2. [.7] 18 2.9 [1.] 19 2.5 [.9] 2 3 [1] 21 2 [1] 22 1. [.4] 23 2.2 [.9] 24 1.7 [.7] 25 1.3 [.5] 29 3 [1].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 26 28 3-7-3-2 315

[7-4] cis- (pg/l) 1 8 6 4 [](pg/l) 14 1.8 [.6] 15.3 [.1] 16.6 [.2] 17.5 [.2] 18.8 [.3] 19 2.4 [.8] 2.9 [.3] 21.3 [.1] 22 1.3 [.4] 23.6 [.2] 24.8 [.3] 25.8 [.3] 29 1.5 [.6] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 26 28 3-7-4-1 cis- 8 [7-4] cis- (pg/g-dry) 6 4 2 [](pg/g-dry) 14 2.1 [.7] 15 3 [.9] 16 2 [.6] 17 1.9 [.64] 18 1.2 [.4] 19 1.6 [.6] 2.6 [.2] 21 1. [.4] 22.9 [.3] 23 1.1 [.4] 24 3 [1] 25.7 [.3] 29 1.7 [.7] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 26 28 3-7-4-2 cis- 316

[7-5] trans- (pg/l) 35 3 25 2 15 1 [](pg/l) 14 1.2 [.4] 15 2 [.5] 16 4 [2] 17 2.5 [.84] 18 3. [1.] 19 5 [2] 2 1.9 [.7] 21 1. [.4] 22 8 [3] 23 1.3 [.5] 24 1.5 [.6] 25 1.5 [.6] 29 3 [1] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 2 26 28 3-7-5-1 trans- [7-5] trans- (pg/g-dry) 14 12 1 8 6 4 [](pg/g-dry) 14 1.5 [.5] 15 2 [.6] 16 2 [.6] 17 1.5 [.54] 18 1.2 [.4] 19 1.7 [.6] 2 2.2 [.8] 21.9 [.3] 22 6 [2] 23.8 [.3] 24 2.4 [.8] 25 1.2 [.4] 29 6 [2] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 26 28 3-7-5-2 trans- 317

[7-1] cis- 2, 1,5 1, 5 [] 14 2.4 [.8] 15 3.9 [1.3] 16 18 [5.8] 17 12 [3.9] 18 4 [1] 19 5 [2] 2 5 [2] 21 4[2] 22 4 [2] 23 3 [1] 24 5 [2] 25 13 [4] 28 3 [1] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 24 3 26 27 29 3-7-1-3 cis- [7-1] cis- 12 pg/m 3 1 8 6 4 2 [] (pg/m 3 ) 14.6 [.2] 15.51 [.17] 16.57 [.19] 17.16 [.54] 18.13 [.4] 19.1 [.4] 2.14 [.5] 21.16 [.6] 22.9 [.3] 23 1.3 [.42] 24 1.5 [.51] 25.7 [.2] 28.9 [.3] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 26 27 29 3-7-1-4 cis- 318

[7-2] trans- 6 5 4 3 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 24 3 26 27 29 3-7-2-3 trans- [7-2] trans- pg/m 3 14 12 1 8 6 4 2 [] (pg/m 3 ) 14.6 [.2] 15.86 [.29] 16.69 [.23] 17.34 [.14] 18.17 [.6] 19.12 [.5] 2.17 [.6] 21.12 [.5] 22 1.2 [.4] 23 1.6 [.53] 24 2.1 [.7] 25.8 [.3] 28 1. [.3] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 26 27 29 3-7-2-4 trans- 319

[7-3] 3 25 2 15 1 5 [] 14 3.6 [1.2] 15 8.4 [2.8] 16 9.2 [3.1] 17 9.3 [3.1] 18 7 [3] 19 6 [2] 2 7 [2] 21 4[1] 22 8 [3] 23 3 [1] 24 3 [1] 25 3 [1] 28 3 [1] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 24 3 26 27 29 3-7-3-3 [7-3] 3 pg/m 3 2.5 2 1.5 1.5 [] (pg/m 3 ) 14.24 [.8] 15.45 [.15] 16.13 [.42] 17.16 [.54] 18.23 [.8] 19.5 [.2] 2.4 [.1] 21.4 [.2] 22.3 [.1] 23.7 [.3] 24.8 [.3] 25.3 [.1] 28.16 [.6] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 26 27 29 3-7-3-4 32

[7-4] cis- 5 4 3 2 1 [] 14 1.2 [.4] 15 4.8 [1.6] 16 3.4 [1.1] 17 4.5 [1.5] 18 3 [1] 19 3 [1] 2 4 [1] 21 3[1] 22 3 [1] 23 1.8 [.7] 24 2 [1] 25 2.2 [.7] 28 1.4 [.6] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 24 3 26 27 29 3-7-4-3 cis- [7-4] cis- pg/m 3 14 12 1 8 6 4 2 [] (pg/m 3 ) 14.3 [.1] 15.26 [.88] 16.72 [.24] 17.8 [.3] 18.15 [.5] 19.3 [.1] 2.3 [.1] 21.4 [.2] 22.11 [.4] 23.15 [.51] 24.12 [.5] 25.7 [.2] 28.14 [.5] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 26 27 29 3-7-4-4 cis- 321

[7-5] trans- 1,2 1, 8 6 4 2 [] 14 2.4 [.8] 15 3.6 [1.2] 16 13 [4.2] 17 6.2 [2.1] 18 3 [1] 19 7 [3] 2 6 [2] 21 3[1] 22 4 [2] 23 3 [1] 24 4 [1] 25 1 [3.4] 28 3 [1] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 24 3 26 27 29 3-7-5-3 trans- [7-5] trans- 1 pg/m 3 8 6 4 2 [] (pg/m 3 ) 14.3 [.1] 15.35 [.12] 16.48 [.16] 17.13 [.44] 18.1 [.3] 19.9 [.3] 2.9 [.3] 21.7 [.3] 22.8 [.3] 23 1.1 [.35] 24 1.2 [.41] 25.5 [.2] 28.7 [.2] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 26 27 29 3-7-5-4 trans- 322

[8] 5 61 9 POPs 16 14 13 57 61 14 14 cis- trans- 15 14 23 24 25 27 29 26 29 47 1 pg/l 47 2 6 pg/l 14 29 cis-47.6 pg/l 47 46 83 pg/l 15 29 trans-47.9 pg/l 47 14 29 cis- trans- [] H14 tr(1.2) tr(1.) 25 nd 1.5 [.5] 97/114 38/38 H15 tr(1.8) tr(1.6) 7 tr(1.) 2 [.5] 36/36 36/36 H16 nd nd 29 nd 5 [2] 9/38 9/38 H17 nd tr(1) 54 nd 3 [1] 25/47 25/47 H18 nd nd 6 nd 5 [2] 5/48 5/48 H19 nd nd 5.2 nd 2.4 [.8] 12/48 12/48 (pg/l) H2 nd nd 4.6 nd 2.1 [.8] 19/48 19/48 H21 tr(.5) nd 17 nd.8 [.3] 2/49 2/49 H22 nd nd 43 nd 2.2 [.7] 4/49 4/49 H23 nd nd 22 nd 1.3 [.5] 6/49 6/49 H26 tr(.2) tr(.2) 1.5 nd.5 [.2] 28/48 28/48 H29 nd nd 6 nd 3 [1] 2/47 2/47 323

cis- [] H15 9.8 11 17 1.2.7 [.2] 36/36 36/36 H16 1 1 77 2 2 [.4] 38/38 38/38 H17 7.1 6.6 59 1..7 [.2] 47/47 47/47 H18 7.6 6.6 47 1.1 2. [.7] 48/48 48/48 H19 6.1 5.8 12 tr(.9) 1.3 [.4] 48/48 48/48 H2 4.7 5. 37 nd.6 [.2] 46/48 46/48 (pg/l) H21 5.5 4.2 72.8.5 [.2] 49/49 49/49 H22 5.9 3.9 71.7.4 [.2] 49/49 49/49 H23 5.8 5.8 16.7.7 [.3] 49/49 49/49 H26 4.9 3.4 56.7.5 [.2] 48/48 48/48 H29 4.7 3.5 83 nd 1.6 [.6] 46/47 46/47 trans- [] H15 nd nd 2 nd 2 [.4] 4/36 4/36 H16 nd nd nd nd.9 [.3] /38 /38 H17 nd nd nd nd.7 [.2] /47 /47 H18 nd nd nd nd 1.8 [.6] /48 /48 H19 nd nd tr(.9) nd 2. [.7] 2/48 2/48 H2 nd nd nd nd 1.9 [.7] /48 /48 (pg/l) H21 nd nd nd nd.7 [.3] /49 /49 H22 nd nd 8. nd 1.3 [.5] 2/49 2/49 H23 nd nd 2.8 nd.8 [.3] 3/49 3/49 H26 nd nd nd nd.8 [.3] /48 /48 H29 nd nd nd nd 2.3 [.9] /47 /47 1 14 2 24 25 27 28 62.3 pg/g-dry 62 53 4 pg/g-dry 14 29 5 5 cis-62.5 pg/g-dry 62 51 15 pg/g-dry 15 29 5 5 5 5 trans-62.8 pg/g-dry 62 324

14 29 cis- trans- [] H14 4.1 3.2 12 nd 1.8 [.6] 167/189 6/63 H15 tr(2.7) tr(2.2) 16 nd 3 [1.] 138/186 53/62 H16 tr(2.8) tr(2.3) 17 nd 3 [.9] 134/189 53/63 H17 3.1 2.8 2 nd 2.5 [.8] 12/189 48/63 H18 5.2 3.9 23 nd 1.9 [.6] 19/192 64/64 H19 tr(1.8) tr(1.5) 11 nd 3. [.7] 143/192 57/64 (pg/g-dry) H2 tr(1) nd 85 nd 4 [1] 59/192 27/64 H21 1.6 1.3 65 nd 1.1 [.4] 144/192 59/64 H22 1.2 tr(.8) 35 nd 1.1 [.4] 51/64 51/64 H23 tr(1.3) tr(1.2) 48 nd 1.8 [.7] 4/64 4/64 H26 tr(1.) tr(.9) 49 nd 1.5 [.5] 38/63 38/63 H29 1.2 1.1 4 nd.9 [.3] 53/62 53/62 cis- (pg/g-dry) trans- (pg/g-dry) [] H15 4 3 16 nd 3 [1] 153/186 55/62 H16 tr(5) tr(3) 23 nd 6 [2] 136/189 52/63 H17 tr(4) tr(3) 14 nd 7 [2] 119/189 49/63 H18 4. 3.2 21 nd 3. [1.] 157/192 58/64 H19 3 tr(2) 27 nd 3 [1] 141/192 53/64 H2 3 2 18 nd 2 [1] 13/192 51/64 H21 2.7 1.9 29 nd.7 [.3] 176/192 63/64 H22 3.1 2.4 3 nd.8 [.3] 62/64 62/64 H23 2.8 2.5 16 nd.6 [.2] 63/64 63/64 H26 2.1 1.7 31 nd.5 [.2] 59/63 59/63 H29 1.9 1.6 15 nd 1.2 [.5] 51/62 51/62 [] H15 nd nd nd nd 9 [3] /186 /62 H16 nd nd tr(2.5) nd 4 [2] 1/189 1/63 H17 nd nd nd nd 5 [2] /189 /63 H18 nd nd 19 nd 7 [2] 2/192 2/64 H19 nd nd 31 nd 1 [4] 2/192 2/64 H2 nd nd nd nd 1.7 [.7] /192 /64 H21 nd nd nd nd 1.4 [.6] /192 /64 H22 nd nd 4 nd 3 [1] 1/64 1/64 H23 nd nd 2.4 nd 2.3 [.9] 2/64 2/64 H26 nd nd 3.6 nd.7 [.3] 1/63 1/63 H29 nd nd nd nd 2. [.8] /62 /62 1 14 21 2 24 25 27 28 325

28 14 28 cis- trans- [] H14 tr(3.5) 4.6 15 nd 4.2 [1.4] 28/38 6/8 H15 tr(2.8) tr(2.4) 14 nd 6.6 [2.2] 16/3 4/6 H16 tr(3.4) 5.2 16 nd 4.1 [1.4] 23/31 6/7 H17 tr(2.9) tr(2.9) 24 nd 6.1 [2.] 18/31 6/7 H18 tr(4) tr(4) 2 nd 6 [2] 23/31 6/7 H19 tr(3) tr(3) 12 nd 6 [2] 2/31 6/7 H2 tr(2) nd 9 nd 6 [2] 13/31 5/7 H21 tr(4) nd 12 nd 5 [2] 14/31 4/7 H22 3 tr(2) 78 nd 3 [1] 5/6 5/6 H23 4 4 51 nd 3 [1] 3/4 3/4 H24 tr(3) tr(3) 13 nd 4 [1] 4/5 4/5 H25 3 tr(2) 19 nd 3 [1] 4/5 4/5 H27 nd nd tr(1.7) nd 3. [1.] 1/3 1/3 H28 nd nd tr(1.4) nd 2.4 [.9] 1/3 1/3 cis- H14 4.2 4.8 2 nd 4.2 [1.4] 57/7 12/14 H15 nd nd 11 nd 6.6 [2.2] 29/7 8/14 H16 tr(2.3) tr(2.1) 46 nd 4.1 [1.4] 5/7 11/14 H17 nd nd 7.6 nd 6.1 [2.] 32/8 8/16 H18 tr(2) nd 8 nd 6 [2] 36/8 8/16 H19 tr(2) nd 7 nd 6 [2] 28/8 6/16 H2 nd nd 9 nd 6 [2] 25/85 7/17 H21 tr(2) nd 8 nd 5 [2] 3/9 11/18 H22 tr(2) tr(2) 5 nd 3 [1] 12/18 12/18 H23 tr(1) tr(1) 7 nd 3 [1] 13/18 13/18 H24 nd tr(1) 5 nd 4 [1] 1/19 1/19 H25 nd nd 12 nd 3 [1] 9/19 9/19 H27 nd nd 9.2 nd 3. [1.] 9/19 9/19 H28 nd nd 5.5 nd 2.4 [.9] 8/19 8/19 H14 tr(1.7) tr(2.8) 5.2 nd 4.2 [1.4] 7/1 2/2 H15 nd nd nd nd 6.6 [2.2] /1 /2 H16 nd nd tr(1.5) nd 4.1 [1.4] 1/1 1/2 H17 nd nd nd nd 6.1 [2.] /1 /2 H18 nd nd nd nd 6 [2] /1 /2 H19 nd nd nd nd 6 [2] /1 /2 H2 nd nd nd nd 6 [2] /1 /2 H21 nd nd nd nd 5 [2] /1 /2 H22 nd --- tr(1) nd 3 [1] 1/2 1/2 H23 --- --- nd nd 3 [1] /1 /1 H24 nd --- nd nd 4 [1] /2 /2 H25 nd --- nd nd 3 [1] /2 /2 H27 --- --- nd nd 3. [1.] /1 /1 H28 nd --- nd nd 2.4 [.9] /2 /2 [] H15 44 29 88 9.7 6.9 [2.3] 3/3 6/6 H16 64 34 84 tr(9.8) 9.9 [3.3] 31/31 7/7 H17 49 2 59 7.4 3.5 [1.2] 31/31 7/7 H18 56 23 1,1 8 4 [1] 31/31 7/7 H19 37 2 1,1 8 4 [1] 31/31 7/7 H2 37 19 51 8 5 [2] 31/31 7/7 H21 59 33 38 1 3 [1] 31/31 7/7 H22 17 26 1,8 9. 2.4 [.9] 6/6 6/6 H23 55 11 32 3.9 2. [.8] 4/4 4/4 H24 48 12 18 6.2 1.5 [.6] 5/5 5/5 H25 28 29 11 4.4 2.1 [.8] 5/5 5/5 H27 21 14 91 7.2 2.1 [.8] 3/3 3/3 H28 23 18 75 9.4 1.9 [.7] 3/3 3/3 326

cis- [] H15 43 43 32 7. 6.9 [2.3] 7/7 14/14 H16 51 49 62 tr(3.3) 9.9 [3.3] 7/7 14/14 H17 41 45 39 4.9 3.5 [1.2] 8/8 16/16 H18 42 48 27 4 4 [1] 8/8 16/16 H19 43 49 39 4 4 [1] 8/8 16/16 H2 39 46 35 tr(3) 5 [2] 85/85 17/17 H21 41 5 31 4 3 [1] 9/9 18/18 H22 39 49 23 5. 2.4 [.9] 18/18 18/18 H23 5 62 54 3.2 2. [.8] 18/18 18/18 H24 41 62 12 6.9 1.5 [.6] 19/19 19/19 H25 42 46 19 7.3 2.1 [.8] 19/19 19/19 H27 33 43 19 3.2 2.1 [.8] 19/19 19/19 H28 29 28 13 3.6 1.9 [.7] 19/19 19/19 H15 54 51 77 37 6.9 [2.3] 1/1 2/2 H16 27 27 35 19 9.9 [3.3] 1/1 2/2 H17 37 34 69 25 3.5 [1.2] 1/1 2/2 H18 33 31 65 24 4 [1] 1/1 2/2 H19 28 27 35 25 4 [1] 1/1 2/2 H2 37 37 56 18 5 [2] 1/1 2/2 H21 22 21 39 16 3 [1] 1/1 2/2 H22 29 --- 36 24 2.4 [.9] 2/2 2/2 H23 --- --- 41 41 2. [.8] 1/1 1/1 H24 16 --- 17 15 1.5 [.6] 2/2 2/2 H25 3 --- 56 16 2.1 [.8] 2/2 2/2 H27 --- --- 2 2 2.1 [.8] 1/1 1/1 H28 91 --- 27 31 1.9 [.7] 2/2 2/2 trans- [] H15 nd nd 48 nd 13 [4.4] 5/3 1/6 H16 nd nd 55 nd 12 [4.] 9/31 2/7 H17 nd nd 37 nd 23 [7.5] 5/31 1/7 H18 nd nd 45 nd 13 [5] 5/31 1/7 H19 nd nd 61 nd 13 [5] 5/31 1/7 H2 nd nd 33 nd 1 [4] 5/31 1/7 H21 tr(3) nd 24 nd 8 [3] 13/31 3/7 H22 3 tr(2) 24 nd 3 [1] 3/6 3/6 H23 nd nd tr(6) nd 7 [3] 1/4 1/4 H24 nd nd tr(4) nd 8 [3] 1/5 1/5 H25 nd nd nd nd 7 [3] /5 /5 H27 nd nd nd nd 7 [3] /3 /3 H28 nd nd nd nd 9 [3] /3 /3 H15 nd nd nd nd 13 [4.4] /7 /14 H16 nd nd tr(1) nd 12 [4.] 2/7 2/14 H17 nd nd nd nd 23 [7.5] /8 /16 H18 nd nd nd nd 13 [5] /8 /16 H19 nd nd nd nd 13 [5] /8 /16 H2 nd nd nd nd 1 [4] /85 /17 H21 nd nd nd nd 8 [3] /9 /18 H22 nd nd nd nd 3 [1] /18 /18 H23 nd nd nd nd 7 [3] /18 /18 H24 nd nd nd nd 8 [3] /19 /19 H25 nd nd nd nd 7 [3] /19 /19 H27 nd nd 1 nd 7 [3] 5/19 5/19 H28 nd nd nd nd 9 [3] /19 /19 H15 nd nd nd nd 13 [4.4] /1 /2 H16 nd nd nd nd 12 [4.] /1 /2 H17 nd nd nd nd 23 [7.5] /1 /2 H18 nd nd nd nd 13 [5] /1 /2 H19 nd nd nd nd 13 [5] /1 /2 H2 nd nd nd nd 1 [4] /1 /2 H21 nd nd nd nd 8 [3] /1 /2 H22 nd --- nd nd 3 [1] /2 /2 H23 --- --- nd nd 7 [3] /1 /1 H24 nd --- nd nd 8 [3] /2 /2 H25 nd --- tr(5) nd 7 [3] 1/2 1/2 H27 --- --- nd nd 7 [3] /1 /1 H28 nd --- nd nd 9 [3] /2 /2 1 14 21 2 25 24 3 26 327

14 28 cis- trans- [] H14 11 14 22.2.12 [.4] 12/12 34/34 H15 27 41 24 1.1 35/35 35/35.25 [.85] H15 1 16 65.39 34/34 34/34 H16 23 36 2.46.23 [.78] H16 11 18 1.53 H17 25 29 19 1.1.16 [.54] H17 6.5 7.9 61.52 H18 2 27 16.88.11 [.4] H18 6.8 7.2 56.32 H19 22 27 32 1.1 36/36 36/36.7 [.3] H19 6.3 8. 74.42 36/36 36/36 H2 2 31 19.92.6 [.2] H2 7.5 12 6.51 (pg/m 3 ) H21 18 3 11.48.4 [.1] H21 6.3 7.8 48.15 H22 17 26 16.69.11 [.4] H22 7.2 9.5 53.22 H23 16 25 11.73 35/35 35/35.3 [.99] H23 6.1 1 56 tr(.13) H24 13 21 58.46 36/36 36/36.41 [.14] H24 3.2 4.9 2 nd 35/36 35/36 H25 11 21 43.46 36/36 36/36.16 [.5] H25 3.1 4.6 22 tr(.1) 36/36 36/36 H27 8.7 11 49.43.19 [.6] 35/35 35/35 H28 12 14 12 tr(.18).22 [.8] cis- [] H15 3.5 3.5 28.45 35/35 35/35.15 [.48] H15 1.3 1.3 6.6.49 34/34 34/34 H16 2.8 2.9 9.7.65.52 [.17] H16 1.1 1.1 7..44 H17 1.5 1.7 11 tr(.1).12 [.44] H17.91.81 2.9.43 H18 1.7 2. 6.7.13.11 [.4] H18.74.88 3.2 nd 36/37 36/37 H19 2.9 2.8 13.54 36/36 36/36.3 [.1] H19.93.82 3..41 36/36 36/36 H2 2.4 2.2 9.9.53.22 [.8] H2.91.84 3..37 (pg/m 3 H21 2.5 2.6 16.37 ).3 [.1] H21 1..91 3.8.42 H22 2.3 2.3 1.38.2 [.1] H22.93.85 4.3.33 H23 2. 2.3 6..29 35/35 35/35.4 [.1] H23.9.9 2.8.35 H24 2. 2.1 6.3.37 36/36 36/36.5 [.2] H24.62.57 1.9.3 36/36 36/36 H25 2. 2.1 7.7.43 36/36 36/36.3 [.1] H25.66.63 1.4.32 36/36 36/36 H27 1.4 1.4 4.7 tr(.4).5 [.2] 35/35 35/35 H28 1.9 1.9 9.1.3.12 [.5] 26 328

trans- [] H15 tr(.36) tr(.38).3 nd 18/35 18/35.99 [.33] H15 nd nd tr(.94) nd 3/34 3/34 H16 nd nd tr(.38) nd 4/37 4/37.6 [.2] H16 nd nd nd nd /37 /37 H17 tr(.1) tr(.12) 1.2 nd 27/37 27/37.16 [.5] H17 nd nd.32 nd 3/37 3/37 H18 nd nd.7 nd 2/37 2/37.3 [.1] H18 nd nd tr(.1) nd 1/37 1/37 H19 nd nd.16 nd 8/36 8/36.14 [.6] H19 nd nd tr(.6) nd 1/36 1/36 H2 nd nd.17 nd 6/37 6/37.16 [.6] H2 nd nd nd nd /37 /37 (pg/m 3 H21 nd nd.18 nd 1/37 1/37 ).14 [.5] H21 nd nd tr(.6) nd 1/37 1/37 H22 nd nd.16 nd 6/37 6/37.16 [.6] H22 nd nd nd nd /37 /37 H23 nd nd.14 nd 5/35 5/35.13 [.5] H23 nd nd nd nd /37 /37 H24 nd nd tr(.8) nd 8/36 8/36.12 [.5] H24 nd nd nd nd /36 /36 H25 nd nd tr(.11) nd 7/36 7/36.12 [.5] H25 nd nd nd nd /36 /36 H27 nd nd nd nd.3 [.1] /35 /35 H28 nd nd tr(.2) nd.3 [.1] 1/37 1/37 26 329

[8-1] (pg/g-dry) 6 5 4 3 2 [](pg/g-dry) 14 1.8 [.6] 15 3 [1.] 16 3 [.9] 17 2.5 [.8] 18 1.9 [.6] 19 3. [.7] 2 4 [1] 21 1.1 [.4] 22 1.1 [.4] 23 1.8 [.7] 26 1.5 [.5] 29 1.5 [.5] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 24 25 27 28 3-8-1-1 [8-2] cis- (pg/l) 12 1 8 6 4 [](pg/l) 15.7 [.2] 16 2 [.4] 17.7 [.2] 18 2. [.7] 19 1.3 [.4] 2.6 [.2] 21.5 [.2] 22.4 [.2] 23.7 [.3] 26.5 [.2] 29 1.6 [.6] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 24 25 27 28 3-8-2-1 cis- 33

[8-2] cis- (pg/g-dry) 6 5 4 3 [](pg/g-dry) 15 3 [1] 16 6 [2] 17 7 [2] 18 3. [1.] 19 3 [1] 2 2 [1] 21.7 [.3] 22.8 [.3] 23.6 [.2] 26.5 [.2] 29 1.2 [.5] 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 14 24 25 27 28 3-8-2-2 cis- [8-3] trans- (pg/g-dry) 2.5 2 1.5 1 [](pg/g-dry) 15 9 [3] 16 4 [2] 17 5 [2] 18 7 [2] 19 1 [4] 2 1.7 [.7] 21 1.4 [.6] 22 3 [1] 23 2.3 [.9] 26.7 [.3] 29 2. [.8].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 14 24 25 27 28 3-8-3-1 trans- 331

[8-1] 5 4 3 2 1 [] 14 4.2 [1.4] 15 6.6 [2.2] 16 4.1 [1.4] 17 6.1 [2.] 18 6 [2] 19 6 [2] 2 6 [2] 21 5[2] 22 3 [1] 23 3 [1] 24 4 [1] 25 3 [1] 27 3. [1.] 28 2.4 [.9] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 3 25 24 4 26 29 5 27 28 1/2 3-8-1-2 [8-1] 3 pg/m 3 25 2 15 1 5 [] (pg/m 3 ) 14.12 [.4] 15.25 [.85] 16.23 [.78] 17.16 [.54] 18.11 [.4] 19.7 [.3] 2.6 [.2] 21.4 [.1] 22.11 [.4] 23.3 [.99] 24.41 [.14] 25.16 [.5] 27.19 [.6] 28.22 [.8] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 26 29 3-8-1-3 332

[8-2] cis- 2 15 1 5 [] 15 6.9 [2.3] 16 9.9 [3.3] 17 3.5 [1.2] 18 4 [1] 19 4 [1] 2 5 [2] 21 3[1] 22 2.4 [.9] 23 2. [.8] 24 1.5 [.6] 25 2.1 [.8] 27 2.1 [.8] 28 1.9 [.7] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 25 24 3 14 26 29 3-8-2-3 cis- [8-2] cis- 4 pg/m 3 3 2 1 [] (pg/m 3 ) 15.15 [.48] 16.52 [.17] 17.12 [.44] 18.11 [.4] 19.3 [.1] 2.22 [.8] 21.3 [.1] 22.2 [.1] 23.4 [.1] 24.5 [.2] 25.3 [.1] 27.5 [.2] 28.12 [.5] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 26 29 3-8-2-4 cis- 333

[9] 14 9 POPs 16 15 14 58 14 2-endo,3-exo,5-endo,6-exo,8,8,1,1- Parlar-262-endo,3-exo,5-endo,6-exo,8,8,9,1,1- Parlar-5 2,2,5,5,8,9,9,1,1- Parlar-62 3 15 21 27 28 29 27 27 15 21 Parlar-26 Parlar-5 Parlar-62 Parlar-26 [] H15 nd nd nd nd 4 [2] /36 /36 H16 nd nd nd nd 9 [3] /38 /38 H17 nd nd nd nd 1 [4] /47 /47 H18 nd nd nd nd 16 [5] /48 /48 (pg/l) H19 nd nd nd nd 2 [5] /48 /48 H2 nd nd nd nd 8 [3] /48 /48 H21 nd nd nd nd 5 [2] /49 /49 Parlar-5 [] (pg/l) Parlar-62 (pg/l) H15 nd nd nd nd 7 [3] /36 /36 H16 nd nd nd nd 2 [7] /38 /38 H17 nd nd nd nd 2 [5] /47 /47 H18 nd nd nd nd 16 [5] /48 /48 H19 nd nd nd nd 9 [3] /48 /48 H2 nd nd nd nd 7 [3] /48 /48 H21 nd nd nd nd 7 [3] /49 /49 [] H15 nd nd nd nd 3 [9] /36 /36 H16 nd nd nd nd 9 [3] /38 /38 H17 nd nd nd nd 7[3] /47 /47 H18 nd nd nd nd 6 [2] /48 /48 H19 nd nd nd nd 7 [3] /48 /48 H2 nd nd nd nd 4 [2] /48 /48 H21 nd nd nd nd 4 [2] /49 /49 334

15 21 Parlar-26 Parlar-5 Parlar-62 Parlar-26 [] H15 nd nd nd nd 9 [3] /186 /62 H16 nd nd nd nd 6 [2] /189 /63 H17 nd nd nd nd 6 [3] /189 /63 H18 nd nd nd nd 12 [4] /192 /64 (pg/g-dry) H19 nd nd nd nd 7 [3] /192 /64 H2 nd nd nd nd 12 [5] /192 /64 H21 nd nd nd nd 1 [4] /192 /64 Parlar-5 [] (pg/g-dry) Parlar-62 (pg/g-dry) H15 nd nd nd nd 2 [5] /186 /62 H16 nd nd nd nd 6 [2] /189 /63 H17 nd nd nd nd 9 [4] /189 /63 H18 nd nd nd nd 24 [7] /192 /64 H19 nd nd nd nd 3 [1] /192 /64 H2 nd nd nd nd 17 [6] /192 /64 H21 nd nd nd nd 12 [5] /192 /64 [] H15 nd nd nd nd 4, [2,] /186 /62 H16 nd nd nd nd 2, [4] /189 /63 H17 nd nd nd nd 2, [7] /189 /63 H18 nd nd nd nd 21 [6] /192 /64 H19 nd nd nd nd 3 [7] /192 /64 H2 nd nd nd nd 9 [4] /192 /64 H21 nd nd nd nd 8 [3] /192 /64 15 21 15 27 Parlar-26 Parlar-5 Parlar- 62 Parlar-26 [] H15 nd nd tr(39) nd 45 [15] 11/3 3/6 H16 nd nd tr(32) nd 42 [14] 15/31 3/7 H17 nd nd tr(28) nd 47 [16] 7/31 4/7 H18 tr(9) tr(12) 25 nd 18 [7] 21/31 5/7 H19 tr(7) tr(8) 2 nd 1 [4] 26/31 6/7 H2 tr(7) tr(8) 22 nd 9 [3] 27/31 7/7 H21 9 9 23 nd 7 [3] 27/31 7/7 H27 tr(1) tr(15) tr(17) nd 23 [9] 2/3 2/3 H15 tr(28) tr(24) 81 nd 45 [15] 44/7 11/14 H16 43 tr(41) 1, nd 42 [14] 54/7 13/14 H17 tr(42) 53 9 nd 47 [16] 5/75 13/16 H18 41 44 88 nd 18 [7] 7/8 15/16 H19 24 32 69 nd 1 [4] 64/8 14/16 H2 35 33 73 nd 9 [3] 79/85 17/17 H21 25 2 69 nd 7 [3] 82/9 18/18 H27 26 28 4 nd 23 [9] 13/19 13/19 H15 12 65 2,5 nd 45 [15] 5/1 1/2 H16 7 34 81 nd 42 [14] 5/1 1/2 H17 86 38 1,2 nd 47 [16] 5/1 1/2 H18 48 29 75 nd 18 [7] 5/1 1/2 H19 34 28 65 nd 1 [4] 5/1 1/2 H2 38 32 1,2 nd 9 [3] 6/1 2/2 H21 26 2 5 nd 7 [3] 6/1 2/2 H27 --- --- tr(1) tr(1) 23 [9] 1/1 1/1 335

Parlar-5 [] H15 tr(12) tr(12) 58 nd 33 [11] 17/3 4/6 H16 tr(15) nd tr(45) nd 46 [15] 15/31 3/7 H17 nd nd tr(38) nd 54 [18] 9/31 4/7 H18 tr(1) 14 32 nd 14 [5] 24/31 6/7 H19 9 1 37 nd 9 [3] 27/31 7/7 H2 tr(7) tr(6) 23 nd 1 [4] 23/31 6/7 H21 9 9 31 nd 8 [3] 27/31 7/7 H27 tr(11) tr(15) tr(16) nd 3 [1] 2/3 2/3 H15 35 34 1,1 nd 33 [11] 55/7 14/14 H16 6 61 1,3 nd 46 [15] 59/7 14/14 H17 tr(52) 66 1,4 nd 54 [18] 55/8 13/16 H18 56 52 1,3 nd 14 [5] 79/8 16/16 H19 35 41 1,1 nd 9 [3] 77/8 16/16 H2 44 45 1, nd 1 [4] 77/85 17/17 H21 3 23 91 nd 8 [3] 85/9 18/18 H27 tr(25) tr(13) 64 nd 3 [1] 13/19 13/19 H15 11 85 3, nd 33 [11] 5/1 1/2 H16 83 44 1, nd 46 [15] 5/1 1/2 H17 1 48 1,5 nd 54 [18] 5/1 1/2 H18 46 38 1, nd 14 [5] 5/1 1/2 H19 34 36 93 nd 9 [3] 5/1 1/2 H2 49 41 1,6 nd 1 [4] 5/1 1/2 H21 29 25 62 nd 8 [3] 5/1 1/2 H27 --- --- nd nd 3 [1] /1 /1 Parlar-62 [] H15 nd nd nd nd 12 [4] /3 /6 H16 nd nd nd nd 98 [33] /31 /7 H17 nd nd nd nd 1 [34] /31 /7 H18 nd nd nd nd 7 [3] /31 /7 H19 nd nd nd nd 7 [3] /31 /7 H2 nd nd nd nd 8 [3] /31 /7 H21 nd nd nd nd 7 [2] /31 /7 H27 nd nd nd nd 15 [6] /3 /3 H15 nd nd 58 nd 12 [4] 9/7 3/14 H16 nd nd 87 nd 98 [33] 24/7 7/14 H17 nd nd 83 nd 1 [34] 23/8 8/16 H18 tr(3) nd 87 nd 7 [3] 28/8 1/16 H19 tr(3) nd 53 nd 7 [3] 22/8 7/16 H2 tr(3) nd 59 nd 8 [3] 31/85 8/17 H21 tr(2) nd 66 nd 7 [2] 24/9 8/18 H27 nd nd 32 nd 15 [6] 2/19 2/19 H15 tr(96) 2 53 nd 12 [4] 5/1 1/2 H16 tr(64) 11 28 nd 98 [33] 5/1 1/2 H17 tr(78) 13 46 nd 1 [34] 5/1 1/2 H18 7 12 43 nd 7 [3] 5/1 1/2 H19 tr(6) 1 3 nd 7 [3] 5/1 1/2 H2 tr(7) 13 36 nd 8 [3] 5/1 1/2 H21 tr(4) 8 21 nd 7 [2] 5/1 1/2 H27 --- --- nd nd 15 [6] /1 /1 1 15 21 2 27 21 3 22 26 336

15 21 Parlar-26 Parlar-5 Parlar-62 [] Parlar-26 H15.31.31.77 tr(.17) 35/35 35/35.2 [.66] H15 tr(.17) tr(.17).27 tr(.91) 34/34 34/34 H16.27.26.46 tr(.17).2 [.66] H16 tr(.15) tr(.15).5 tr(.94) H17 nd nd nd nd /37 /37.3 [.1] H17 nd nd nd nd /37 /37 H18 nd nd nd nd /37 /37 (pg/m 3 1.8 [.6] ) H18 nd nd nd nd /37 /37 H19 nd nd tr(.3) nd 18/36 18/36.6 [.2] H19 nd nd nd nd /36 /36 H2 tr(.21).22.58 tr(.12).22 [.8] H2 tr(.11) tr(.12) tr(.2) nd 36/37 36/37 H21 tr(.18) tr(.19).26 tr(.11).23 [.9] H21 tr(.12) tr(.13).27 nd 33/37 33/37 [] Parlar-5 H15 nd nd tr(.37) nd 2/35 2/35.81 [.27] H15 nd nd nd nd /34 /34 H16 nd nd nd nd /37 /37 1.2 [.4] H16 nd nd nd nd /37 /37 H17 nd nd nd nd /37 /37.6 [.2] H17 nd nd nd nd /37 /37 H18 nd nd nd nd /37 /37 (pg/m 3 1.6 [.5] ) H18 nd nd nd nd /37 /37 H19 nd tr(.1) tr(.2) nd 29/36 29/36.3 [.1] H19 nd nd nd nd /36 /36 H2 nd nd tr(.19) nd 15/37 15/37.25 [.9] H2 nd nd nd nd /37 /37 H21 nd nd tr(.1) nd 11/37 11/37.3 [.1] H21 nd nd tr(.1) nd 1/37 1/37 [] Parlar-62 H15 nd nd nd nd /35 /35 1.6 [.52] H15 nd nd nd nd /34 /34 H16 nd nd nd nd /37 /37 2.4 [.81] H16 nd nd nd nd /37 /37 H17 nd nd nd nd /37 /37 1.2 [.4] H17 nd nd nd nd /37 /37 H18 nd nd nd nd /37 /37 (pg/m 3 8 [3] ) H18 nd nd nd nd /37 /37 H19 nd nd nd nd /36 /36 1.5 [.6] H19 nd nd nd nd /36 /36 H2 nd nd nd nd /37 /37 1.6 [.6] H2 nd nd nd nd /37 /37 H21 nd nd nd nd /37 /37 1.6 [.6] H21 nd nd nd nd /37 /37 337

[9-1] Parlar-26 5 4 3 2 [] 15 45 [15] 16 42 [14] 17 47 [16] 18 18 [7] 19 1 [4] 2 9 [3] 21 7[3] 27 23[9] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 25 21 3 14 22 26 28 29 4 15 17 1/2 3-9-1-1 Parlar-26 [9-1] Parlar-26 pg/m 3.35.3.25.2.15 [] (pg/m 3 ) 15.2 [.66] 16.2 [.66] 17.3 [.1] 18 1.8 [.6] 19.6 [.2] 2.22 [.8] 21.23 [.9].1.5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 22 29 2 17 18 19 1/2 3-9-1-2 Parlar-26 338

[9-2] Parlar-5 7 6 5 4 3 [] 15 33 [11] 16 46 [15] 17 54 [18] 18 14 [5] 19 9 [3] 2 1 [4] 21 8[3] 27 3 [1] 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 25 21 3 14 22 26 28 29 3-9-2-1 Parlar-5 339

[1] 14 9 POPs 16 15 14 58 14 15 21 23 24 29 23 23 15 23 [] (pg/l) 22 H15 tr(.13) tr(.12).8 nd.3 [.9] 25/36 25/36 H16 nd nd 1.1 nd.4 [.2] 18/38 18/38 H17 nd nd 1. nd.4 [.1] 14/47 14/47 H18 nd nd.7 nd 1.6 [.5] 1/48 1/48 H19 nd nd tr(.5) nd 1.1 [.4] 2/48 2/48 H2 nd nd.7 nd.6 [.2] 4/48 4/48 H21 nd nd.5 nd.4 [.2] 8/49 8/49 H23 nd nd.8 nd.5 [.2] 3/49 3/49 15 23 [] (pg/g-dry) H15 2 tr(1.6) 1,5 nd 2 [.4] 137/186 51/62 H16 2 tr(1.6) 22 nd 2 [.5] 153/189 55/63 H17 1.8 1.2 5,3 nd.9 [.3] 134/189 48/63 H18 1.7 1.2 64 nd.6 [.2] 156/192 57/64 H19 1.5.9 2 nd.9 [.3] 147/192 55/64 H2 1.4 1.1 82 nd.7 [.3] 117/192 48/64 H21 1.4 1.3 62 nd 1. [.4] 126/192 49/64 H23 1.2.9 1,9 nd.9 [.4] 42/64 42/64 1 15 21 2 22 34

15 23 [] H15 4.9 4.2 19 tr(1.6) 2.4 [.81] 3/3 6/6 H16 4.4 4.3 12 tr(1.1) 2.5 [.82] 31/31 7/7 H17 5.4 5.2 2 tr(1.9) 3. [.99] 31/31 7/7 H18 5 4 19 tr(2) 3 [1] 31/31 7/7 H19 5 4 18 tr(2) 3 [1] 31/31 7/7 H2 4 tr(3) 18 tr(2) 4 [1] 31/31 7/7 H21 5.9 5.2 21 tr(1.7) 2.1 [.8] 31/31 7/7 H23 1 7.1 44 5.2 1.9 [.8] 4/4 4/4 H15 8.3 9. 25 tr(1.7) 2.4 [.81] 7/7 14/14 H16 13 11 18 3.8 2.5 [.82] 7/7 14/14 H17 13 13 78 tr(1.) 3. [.99] 8/8 16/16 H18 11 1 53 tr(2) 3 [1] 8/8 16/16 H19 9 11 36 tr(1) 3 [1] 8/8 16/16 H2 11 13 48 tr(1) 4 [1] 85/85 17/17 H21 8.6 9.6 37 tr(.9) 2.1 [.8] 9/9 18/18 H23 12 15 41 tr(1.3) 1.9 [.8] 18/18 18/18 H15 12 15 45 31 2.4 [.81] 1/1 2/2 H16 61 64 11 33 2.5 [.82] 1/1 2/2 H17 77 66 18 41 3. [.99] 1/1 2/2 H18 77 7 28 39 3 [1] 1/1 2/2 H19 57 59 1 32 3 [1] 1/1 2/2 H2 74 68 26 27 4 [1] 1/1 2/2 H21 49 --- 79 32 2.1 [.8] 1/1 2/2 H23 --- --- 58 58 1.9 [.8] 1/1 1/1 1 15 21 2 22 15 23 [] H15.11.12.19.47.84 35/35 35/35 H15.44.43.99.24 [.28] 34/34 34/34 H16.99.11.16 tr(.42).5 [.17] H16 tr(.46) tr(.47).23 tr(.19) H17 tr(.9) tr(.9).24 tr(.5).1 [.3] H17 tr(.4) tr(.4) tr(.8) nd 29/37 29/37 H18 tr(.7) tr(.1).22 nd 29/37 29/37.13 [.4] H18 tr(.7) tr(.7) 2.1 nd 27/37 27/37 (pg/m 3 ) H19.11.11.28.4 36/36 36/36.3 [.1] H19.4.4.9 tr(.2) 36/36 36/36 H2.9.9.25.3.3 [.1] H2.5.4.8.3 H21.12.13.48.49.15 [.6] H21.58.54.18.3 H23.14.13.25.8 35/35 35/35.4 [.1] H23.7.7.11 tr(.3) 22 341

[1] (pg/g-dry) 2.5 2 1.5 1 [](pg/g-dry) 15 2 [.4] 16 2 [.5] 17.9 [.3] 18.6 [.2] 19.9 [.3] 2.7 [.3] 21 1. [.4] 23.9 [.4].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 14 22 24 29 3-1-1 [1] 14 12 1 8 6 [] 15 2.4 [.81] 16 2.5 [.82] 17 3. [.99] 18 3 [1] 19 3 [1] 2 4 [1] 21 2.1 [.8] 23 1.9 [.8] 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 14 22 24 29 3-1-2 342

[1].16 pg/m 3.12.8 [] (pg/m 3 ) 15.84 [.28] 16.5 [.17] 17.1 [.3] 18.13 [.4] 19.3 [.1] 2.3 [.1] 21.15 [.6] 23.4 [.1].4 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 22 24 29 3-1-3 343

[11] HCH HCH 46 21 5 POPs 4 COP4HCH α-hch β-hch γ-hch 22 4 HCH α-β-γ- δ- 4 13 α- β- 61 1 61 13 53 8 1 12 13 γ- 9 δ- 5 14 α- β- 14 α- β- γ- δ- 15 28 α-hch47.4 pg/l 47 3.7 68 pg/l 14 29 β-hch47.7 pg/l 47 12 83 pg/l 14 29 γ-hch47.5 pg/l 47 2.1 19 pg/l 15 29 δ-hch47.4 pg/l 47 tr(.4) 69 pg/l 344

14 29 α-hch β-hch γ-hch δ-hch α-hch [] H14 86 76 6,5 1.9.9 [.3] 114/114 38/38 H15 12 12 97 13 3 [.9] 36/36 36/36 H16 15 145 5,7 13 6 [2] 38/38 38/38 H17 9 81 66 16 4 [1] 47/47 47/47 H18 11 9 2,1 25 3 [1] 48/48 48/48 H19 76 73 72 13 1.9 [.6] 48/48 48/48 H2 78 75 1,1 9 4 [2] 48/48 48/48 H21 74 73 56 14 1.2 [.4] 49/49 49/49 (pg/l) H22 94 75 1,4 14 4 [1] 49/49 49/49 H23 67 6 1, 11 7 [3] 49/49 49/49 H24 65 56 2,2 9.5 1.4 [.5] 48/48 48/48 H25 57 55 1,9 9 7 [2] 48/48 48/48 H26 47 41 7 7.3 4.5 [1.5] 48/48 48/48 H27 48 4 61 8.7 1.2 [.4] 48/48 48/48 H28 38 36 64 5.1 1.1 [.4] 48/48 48/48 H29 47 45 68 3.7.9 [.4] 47/47 47/47 β-hch [] (pg/l) γ-hch (pg/l) H14 21 18 1,6 24.9 [.3] 114/114 38/38 H15 25 24 1,7 14 3 [.7] 36/36 36/36 H16 26 25 3,4 31 4 [2] 38/38 38/38 H17 2 17 2,3 25 2.6 [.9] 47/47 47/47 H18 2 16 2, 42 1.7 [.6] 48/48 48/48 H19 17 15 1,3 18 2.7[.9] 48/48 48/48 H2 15 15 1,8 15 1. [.4] 48/48 48/48 H21 15 15 1,1 18.6 [.2] 49/49 49/49 H22 18 16 2,5 33 2. [.7] 49/49 49/49 H23 13 12 84 28 2. [.8] 49/49 49/49 H24 15 13 82 17 1.4 [.5] 48/48 48/48 H25 13 13 1,1 2 7 [2] 48/48 48/48 H26 1 11 1,1 11 1. [.4] 48/48 48/48 H27 13 12 1,1 21 1.2 [.4] 48/48 48/48 H28 1 96 1,1 12 1.2 [.4] 48/48 48/48 H29 1 11 83 12 1.8 [.7] 47/47 47/47 [] H15 92 9 37 32 7 [2] 36/36 36/36 H16 91 76 8,2 21 2 [7] 38/38 38/38 H17 48 4 25 tr(8) 14 [5] 47/47 47/47 H18 44 43 46 tr(9) 18 [6] 48/48 48/48 H19 34 32 29 5.2 2.1 [.7] 48/48 48/48 H2 34 32 34 4 3 [1] 48/48 48/48 H21 32 26 28 5.1.6 [.2] 49/49 49/49 H22 26 22 19 tr(5) 6 [2] 49/49 49/49 H23 23 2 17 3 3 [1] 49/49 49/49 H24 22 21 44 3. 1.3 [.4] 48/48 48/48 H25 21 17 56 3.2 2.7 [.8] 48/48 48/48 H26 18 18 35 3.5 1.2 [.4] 48/48 48/48 H27 17 15 11 2.6.9 [.3] 48/48 48/48 H28 14 13 13 1.8.8 [.3] 48/48 48/48 H29 17 16 19 2.1 1.4 [.5] 47/47 47/47 δ-hch [] H15 14 14 2 tr(1.1) 2 [.5] 36/36 36/36 H16 24 29 67 tr(1.4) 2 [.7] 38/38 38/38 H17 1.8 nd 62 nd 1.5 [.5] 23/47 23/47 H18 24 18 1, 2.2 2. [.8] 48/48 48/48 H19 11 9.7 72 tr(.7) 1.2 [.4] 48/48 48/48 H2 11 1 1,9 tr(1.1) 2.3 [.9] 48/48 48/48 H21 1 11 45 tr(.7).9 [.4] 49/49 49/49 (pg/l) H22 16 17 78.9.8 [.3] 49/49 49/49 H23 8.6 8.9 3.7.4 [.2] 49/49 49/49 H24 7.9 6.7 22 tr(.5) 1.1 [.4] 48/48 48/48 H25 8.2 8.9 32 tr(.6) 1.1 [.4] 48/48 48/48 H26 7.1 6.5 59.7.4 [.2] 48/48 48/48 H27 7.2 7.4 31.8.3 [.1] 48/48 48/48 H28 5.5 6. 92 tr(.5).8 [.3] 48/48 48/48 H29 8.2 8.2 69 tr(.4) 1. [.4] 47/47 47/47 14 345

α-hch62.2 pg/g-dry 62 1. 1,9 pg/g-dry 14 29 β-hch62.6 pg/g-dry 62 5.7 3,4 pg/g-dry 14 29 γ-hch62.4 pg/g-dry 62 tr(.4) 1,9 pg/g-dry 15 29 δ-hch62.2 pg/g-dry 62 tr(.2) 1,7 pg/g-dry 15 29 14 29 α-hch β-hch γ-hch δ-hch α-hch [] H14 15 17 8,2 2. 1.2 [.4] 189/189 63/63 H15 16 17 9,5 2 2 [.5] 186/186 62/62 H16 16 18 5,7 tr(1.5) 2 [.6] 189/189 63/63 H17 14 16 7, 3.4 1.7 [.6] 189/189 63/63 H18 14 16 4,3 tr(2) 5 [2] 192/192 64/64 H19 14 15 12, tr(1.3) 1.8 [.6] 192/192 64/64 H2 14 19 5,2 nd 1.6 [.6] 191/192 64/64 H21 12 12 6,3 nd 1.1 [.4] 191/192 64/64 (pg/g-dry) H22 14 14 3,7 3.1 2. [.8] 64/64 64/64 H23 12 14 5,1 1.6 1.5 [.6] 64/64 64/64 H24 1 1 3,9 tr(1.1) 1.6 [.5] 63/63 63/63 H25 94 98 3,2 tr(.6) 1.5 [.5] 63/63 63/63 H26 84 93 4,3 nd 2.4 [.8] 62/63 62/63 H27 97 12 9,6 1.1.7 [.3] 62/62 62/62 H28 64 77 5, 1.1.9 [.3] 62/62 62/62 H29 77 86 1,9 1..5 [.2] 62/62 62/62 β-hch [] (pg/g-dry) H14 23 23 11, 3.9.9 [.3] 189/189 63/63 H15 25 22 39, 5 2 [.7] 186/186 62/62 H16 24 23 53, 4 3 [.8] 189/189 63/63 H17 2 22 13, 3.9 2.6 [.9] 189/189 63/63 H18 19 21 21, 2.3 1.3 [.4] 192/192 64/64 H19 2 19 59, 1.6.9 [.3] 192/192 64/64 H2 19 2 8,9 2.8.8 [.3] 192/192 64/64 H21 18 17 1, 2.4 1.3 [.5] 192/192 64/64 H22 23 21 8,2 11 2.4 [.8] 64/64 64/64 H23 18 21 14, 3 3 [1] 64/64 64/64 H24 16 17 8,3 3.7 1.5 [.6] 63/63 63/63 H25 16 17 6,9 4.5.4 [.1] 63/63 63/63 H26 14 14 7,2 2.9.9 [.3] 63/63 63/63 H27 16 17 5,9 2.5.8 [.3] 62/62 62/62 H28 13 16 6, 3.7.9 [.3] 62/62 62/62 H29 14 11 3,4 5.7 1.5 [.6] 62/62 62/62 346

γ-hch (pg/g-dry) δ-hch (pg/g-dry) [] H15 51 47 4, tr(1.4) 2 [.4] 186/186 62/62 H16 53 48 4,1 tr(.8) 2 [.5] 189/189 63/63 H17 49 46 6,4 tr(1.8) 2. [.7] 189/189 63/63 H18 48 49 3,5 tr(1.4) 2.1 [.7] 192/192 64/64 H19 42 41 5,2 tr(.6) 1.2 [.4] 192/192 64/64 H2 4 43 2,2 tr(.7).9 [.4] 192/192 64/64 H21 38 43 3,8 nd.6 [.2] 191/192 64/64 H22 35 3 2,3 tr(1.5) 2. [.7] 64/64 64/64 H23 35 42 3,5 nd 3 [1] 62/64 62/64 H24 3 29 3,5 nd 1.3 [.4] 61/63 61/63 H25 33 35 2,1.9.6 [.2] 63/63 63/63 H26 27 3 2,6 nd 2.7 [.9] 61/63 61/63 H27 29 35 2,8 tr(.3).5 [.2] 62/62 62/62 H28 2 25 3,1 tr(.7).8 [.3] 62/62 62/62 H29 23 25 1,9 tr(.4) 1. [.4] 62/62 62/62 [] H15 42 46 5,4 nd 2 [.7] 18/186 61/62 H16 55 55 5,5 tr(.5) 2 [.5] 189/189 63/63 H17 52 63 6,2 nd 1. [.3] 188/189 63/63 H18 45 47 6, nd 1.7 [.6] 189/192 64/64 H19 26 28 5,4 nd 5 [2] 165/192 6/64 H2 41 53 3,3 nd 2 [1] 186/192 64/64 H21 36 37 5, nd 1.2 [.5] 19/192 64/64 H22 39 4 3,8 1.3 1.2 [.5] 64/64 64/64 H23 37 47 5, nd 1.4 [.5] 63/64 63/64 H24 28 28 3,1 nd.8 [.3] 62/63 62/63 H25 31 29 2,5.4.3 [.1] 63/63 63/63 H26 27 26 3,9.4.4 [.1] 63/63 63/63 H27 27 28 2,9 tr(.4).5 [.2] 62/62 62/62 H28 2 24 6,1 nd.5 [.2] 6/62 6/62 H29 25 22 1,7 tr(.2).6 [.2] 62/62 62/62 14 21 α-hch3 1 pg/g-wet 3 6 32pg/g-wet 19 1 pg/g-wet 19 18 13pg/g-wet 2 1 pg/g-wet 2 7 93pg/g-wet 14 29 β-hch3 1 pg/g-wet 3 21 6pg/g-wet 19 1 pg/gwet 19 4 29pg/g-wet 2 1 pg/g-wet 2 3 3,5pg/g-wet γ-hch3 1 pg/g-wet 3 tr(2) 11pg/g-wet 19 1 pg/g-wet 19 16 3pg/g-wet 2 1 pg/g-wet 2 tr(1) 2pg/g-wet 15 29 347

5 5 δ-hch3.9 pg/g-wet 3 tr(1) 3pg/g-wet 19.9 pg/g-wet 19 15 23pg/g-wet 2.9 pg/g-wet 2 1 tr(1)pg/gwet 15 28 5 5 14 29 α-hch β-hch γ-hch δ-hch α-hch [] H14 67 64 1,1 12 4.2 [1.4] 38/38 8/8 H15 45 3 61 9.9 1.8 [.61] 3/3 6/6 H16 56 25 1,8 tr(12) 13 [4.3] 31/31 7/7 H17 38 25 1,1 tr(7.1) 11 [3.6] 31/31 7/7 H18 3 21 39 6 3 [1] 31/31 7/7 H19 31 17 1,4 8 7 [2] 31/31 7/7 H2 26 16 38 7 6 [2] 31/31 7/7 H21 45 21 2,2 9 5 [2] 31/31 7/7 H22 35 2 73 13 3 [1] 6/6 6/6 H23 64 33 1,2 13 3 [1] 4/4 4/4 H24 23 12 34 4. 3.7 [1.2] 5/5 5/5 H25 3 25 69 6 3 [1] 5/5 5/5 H26 16 16 39 7 3 [1] 3/3 3/3 H27 11 15 25 3.5 3. [1.] 3/3 3/3 H28 13 2 22 5 3 [1] 3/3 3/3 H29 15 16 32 6 3 [1] 3/3 3/3 H14 57 56 59 tr(1.9) 4.2 [1.4] 7/7 14/14 H15 43 58 59 2.6 1.8 [.61] 7/7 14/14 H16 57 55 2,9 nd 13 [4.3] 63/7 14/14 H17 42 43 1, nd 11 [3.6] 75/8 16/16 H18 44 53 36 tr(2) 3 [1] 8/8 16/16 H19 39 4 73 tr(2) 7 [2] 8/8 16/16 H2 36 47 41 nd 6 [2] 84/85 17/17 H21 39 32 83 tr(2) 5 [2] 9/9 18/18 H22 27 39 25 tr(1) 3 [1] 18/18 18/18 H23 37 54 69 tr(2) 3 [1] 18/18 18/18 H24 24 32 17 nd 3.7 [1.2] 18/19 18/19 H25 32 47 32 tr(2) 3 [1] 19/19 19/19 H26 26 4 21 nd 3 [1] 18/19 18/19 H27 18 26 18 tr(1.3) 3. [1.] 19/19 19/19 H28 15 17 81 nd 3 [1] 18/19 18/19 H29 2 29 13 nd 3 [1] 18/19 18/19 H14 17 13 36 93 4.2 [1.4] 1/1 2/2 H15 73 74 23 3 1.8 [.61] 1/1 2/2 H16 19 8 1,6 58 13 [4.3] 1/1 2/2 H17 76 77 85 67 11 [3.6] 1/1 2/2 H18 76 75 1 55 3 [1] 1/1 2/2 H19 75 59 21 43 7 [2] 1/1 2/2 H2 48 48 61 32 6 [2] 1/1 2/2 H21 43 42 56 34 5 [2] 1/1 2/2 H22 26 --- 43 16 3 [1] 2/2 2/2 H23 --- --- 48 48 3 [1] 1/1 1/1 H24 35 --- 39 32 3.7 [1.2] 2/2 2/2 H25 46 --- 13 16 3 [1] 2/2 2/2 H26 61 --- 22 17 3 [1] 2/2 2/2 H27 --- --- 13 13 3. [1.] 1/1 1/1 H28 63 --- 17 23 3 [1] 2/2 2/2 H29 81 --- 93 7 3 [1] 2/2 2/2 348

14 29 α-hch β-hch γ-hch δ-hch β-hch [] H14 88 62 1,7 32 12 [4] 38/38 8/8 H15 78 5 1,1 23 9.9 [3.3] 3/3 6/6 H16 1 74 1,8 22 6.1 [2.] 31/31 7/7 H17 85 56 2, 2 2.2 [.75] 31/31 7/7 H18 81 7 88 11 3 [1] 31/31 7/7 H19 79 56 1,8 21 7 [3] 31/31 7/7 H2 73 51 1,1 23 6 [2] 31/31 7/7 H21 83 55 1,6 27 6 [2] 31/31 7/7 H22 89 56 1,5 27 3 [1] 6/6 6/6 H23 13 68 2, 39 3 [1] 4/4 4/4 H24 65 37 98 15 2. [.8] 5/5 5/5 H25 61 47 71 17 2.2 [.8] 5/5 5/5 H26 4 35 64 28 2.4 [.9] 3/3 3/3 H27 34 45 69 13 3. [1.] 3/3 3/3 H28 37 47 5 21 3 [1] 3/3 3/3 H29 39 47 6 21 3 [1] 3/3 3/3 γ-hch H14 11 12 1,8 tr(5) 12 [4] 7/7 14/14 H15 81 96 1,1 tr(3.5) 9.9 [3.3] 7/7 14/14 H16 11 14 1,1 tr(3.9) 6.1 [2.] 7/7 14/14 H17 95 11 1,3 6.7 2.2 [.75] 8/8 16/16 H18 89 11 1,1 4 3 [1] 8/8 16/16 H19 11 12 81 7 7 [3] 8/8 16/16 H2 94 15 75 tr(4) 6 [2] 85/85 17/17 H21 98 13 97 tr(5) 6 [2] 9/9 18/18 H22 81 11 76 5 3 [1] 18/18 18/18 H23 1 14 71 4 3 [1] 18/18 18/18 H24 72 1 51 6.5 2. [.8] 19/19 19/19 H25 8 11 42 7.2 2.2 [.8] 19/19 19/19 H26 75 14 46 4.4 2.4 [.9] 19/19 19/19 H27 56 94 39 6. 3. [1.] 19/19 19/19 H28 41 65 2 5 3 [1] 19/19 19/19 H29 54 86 29 4 3 [1] 19/19 19/19 H14 3, 3, 7,3 1,6 12 [4] 1/1 2/2 H15 3,4 3,9 5,9 1,8 9.9 [3.3] 1/1 2/2 H16 2,3 2,1 4,8 1,1 6.1 [2.] 1/1 2/2 H17 2,5 2,8 6, 93 2.2 [.75] 1/1 2/2 H18 2,1 2,4 4,2 1,1 3 [1] 1/1 2/2 H19 2, 1,9 3,2 1,4 7 [3] 1/1 2/2 H2 2,4 2, 5,6 1,3 6 [2] 1/1 2/2 H21 1,6 1,4 4,2 87 6 [2] 1/1 2/2 H22 1,6 --- 2,8 91 3 [1] 2/2 2/2 H23 --- --- 4,5 4,5 3 [1] 1/1 1/1 H24 1,4 --- 2,6 73 2. [.8] 2/2 2/2 H25 1,4 --- 3, 61 2.2 [.8] 2/2 2/2 H26 29 --- 3,6 24 2.4 [.9] 2/2 2/2 H27 --- --- 57 57 3. [1.] 1/1 1/1 H28 1,4 --- 2,6 79 3 [1] 2/2 2/2 H29 1, --- 3,5 3 3 [1] 2/2 2/2 [] H15 19 18 13 5.2 3.3 [1.1] 3/3 6/6 H16 tr(24) tr(16) 23 nd 31 [1] 28/31 7/7 H17 23 13 37 tr(5.7) 8.4 [2.8] 31/31 7/7 H18 18 12 14 7 4 [2] 31/31 7/7 H19 16 1 45 tr(4) 9 [3] 31/31 7/7 H2 12 1 98 tr(3) 9 [3] 31/31 7/7 H21 14 12 89 tr(3) 7 [3] 31/31 7/7 H22 14 9 15 5 3 [1] 6/6 6/6 H23 26 17 32 5 3 [1] 4/4 4/4 H24 8.1 3.5 68 3. 2.3 [.9] 5/5 5/5 H25 7.2 3.9 31 tr(2.1) 2.4 [.9] 5/5 5/5 H26 7.4 4.8 18 4.6 2.2 [.8] 3/3 3/3 H27 7.3 7.8 14 tr(3.6) 4.8 [1.6] 3/3 3/3 H28 6 5 11 4 3 [1] 3/3 3/3 H29 4 3 11 tr(2) 3 [1] 3/3 3/3 349

γ-hch δ-hch [] H15 16 22 13 tr(1.7) 3.3 [1.1] 7/7 14/14 H16 tr(28) tr(24) 66 nd 31 [1] 55/7 11/14 H17 17 17 23 nd 8.4 [2.8] 78/8 16/16 H18 19 22 97 tr(2) 4 [2] 8/8 16/16 H19 15 15 19 nd 9 [3] 71/8 15/16 H2 13 16 96 nd 9 [3] 7/85 15/17 H21 14 12 18 nd 7 [3] 81/9 17/18 H22 9 13 56 tr(1) 3 [1] 18/18 18/18 H23 12 15 16 tr(1) 3 [1] 18/18 18/18 H24 7.8 12 43 nd 2.3 [.9] 18/19 18/19 H25 8.6 12 81 nd 2.4 [.9] 17/19 17/19 H26 8.4 14 45 nd 2.2 [.8] 16/19 16/19 H27 6.1 7.9 42 nd 4.8 [1.6] 14/19 14/19 H28 5 5 43 nd 3 [1] 18/19 18/19 H29 5.9 9 3 nd 3 [1] 16/19 16/19 H15 14 19 4 3.7 3.3 [1.1] 1/1 2/2 H16 64 tr(21) 1,2 tr(11) 31 [1] 1/1 2/2 H17 18 2 32 9.6 8.4 [2.8] 1/1 2/2 H18 16 17 29 8 4 [2] 1/1 2/2 H19 21 14 14 tr(8) 9 [3] 1/1 2/2 H2 12 14 19 tr(5) 9 [3] 1/1 2/2 H21 11 11 21 tr(6) 7 [3] 1/1 2/2 H22 1 --- 23 4 3 [1] 2/2 2/2 H23 --- --- 26 26 3 [1] 1/1 1/1 H24 11 --- 19 6.3 2.3 [.9] 2/2 2/2 H25 6. --- 24 tr(1.5) 2.4 [.9] 2/2 2/2 H26 1 --- 24 4.4 2.2 [.8] 2/2 2/2 H27 --- --- nd nd 4.8 [1.6] /1 /1 H28 5 --- 14 tr(2) 3 [1] 2/2 2/2 H29 4.5 --- 2 tr(1) 3 [1] 2/2 2/2 [] H15 7.4 tr(2.6) 1,3 nd 3.9 [1.3] 29/3 6/6 H16 6.3 tr(2.1) 1,5 nd 4.6 [1.5] 25/31 6/7 H17 5.4 tr(2.1) 1,6 nd 5.1 [1.7] 23/31 6/7 H18 6 tr(2) 89 tr(1) 3 [1] 31/31 7/7 H19 4 nd 75 nd 4 [2] 12/31 4/7 H2 tr(3) nd 61 nd 6 [2] 7/31 3/7 H21 tr(4) nd 7 nd 5 [2] 14/31 4/7 H22 4 tr(2) 87 nd 3 [1] 5/6 5/6 H23 9 tr(2) 1,4 tr(1) 3 [1] 4/4 4/4 H24 3 tr(1) 58 nd 3 [1] 3/5 3/5 H25 3 tr(1) 23 nd 3 [1] 3/5 3/5 H26 tr(1) tr(2) 3 nd 3 [1] 2/3 2/3 H27 nd nd tr(1.5) nd 2.1 [.8] 1/3 1/3 H28 tr(1) tr(1) tr(2) tr(1) 3 [1] 3/3 3/3 H29 tr(1.7) tr(1.6) 3 tr(1) 2.3 [.9] 3/3 3/3 H15 tr(3.6) 4. 16 nd 3.9 [1.3] 59/7 13/14 H16 tr(4.2) tr(3.5) 27 nd 4.6 [1.5] 54/7 11/14 H17 tr(3.2) tr(3.1) 32 nd 5.1 [1.7] 55/8 12/16 H18 4 3 35 nd 3 [1] 72/8 16/16 H19 tr(3) tr(2) 31 nd 4 [2] 42/8 1/16 H2 tr(4) tr(3) 77 nd 6 [2] 54/85 12/17 H21 tr(3) tr(3) 18 nd 5 [2] 57/9 13/18 H22 tr(2) tr(2) 36 nd 3 [1] 13/18 13/18 H23 3 4 19 nd 3 [1] 14/18 14/18 H24 tr(2) tr(2) 12 nd 3 [1] 14/19 14/19 H25 3 tr(2) 4 nd 3 [1] 14/19 14/19 H26 tr(2) tr(2) 23 nd 3 [1] 14/19 14/19 H27 tr(1.7) tr(1.8) 17 nd 2.1 [.8] 12/19 12/19 H28 tr(2) tr(2) 1 nd 3 [1] 17/19 17/19 H29 2.4 2.4 23 nd 2.3 [.9] 15/19 15/19 35

δ-hch [] H15 19 18 31 12 3.9 [1.3] 1/1 2/2 H16 3 14 26 6.4 4.6 [1.5] 1/1 2/2 H17 16 15 3 1 5.1 [1.7] 1/1 2/2 H18 13 12 21 9 3 [1] 1/1 2/2 H19 12 1 22 4 4 [2] 1/1 2/2 H2 9 8 31 tr(3) 6 [2] 1/1 2/2 H21 5 6 9 tr(3) 5 [2] 1/1 2/2 H22 12 --- 13 11 3 [1] 2/2 2/2 H23 --- --- 5 5 3 [1] 1/1 1/1 H24 4 --- 7 tr(2) 3 [1] 2/2 2/2 H25 3 --- 4 tr(2) 3 [1] 2/2 2/2 H26 tr(2) --- 3 tr(1) 3 [1] 2/2 2/2 H27 --- --- nd nd 2.1 [.8] /1 /1 H28 tr(1) --- tr(2) tr(1) 3 [1] 2/2 2/2 H29 nd --- tr(1) nd 2.3 [.9] 1/2 1/2 1 14 21 2 25 24 α-hch37.3 pg/m 3 37 4.9 7pg/m 3 β-hch37.4 pg/m 3 37.67 59pg/m 3 21 29 γ-hch37.4 pg/m 3 37.84 93pg/m 3 21 29 δ-hch37.3 pg/m 3 37 36 46pg/m 3 HCH 15 2 HCH HCH 遡 21 29 α-hch β-hch γ-hch δ-hch α-hch [] H21 58 58 34 19.12 [.5] H21 21 18 4 7.8 H22 46 51 28 14 1.4 [.47] H22 19 16 41 6.8 H23 43 44 41 9.5 35/35 35/35 2.5 [.83] H23 18 15 68 6.5 H24 37 37 25 15 36/36 36/36 (pg/m 3 2.1 [.7] ) H24 12 11 12 4.4 36/36 36/36 H25 36 39 22 13 36/36 36/36 5.2 [1.7] H25 1 8.8 75 tr(3.9) 36/36 36/36 H26 44 4 65 14.19 [.6] 36/36 36/36 H27 33 32 3 8.8.17 [.6] 35/35 35/35 H28 39 35 52 5.4.17 [.7] H29 36 37 7 4.9.8 [.3] 351

β-hch (pg/m 3 ) γ-hch (pg/m 3 ) δ-hch (pg/m 3 ) [] H21 5.6 5.6 28.96.9 [.3] H21 1.8 1.8 24.31 H22 5.6 6.2 34.89.27 [.9] H22 1.7 1.7 29 tr(.26) H23 5. 5.2 49.84 35/35 35/35.39 [.13] H23 1.7 1.7 91 tr(.31) H24 5. 5.5 32.65 36/36 36/36.36 [.12] H24.93 1.1 8.5 tr(.26) 36/36 36/36 H25 4.7 5.7 37.66 36/36 36/36.21 [.7] H25.97.95 6.7 tr(.17) 36/36 36/36 H26 5.4 6.8 74.57.24 [.8] 36/36 36/36 H27 3. 3. 34.36.25 [.8] 35/35 35/35 H28 4.8 5.6 64.3.3 [.1] H29 4.1 5.1 59.67.11 [.4] [] H21 17 19 65 2.9.6 [.2] H21 5.6 4.6 55 1.5 H22 14 16 66 2.3.35 [.12] H22 4.8 4.4 6 1.1 H23 14 17 98 2.7 35/35 35/35 1.6 [.52] H23 5.1 4.8 67 tr(1.1) H24 13 15 55 2.3 36/36 36/36.95 [.32] H24 3.1 3.2 19 tr(.63) 36/36 36/36 H25 12 14 58 tr(2.) 36/36 36/36 2.2 [.7] H25 2.8 3. 12 nd 34/36 34/36 H26 14 16 1 1.7.17 [.6] 36/36 36/36 H27 8.3 1 51 1.4.19 [.6] 35/35 35/35 H28 12 13 89.79.18 [.7] H29 1 11 93.84.1 [.4] [] H21 1.3 1.3 21.9.4 [.2] H21.36.33 2.4 H22 1.4 1.3 25.11.5 [.2] H22.38.35 22.5 H23 1.1 1.1 33.11 35/35 35/35.63 [.21] H23.35.34 26 tr(.5) H24 1. 1.3 2 tr(.6) 36/36 36/36.7 [.3] H24.18.19 7.3 nd 35/36 35/36 H25 1. 1.1 2 tr(.5) 36/36 36/36.8 [.3] H25.17.17 5.3 nd 34/36 34/36 H26 1.2 1.3 5 tr(.7).19 [.6] 36/36 36/36 H27.55.71 22 nd.15 [.5] 32/35 32/35 H28 1. 1.2 46 nd.2 [.8] 35/37 35/37 H29.8.92 46 nd.8 [.3] 36/37 36/37 352

[11-1] α-hch (pg/l) 16 12 8 4 [](pg/l) 14.9 [.3] 15 3 [.9] 16 6 [2] 17 4 [1] 18 3 [1] 19 1.9 [.6] 2 4[2] 21 1.2 [.4] 22 4 [1] 23 7 [3] 24 1.4 [.5] 25 7 [2] 26 4.5 [1.5] 27 1.2 [.4] 28 1.1 [.4] 29.9 [.4] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 3-11-1-1 α-hch [11-1] α-hch (pg/g-dry) 2 15 1 5 [](pg/g-dry) 14 1.2 [.4] 15 2 [.5] 16 2 [.6] 17 1.7 [.6] 18 5 [2] 19 1.8 [.6] 2 1.6 [.6] 21 1.1 [.4] 22 2. [.8] 23 1.5 [.6] 24 1.6 [.5] 25 1.5 [.5] 26 2.4 [.8] 27.7 [.3] 28.9 [.3] 29.5 [.2] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 21 3-11-1-2 α-hch 353

[11-1] α-hch 8 6 4 2 [] 14 4.2 [1.4] 15 1.8 [.61] 16 13 [4.3] 17 11 [3.6] 18 3 [1] 19 7 [2] 2 6 [2] 21 5[2] 22 3 [1] 23 3 [1] 24 3.7 [1.2] 25 3 [1] 26 3 [1] 27 3. [1.] 28 3[1] 29 3[1] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 24 3-11-1-3 α-hch [11-1] α-hch pg/m 3 6 5 4 3 2 [] (pg/m 3 ) 21.12 [.5] 22 1.4 [.47] 23 2.5 [.83] 24 2.1 [.7] 25 5.2 [1.7] 26.19 [.16] 27.17 [.6] 28.17 [.7] 29.8 [.3] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-11-1-4 α-hch 354

[11-2] β-hch (pg/l) 3 25 2 15 1 5 [](pg/l) 14.9 [.3] 15 3 [.7] 16 4 [2] 17 2.6 [.9] 18 1.7 [.6] 19 2.7 [.9] 2 1. [.4] 21.6 [.2] 22 2. [.7] 23 2. [.8] 24 1.4 [.5] 25 7 [2] 26 1. [.4] 27 1.2 [.4] 28 1.2 [.4] 29 1.8 [.7] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 3-11-2-1 β-hch [11-2] β-hch (pg/g-dry) 3 25 2 15 1 [](pg/g-dry) 14.9 [.3] 15 2 [.7] 16 3 [.8] 17 2.6 [.9] 18 1.3 [.4] 19.9 [.3] 2.8 [.3] 21 1.3 [.5] 22 2.4 [.8] 23 3 [1] 24 1.5 [.6] 25.4 [.1] 26.9 [.3] 27.8 [.3] 28.9 [.3] 29 1.5 [.6] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 14 21 3-11-2-2 β-hch 355

14 12 1 8 6 4 2 [11-2] β-hch 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 14 21 2 25 24 3-11-2-3 β-hch [] 14 12 [4] 15 9.9 [3.3] 16 6.1 [2.] 17 2.2 [.75] 18 3 [1] 19 7 [3] 2 6 [2] 21 6[2] 22 3 [1] 23 3 [1] 24 2 [.8] 25 2.2 [.8] 26 2.4 [.9] 27 3. [1.] 28 3 [1] 29 3 [1] [11-2] β-hch 6 pg/m 3 5 4 3 2 [] (pg/m 3 ) 21.9 [.3] 22.27 [.9] 23.39 [.13] 24.36 [.12] 25.21 [.7] 26.24 [.8] 27.25 [.8] 28.3 [.1] 29.11 [.4] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-11-2-4 β-hch 356

[11-3] γ-hch (pg/l) 1 8 6 4 2 [](pg/l) 15 7 [2] 16 2 [7] 17 14 [5] 18 18 [6] 19 2.1 [.7] 2 3 [1] 21.6 [.2] 22 6 [2] 23 3 [1] 24 1.3 [.4] 25 2.7 [.8] 26 1.2 [.4] 27.9 [.3] 28.8 [.3] 29 1.4 [.5] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-11-3-1 γ-hch [11-3] γ-hch (pg/g-dry) 6 5 4 3 2 [](pg/g-dry) 15 2 [.4] 16 2 [.5] 17 2. [.7] 18 2.1 [.7] 19 1.2 [.4] 2.9 [.4] 21.6 [.2] 22 2. [.7] 23 3 [1] 24 1.3 [.4] 25.6 [.2] 26 2.7 [.9] 27.5 [.2] 28.8 [.3] 29 1. [.4] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 γ-hch 14 2 15 21 3-11-3-2 γ-hch 357

[11-3] γ-hch 3 25 2 15 1 5 [] 15 3.3 [1.1] 16 31 [1] 17 8.4 [2.8] 18 4 [2] 19 9 [3] 2 9 [3] 21 7[3] 22 3 [1] 23 3 [1] 24 2.3 [.9] 25 2.4 [.9] 26 2.2 [.8] 27 4.8 [1.6] 28 3 [1] 29 3 [1] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 25 24 3-11-3-3 γ-hch [11-3] γ-hch 2 pg/m 3 15 1 [] (pg/m 3 ) 21.6 [.2] 22.35 [.12] 23 1.6 [.52] 24.95 [.32] 25 2.2[.7] 26.17 [.6] 27.19 [.6] 28.18 [.7] 29.1 [.4] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-11-3-4 γ-hch 358

[11-4] δ-hch (pg/l) 25 2 15 1 5 [](pg/l) 15 2 [.5] 16 2 [.7] 17 1.5 [.5] 18 2. [.8] 19 1.2 [.4] 2 2.3 [.9] 21.9 [.4] 22.8 [.3] 23.4 [.2] 24 1.1 [.4] 25 1.1 [.4] 26.4 [.2] 27.3 [.1] 28.8 [.3] 29 1. [.4] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-11-4-1 δ-hch [11-4] δ-hch (pg/g-dry) 6 5 4 3 2 1 [](pg/g-dry) 15 2 [.7] 16 2 [.5] 17 1. [.3] 18 1.7 [.6] 19 5 [2] 2 2 [1] 21 1.2 [.5] 22 1.2 [.5] 23 1.4 [.5] 24.8 [.3] 25.3 [.1] 26.4 [.1] 27.5 [.2] 28.5 [.2] 29.6 [.2] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 δ-hch 14 2 15 21 3-11-4-2 δ-hch 359

[11-4] δ-hch 1 8 6 4 2 [] 15 3.9 [1.3] 16 4.6 [1.5] 17 5.1 [1.7] 18 3 [1] 19 4 [2] 2 6 [2] 21 5[2] 22 3 [1] 23 3 [1] 24 3 [1] 25 3 [1] 26 3 [1] 27 2.1 [.8] 28 3 [1] 29 2.3 [.9] 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 15 21 2 25 24 3 27 1/2 3-11-4-3 δ-hch [11-4] δ-hch 1.6 pg/m 3 1.2.8 [] (pg/m 3 ) 21.4 [.2] 21.5 [.2] 23.63 [.21] 24.7 [.3] 25.8 [.3] 26.19 [.6] 27.15 [.5] 28.2 [.8] 29.8 [.3].4 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-11-4-4 δ-hch 36

[12] 21 5 POPs 4 COP4 22 4 2 14 15 14 2 22 23 24 29 23 23 2 23 [] (pg/l) 21 H2 nd nd.76 nd.14 [.5] 13/46 13/46 H22 tr(.4) nd 1.6 nd.9 [.4] 13/49 13/49 H23 nd nd.7 nd.2 [.5] 15/49 15/49 2 23 [] (pg/g-dry) H2 nd nd 5.8 nd.42 [.16] 23/129 1/49 H22 nd nd 2.8 nd.4 [.2] 9/64 9/64 H23 nd nd 1.5 nd.4 [.2] 9/64 9/64 1 2 2 21 2 23 [] H2 nd nd nd nd 5.6 [2.2] /31 /7 H22 nd nd nd nd 5.9 [2.3] /6 /6 H23 nd nd nd nd.5 [.2] /4 /4 H2 nd nd nd nd 5.6 [2.2] /85 /17 H22 nd nd nd nd 5.9 [2.3] /18 /18 H23 nd nd nd nd.5 [.2] /18 /18 H2 nd nd nd nd 5.6 [2.2] /1 /2 H22 nd --- nd nd 5.9 [2.3] /2 /2 H23 --- --- nd nd.5 [.2] /1 /1 1 2 2 21 361

22 23 [] H22 nd nd nd nd /37 /37.4 [.2] H22 nd nd nd nd /37 /37 (pg/m 3 ) H23 nd nd nd nd /35 /35.4 [.2] H23 nd nd nd nd /37 /37 362

[13] 21 5 POPs 4 COP4 22 4 21 13 14 15 16 14 21 22 23 27 28 29 27 27 21 23 [] H21 nd nd nd nd 5.7 [2.2] /49 /49 H22 nd nd nd nd 3 [1] /49 /49 (pg/l) H23 nd nd nd nd 2.2 [.9] /49 /49 21 23 [][] 21 27 [] H21 nd nd 12 nd 1.1 [.4] 45/19 21/64 H22 nd nd 18 nd 1.5 [.6] 1/64 1/64 (pg/g-dry) H23 nd nd 6.3 nd 3.6 [1.4] 8/64 8/64 H27 nd nd 15 nd.8 [.3] 9/62 9/62 1 21 2 21 23 [][] 3 24 26 21 27 [] H21 nd nd tr(.53) nd 1.3 [.43] 1/31 1/7 H22 nd nd nd nd 24 [1] /6 /6 H23 nd nd nd nd 3 [1] /4 /4 H27 nd nd nd nd 14 [5] /3 /3 H21 tr(.49) tr(.43) 6. nd 1.3 [.43] 46/9 12/18 H22 nd nd nd nd 24 [1] /18 /18 H23 nd nd 3 nd 3 [1] 5/18 5/18 H27 nd nd nd nd 14 [5] /19 /19 363

[] H21 1.6 1.6 2.1 tr(1.2) 1.3 [.43] 1/1 2/2 H22 nd --- nd nd 24 [1] /2 /2 H23 --- --- 3 3 3 [1] 1/1 1/1 H27 --- --- nd nd 14 [5] /1 /1 1 21 2 21 22 [][] 3 27 23 4 24 26 22 27 [] H22 nd nd nd nd /37 /37.3 [.1] H22 nd nd nd nd /37 /37 (pg/m 3 H23 nd nd nd nd /35 /35 ).3 [.1] H23 nd nd nd nd /37 /37 H27 nd nd 1.1 nd.6 [.2] 2/35 2/35 24 26 364

[14] 4 1 21 5 POPs 4 COP4 22 4 29 4 5 POPs 8 COP8 2 13 52 1 62 63 6 8 1 8 1 13 1 7 14 14 1 15 6 8 1 16 5 1 7 17 1 2 3 4 5 6 7 9 1 14 4 1 2 21 22 24 26 29 47 3 pg/l 47 44 12 pg/l 47 1 pg/l 47 24 8 pg/l 21 29 47 3 pg/l 47 1 tr(6)pg/l 47 5 pg/l 47 1 3 pg/l 47 1 pg/l 47 22 33 pg/l 47 3 pg/l 47 365

37 46 pg/l 47 8 pg/l 47 46 4,1 pg/l 21 29 4 1 [] H21 17 16 16 nd 8 [3] 44/49 44/49 H22 nd nd 39 nd 9 [3] 17/49 17/49 H23 11 1 18 nd 4 [2] 48/49 48/49 H24 tr(3) tr(3) 22 nd 4 [1] 47/48 47/48 (pg/l) H26 tr(6) tr(6) 51 tr(4) 8 [3] 48/48 48/48 H27 4.3 4.1 4 tr(1.2) 3.6 [1.2] 48/48 48/48 H28 5 tr(5) 47 tr(3) 5 [2] 48/48 48/48 H29 tr(4) tr(4) 12 nd 9 [3] 44/47 44/47 (pg/l) (pg/l) (pg/l) (pg/l) (pg/l) [] H21 11 12 87 nd 11 [4] 43/49 43/49 H22 tr(1) tr(1) 13 nd 3 [1] 25/49 25/49 H23 5 4 18 nd 3 [1] 48/49 48/49 H24 tr(1) tr(1) 2 nd 2 [1] 32/48 32/48 H26 nd nd 39 nd 4 [2] 19/48 19/48 H27 tr(3.) tr(3.2) 31 nd 6.3 [2.1] 34/48 34/48 H28 tr(1.5) tr(1.3) 36 nd 2.4 [.9] 39/48 39/48 H29 nd tr(1) 8 nd 3 [1] 24/47 24/47 [] H21 tr(.9) tr(.7) 18 nd 1.4 [.6] 26/49 26/49 H22 nd nd 51 nd 4 [2] 16/49 16/49 H23 tr(1) nd 39 nd 3 [1] 21/49 21/49 H24 nd nd 7 nd 3 [1] 6/48 6/48 H26 nd nd 8 nd 4 [1] 1/48 1/48 H27 nd nd 12 nd 1.5 [.6] 5/48 5/48 H28 nd nd 9.1 nd 2.1 [.8] 9/48 9/48 H29 nd nd tr(6) nd 7 [3] 1/47 1/47 [] H21 nd nd 4 nd 4 [2] 9/49 9/49 H22 nd nd 14 nd 3 [1] 17/49 17/49 H23 nd nd 14 nd 6 [2] 14/49 14/49 H24 nd nd 1 nd 4 [1] 9/48 9/48 H26 nd nd 8 nd 8 [3] 3/48 3/48 H27 nd nd 28 nd 2. [.8] 9/48 9/48 H28 nd nd 11 nd 7 [3] 1/48 1/48 H29 nd nd 3 nd 14 [5] 1/47 1/47 [] H21 3. 3.9 56 nd 1.4 [.6] 37/49 37/49 H22 tr(2) tr(2) 69 nd 3 [1] 4/49 4/49 H23 4 3 98 nd 2 [1] 44/49 44/49 H24 tr(2) nd 35 nd 4 [2] 16/48 16/48 H26 2.5 3.7 38 nd 1.6 [.6] 33/48 33/48 H27 2.3 3.1 36 nd 1.5 [.6] 31/48 31/48 H28 5.8 7.5 23 nd.8 [.3] 44/48 44/48 H29 tr(2) nd 33 nd 2 [1] 22/47 22/47 [] H21 tr(46) tr(38) 5 nd 91 [3] 32/49 32/49 H22 tr(17) tr(13) 62 nd 21 [7] 39/49 39/49 H23 33 24 92 nd 1 [4] 47/49 47/49 H24 tr(21) tr(19) 32 nd 4 [13] 3/48 3/48 H26 37 38 59 nd 6 [2] 47/48 47/48 H27 36 33 33 nd 6 [2] 47/48 47/48 H28 43 45 3,9 tr(2) 4 [1] 48/48 48/48 H29 17 26 46 nd 7 [3] 37/47 37/47 366

[] H21 tr(31) tr(22) 3,4 nd 6 [2] 26/49 26/49 H22 tr(25) tr(2) 13, nd 3 [1] 31/49 31/49 H23 2 14 58, nd 6 [2] 45/49 45/49 H24 tr(4) tr(32) 12, nd 66 [22] 31/48 31/48 (pg/l) H26 2 23 5,6 tr(14) 22 [9] 48/48 48/48 H27 72 57 13, 14 18 [7] 48/48 48/48 H28 21 16 34, tr(12) 14 [6] 48/48 48/48 H29 15 21 4,1 nd 24 [8] 46/47 46/47 25 62 4 pg/g-dry 62 44 57 pg/g-dry 21 29 5 62 4 pg/g-dry 62 37 56 pg/g-dry 62 2 pg/g-dry 62 44 57 pg/g-dry 21 29 5 62 6 pg/g-dry 62 36 58 pg/g-dry 62 2 pg/g-dry 62 48 1,9 pg/g-dry 21 29 5 62 5 pg/g-dry 62 61 29, pg/g-dry 21 29 5 62 1 pg/g-dry 62 tr(27) 58,pg/g-dry 21 29 4 1 [] H21 tr(6) tr(44) 1,4 nd 69 [23] 131/192 51/64 H22 35 38 91 nd 6 [2] 57/64 57/64 H23 32 3 2,6 nd 3 [1] 47/64 47/64 H24 27 37 4,5 nd 2 [1] 6/63 6/63 (pg/g-dry) H26 tr(24) tr(19) 55 nd 27 [9] 44/63 44/63 H27 3 28 1,4 nd 21 [7] 44/62 44/62 H28 tr(21) tr(16) 39 nd 33 [11] 35/62 35/62 H29 13 1 57 nd 9 [4] 44/62 44/62 367

[] H21 36 24 1,7 nd 24 [8] 146/192 57/64 H22 26 23 74 nd 5 [2] 58/64 58/64 H23 24 18 4,7 nd 5 [2] 62/64 62/64 H24 21 21 2,9 nd 2.4 [.9] 62/63 62/63 (pg/g-dry) H26 16 14 57 nd 6 [2] 53/63 53/63 H27 23 2 1,3 nd 18 [6] 44/62 44/62 H28 13 tr(1) 4 nd 12 [4] 46/62 46/62 H29 1 tr(5.5) 56 nd 9 [4] 37/62 37/62 [] H21 21 21 2,6 nd 5 [2] 139/192 53/64 H22 23 23 77 nd 4 [2] 57/64 57/64 H23 31 42 2, nd 9 [3] 52/64 52/64 H24 15 19 1,7 nd 3 [1] 48/63 48/63 (pg/g-dry) H26 21 27 73 nd 5 [2] 5/63 5/63 H27 11 15 82 nd 3 [1] 42/62 42/62 H28 17 19 6 nd 8 [3] 4/62 4/62 H29 16 24 57 nd 6 [2] 44/62 44/62 [] H21 3 25 16, nd 9 [4] 125/192 51/64 H22 28 18 93 nd 4 [2] 58/64 58/64 H23 29 32 2,4 nd 7 [3] 55/64 55/64 H24 34 32 4,4 nd 4 [2] 48/63 48/63 (pg/g-dry) H26 19 tr(14) 68 nd 16 [6] 41/63 41/63 H27 16 21 1,8 nd 3 [1] 44/62 44/62 H28 16 17 1,1 nd 6 [2] 44/62 44/62 H29 18 16 58 nd 15 [6] 36/62 36/62 [] H21 21 96 11, nd 1.2 [.5] 182/192 63/64 H22 71 76 1,8 nd 1 [4] 6/64 6/64 H23 57 64 36, nd 1 [4] 55/64 55/64 H24 78 74 15, nd 19 [6] 47/63 47/63 (pg/g-dry) H26 52 58 2, nd 12 [4] 55/63 55/63 H27 58 tr(44) 1,4 nd 48 [16] 41/62 41/62 H28 51 49 1,4 nd 6 [2] 55/62 55/62 H29 38 58 1,9 nd 5 [2] 48/62 48/62 [] H21 1,1 71 23, nd 9 [4] 181/192 64/64 H22 36 43 26, nd 24 [9] 6/64 6/64 H23 71 63 7, nd 23 [9] 62/64 62/64 H24 36 38 84, nd 34 [11] 52/63 52/63 (pg/g-dry) H26 47 47 42, nd 6 [2] 6/63 6/63 H27 3 42 11, nd 24 [8] 55/62 55/62 H28 43 39 26, nd 27 [9] 6/62 6/62 H29 4 49 29, nd 15 [5] 61/62 61/62 [] H21 6, 4,8 88, tr(3) 6 [2] 192/192 64/64 H22 5,1 4,2 7, nd 22 [8] 6/64 6/64 H23 4,2 4,7 7, nd 4 [2] 62/64 62/64 H24 5,7 6,3 76, nd 27 [89] 6/63 6/63 (pg/g-dry) H26 5,6 5, 98, nd 24 [8] 61/63 61/63 H27 6,6 7,2 49, 4 4 [2] 62/62 62/62 H28 4,7 5,1 94, nd 12 [41] 61/62 61/62 H29 4,6 5,7 58, tr(27) 3 [1] 62/62 62/62 1 21 2 25 3 6 pg/gwet 3 23 2pg/g-wet 19 6 pg/g-wet 19 tr(7) 36pg/g-wet 2 6 pg/g-wet 2 26 66pg/g-wet 2 29 368

3 5 pg/gwet 3 tr(6) 62pg/g-wet 19 5 pg/g-wet 19 18 87pg/g-wet 2 5 pg/g-wet 2 12 5pg/g-wet 3 7 pg/gwet 3 2 36pg/g-wet 19 7 pg/g-wet 19 18 21pg/g-wet 2 7 pg/g-wet 2 51 1,pg/g-wet 3 8 pg/gwet 3 1 tr(9)pg/g-wet 19 8 pg/g-wet 19 1 55pg/g-wet 2 8 pg/g-wet 2 tr(18) 44pg/g-wet 3 8 pg/gwet 3 1 tr(9)pg/g-wet 19 8 pg/g-wet 19 9 88pg/g-wet 2 8 pg/g-wet 2 25 72pg/g-wet 3 2 pg/g-wet 3 19 2 pg/g-wet 19 1 68pg/g-wet 2 2 pg/g-wet 2 3 8 pg/g-wet 3 1 tr(18)pg/g-wet 19 8 pg/g-wet 19 1 2,1pg/g-wet 2 8 pg/g-wet 2 2 29 4 1 [] H2 73 61 38 2 5.9 [2.2] 31/31 7/7 H22 59 73 31 nd 43 [16] 5/6 5/6 H23 96 12 49 26 16 [6] 4/4 4/4 H24 59 44 19 24 19 [7] 5/5 5/5 H26 56 38 14 33 15 [6] 3/3 3/3 H27 48 38 89 32 15 [6] 3/3 3/3 H28 42 32 98 23 13 [5] 3/3 3/3 H29 47 23 2 23 16 [6] 3/3 3/3 369

[] H2 12 11 1,3 9.8 5.9 [2.2] 85/85 17/17 H22 16 17 74 tr(16) 43 [16] 18/18 18/18 H23 11 11 86 tr(9) 16 [6] 18/18 18/18 H24 12 14 65 tr(1) 19 [7] 19/19 19/19 H26 15 16 1,3 18 15 [6] 19/19 19/19 H27 9 82 58 tr(14) 15 [6] 19/19 19/19 H28 76 53 39 tr(1) 13 [5] 19/19 19/19 H29 8 73 36 tr(7) 16 [6] 19/19 19/19 H2 17 19 1,2 32 5.9 [2.2] 1/1 2/2 H22 14 --- 27 72 43 [16] 2/2 2/2 H23 --- --- 67 67 16 [6] 1/1 1/1 H24 73 --- 11 49 19 [7] 2/2 2/2 H26 19 --- 48 78 15 [6] 2/2 2/2 H27 --- --- 36 36 15 [6] 1/1 1/1 H28 17 --- 47 62 13 [5] 2/2 2/2 H29 13 --- 66 26 16 [6] 2/2 2/2 [] H2 32 27 94 tr(11) 16 [5.9] 31/31 7/7 H22 32 37 98 tr(9) 14 [6] 6/6 6/6 H23 51 6 16 tr(12) 15 [6] 4/4 4/4 H24 28 24 67 tr(8) 18 [6] 5/5 5/5 H26 3 37 41 18 12 [5] 3/3 3/3 H27 18 19 2 16 13 [5] 3/3 3/3 H28 11 9 2 tr(8) 9 [4] 3/3 3/3 H29 18 16 62 tr(6) 12 [5] 3/3 3/3 H2 3 37 28 nd 16 [5.9] 72/85 16/17 H22 51 54 2 nd 14 [6] 16/18 16/18 H23 39 39 3 nd 15 [6] 17/18 17/18 H24 37 54 18 nd 18 [6] 17/19 17/19 H26 41 47 57 nd 12 [5] 18/19 18/19 H27 22 17 14 nd 13 [5] 18/19 18/19 H28 18 14 87 tr(4) 9 [4] 19/19 19/19 H29 23 28 87 nd 12 [5] 18/19 18/19 H2 15 13 44 52 16 [5.9] 1/1 2/2 H22 15 --- 2 12 14 [6] 2/2 2/2 H23 --- --- 11 11 15 [6] 1/1 1/1 H24 85 --- 11 66 18 [6] 2/2 2/2 H26 1 --- 32 31 12 [5] 2/2 2/2 H27 --- --- 22 22 13 [5] 1/1 1/1 H28 88 --- 3 26 9 [4] 2/2 2/2 H29 77 --- 5 12 12 [5] 2/2 2/2 [] H2 19 16 82 tr(5.3) 14 [5.] 31/31 7/7 H22 8 16 26 nd 8 [3] 4/6 4/6 H23 38 41 81 2 1 [4] 4/4 4/4 H24 21 23 13 tr(6) 1 [4] 5/5 5/5 H26 23 21 52 11 1 [4] 3/3 3/3 H27 tr(9) tr(6) 41 nd 12 [5] 2/3 2/3 H28 tr(13) tr(13) 4 nd 21 [8] 2/3 2/3 H29 tr(14) 2 36 nd 17 [7] 2/3 2/3 H2 46 51 31 nd 14 [5.] 83/85 17/17 H22 39 47 4 nd 8 [3] 16/18 16/18 H23 53 5 43 nd 1 [4] 17/18 17/18 H24 55 71 32 nd 1 [4] 18/19 18/19 H26 6 61 1,1 nd 1 [4] 18/19 18/19 H27 44 45 25 nd 12 [5] 18/19 18/19 H28 42 36 19 nd 21 [8] 18/19 18/19 H29 49 49 21 nd 17 [7] 18/19 18/19 H2 14 12 38 62 14 [5.] 1/1 2/2 H22 11 --- 14 86 8 [3] 2/2 2/2 H23 --- --- 96 96 1 [4] 1/1 1/1 H24 15 --- 32 72 1 [4] 2/2 2/2 H26 17 --- 68 42 1 [4] 2/2 2/2 H27 --- --- 3 3 12 [5] 1/1 1/1 H28 22 --- 74 68 21 [8] 2/2 2/2 H29 23 --- 1, 51 17 [7] 2/2 2/2 37

[] H2 tr(8.5) tr(7.6) 35 nd 18 [6.7] 2/31 7/7 H22 nd nd tr(1) nd 3 [1] 1/6 1/6 H23 14 26 44 nd 11 [4] 3/4 3/4 H24 tr(8) tr(6) 59 nd 12 [5] 3/5 3/5 H26 nd nd 13 nd 12 [5] 1/3 1/3 H27 nd nd tr(11) nd 12 [5] 1/3 1/3 H28 nd nd tr(8) nd 13 [5] 1/3 1/3 H29 nd nd tr(9) nd 22 [8] 1/3 1/3 H2 tr(11) tr(8.1) 77 nd 18 [6.7] 44/85 1/17 H22 nd nd 4 nd 3 [1] 4/18 4/18 H23 13 21 13 nd 11 [4] 13/18 13/18 H24 tr(11) 18 12 nd 12 [5] 11/19 11/19 H26 tr(1) 13 28 nd 12 [5] 1/19 1/19 H27 nd nd 44 nd 12 [5] 4/19 4/19 H28 tr(9) tr(7) 85 nd 13 [5] 11/19 11/19 H29 tr(11) tr(12) 55 nd 22 [8] 1/19 1/19 H2 35 35 53 19 18 [6.7] 1/1 2/2 H22 tr(19) --- 7 nd 3 [1] 1/2 1/2 H23 --- --- 44 44 11 [4] 1/1 1/1 H24 63 --- 28 14 12 [5] 2/2 2/2 H26 19 --- 15 nd 12 [5] 1/2 1/2 H27 --- --- tr(11) tr(11) 12 [5] 1/1 1/1 H28 65 --- 22 19 13 [5] 2/2 2/2 H29 89 --- 44 tr(18) 22 [8] 2/2 2/2 [] H2 nd nd 1 nd 9.6 [3.6] 15/31 6/7 H22 nd nd tr(1) nd 11 [4] 2/6 2/6 H23 7 9 29 nd 7 [3] 3/4 3/4 H24 8 tr(7) 25 nd 8 [3] 4/5 4/5 H26 tr(9.2) 11 14 tr(5) 11 [4] 3/3 3/3 H27 nd nd nd nd 14 [5] /3 /3 H28 nd nd nd nd 16 [6] /3 /3 H29 nd nd tr(9) nd 2 [8] 1/3 1/3 H2 tr(5.7) nd 73 nd 9.6 [3.6] 35/85 7/17 H22 tr(6) nd 1 nd 11 [4] 8/18 8/18 H23 tr(6) tr(7) 15 nd 7 [3] 1/18 1/18 H24 tr(7) 8 16 nd 8 [3] 12/19 12/19 H26 14 13 54 nd 11 [4] 15/19 15/19 H27 tr(7) nd 6 nd 14 [5] 9/19 9/19 H28 tr(8) nd 86 nd 16 [6] 9/19 9/19 H29 tr(9.7) nd 88 nd 2 [8] 9/19 9/19 H2 42 41 64 3 9.6 [3.6] 1/1 2/2 H22 41 --- 65 26 11 [4] 2/2 2/2 H23 --- --- 66 66 7 [3] 1/1 1/1 H24 13 --- 42 4 8 [3] 2/2 2/2 H26 17 --- 14 nd 11 [4] 1/2 1/2 H27 --- --- tr(5) tr(5) 14 [5] 1/1 1/1 H28 65 --- 22 19 16 [6] 2/2 2/2 H29 13 37 72 25 2 [8] 2/2 2/2 [] H2 nd nd tr(23) nd 35 [13] 5/31 1/7 H22 tr(16) tr(15) 6 nd 3 [1] 5/6 5/6 H23 tr(12) tr(11) 4 nd 22 [9] 3/4 3/4 H24 tr(15) 25 45 nd 24 [9] 3/5 3/5 H26 4 tr(2) 11 tr(2) 3 [1] 3/3 3/3 H27 nd nd tr(11) nd 23 [9] 1/3 1/3 H28 nd nd nd nd 36 [14] /3 /3 H29 nd nd nd nd 5 [2] /3 /3 H2 nd nd tr(15) nd 35 [13] 2/85 2/17 H22 nd nd 4 nd 3 [1] 3/18 3/18 H23 nd nd tr(15) nd 22 [9] 5/18 5/18 H24 nd nd 54 nd 24 [9] 9/19 9/19 H26 tr(1) tr(2) 4 nd 3 [1] 16/19 16/19 H27 nd nd 35 nd 23 [9] 6/19 6/19 H28 nd nd tr(22) nd 36 [14] 3/19 3/19 H29 nd nd 68 nd 5 [2] 1/19 1/19 371

[] H2 tr(21) tr(2) tr(33) nd 35 [13] 9/1 2/2 H22 32 --- 5 tr(2) 3 [1] 2/2 2/2 H23 --- --- 62 62 22 [9] 1/1 1/1 H24 1 --- 15 67 24 [9] 2/2 2/2 H26 tr(1) --- tr(2) tr(1) 3 [1] 2/2 2/2 H27 --- --- tr(12) tr(12) 23 [9] 1/1 1/1 H28 nd --- tr(21) nd 36 [14] 1/2 1/2 H29 nd --- nd nd 5 [2] /2 /2 [] H2 nd nd tr(17) nd 22 [74] 8/31 3/7 H22 nd nd tr(19) nd 27 [97] 2/6 2/6 H23 nd nd 24 nd 23 [8] 1/4 1/4 H24 12 17 48 nd 12 [5] 4/5 4/5 H26 22 tr(15) 57 tr(12) 17 [6] 3/3 3/3 H27 nd nd tr(7) nd 17 [7] 1/3 1/3 H28 nd nd tr(11) nd 3 [1] 1/3 1/3 H29 nd nd tr(18) nd 21 [8] 1/3 1/3 H2 nd nd 23 nd 22 [74] 5/76 4/16 H22 nd nd tr(15) nd 27 [97] 2/18 2/18 H23 nd nd tr(9) nd 23 [8] 2/18 2/18 H24 tr(59) tr(6) 38 nd 12 [5] 11/19 11/19 H26 tr(75) tr(7) 3 nd 17 [6] 13/19 13/19 H27 nd nd 38 nd 17 [7] 5/19 5/19 H28 nd nd tr(19) nd 3 [1] 7/19 7/19 H29 nd nd 2,1 nd 21 [8] 1/19 1/19 H2 nd nd tr(11) nd 22 [74] 4/1 1/2 H22 nd --- nd nd 27 [97] /2 /2 H23 --- --- tr(17) tr(17) 23 [8] 1/1 1/1 H24 25 --- 26 24 12 [5] 2/2 2/2 H26 tr(65) --- tr(14) nd 17 [6] 1/2 1/2 H27 --- --- tr(9) tr(9) 17 [7] 1/1 1/1 H28 nd --- nd nd 3 [1] /2 /2 H29 nd --- nd nd 21 [8 ] /2 /2 1 2 2 26 24 3 21 25 37.5 pg/m 3 37.6 4.1pg/m 3 21 29 37.4 pg/m 3 37 33 3.4pg/m 3 37.1 pg/m 3 37 11 2.1pg/m 3 37.2 pg/m 3 37 1 3.2pg/m 3 37.7 pg/m 3 37 28 5.7pg/m 3 37.2 pg/m 3 37 31 4pg/m 3 37.8 pg/m 3 37 34 14pg/m 3 372

21 29 4 1 [] H21.89.8 18.11.11 [.4] H21.4.37 7.1 tr(.4) H22.79.57 5.15.12 [.5] H22.4.35 25 tr(.9) H23.8.72 9.3 tr(.11) 35/35 35/35.18 [.7] H23.36.34 7. nd 35/37 35/37 (pg/m 3 ) H24.7.7 5.7 nd 35/36 35/36.3 [.1] H24 tr(.2) tr(.2) 1.7 nd 25/36 25/36 H26.53.47 2.3 tr(.9).28 [.9] 36/36 36/36 H27 tr(.3) tr(.3) 2.7 nd.4 [.1] 3/35 3/35 H28.5.4 28 nd.4 [.2] 3/37 3/37 H29.39.34 4.1 tr(.6).15 [.5] [] H21.2.19 18 nd 33/37 33/37.16 [.6] H21.19.16 1 nd 29/37 29/37 H22.2.17 45 nd 35/37 35/37.12 [.5] H22.2.22 28 nd 34/37 34/37 H23.19.17 8.8 nd 31/35 31/35.16 [.6] H23.16 tr(.14) 2.6 nd 31/37 31/37 (pg/m 3 ) H24 tr(.13) tr(.12) 2.4 nd 3/36 3/36.14 [.6] H24 tr(.9) tr(.9).77 nd 26/36 26/36 H26 tr(.13) tr(.14).8 nd.28 [.9] 25/36 25/36 H27 nd nd.9 nd.6 [.2] 6/35 6/35 H28 nd nd 28 nd.4 [.2] 6/37 6/37 H29.11.1 3.4 nd.1 [.4] 33/37 33/37 [] H21 tr(.11) tr(.11) 2. nd 19/37 19/37.22 [.9] H21 tr(.2).22 27 nd 24/37 24/37 H22 tr(.14) tr(.13) 4.9 nd 29/37 29/37.16 [.6] H22.24.27 5.4 nd 31/37 31/37 H23 tr(.11) tr(.1) 1.2 nd 28/35 28/35.14 [.5] H23.16.18 1.7 nd 3/37 3/37 (pg/m 3 ) H24 nd nd 3.1 nd 9/36 9/36.3 [.1] H24 tr(.1) tr(.1).5 nd 22/36 22/36 H26 nd nd.4 nd.4 [.1] 5/36 5/36 H27 nd nd 2. nd 1.1 [.4] 3/35 3/35 H28 nd nd 2.7 nd.6 [.2] 3/37 3/37 H29 nd nd 2.1 nd.3 [.1] 11/37 11/37 [] H21 tr(.1) nd 1.7 nd 17/37 17/37.3 [.1] H21 tr(.2).3 2 nd 25/37 25/37 H22 tr(.2) tr(.1) 1.4 nd 24/37 24/37.3 [.1] H22.3.4 11 nd 28/37 28/37 H23 tr(.1) tr(.1) 1.1 nd 2/35 2/35.3 [.1] H23 tr(.2) tr(.2) 2.3 nd 25/37 25/37 (pg/m 3 ) H24 nd nd 1.8 nd 6/36 6/36.5 [.2] H24 nd nd.7 nd 8/36 8/36 H26 nd nd tr(.4) nd.7 [.2] 2/36 2/36 H27 nd nd tr(.6) nd 1.3 [.4] 2/35 2/35 H28 nd nd 1.3 nd 1.1 [.4] 1/37 1/37 H29 nd nd 3.2 nd.4 [.2] 1/37 1/37 [] H21 tr(.2).3 1.6 nd 23/37 23/37.3 [.1] H21.3.4 7.1 nd 26/37 26/37 H22.25.3 2.3 nd 3/37 3/37.15 [.6] H22.4.52 6.9 nd 32/37 32/37 H23.24.31 1.9 nd 27/35 27/35.2 [.8] H23.35.44 7. nd 3/37 3/37 (pg/m 3 ) H24 tr(.2) tr(.2) 1.2 nd 29/36 29/36.3 [.1] H24.3.4 1.2 nd 3/36 3/36 H26 tr(.1) tr(.1).7 nd.4 [.1] 22/36 22/36 H27 nd nd 3.8 nd 1.1 [.4] 9/35 9/35 H28 nd nd 1.6 nd.6 [.2] 18/37 18/37 H29 tr(.19).23 5.7 nd.21 [.7] 28/37 28/37 25 373

(pg/m 3 ) [] H21 tr(.7) tr(.7) 3. nd 22/37 22/37 1.8 [.6] H21 tr(1.) tr(.8) 3.9 nd 27/37 27/37 H22 nd nd 24 nd 12/37 12/37 3.7 [1.2] H22 tr(1.2) tr(1.3) 7.1 nd 22/37 22/37 H23 tr(.8).9 3.9 nd 29/35 29/35.9 [.4] H23 1.1 1.1 14 nd 3/37 3/37 H24 tr(.5) tr(.5) 5.1 nd 24/36 24/36 1.2 [.4] H24 tr(.9) tr(1.1) 4.7 nd 3/36 3/36 H26 nd nd tr(3) nd 4 [1] 7/36 7/36 H27 nd nd 12 nd 3.2 [1.1] 14/35 14/35 H28 tr(.9) tr(.9) 11 nd 1.4 [.5] 28/37 28/37 H29.8.8 4 nd.6 [.2] 31/37 31/37 [] H21 tr(7) tr(9) 31 nd 28/37 28/37 16 [5] H21 tr(1) tr(11) 45 nd 29/37 29/37 H22 nd nd 29 nd 1/37 1/37 27 [9.1] H22 tr(11) tr(12) 88 nd 21/37 21/37 H23 tr(8.2) tr(9.) 3 nd 31/35 31/35 12 [4.] H23 tr(8.4) tr(9.) 44 nd 29/37 29/37 (pg/m 3 ) H24 nd nd 31 nd 17/36 17/36 16 [5] H24 tr(1) tr(12) 73 nd 28/36 28/36 H26 tr(4.7) tr(5.) 64 nd 9 [3] 24/36 24/36 H27 4.2 4.3 61 nd 2.2 [.7] 3/35 3/35 H28 5 5 86 nd 3 [1] 35/37 35/37 H29 4.2 4.4 14 nd 2.4 [.8] 34/37 34/37 25 374

[14-1] 2 15 [](pg/l) 21 8[3] 22 9[3] 23 4 [2] 24 4 [1] 26 8 [3] 27 3.6 [1.2] 28 5 [2] (pg/l) 1 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 22 1/2 3-14-1-1 [14-1] (pg/g-dry) 7 6 5 4 3 [](pg/g-dry) 21 69 [23] 22 6[2] 23 3 [1] 24 2 [1] 26 27 [9] 27 21 [7] 28 33 [11] 29 9 [4] 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-1-2 375

[14-1] 2 15 1 [] 2 5.9 [2.2] 22 43 [16] 23 16 [6] 24 19 [7] 26 15 [6] 27 15 [6] 28 13 [5] 29 16 [6] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 26 24 2 21 25 3-14-1-3 [14-1] 1 pg/m 3.8.6.4 [] (pg/m 3 ) 21.11 [.4] 22.12 [.5] 23.18 [.7] 24.3 [.1] 26.28 [.9] 27.4 [.1] 28.4 [.2] 29.15 [.5].2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-1-4 376

[14-2] 12 1 8 [](pg/l) 21 11 [4] 22 3[1] 23 3 [1] 24 2 [1] 26 4 [2] 27 6.3 [2.1] 28 2.4 [.9] 29 3 [1] (pg/l) 6 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 26 1/2 3-14-2-1 [14-2] (pg/g-dry) 4 3 2 [](pg/g-dry) 21 24 [8] 22 5[2] 23 5 [2] 24 2.4 [.9] 26 6 [2] 27 18 [6] 28 12 [4] 29 9 [4] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-2-2 377

[14-2] 6 5 4 3 2 [] 2 16 [5.9] 22 14 [6] 23 15 [6] 24 18 [6] 26 12 [5] 27 13 [5] 28 9 [4] 29 12 [5] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 26 24 2 21 25 3-14-2-3 [14-2].25 pg/m 3.2.15.1 [] (pg/m 3 ) 21.16 [.6] 22.12 [.5] 23.16 [.6] 24.14 [.6] 26.28 [.9] 27.6 [.2] 28.4 [.2] 29.15 [.5].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 27 29 1/2 3-14-2-4 378

[14-3] (pg/g-dry) 4 3 2 [](pg/g-dry) 21 5 [2] 22 4[2] 23 9 [3] 24 3 [1] 26 5 [2] 27 3 [1] 28 8 [3] 29 6 [2] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-3-1 [14-3] 7 6 5 4 3 [] 2 14 [5.] 22 8[3] 23 1 [4] 24 1 [4] 26 1 [4] 27 12 [5] 28 21 [8] 29 17 [7] 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 26 24 2 21 25 3-14-3-2 379

[14-4] (pg/g-dry) 4 3 2 [](pg/g-dry) 21 9 [4] 22 4[2] 23 7 [3] 24 4 [2] 26 16 [6] 27 3 [1] 28 6 [2] 29 15 [6] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-4-1 [14-5] 6 5 4 [](pg/l) 21 1.4 [.6] 22 3[1] 23 2 [1] 24 4 [2] 26 1.6 [.6] 27 1.5 [.6] 28.8 [.3] 29 2 [1] (pg/l) 3 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-5-1 38

[14-5] (pg/g-dry) 25 2 15 1 [](pg/g-dry) 21 1.2 [.5] 22 1 [4] 23 1 [4] 24 19 [6] 26 12 [4] 27 48 [16] 28 6 [2] 29 5 [2] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-5-2 [14-5] 16 12 8 [] 2 9.6 [3.6] 22 11 [4] 23 7 [3] 24 8 [3] 26 11 [4] 27 14 [5] 28 16 [6] 29 2 [8] 4 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 2 26 24 3 21 25 3-14-5-3 381

[14-5].5 pg/m 3.4.3.2 [] (pg/m 3 ) 21.3 [.1] 22.15 [.6] 23.2 [.8] 24.3 [.1] 26.4 [.1] 27 1.1 [.4] 28.6 [.2] 29.21 [.7].1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 27 28 1/2 3-14-5-4 [14-6] 5 4 3 [](pg/l) 21 91 [3] 22 21 [7] 23 1 [4] 24 4 [13] 26 6 [2] 27 6 [2] 28 4 [1] 29 7 [3] (pg/l) 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-6-1 382

[14-6] (pg/g-dry) 1,2 1, 8 6 [](pg/g-dry) 21 9 [4] 22 24 [9] 23 23 [9] 24 34 [11] 26 6 [2] 27 24 [8] 28 27 [9] 29 15 [5] 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-6-2 [14-6] 1.4 pg/m 3 1.2 1.8.6 [] (pg/m 3 ) 21 1.8 [.6] 22 3.7 [1.2] 23.9 [.4] 24 1.2 [.4] 26 4 [1] 27 3.2 [1.1] 28 1.4 [.5] 29.6 [.2].4.2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 22 26 27 1/2 3-14-6-3 383

[14-7] 8 6 [](pg/l) 21 6 [2] 22 3 [1] 23 6 [2] 24 66 [22] 26 22 [9] 27 18 [7] 28 14 [6] 29 24 [8] (pg/l) 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-7-1 [14-7] (pg/g-dry) 8, 6, 4, [](pg/g-dry) 21 6 [2] 22 22 [8] 23 4 [2] 24 27 [89] 26 24 [8] 27 4 [2] 28 12 [41] 29 3 [1] 2, 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-14-7-2 384

[14-7] pg/m 3 12 1 8 6 4 [] (pg/m 3 ) 21 16 [5] 22 27 [9.1] 23 12 [4.] 24 16 [5] 26 9 [3] 27 2.2 [.7] 28 3 [1] 29 2.4 [.8] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 22 24 1/2 3-14-7-3 385

[15] PFOS PFOS 21 5 POPs 4 COP4 22 4 ( -1-) ( -1-) 21 14 14 15 16 17 14 ( -1- ) 21 22 24 25 26 28 29 3 4 pg/g-wet 3 2 16pg/g-wet 19 4 pg/gwet 19 tr(4) 11,pg/g-wet 2 4 pg/g-wet 2 3, 32,pg/g-wet 21 29 PFOS [] PFOS H21 24 28 64 nd 19 [7.4] 17/31 5/7 H22 72 85 68 nd 25 [9.6] 5/6 5/6 H23 38 44 1 16 1 [4] 4/4 4/4 H24 27 21 16 tr(4) 7 [3] 5/5 5/5 H26 8 6 93 nd 5 [2] 2/3 2/3 H27 7 tr(2) 21 nd 4 [2] 2/3 2/3 H28 11 tr(6) 16 nd 9 [3] 2/3 2/3 H29 22 34 16 nd 12 [4] 2/3 2/3 H21 22 23 15, nd 19 [7.4] 83/9 17/18 H22 39 48 15, nd 25 [9.6] 17/18 17/18 H23 82 95 3,2 nd 1 [4] 16/18 16/18 H24 11 13 7,3 tr(5) 7 [3] 19/19 19/19 H26 82 83 4,6 nd 5 [2] 18/19 18/19 H27 91 9 2,5 nd 4 [2] 18/19 18/19 H28 79 8 5,2 nd 9 [3] 18/19 18/19 H29 15 15 11, tr(4) 12 [4] 19/19 19/19 386

PFOS [] H21 3 36 89 37 19 [7.4] 1/1 2/2 H22 1,3 --- 3, 58 25 [9.6] 2/2 2/2 H23 --- --- 11 11 1 [4] 1/1 1/1 H24 16 --- 41 63 7 [3] 2/2 2/2 H26 4,6 --- 11, 19 5 [2] 2/2 2/2 H27 --- --- 79 79 4 [2] 1/1 1/1 H28 3,6 --- 9,1 1,4 9 [3] 2/2 2/2 H29 9,8 --- 32, 3, 12 [4] 2/2 2/2 1 21 2 26 24 3 25 37.1 pg/m 3 37 1.1 8.9pg/m 3 22 29 22 29 PFOS [] PFOS H22 5.2 5.9 14 1.6.4 [.1] H22 4.7 4.4 15 1.4 H23 4.4 4.2 1.9 35/35 35/35.5 [.2] H23 3.7 3.8 9.5 1.3 H24 3.6 3.8 8.9 1.3 36/36 36/36 (pg/m 3 ) H24 2.7 3. 5.9 1..5 [.2] 36/36 36/36 H25 4.6 5.2 9.6 1.2 36/36 36/36.3 [.1] H25 3.7 3.9 7.4 1.6 36/36 36/36 H26 3.1 3.2 8.6.52.17 [.6] 36/36 36/36 H27 2.8 2.6 8.8.59.19 [.6] 35/35 35/35 H28 3.1 2.4 9.3.7.6 [.2] H29 2.9 2.7 8.9 1.1.3 [.1] 387

28 21 28 PFOS [] PFOS (pg/l) 25 H21 73 58 14, tr(26) 37 [14] 49/49 49/49 H22 49 38 23, tr(37) 5 [2] 49/49 49/49 H23 48 36 1, tr(2) 5 [2] 49/49 49/49 H24 55 51 14, 39 31 [12] 48/48 48/48 H26 46 41 7,5 nd 5 [2] 47/48 47/48 H27 63 49 4,7 12 29 [11] 48/48 48/48 H28 33 3 14, tr(23) 5 [2] 48/48 48/48 21 28 PFOS [] PFOS (pg/g-dry) H21 78 97 1,9 nd 9.6 [3.7] 18/19 64/64 H22 82 1 1,7 tr(3) 5 [2] 64/64 64/64 H23 92 11 1,1 nd 5 [2] 63/64 63/64 H24 68 84 1,2 tr(7) 9 [4] 63/63 63/63 H26 59 79 98 nd 5 [2] 62/63 62/63 H27 91 88 2,2 7 3 [1] 62/62 62/62 H28 54 61 69 5 5 [2] 62/62 62/62 1 21 2 25 388

[15] PFOS 5 4 3 2 [] 21 19 [7.4] 22 25 [9.6] 23 1 [4] 24 7 [3] 26 5 [2] 27 4 [2] 28 9 [3] 29 12 [4] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 26 24 2 25 3-15-1 PFOS [15] PFOS pg/m 3 6 5 4 3 2 [] (pg/m 3 ) 22.4 [.1] 23.5 [.2] 24.5 [.2] 25.3 [.1] 26.17 [.6] 27.19 [.6] 28.6 [.2] 29.3 [.1] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-15-2 PFOS 389

[15] PFOS (pg/l) 8 6 4 [](pg/l) 21 37 [14] 22 5 [2] 23 5 [2] 24 31 [12] 26 5 [2] 27 29 [11] 28 5 [2] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-15-3 PFOS [15] PFOS (pg/g-dry) 1 8 6 4 [](pg/g-dry) 21 9.6 [3.7] 22 5[2] 23 5 [2] 24 9 [4] 26 5 [2] 27 3 [1] 28 5 [2] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-15-4 PFOS 39

[16] PFOA PFOA PFOS POPs POPs 21 14 14 15 16 17 14 21 22 24 25 26 28 29 3 4 pg/g-wet 3 2 18pg/g-wet 19 4 pg/gwet 19 12 79pg/g-wet 2 4 pg/g-wet 2 85 68pg/g-wet 21 29 PFOA PFOA [] H21 tr(2) tr(21) 94 nd 25 [9.9] 27/31 7/7 H22 28 33 76 nd 26 [9.9] 5/6 5/6 H23 tr(19) tr(22) tr(4) nd 41 [14] 3/4 3/4 H24 tr(21) tr(23) 46 nd 38 [13] 4/5 4/5 H26 tr(4) tr(6) 1 nd 1 [3] 2/3 2/3 H27 tr(6.5) tr(6.3) 26 nd 1 [3.4] 2/3 2/3 H28 4 7 9 nd 4 [2] 2/3 2/3 H29 tr(6.3) tr(7) 18 nd 12 [4] 2/3 2/3 H21 tr(23) tr(19) 49 nd 25 [9.9] 74/9 17/18 H22 tr(13) tr(11) 95 nd 26 [9.9] 13/18 13/18 H23 nd nd 51 nd 41 [14] 7/18 7/18 H24 tr(35) tr(32) 86 nd 38 [13] 18/19 18/19 H26 tr(6) tr(4) 85 nd 1 [3] 11/19 11/19 H27 tr(5.7) tr(5.3) 99 nd 1 [3.4] 11/19 11/19 H28 4 tr(3) 2 tr(2) 4 [2] 19/19 19/19 H29 tr(6.4) tr(4) 79 nd 12 [4] 12/19 12/19 391

PFOA [] H21 32 29 58 tr(16) 25 [9.9] 1/1 2/2 H22 38 --- 48 3 26 [9.9] 2/2 2/2 H23 --- --- nd nd 41 [14] /1 /1 H24 tr(27) --- tr(28) tr(26) 38 [13] 2/2 2/2 H26 62 --- 2,6 nd 1 [3] 1/2 1/2 H27 --- --- 31 31 1 [3.4] 1/1 1/1 H28 13 --- 32 52 4 [2] 2/2 2/2 H29 24 --- 68 85 12 [4] 2/2 2/2 1 21 2 26 24 3 25 37 1.1 pg/m 3 37 2 15pg/m 3 22 29 PFOA PFOA [] H22 25 26 21 4..5 [.2] H22 14 14 13 2.4 H23 2 18 24 tr(3.5) 35/35 35/35 5.4 [1.8] H23 12 11 97 nd 36/37 36/37 H24 11 12 12 1.9 36/36 36/36.7 [.2] H24 6.9 6. 48 1.6 36/36 36/36 (pg/m 3 ) H25 23 23 19 3.2 36/36 36/36 1.8 [.6] H25 14 14 53 3. 36/36 36/36 H26 28 29 21 5.4.4 [.1] 36/36 36/36 H27 19 17 26 tr(3.7) 4.2 [1.4] 35/35 35/35 H28 17 15 14 3.2 1.3 [.4] H29 14 13 15 tr(2.) 3.3 [1.1] 28 21 28 PFOA PFOA [] H21 1,6 1,3 31, 25 59 [23] 49/49 49/49 H22 2,7 2,4 23, 19 6 [2] 49/49 49/49 H23 2, 1,7 5, 38 5 [2] 49/49 49/49 H24 1,4 1,1 26, 24 17 [55] 48/48 48/48 (pg/l) H26 1,4 1,4 26, 14 5 [2] 48/48 48/48 H27 1,4 1,2 17, 31 56 [22] 48/48 48/48 H28 1,3 1,2 21, 26 5 [2] 48/48 48/48 25 21 28 PFOA PFOA (pg/g-dry) [] H21 27 24 5 nd 8.3 [3.3] 182/19 64/64 H22 28 33 18 nd 12 [5] 62/64 62/64 H23 1 93 1,1 22 5 [2] 64/64 64/64 H24 51 48 28 12 4 [2] 63/63 63/63 H26 44 5 19 tr(6) 11 [5] 63/63 63/63 H27 48 48 27 8 3 [1] 62/62 62/62 H28 27 27 19 nd 9 [4] 61/62 61/62 1 21 2 25 392

[16] PFOA 4 3 2 [] 21 25 [9.9] 22 26 [9.9] 23 41 [14] 24 38 [13] 26 1 [3] 27 1 [3.4] 28 4 [2] 29 12 [4] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 26 24 2 25 3 23 1/2 3-16-1 PFOA [16] PFOA pg/m 3 3 25 2 15 1 [] (pg/m 3 ) 22.5 [.2] 23 5.4 [1.8] 24.7 [.2] 25 1.8 [.6] 26.4 [.1] 27 4.2 [1.4] 28 1.3 [.4] 29 3.3 [1.1] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 3-16-2 PFOA 393

[16] PFOA 3, 2,5 2, [](pg/l) 21 59 [23] 22 6 [2] 23 5 [2] 24 17 [55] 26 5 [2] 27 56 [22] 28 5 [2] (pg/l) 1,5 1, 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-16-3 PFOA [16] PFOA 12 1 8 [](pg/g-dry) 21 8.3 [3.3] 22 12 [5] 23 5 [2] 24 4 [2] 26 11 [5] 27 3 [1] 28 9 [4] (pg/g-dry) 6 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-16-4 PFOA 394

[17] 21 5 POPs 4 COP4 22 4 13 55 56 61 63 2 4 8 11 14 19 22 27 29 21 28 47.6 pg/l 47 2. 14 pg/l 19 29 [] H19 nd nd nd nd 3,3 [1,3] /48 /48 H22 8 5 1 tr(1) 4 [1] 49/49 49/49 H23 11 11 17 2.6 2.4 [.9] 49/49 49/49 H24 14 11 17 3 3 [1] 48/48 48/48 (pg/l) H25 12 1 17 tr(3) 4 [1] 48/48 48/48 H26 1 7. 18 2.8.8 [.3] 48/48 48/48 H27 13 11 18 3. 1.5 [.5] 48/48 48/48 H29 8.8 5.9 14 2. 1.4 [.6] 47/47 47/47 2 21 62.5 pg/g-dry 62 1.3 2,8 pg/g-dry 19 29 [] H19 tr(46) nd 2,4 nd 86 [33] 79/192 35/64 H22 9 95 4,2 1..9 [.3] 64/64 64/64 H23 95 76 4,5 3 5 [2] 64/64 64/64 H24 33 33 1,1 nd 2.5 [.8] 62/63 62/63 H25 84 98 3,8 2.2 2.1 [.7] 63/63 63/63 (pg/g-dry) H26 7 78 3,6 tr(1.2) 2.4 [.8] 63/63 63/63 H27 65 69 2,6 2.4 1.5 [.5] 62/62 62/62 H28 62 71 3,7 tr(1.1) 1.8 [.6] 62/62 62/62 H29 61 61 2,8 1.3 1.2 [.5] 62/62 62/62 1 19 2 2 21 395

3 1 pg/g-wet 3 14 22pg/g-wet 19 1 pg/g-wet 19 4 17pg/g-wet 2 1 pg/g-wet 2 35 47pg/g-wet 19 29 [] H19 nd nd tr(15) nd 18 [61] 1/31 1/7 H22 18 16 11 5.9 1.9 [.7] 6/6 6/6 H23 28 16 26 1 4 [1] 4/4 4/4 H24 16 9.7 11 tr(5.8) 8.1 [2.7] 5/5 5/5 H25 nd nd 87 nd 78 [26] 1/5 1/5 H26 14 11 23 1 9.3 [3.1] 3/3 3/3 H27 tr(11) tr(9.7) 18 tr(7.4) 12 [4.] 3/3 3/3 H28 tr(13) tr(12) 15 tr(11) 15 [5.1] 3/3 3/3 H29 18 19 22 14 4 [1] 3/3 3/3 H19 nd nd 48 nd 18 [61] 36/8 1/16 H22 42 37 23 5.6 1.9 [.7] 18/18 18/18 H23 36 37 22 5 4 [1] 18/18 18/18 H24 29 37 19 tr(5.) 8.1 [2.7] 19/19 19/19 H25 tr(35) tr(4) 16 nd 78 [26] 11/19 11/19 H26 38 51 28 nd 9.3 [3.1] 18/19 18/19 H27 26 4 23 nd 12 [4.] 18/19 18/19 H28 19 22 15 nd 15 [5.1] 16/19 16/19 H29 29 32 17 4 4 [1] 19/19 19/19 H19 tr(14) tr(14) 21 tr(89) 18 [61] 1/1 2/2 H22 91 --- 17 49 1.9 [.7] 2/2 2/2 H23 --- --- 52 52 4 [1] 1/1 1/1 H24 77 --- 13 46 8.1 [2.7] 2/2 2/2 H25 3 --- 39 23 78 [26] 2/2 2/2 H26 56 --- 56 tr(5.6) 9.3 [3.1] 2/2 2/2 H27 --- --- 53 53 12 [4.] 1/1 1/1 H28 24 --- 57 1 15 [5.1] 2/2 2/2 H29 13 --- 47 35 4 [1] 2/2 2/2 1 19 2 25 24 3 2 21 396

37.1 pg/m 3 37 32 2pg/m 3 19 29 [] H19 85 83 31 18 78/78 26/26 12 [4.8] H19 6 55 22 27 75/75 25/25 H21 63 64 21 2 111/111 37/37 6.4 [2.5] H21 25 22 12 tr(5.) 111/111 37/37 H22 68 73 14 36 1.2 [.5] H22 7 69 18 37 H23 61 6 14 3 35/35 35/35 2.1 [.7] H23 59 57 18 26 (pg/m 3 ) H24 58 57 15 31 36/36 36/36 1.8 [.6] H24 55 55 12 27 36/36 36/36 H25 55 58 16 27 36/36 36/36 1.7 [.6] H25 55 52 11 34 36/36 36/36 H26 83 86 21 39.9 [.3] 36/36 36/36 H27 67 68 17 34.6 [.2] 35/35 35/35 H28 75 75 22 33.5 [.2] H29 71 69 2 32.3 [.1] 2 397

[17] 16 12 [](pg/l) 19 3,3 [1,3] 22 4[1] 23 2.4 [.9] 24 3 [1] 25 4 [1] 26.8 [.3] 27 1.5 [.5] 29 1.4 [.6] (pg/l) 8 4 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 19 2 2 21 28 3-17-1 [17] (pg/g-dry) 1 8 6 4 [](pg/g-dry) 19 86 [33] 22.9 [.3] 23 5 [2] 24 2.5 [.8] 25 2.1 [.7] 26 2.4 [.8] 27 1.5 [.5] 28 1.8 [.6] 29 1.2 [.5] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 19 2 2 21 3-17-2 398

[17] 5 4 3 2 [] 19 18 [61] 22 1.9 [.7] 23 4 [1] 24 8.1 [2.7] 25 78 [26] 26 9.3 [3.1] 27 12 [4.] 28 15 [5.1] 29 4 [1] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 19 2 25 24 3 2 21 4 19 25 1/2 3-17-3 [17] 1 pg/m 3 8 6 4 [] (pg/m 3 ) 19 12 [4.8] 21 6.4 [2.5] 22 1.2 [.5] 23 2.1 [.7] 24 1.8 [.6] 25 1.7 [.6] 26.9 [.3] 27.6 [.2] 28.5 [.2] 29.3 [.1] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 2 3-17-4 399

[18] 23 4 POPs 5 COP5 26 5 23 13 57 4 14 23 24 26 27 28 29 28 28 23 24 α- β- α- [] H23 nd nd 18 nd 12 [5] 2/49 2/49 (pg/l) H24 nd nd 3 nd 27 [1] 3/48 3/48 β- [] H23 nd nd 27 nd 22 [9] 8/49 8/49 (pg/l) H24 nd nd tr(12) nd 24 [9] 1/48 1/48 23 24 α- β- α- [] H23 tr(13) tr(11) 48 nd 3 [1] 35/64 35/64 (pg/g-dry) H24 nd nd 48 nd 13 [5] 19/63 19/63 β- [] H23 tr(5) tr(4) 24 nd 9 [4] 38/64 38/64 (pg/g-dry) H24 nd nd 25 nd 13 [5] 8/63 8/63 23 27 α- β- α- [] H23 62 12 33 nd 5 [2] 3/4 3/4 H24 tr(54) tr(61) 2 nd 71 [24] 4/5 4/5 H26 tr(2) nd 13 nd 6 [2] 1/3 1/3 H27 nd nd 13 nd 12 [38] 1/3 1/3 H23 tr(2) tr(2) 14 nd 5 [2] 1/18 1/18 H24 nd nd tr(54) nd 71 [24] 6/19 6/19 H26 nd nd tr(3) nd 6 [2] 1/19 1/19 H27 nd nd tr(49) nd 12 [38] 1/19 1/19 H23 --- --- nd nd 5 [2] /1 /1 H24 nd --- nd nd 71 [24] /2 /2 H26 nd --- nd nd 6 [2] /2 /2 H27 --- --- nd nd 12 [38] /1 /1 4

β- [] H23 16 26 52 4 11 [4] 4/4 4/4 H24 15 16 43 nd 14 [5] 4/5 4/5 H26 nd nd 23 nd 19 [6] 1/3 1/3 H27 nd nd tr(22) nd 32 [11] 1/3 1/3 H23 nd nd 37 nd 11 [4] 9/18 9/18 H24 nd nd 15 nd 14 [5] 6/19 6/19 H26 nd nd tr(8) nd 19 [6] 3/19 3/19 H27 nd nd tr(11) nd 32 [11] 1/19 1/19 H23 --- --- nd nd 11 [4] /1 /1 H24 nd --- tr(7) nd 14 [5] 1/2 1/2 H26 nd --- tr(8) nd 19 [6] 1/2 1/2 H27 --- --- nd nd 32 [11] /1 /1 1 26 24 2 25 23 28 α- β- α- [] H23 26 24 19 tr(7.8) 35/35 35/35 12 [4.] H23 tr(9.6) tr(9.8) 45 nd 35/37 35/37 H24 23 22 98 tr(6.) 36/36 36/36 16 [5.3] (pg/m 3 H24 nd nd 19 nd 15/36 15/36 ) H26 2 23 9 2.6.8 [.3] 36/36 36/36 H27 1 11 14 1.6 1. [.3] 35/35 35/35 H28 8.9 9.3 46 1..8 [.3] β- [] H23 2.1 1.8 11 nd 34/35 34/35 1.2 [.39] H23 tr(.8) tr(.9) 8.3 nd 31/37 31/37 H24 1.3 1.3 18 nd 33/36 33/36 1.2 [.4] (pg/m 3 H24 nd nd 1.7 nd 17/36 17/36 ) H26 1.3 1.4 6.1 nd 1.2 [.4] 33/36 33/36 H27.7.6 38 nd.5 [.2] 33/35 33/35 H28.8 tr(.7) 3.3 nd.8 [.3] 34/37 34/37 25 41

[18-1] α- 4 pg/m 3 3 2 [] (pg/m 3 ) 23 12 [4.] 24 16 [5.3] 26.8 [.3] 27 1. [.4] 28.8 [.3] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 24 1/2 3-18-1-1 α- [18-2] β- pg/m 3 3 2.5 2 1.5 1 [] (pg/m 3 ) 23 1.2 [.39] 24 1.2 [.4] 26 1.2 [.4] 27.5 [.2] 28.8 [.3].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 24 1/2 3-18-2-1 β- 42

[19] 1,2,5,6,9,1-1,2,5,6,9,1-25 4 5 POPs 6 COP6 α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9,1-26 5 23 13 62 14 15 16 14 α-1,2,5,6,9,1-β-1,2,5,6,9,1- γ-1,2,5,6,9,1- δ-1,2,5,6,9,1- ε-1,2,5,6,9,1-23 24 26 27 28 α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9,1-29 α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1-3 9 pg/g-wet 3 86 43pg/g-wet 19 9 pg/g-wet 19 tr(9) 7,8pg/g-wet 2 9 pg/g-wet 2 5 2,2pg/g-wet β-1,2,5,6,9,1-3 9 pg/g-wet 3 1 36pg/g-wet 19 9 pg/g-wet 19 2 tr(12)pg/g-wet 2 9 pg/g-wet 2 γ-1,2,5,6,9,1-3 9 pg/g-wet 3 tr(2) 2pg/g-wet 19 9 pg/g-wet 19 12 12pg/g- 43

wet 2 9 pg/g-wet 2 1 tr(18)pg/g-wet 23 29 α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1- [] H23 1,1 1,2 13, tr(86) 17 [7] 1/1 4/4 H24 53 48 2,5 19 5 [2] 5/5 5/5 H26 27 27 38 2 3 [1] 3/3 3/3 H27 26 2 56 15 3 [1] 3/3 3/3 H28 14 14 18 11 22 [9] 3/3 3/3 H29 19 2 43 86 24 [9] 3/3 3/3 H23 77 85 69, nd 17 [7] 41/51 16/17 H24 51 56 8,7 nd 5 [2] 18/19 18/19 H26 24 29 15, nd 3 [1] 18/19 18/19 H27 16 18 3, nd 3 [1] 18/19 18/19 H28 11 14 1,1 tr(12) 22 [9] 19/19 19/19 H29 14 14 7,8 tr(9) 24 [9 ] 19/19 19/19 H23 2 nd 53 nd 17 [7] 1/3 1/1 H24 12 --- 1,4 nd 5 [2] 1/2 1/2 H26 48 --- 1,8 13 3 [1] 2/2 2/2 H27 --- --- 8 8 3 [1] 1/1 1/1 H28 4 --- 1,6 1 22 [9] 2/2 2/2 H29 33 --- 2,2 5 24 [9 ] 2/2 2/2 β-1,2,5,6,9,1- [] H23 tr(7) tr(85) 24 nd 98 [4] 7/1 3/4 H24 tr(25) 4 9 nd 4 [1] 4/5 4/5 H26 tr(1) tr(1) tr(2) tr(1) 3 [1] 3/3 3/3 H27 tr(1) tr(1) 3 nd 3 [1] 2/3 2/3 H28 nd tr(8) tr(9) nd 21 [8] 2/3 2/3 H29 tr(9) nd 36 nd 23 [9] 1/3 1/3 H23 nd nd 76 nd 98 [4] 11/51 5/17 H24 nd nd 4 nd 4 [1] 8/19 8/19 H26 nd nd 3 nd 3 [1] 5/19 5/19 H27 nd nd tr(2) nd 3 [1] 2/19 2/19 H28 nd nd tr(12) nd 21 [8] 3/19 3/19 H29 nd nd tr(12) nd 23 [9] 2/19 2/19 H23 nd nd nd nd 98 [4] /3 /1 H24 nd --- nd nd 4 [1] /2 /2 H26 nd --- nd nd 3 [1] /2 /2 H27 --- --- nd nd 3 [1] /1 /1 H28 nd --- nd nd 21 [8] /2 /2 H29 nd nd nd nd 23 [9] /2 /2 γ-1,2,5,6,9,1- [] H23 44 47 3,3 nd 21 [8] 8/1 4/4 H24 17 18 91 3 3 [1] 5/5 5/5 H26 6 6 11 3 3 [1] 3/3 3/3 H27 7 9 2 tr(2) 3 [1] 3/3 3/3 H28 37 39 61 tr(21) 24 [9] 3/3 3/3 H29 49 3 2 tr(2) 24 [9] 3/3 3/3 H23 21 tr(9) 5, nd 21 [8] 26/51 1/17 H24 75 8 1,6 nd 3 [1] 16/19 16/19 H26 3 tr(2) 2,8 nd 3 [1] 12/19 12/19 H27 tr(2) tr(1) 23 nd 3 [1] 1/19 1/19 H28 tr(16) tr(13) 16 nd 24 [9] 11/19 11/19 H29 tr(16) tr(18) 12 nd 24 [9] 12/19 12/19 H23 tr(18) nd 46 nd 21 [8] 1/3 1/1 H24 31 --- 19 nd 3 [1] 1/2 1/2 H26 tr(1) --- tr(1) tr(1) 3 [1] 2/2 2/2 H27 --- --- tr(1) tr(1) 3 [1] 1/1 1/1 H28 tr(1) --- tr(2) nd 24 [9] 1/2 1/2 H29 tr(9) --- tr(18) nd 24 [9] 1/2 1/2 1 23 2 26 24 3 25 44

23 27 δ-1,2,5,6,9,1- ε-1,2,5,6,9,1- δ-1,2,5,6,9,1- [] H23 nd nd nd nd 14 [6] /1 /4 H24 nd nd nd nd 5 [2] /5 /5 H26 nd nd nd nd 3 [1] /3 /3 H27 nd nd nd nd 3 [1] /3 /3 ε-1,2,5,6,9,1- H23 nd nd nd nd 14 [6] /51 /17 H24 nd nd nd nd 5 [2] /19 /19 H26 nd nd nd nd 3 [1] /19 /19 H27 nd nd tr(2) nd 3 [1] 1/19 1/19 H23 nd nd nd nd 14 [6] /3 /1 H24 nd --- nd nd 5 [2] /2 /2 H26 nd --- nd nd 3 [1] /2 /2 H27 --- --- nd nd 3 [1] /1 /1 [] H23 nd nd nd nd 14 [6] /1 /4 H24 nd nd tr(3) nd 4 [2] 1/5 1/5 H26 nd nd tr(2) nd 3 [1] 1/3 1/3 H27 nd nd tr(1) nd 3 [1] 1/3 1/3 H23 nd nd nd nd 14 [6] /51 /17 H24 nd nd tr(3) nd 4 [2] 3/19 3/19 H26 nd nd 8 nd 3 [1] 3/19 3/19 H27 nd nd tr(1) nd 3 [1] 1/19 1/19 H23 nd nd nd nd 14 [6] /3 /1 H24 nd --- nd nd 4 [2] /2 /2 H26 nd --- nd nd 3 [1] /2 /2 H27 --- --- nd nd 3 [1] /1 /1 1 23 2 26 24 3 25 α-1,2,5,6,9,1-37.1 pg/m 3 37 36 3.3pg/m 3 β-1,2,5,6,9,1-37.1 pg/m 3 37 33.8pg/m 3 γ-1,2,5,6,9,1-37.1 pg/m 3 37 2.8pg/m 3 24 29 α-1,2,5,6,9,1-β- 1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1- [] H24 1.7 2.2 13 nd 31/36 31/36.6 [.2] H24 2.9 3. 63 nd 35/36 35/36 H26 tr(.6) tr(.7) 3.1 nd 1.2 [.4] 25/36 25/36 (pg/m 3 ) H27 tr(.6) tr(.7) 3 nd.9 [.3] 26/35 26/35 H28.5.5 2.4 tr(.1).3 [.1] H29.5.5 3.3 nd.3 [.1] 36/37 36/37 β-1,2,5,6,9,1- (pg/m 3 ) [] H24.5.5 29 nd 3/36 3/36.3 [.1] H24.8.8 18 nd 35/36 35/36 H26 nd nd tr(.8) nd 1. [.3] 8/36 8/36 H27 nd nd 3.9 nd.8 [.3] 7/35 7/35 H28 tr(.1) tr(.1).7 nd.3 [.1] 21/37 21/37 H29 tr(.2) tr(.1 ).8 nd.3 [.1] 33/37 33/37 45

γ-1,2,5,6,9,1- (pg/m 3 ) [] H24 1.6 1.7 28 nd 31/36 31/36.3 [.1] H24 2.1 1.8 84 nd 35/36 35/36 H26 nd nd tr(1.2) nd 1.3 [.4] 4/36 4/36 H27 nd nd 4.4 nd.8 [.3] 11/35 11/35 H28 tr(.1) nd 1.4 nd.3 [.1] 16/37 16/37 H29 tr(.1) tr(.1).8 nd.3 [.1] 2/37 2/37 25 23 27 δ-1,2,5,6,9,1- ε- 1,2,5,6,9,1- δ-1,2,5,6,9,1- [] H24 nd nd.8 nd 1/36 1/36.4 [.2] H24 nd nd 1.1 nd 1/36 1/36 (pg/m 3 ) H26 nd nd nd nd 1.8 [.6] /36 /36 H27 nd nd 1.9 nd 1.9 [.6] 1/35 1/35 ε-1,2,5,6,9,1- (pg/m 3 ) [] H24 nd nd nd nd /36 /36.6 [.2] H24 nd nd tr(.5) nd 1/36 1/36 H26 nd nd nd nd.9 [.3] /36 /36 H27 nd nd nd nd.9 [.3] /35 /35 25 46

26 23 26 1,2,5,6,9,1- α-1,2,5,6,9,1- [] H23 nd nd 6,3 nd 1,5 [6] 4/47 4/47 (pg/l) H26 nd nd 1,6 nd 1,5 [6] 1/48 1/48 β-1,2,5,6,9,1- [] H23 nd nd 1,3 nd 1,3 [5] 4/47 4/47 (pg/l) H26 nd nd tr(3) nd 5 [2] 1/48 1/48 γ-1,2,5,6,9,1- [] H23 nd nd 65, nd 1,2 [5] 5/47 5/47 (pg/l) H26 nd nd nd nd 7 [3] /48 /48 δ-1,2,5,6,9,1- [] H23 nd nd nd nd 79 [3] /47 /47 (pg/l) H26 nd nd nd nd 6 [2] /48 /48 ε-1,2,5,6,9,1- [] H23 nd nd nd nd 74 [3] /47 /47 (pg/l) H26 nd nd nd nd 4 [2] /48 /48 24 25 23 28 α-1,2,5,6,9,1-β- 1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1- [] H23 43 nd 24, nd 42 [28] 78/186 35/62 H24 31 28 22, nd 18 [7] 47/63 47/63 (pg/g-dry) H27 39 41 27, nd 15 [6] 47/62 47/62 H28 26 21 27, nd 13 [6] 43/62 43/62 β-1,2,5,6,9,1- (pg/g-dry) γ-1,2,5,6,9,1- (pg/g-dry) δ-1,2,5,6,9,1- (pg/g-dry) ε-1,2,5,6,9,1- (pg/g-dry) [] H23 nd nd 14, nd 25 [17] 48/186 21/62 H24 tr(93) nd 8,9 nd 15 [6] 29/63 29/63 H27 12 92 7,6 nd 15 [6] 33/62 33/62 H28 tr(87) nd 7,4 nd 13 [5] 31/62 31/62 [] H23 67 nd 57, nd 4 [26] 89/186 36/62 H24 42 33 55, nd 16 [6] 52/63 52/63 H27 33 45 6, nd 11 [42] 48/62 48/62 H28 25 19 5, nd 15 [6] 42/62 42/62 [] H23 nd nd 8 nd 35 [25] 11/186 6/62 H24 nd nd 68 nd 3 [1] 5/63 5/63 H27 nd nd nd nd 18 [7] /62 /62 [] H23 nd nd tr(26) nd 28 [21] 2/186 1/62 H24 nd nd 31 nd 15 [6] 7/63 7/63 H27 nd nd nd nd 13 [51] /62 /62 1 23 2 25 26 47

[19-1] α-1,2,5,6,9,1-1,2 1, 8 6 [] 23 17 [7] 24 5 [2] 26 3 [1] 27 3 [1] 28 22 [9] 29 24 [9] 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 23 3 26 24 2 25 3-19-1-1 α-1,2,5,6,9,1- [19-1] α-1,2,5,6,9,1- pg/m 3 3 2.5 2 1.5 1 [] (pg/m 3 ) 24.6 [.2] 26 1.2 [.4] 27.9 [.3] 28.3 [.1] 29.3 [.1].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 25 3-19-1-2 α-1,2,5,6,9,1-48

[19-2] β-1,2,5,6,9,1-8 6 4 [] 23 98 [4] 24 4 [1] 26 3 [1] 27 3 [1] 28 21 [8] 29 23 [9] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 23 2 3 26 24 4 25 5 28 1/2 3-19-2-1 β-1,2,5,6,9,1- [19-2] β-1,2,5,6,9,1-1 pg/m 3.8.6.4 [] (pg/m 3 ) 24.3 [.1] 26 1. [.3] 27.8 [.3] 28.3 [.1] 29.3 [.1].2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 26 27 1/2 3-19-2-2 β-1,2,5,6,9,1-49

[19-3] γ-1,2,5,6,9,1-5 4 3 2 [] 23 21 [8] 24 3 [1] 26 3 [1] 27 3 [1] 28 24 [9] 29 24 [9] 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 23 2 26 24 3 25 3-19-3-1 γ-1,2,5,6,9,1- [19-3] γ-1,2,5,6,9,1-2.5 pg/m 3 2 1.5 1 [] (pg/m 3 ) 24.3 [.1] 26 1.4 [.4] 27.8 [.3] 28.3 [.1] 29.3 [.1].5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 25 2 26 27 1/2 3-19-3-2 γ-1,2,5,6,9,1-41

[19-1] α-1,2,5,6,9,1-5 4 [](pg/g-dry) 23 42 [28] 24 18 [7] 27 15 [6] 28 13 [6] (pg/g-dry) 3 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 23 2 25 26 29 3-19-1-3 α-1,2,5,6,9,1- [19-2] β-1,2,5,6,9,1-14 12 [](pg/g-dry) 23 25 [17] 24 15 [6] 27 15 [6] 28 13 [5] 1 (pg/g-dry) 8 6 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 23 2 25 26 29 2 23 1/2 3-19-2-3 β-1,2,5,6,9,1-411

[19-3] γ-1,2,5,6,9,1-7 6 5 [](pg/g-dry) 23 4 [26] 24 16 [6] 27 11 [42] 28 15 [6] (pg/g-dry) 4 3 2 1 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 23 2 25 26 29 3-19-3-3 γ-1,2,5,6,9,1-412

[2] 3 54 8 POPs 27 5 7 COP7 2 8 2 28 4 13 55 6 62 3 5 14 1 8 18 2 26 27 28 29 62 9.1pg/g-dry 62 tr(16) 32, pg/g-dry 2 29 [] H2 41 4 28, nd 84 [3] 166/189 58/63 H28 76 87 16, nd 59 [2] 59/62 59/62 (pg/g-dry) H29 63 8 32, tr(16) 27 [9.1] 62/62 62/62 1 2 2[] [] 3 21 27 3 12pg/g-wet 3 2 1,4pg/g-wet 19 12pg/g-wet 19 17 36pg/g-wet 2 12pg/g-wet 2 tr(18) 46pg/g-wet 18 29 [] H18 98 73 1.2 tr(19) 27 [11] 31/31 7/7 H2 94 73 1,3 tr(11) 26 [1] 31/31 7/7 H27 7 67 58 nd 54 [18] 2/3 2/3 H28 72 tr(49) 79 nd 57 [19] 2/3 2/3 H29 46 68 1,4 nd 33 [12] 2/3 2/3 413

[] H18 72 49 2,7 nd 27 [11] 78/8 16/16 H2 59 4 2,2 nd 26 [1] 79/85 17/17 H27 tr(5) 85 39 nd 54 [18] 13/19 13/19 H28 tr(44) tr(48) 34 nd 57 [19] 13/19 13/19 H29 32 51 36 nd 33 [12] 17/19 17/19 H18 tr(17) tr(18) 27 tr(11) 27 [11] 1/1 2/2 H2 tr(1) nd tr(22) nd 26 [1] 5/1 1/2 H27 --- --- tr(2) tr(2) 54 [18] 1/1 1/1 H28 13 --- 32 tr(49) 57 [19] 2/2 2/2 H29 91 --- 46 tr(18) 33 [12] 2/2 2/2 1 18 2 2[] [] 3 27 2 4 19 21 26 37.24pg/m 3 37 7 92pg/m 3 2 29 [] H2 2 23 66 35 22/22 22/22 4. [1.3] H2 tr(9.6) tr(9.8) 45 nd 36/36 36/36 (pg/m 3 H26 11 13 1,6 5.4 2.8 [1.] 36/36 36/36 ) H28 11 13 66 9..79 [.28] H29 11 12 92 7.67 [.24] 1[] [] 2 21 25 27 2 2 [] H2 nd nd 18 nd 85[3] 9/48 9/48 (pg/l) [] [] 414

[2] 8 [](pg/g-dry) 2 84 [3] 28 59 [2] 29 27 [9.1] 6 (pg/g-dry) 4 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 2 2 21 27 3-2-1 [2] 1 8 6 4 [] 18 27 [11] 2 26 [1] 27 54 [18] 28 59 [19] 29 33 [12] 2 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 18 2 2 27 2 3 19 21 26 3-2-2 415

[2] 25 pg/m 3 2 15 1 [] (pg/m 3 ) 2 4. [1.3] 26 2.8 [1.] 28.79 [.28] 29.67 [.24] 5 14 15 16 17 18 19 2 21 22 23 24 25 26 27 28 29 1 2 3 21 25 27 3-2-3 416

[21] -1,3- -1,3-17 4 1 POPs 27 5 7 COP7 19 14 56 14 19 14 19 25 27 29 37 2pg/m 3 37 1,1 23,pg/m 3 27 29-1,3- - [] 1,3- H27 1,1 1,2 3,5 45 29 [11] 12/12 34/34 (pg/m 3 H28 85 8 4,3 51 6 [2] 111/111 37/37 ) H29 4,2 4, 23, 1,1 6 [2] 25 19 25-1,3- - [] 1,3- H19 nd nd nd nd 87 [34] /48 /48 (pg/l) H25 nd nd tr(43) nd 94 [37] 1/48 1/48 2 24 19 25-1,3- - [] 1,3- H19 nd nd 1,3 nd 22 [8.5] 22/192 1/64 (pg/g-dry) H25 nd nd 1,6 nd 9.9 [3.8] 4/189 2/63 1 2 2 24 417

19 25-1,3- - [] 1,3- H19 nd nd nd nd 36 [12] /31 /7 H25 nd nd tr(7.1) nd 9.4 [3.7] 3/13 1/5 H19 nd nd nd nd 36 [12] /8 /16 H25 nd nd 59 nd 9.4 [3.7] 7/57 4/19 H19 nd nd nd nd 36 [12] /1 /2 H25 nd nd nd nd 9.4 [3.7] /6 /2 1 2 25 19 3 2 24 418

[22] 27 5 POPs 7 COP7 28 1 1 27 13 49 8 14 17 14 27 28 29 47 1 pg/l 47 43 3,5 pg/l 47 5 pg/l 47 32 1, pg/l 27 29 [] H27 tr(13) tr(9) 26, nd 26 [85] 25/48 25/48 (pg/l) H29 86 11 3,5 nd 3 [1] 43/47 43/47 [] (pg/l) H29 tr(1) tr(8) 1, nd 14 [5] 32/47 32/47 1 28 62 2 pg/g-dry 62 8 7,4 pg/g-dry 62 2 pg/g-dry 62 61 19 pg/g-dry 419

29 [] H29 35 39 7,4 8 4 [2] 62/62 62/62 (pg/g) [] H29 34 32 19 nd 5 [2] 61/62 61/62 (pg/g) 3 12 pg/g-wet 3 1 tr(35)pg/g-wet 19 12 pg/g-wet 19 14 11pg/g-wet 2 12 pg/g-wet 2 3 11,pg/g-wet 3 1 pg/g-wet 3 tr(2) 36pg/g-wet 19 1 pg/g-wet 19 tr(1) 12pg/g-wet 2 1 pg/g-wet 2 11 47pg/g-wet 28 29 [] H28 tr(45) tr(46) 65 tr(3) 63 [21] 3/3 3/3 H29 nd nd tr(35) nd 36 [12] 1/3 1/3 H28 1 13 99 nd 63 [21] 18/19 18/19 H29 tr(15) tr(15) 11 nd 36 [12] 14/19 14/19 H28 1,2 --- 3,1 44 63 [21] 2/2 2/2 H29 1,8 --- 11, 3 36 [12] 2/2 2/2 [] H28 7 3 35 3 3 [1] 3/3 3/3 H29 6 tr(3) 36 tr(2) 4 [1] 3/3 3/3 H28 8 6 1 tr(1) 3 [1] 19/19 19/19 H29 6.7 5 12 tr(1) 4 [1] 19/19 19/19 H28 12 --- 14 1 3 [1] 2/2 2/2 H29 23 29 47 11 4 [1] 2/2 2/2 42

37.2 pg/m 3 37.7 33pg/m 3 37.5 pg/m 3 37 6 21pg/m 3 28 29 [] H28 6.3 6. 25.6.5 [.2] (pg/m 3 ) H29 4.6 4.8 33.7.6 [.2] [] H28 39 42 22 3.4 1. [.4] (pg/m 3 ) H29 34 36 21 6 1.2 [.5] 421

[23] 28 4 5 POPs 8 COP8 28 14 16 17 28 29 47 1,1 pg/l 47 1 tr(1,6)pg/l 47 5 pg/l 47 13 3,1 pg/l 47 1,1 pg/l 47 4 1, pg/l 47 1,2 pg/l 47 7 1, pg/l 29 (pg/l) [] H29 nd nd tr(1,6) nd 3,3 [1,1] 1/47 1/47 [] H29 (pg/l) nd nd 3,1 nd 1,5 [5] 13/47 13/47 (pg/l) [] H29 nd nd 1, nd 3,3 [1,1] 4/47 4/47 [] H29 (pg/l) nd nd 1, nd 3,6 [1,2] 7/47 7/47 5 9 62 4, pg/g-dry 62 12 422

17, pg/g-dry 62 4, pg/g-dry 62 19 37, pg/g-dry 62 4, pg/g-dry 62 19 44, pg/g-dry 62 5, pg/g-dry 62 18 94, pg/g-dry 29 (pg/g-dry) [] H29 nd nd 17, nd 1, [4,] 12/62 12/62 [] H29 (pg/g-dry) nd nd 37, nd 1, [4,] 19/62 19/62 (pg/g-dry) [] H29 nd nd 44, nd 11, [4,] 19/62 19/62 [] H29 (pg/g-dry) nd nd 94, nd 12, [5,] 18/62 18/62 5 9 3 2 pg/g-wet 3 2 1,8pg/g-wet 19 2 pg/g-wet 19 16 2,1pg/g-wet 2 2 pg/g-wet 2 1 1,6pg/g-wet 3 3 pg/g-wet 3 tr(3) 11,pg/g-wet 19 3 pg/g-wet 19 16 24,pg/g-wet 2 3 pg/g-wet 2 8 31,pg/g-wet 3 3 pg/g-wet 3 1,3 4,7pg/g-wet 19 3 pg/g-wet 19 18 19,pg/g-wet 2 3 pg/g-wet 2 1,2 25,pg/g-wet 3 2 pg/g-wet 3 tr(3) 3,1pg/g-wet 19 2 pg/g-wet 19 8 4,1pg/g-wet 423

2 2 pg/g-wet 2 1 8,1pg/g-wet 28 29 [] H28 tr(7) tr(7) 2,2 nd 1,3 [5] 2/3 2/3 H29 67 1,7 1,8 nd 5 [2 ] 2/3 2/3 H28 tr(6) tr(7) 2,8 nd 1,3 [5] 13/19 13/19 H29 tr(41) tr(4) 2,1 nd 5 [2 ] 16/19 16/19 H28 tr(1,) --- 1,3 tr(8) 1,3 [5] 2/2 2/2 H29 tr(4) --- 1,6 nd 5 [2 ] 1/2 1/2 [] H28 tr(2,9) tr(2,) 6, tr(2,) 3, [1,] 3/3 3/3 H29 2,2 3,4 11, tr(3) 8 [3 ] 3/3 3/3 H28 tr(2,9) tr(2,) 15, nd 3, [1,] 18/19 18/19 H29 1,9 1,1 24, nd 8 [3 ] 16/19 16/19 H28 4,9 --- 8, 3, 3, [1,] 2/2 2/2 H29 5, --- 31, 8 8 [3 ] 2/2 2/2 [] H28 tr(1,4) tr(1,5) tr(1,8) tr(1,1) 2,1 [7] 3/3 3/3 H29 2, 1,4 4,7 1,3 9 [3 ] 3/3 3/3 H28 tr(1,8) tr(1,8) 8,7 nd 2,1 [7] 17/19 17/19 H29 2,1 2,1 19, nd 9 [3 ] 18/19 18/19 H28 3,8 --- 6,6 2,2 2,1 [7] 2/2 2/2 H29 5,5 --- 25, 1,2 9 [3 ] 2/2 2/2 [] H28 tr(7) tr(7) tr(9) tr(5) 1,1 [4] 3/3 3/3 H29 87 7 3,1 tr(3) 5 [2 ] 3/3 3/3 H28 tr(8) tr(8) 4,9 nd 1,1 [4] 17/19 17/19 H29 tr(29) nd 4,1 nd 5 [2 ] 8/19 8/19 H28 1,4 --- 1,5 1,4 1,1 [4] 2/2 2/2 H29 9 --- 8,1 nd 5 [2 ] 1/2 1/2 5 9 37 5 pg/m 3 37 7 1,5pg/m 3 37 6 pg/m 3 37 9 2,3pg/m 3 37 3 pg/m 3 37 3 73pg/m 3 37 4 pg/m 3 37 35 1,6pg/m 3 28 29 [] H28 tr(17) tr(2) 94 nd 29 [11] 24/37 24/37 (pg/m 3 ) H29 37 38 1,5 tr(7) 14 [5] 424

[] H28 tr(35) tr(32) 3,2 nd 61 [24] 2/37 2/37 (pg/m 3 ) H29 5 51 2,3 tr(9) 19 [6] [] H28 nd nd 74 nd 43 [17] 7/37 7/37 (pg/m 3 ) H29 19 19 73 tr(3) 1 [3] [] H28 nd nd 51 nd 32 [12] 13/37 13/37 (pg/m 3 ) H29 15 16 1,6 nd 12 [4] 35/37 35/37 4 7 425

[24] 16 17 4 POPs POPs 18 14 16 14 18 2 28 29 28 28 2 (pg/l) [] H2 nd nd 76 nd 25 [1] 13/48 13/48 2 [] H2 nd nd 46 nd 16 [63] 13/63 3/186 (pg/g-dry) 18 2 [] H18 tr(58) tr(7) 24 nd 92 [36] 22/31 5/7 H2 tr(11) 12 21 nd 12 [48] 28/31 7/7 H18 nd nd 29 nd 92 [36] 5/8 1/16 H2 tr(62) tr(77) 27 nd 12 [48] 55/85 14/17 H18 nd nd nd nd 92 [36] /1 /2 H2 nd nd 3 nd 12 [48] 1/1 1/2 28 (pg/m 3 ) H28 [] nd nd 1. nd.5 [.2] 1/37 1/37 426

i) (http://www.env.go.jp/chemi/kurohon/) ii) (http://www.env.go.jp/chemi/kurohon/) iii) (http://www.env.go.jp/chemi/kurohon/) iv) (http://www.env.go.jp/chemi/kurohon/) 427