/ 3 1 / 3 / 3 1 /

Transcription

1 /31/ 3/31/

2 [1] PCB [2] HCB [3] [4] [5] DDT [6-1] p,p'-ddt [6-2] p,p'-dde pg/l ( ) nd 2,4 (46/47) (47/47) pg/g-dry ( ) nd 61, (61/62) 4,6 3 11, (62/62) 82 [6] [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7] [8] [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans (47/47) tr(2) 15 (47/47) nd 12 (19/47) tr(.6) 36 (47/47) tr(2) 12 (47/47) nd 6 (2/47) nd 83 (46/47) nd (/47) nd nd 4.7 nd nd 2,8 (61/62) tr(1) 3, (62/62) nd 78 (41/62) nd 1,5 (61/62) nd 2,6 (61/62) nd 4 (53/62) nd 15 (51/62) nd (/62) tr(1) nd [9-1] Parlar-26 [9] [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch [11] [11-3] γ-hch [11-4] δ-hch [12] (47/47) (47/47) (47/47) tr(.4) 69 (47/47) ,9 (62/62) 5.7 3,4 (62/62) tr(.4) 1,9 (62/62) tr(.2) 1,7 (62/62) [13] 1 nd 1/2 2 3 tr(x)x

3 4 1 [14-1] [14-2] [14-3] [14] [14-4] [14-5] [14-6] [14-7] [15] PFOS [16] PFOA [17] [18-1] α- [18] [18-2] β- 1,2,5,6,9,1- [19-1] α-1,2,5,6,9,1- [19-2] β-1,2,5,6,9,1- [19] [19-3] γ-1,2,5,6,9,1- [19-4] δ-1,2,5,6,9,1- [19-5] ε-1,2,5,6,9,1- [2] [21] -1,3- [22] [22-1] [22-2] [23-1] [23-2] [23] [23-3] [23-4] ( ) nd 12 (44/47) nd 8 (24/47) nd tr(6) (1/47) nd 3 (1/47) nd 33 (22/47) nd 46 (37/47) nd 4,1 (46/47) (47/47) nd 3,5 (43/47) nd 1, (32/47) nd tr(1,6) (1/47) nd 3,1 (13/47) nd 1, (4/47) nd 1, (7/47) pg/l tr(4) nd nd nd tr(2) tr(1) nd nd nd nd pg/g-dry ( ) nd 57 (44/62) nd 56 (37/62) nd 57 (44/62) nd 58 (36/62) nd 1,9 (48/62) nd 29, (61/62) tr(27) 58, (62/62) 1.3 2,8 (62/62) tr(16) 32, (62/62) 8 7,4 (62/62) nd 19 (61/62) nd 17, (12/62) nd 37, (19/62) nd 44, (19/62) nd 94, (18/62) , nd nd nd nd [24] 1 nd 1/2 2 3 tr(x)x

4 [1] PCB [2] HCB [3] [4] [5] DDT [6-1] p,p'-ddt [6-2] p,p'-dde pg/g-wet pg/m 3 ( ) ( ) ( ) ( ) 5 19, 86 16, 4, 38, 26 3,3 2,5 1, 39, (3/3) (19/19) (2/2) (37/37) ,1 23 4, ,1 (3/3) (19/19) (2/2) (37/37) 13 [6] [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7] [7-2] trans- [7-3] [8] [9] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch [11] [11-3] γ-hch [11-4] δ-hch [12] [13] 6 32 (3/3) 21 6 (3/3) tr(2) 11 (3/3) tr(1) 3 (3/3) tr(1.7) nd 13 (18/19) 4 29 (19/19) nd 3 (16/19) nd 23 (15/19) (2/2) 3 3,5 (2/2) tr(1) 2 (2/2) nd tr(1) (1/2) 1 nd 1/2 2 3 tr(x)x , 4.5 nd (37/37) (37/37) (37/37) nd 46 (36/37)

5 4 1 [14-1] 23 2 (3/3) [14-2] tr(6) 62 (3/3) [14-3] nd 36 (2/3) [14] [14-4] nd tr(9) (1/3) [14-5] nd tr(9) (1/3) [14-6] nd (/3) [14-7] nd tr(18) (1/3) [15] nd 16 PFOS (2/3) [16] nd 18 PFOA (2/3) [17] (3/3) [18-1] α- [18] [18-2] β- 1,2,5,6,9,1- [19-1] α-1,2,5,6,9, (3/3) [19-2] β-1,2,5,6,9,1- nd 36 (1/3) [19] [19-3] γ-1,2,5,6,9,1- tr(2) 2 (3/3) [19-4] δ-1,2,5,6,9,1- [19-5] ε-1,2,5,6,9,1- nd 1,4 [2] (2/3) [21] -1,3- [22] [22-1] nd tr(35) (1/3) [22-2] tr(2) 36 (3/3) nd 1,8 [23-1] (2/3) [23-2] tr(3) 11, [23] (3/3) 1,3 4,7 [23-3] (3/3) tr(3) 3,1 [23-4] (3/3) [24] pg/g-wet pg/m 3 ( ) ( ) ( ) ( ) tr(14) nd nd nd nd 22 tr(6.3) tr(9) nd ,2 2, 87 tr(7) 36 (19/19) nd 87 (18/19) nd 21 (18/19) nd 55 (1/19) nd 88 (9/19) nd 68 (1/19) nd 2,1 (1/19) tr(4) 11, (19/19) nd 79 (12/19) 4 17 (19/19) tr(9) 7,8 (19/19) nd tr(12) (2/19) nd 12 (12/19) nd 36 (17/19) nd 11 (14/19) tr(1) 12 (19/19) nd 2,1 (16/19) nd 24, (16/19) nd 19, (18/19) nd 4,1 (8/19) tr(11) tr(9.7) nd nd 15 tr(6.4) nd tr(16) 32 tr(15) 6.7 tr(41) 1,9 2, (2/2) 12 5 (2/2) 51 1, (2/2) tr(18) 44 (2/2) (2/2) nd (/2) nd (/2) 3, 32, (2/2) (2/2) (2/2) 5 2,2 (2/2) nd (/2) nd tr(18) (1/2) tr(18) 46 (2/2) 3 11, (2/2) (2/2) nd 1,6 (1/2) 8 31, (2/2) 1,2 25, (2/2) nd 8,1 (1/2) nd nd 9, nd tr(9) 91 1,8 23 tr(4) 5, 5, (37/37) nd 3.4 (33/37) nd 2.1 (11/37) nd 3.2 (1/37) nd 5.7 (28/37) nd 4 (31/37) nd 14 (34/37) (37/37) 2 15 (37/37) 32 2 (37/37) nd 3.3 (36/37) nd.8 (33/37) nd.8 (2/37) 7 92 (37/37) 1,1 23, (37/37).7 33 (37/37) 6 21 (37/37) 7 1,5 (37/37) 9 2,3 (37/37) 3 73 (37/37) nd 1,6 (35/37) nd nd tr(.19) nd 1/2 tr(x)x -1,3-3/ tr(29) tr(.2) tr(.1) 11 4,

6 9 29 [1] PCB [2] HCB pg/l pg/g-dry pg/g-wet pg/m 3 [3] [4] [5] DDT [6-1] p,p'-ddt [6-2] p,p'-dde 16 [5.5] 2.1 [.8] 14 [5.] 3 [1] 68 [23] 3.9 [1.3] 7. [2.3].5 [.2] [6] [6-3] p,p'-ddd [7] [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9] [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch [11] [11-3] γ-hch [11-4] δ-hch [12] 2 [1] 3 [1] 4 [2] 1.5 [.6] 3 [1] 3 [1] 1.6 [.6] 2.3 [.9].9 [.4] 1.8 [.7] 1.4 [.5] 1. [.4] 4.8 [1.6] 4 [1] 3 [1] 1.7 [.7] 6 [2].9 [.3] 1.2 [.5] 2. [.8].5 [.2] 1.5 [.6] 1. [.4].6 [.2] [13] 1 2[] 3 4 3[1] 3[1] 3[1] 2.3 [.9].8 [.3].11 [.4].1 [.4].8 [.3] 245

7 pg/l pg/g-dry pg/g-wet pg/m [14-1] 9 [3] 9 [4] 16 [6].15 [.5] [14-2] 3 [1] 9 [4] 12 [5].1 [.4] [14-3] [14] [3] [2] [7] [.1] [14-4] 14 [5] 15 [6] 22 [8].4 [.2] [14-5] 2 [1] 5 [2] 2 [8].21 [.7] [14-6] 7 [3] 15 [5] 5 [2].6 [.2] [14-7] [15] PFOS [16] PFOA [17] [18-1] α- [18] [18-2] β- 1,2,5,6,9,1- [19-1] α-1,2,5,6,9,1- [19-2] β-1,2,5,6,9,1- [19] [19-3] γ-1,2,5,6,9,1- [19-4] δ-1,2,5,6,9,1- [19-5] ε-1,2,5,6,9,1- [2] [21] -1,3- [22] [22-1] [22-2] [23-1] [23-2] [23] [23-3] [23-4] [24] 24 [8] 1.4 [.6] 3 [1] 14 [5] 3,3 [1,1] 1,5 [5] 3,3 [1,1] 3,6 [1,2] 3 [1] 1.2 [.5] 27 [9.1] 4 [2] 5 [2] 1, [4,] 1, [4,] 11, [4,] 12, [5,] 1 2[] [8] 12 [4] 12 [4] 4 [1] 24 [9] 23 [9] 24 [9] 33 [12] 36 [12] 4 [1] 5 [2] 8 [3] 9 [3] 5 [2] 2.4 [.8].3 [.1] 3.3 [1.1].3 [.1].3 [.1].3 [.1].3 [.1].67 [.24] 6 [2].6 [.2] 1.2 [.5] 14 [5] 19 [6] 1 [3] 12 [4] 246

8 [1] PCB [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis [7-2] trans- [7-3] X X X [7-4] cis- [7-5] trans [8-1] X X X X [8-2] cis- [8-3] trans- X X X X X [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] [11] HCH [11-1] α-hch [11-2] β-hch [11-3] γ-hch [11-4] δ-hch * * X 1 AIC 95 2 X

9 [14] [14-1] [14-2] [14-3] [14-4] [14-5] X X X X X X X X X X X X X X X X X X X X [14-6] * * X X [14-7] * * X X [17] 1 AIC 95 2 X

10 [1] PCB [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans [7-3] X * X [7-4] cis- [7-5] trans [8-1] X X [8-2] cis- * X [8-3] trans- X X X X X [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] [11] HCH [11-1] α-hch [11-2] β-hch [11-3] γ-hch [11-4] δ-hch 1 AIC 95 2 X

11 [14] [14-1] * [14-2] X [14-3] X [14-4] * X * [14-5] X [14-6] [14-7] [17] 1 AIC 95 2 X

12 [1] PCB [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] [11] HCH [11-1] α-hch [11-2] β-hch [11-3] γ-hch [11-4] δ-hch X 1 AIC 95 2 X

13 [14] [15] [14-1] [14-2] [14-3] [14-4] [14-5] [14-6] [14-7] PFOS [16] PFOA X X X X X X X X [17] X * 1 AIC 95 2 X 3 2 PFOSPFOA X X X X 252

14 [1] PCB [2] HCB [3] [4] [5] [6] [7] [8] [9] DDT [6-1] p,p'-ddt [6-2] p,p'-dde [6-3] p,p'-ddd [6-4] o,p'-ddt [6-5] o,p'-dde [6-6] o,p'-ddd [7-1] cis- [7-2] trans- [7-3] [7-4] cis- [7-5] trans- [8-1] [8-2] cis- [8-3] trans- [9-1] Parlar-26 [9-2] Parlar-5 [9-3] Parlar-62 [1] HCH [11-1] α-hch [11-2] β-hch 19 [11] 1 1 [11-3] γ-hch [11-4] δ-hch 1 AIC HCH

15 [14-1] [14-2] X [14] [14-3] X [14-4] X [14-5] X [14-6] X [14-7] X [15] PFOS [16] PFOA [17] 1 AIC 95 2 X 3 21 PFOSPFOA

16 茨 255

17 PCB HCB HCH 4 1 PFOSPFOA 1,2,5,6,9,1- α-1,2,5,6,9,1-β- 1,2,5,6,9,1- γ-1,2,5,6,9,1- -1,3- trans ,2,5,6,9,1- β-1,2,5,6,9,1-256

18 [1] PCB PCB 49 6 POPs pg/l ,4pg/L PCB [] PCB (pg/l) H , [2.5] 114/114 38/38 H , [2.5] 36/36 36/36 H , [5.] 38/38 38/38 H , [3.2] 47/47 47/47 H , [3] 48/48 48/48 H , [2.9] 48/48 48/48 H , [3.] 48/48 48/48 H , [4] 48/48 48/48 H ,2 nd 73 [24] 41/49 41/49 H , [1.7] 49/49 49/49 H , [15] 48/48 48/48 H ,6 tr(13) 25 [8] 48/48 48/48 H , [2.9] 48/48 48/48 H , [7.3] 48/48 48/48 H ,1 tr(7.2) 8.4 [2.8] 48/48 48/48 H ,4 nd 16 [5.5] 46/47 46/ [] [] pg/g-dry ,pg/g-dry

19 14 29 PCB [] PCB (pg/g-dry) H14 11, 11, 63, 39 1 [3.5] 189/189 63/63 H15 9,4 9,5 5,6, 39 1 [3.2] 186/186 62/62 H16 8,4 7,6 1,3, [2.6] 189/189 63/63 H17 8,6 7,1 69, [2.1] 189/189 63/63 H18 8,8 6,6 69, 36 4 [1] 192/192 64/64 H19 7,4 6,8 82, [1.5] 192/192 64/64 H2 8,7 8,9 63, [1.2] 192/192 64/64 H21 7,6 7,1 1,7, [2.1] 192/192 64/64 H22 6,5 7,8 71, nd 66 [22] 56/64 56/64 H23 6,3 7,4 95, [4.5] 64/64 64/64 H24 5,7 6,7 64, tr(32) 51 [18] 63/63 63/63 H25 6,2 8, 65, tr(43) 44 [13] 62/62 62/62 H26 4,9 5,5 44, tr(35) 61 [21] 63/63 63/63 H27 6,4 7,5 1,1, nd 62 [22] 61/62 61/62 H28 5,3 5,3 77, tr(21) 53 [18] 62/62 62/62 H29 4,6 6,2 61, nd 14 [5.] 61/62 61/ [] [] 3 23pg/g-wet ,pg/g-wet 19 23pg/gwet ,pg/g-wet 2 23pg/g-wet 2 4, 38,pg/gwet PCB PCB [] H14 8,8 28, 16, 2 25 [8.4] 38/38 8/8 H15 11, 9,6 13, 1, 5 [17] 3/3 6/6 H16 11, 11, 15, 1,5 85 [29] 31/31 7/7 H17 11, 13, 85, [23] 31/31 7/7 H18 8,5 8,6 77, [14] 31/31 7/7 H19 9, 11, 66, [18] 31/31 7/7 H2 8,6 8,6 69, [17] 31/31 7/7 H21 8,7 11, 62, [11] 31/31 7/7 H22 9,2 11, 46, 1,5 52 [2] 6/6 6/6 H23 8,9 17, 65, [74] 4/4 4/4 H24 6,6 12, 34, [11] 5/5 5/5 H25 5,2 7,8 44, [14] 5/5 5/5 H26 2,9 2,6 15, 6 95 [31] 3/3 3/3 H27 2,4 2,5 9, [17] 3/3 3/3 H28 2,3 2,3 12, 42 6 [2] 3/3 3/3 H29 2,5 1,6 19, 5 68 [23] 3/3 3/3 258

20 PCB [] H14 17, 8,1 55, 1,5 25 [8.4] 7/7 14/14 H15 11, 9,6 15, 87 5 [17] 7/7 14/14 H16 15, 1, 54, [29] 7/7 14/14 H17 14, 8,6 54, 8 69 [23] 8/8 16/16 H18 13, 9, 31, [14] 8/8 16/16 H19 11, 6,2 53, [18] 8/8 16/16 H2 12, 9,1 33, 1,2 47 [17] 85/85 17/17 H21 12, 12, 29, [11] 9/9 18/18 H22 13, 1, 26, [2] 18/18 18/18 H23 14, 12, 25, 9 22 [74] 18/18 18/18 H24 13, 14, 13, [11] 19/19 19/19 H25 14, 13, 27, 1, 44 [14] 19/19 19/19 H26 13, 1, 23, [31] 19/19 19/19 H27 11, 7,7 18, 1,3 52 [17] 19/19 19/19 H28 11, 8,4 15, 1,2 6 [2] 19/19 19/19 H29 1, 8,3 16, [23] 19/19 19/19 H14 12, 14, 22, 4,8 25 [8.4] 1/1 2/2 H15 19, 22, 42, 6,8 5 [17] 1/1 2/2 H16 9, 9,4 13, 5,9 85 [29] 1/1 2/2 H17 1, 9,7 19, 5,6 69 [23] 1/1 2/2 H18 12, 9,8 48, 5,6 42 [14] 1/1 2/2 H19 7,6 7,8 15, 3,9 46 [18] 1/1 2/2 H2 9,7 7,4 56, 3, 47 [17] 1/1 2/2 H21 5,9 5,7 9,5 3,9 32 [11] 1/1 2/2 H22 7, ,1 6,6 52 [2] 2/2 2/2 H ,4 5,4 22 [74] 1/1 1/1 H24 5, ,2 5,6 34 [11] 2/2 2/2 H25 36, , 25, 44 [14] 2/2 2/2 H26 46, , 15, 95 [31] 2/2 2/2 H , 5, 52 [17] 1/1 1/1 H28 31, --- 1, 9,8 6 [2] 2/2 2/2 H29 39, 19, 38, 4, 68 [23] 2/2 2/ [] [] pg/m ,3pg/m

21 14 29 PCB [] PCB H [33] 12/12 34/34 H , /35 35/ [2.2] H /34 34/34 H , [.98] H ,5 2 H , [.14] H H , [.3] H H /24 24/24.37 [.13] H /22 22/22 H /22 22/22.8 [.3] H , /36 36/36 pg/m 3 H , /34 34/34.75 [.26] H /34 34/34 H /35 35/ [2.5] H /35 35/35 H /35 35/35 18 [5.9] H tr(17) H /35 35/35 26 [8.5] H tr(16) 35/35 35/35 H , /35 35/35 2 [6.5] H tr(19) 35/35 35/35 H , [1.4] 36/36 36/36 H [2.] 35/35 35/35 H , [2.7] H , [2.3] 1[] []

22 [1] PCB (pg/l) [](pg/l) [2.5] [2.5] [5.] 17 1 [3.2] 18 9 [3] [2.9] [3.] 21 1 [4] [24] [1.7] [15] [8] [2.9] [7.3] [2.7] [5.5] PCB [1] PCB (pg/g-dry) 12, 1, 8, 6, 4, 2, [] (pg/g-dry) 14 1 [3.5] 15 1 [3.2] [2.6] [2.1] 18 4 [1] [1.5] [1.2] [2.1] [22] [4.5] [18] [13] [21] [22] [18] [5.] PCB 261

23 [1] PCB 2, 15, 1, 5, [] [8.4] 15 5 [17] [29] [23] [14] [18] 2 47 [17] [11] [2] [74] [11] [14] [31] [17] 28 6 [2] [23] PCB [1] PCB 3 pg/m PCB [] (pg/m 3 ) [33] [2.2] [.98] [.14] 18.8 [.3] [.13] 2.8 [.3] [.26] [2.5] [5.9] [8.5] 25 2 [6.5] [1.4] [2.] [2.7] [2.3] 262

24 [2] HCB HCB 54 8 POPs pg/l pg/l HCB HCB [] H , [.2] 114/114 38/38 H [2] 36/36 36/36 H16 3 tr(29) 18 tr(11) 3 [8] 38/38 38/38 H tr(6) 15 [5] 47/47 47/47 H18 16 tr(12) 19 nd 16 [5] 46/48 46/48 H tr(4) 8 [3] 48/48 48/48 H [1] 48/48 48/48 H [.2] 49/49 49/49 (pg/l) H22 tr(1) tr(8) 12 nd 13 [4] 39/49 39/49 H tr(3) 5 [2] 49/49 49/49 H [.7] 48/48 48/48 H tr(4) 7 [2] 48/48 48/48 H [.4] 48/48 48/48 H [.6] 48/48 48/48 H [.3] 48/48 48/48 H [.8] 47/47 47/ pg/g-dry , pg/g-dry

25 14 29 HCB HCB [] H , [.3] 189/189 63/63 H , 5 4 [2] 186/186 62/62 H , tr(6) 7 [3] 189/189 63/63 H , 13 3 [1] 189/189 63/63 H , [1.] 192/192 64/64 H , nd 5 [2] 191/192 64/64 H , [.8] 192/192 64/64 H , nd 1.8 [.7] 19/192 64/64 (pg/g-dry) H , 4 3 [1] 64/64 64/64 H , 11 7 [3] 64/64 64/64 H , 3 3 [1] 63/63 63/63 H , [1.8] 63/63 63/63 H ,6 tr(4) 6 [2] 63/63 63/63 H , 4 3 [1] 62/62 62/62 H ,4 4 3 [1] 62/62 62/62 H , 3 3 [1] 62/62 62/ pg/g-wet pg/g-wet pg/g-wet ,1pg/g-wet pg/g-wet ,9pg/g-wet HCB HCB [] H [.6] 38/38 8/8 H tr(21) 23 [7.5] 3/3 6/6 H [4.6] 31/31 7/7 H [3.8] 31/31 7/7 H [1] 31/31 7/7 H [3] 31/31 7/7 H [3] 31/31 7/7 H [2] 31/31 7/7 H tr(4) 5 [2] 6/6 6/6 H [1] 4/4 4/4 H [2.8] 5/5 5/5 H nd 31 [1] 4/5 4/5 H [3] 3/3 3/3 H tr(14) 2 [6.5] 3/3 3/3 H [2.7] 3/3 3/3 H [1.3] 3/3 3/3 H [.6] 7/7 14/14 H , [7.5] 7/7 14/14 H , [4.6] 7/7 14/14 H , [3.8] 8/8 16/16 H , [1] 8/8 16/16 H , [3] 8/8 16/16 H , [3] 85/85 17/17 H , 29 4 [2] 9/9 18/18 H , [2] 18/18 18/18 H , [1] 18/18 18/18 H , [2.8] 19/19 19/19 H , [1] 19/19 19/19 H , [3] 19/19 19/19 H , [6.5] 19/19 19/19 H , [2.7] 19/19 19/19 H , [1.3] 19/19 19/19 264

26 HCB [] H14 1, 1,2 1, [.6] 1/1 2/2 H15 1,8 2, 4, [7.5] 1/1 2/2 H ,3 2, [4.6] 1/1 2/2 H17 1, 1,1 2, [3.8] 1/1 2/2 H ,1 2, [1] 1/1 2/2 H ,1 2, 42 7 [3] 1/1 2/2 H2 88 1,1 2, [3] 1/1 2/2 H ,5 4 4 [2] 1/1 2/2 H ,9 5 5 [2] 2/2 2/2 H [1] 1/1 1/1 H , [2.8] 2/2 2/2 H25 3, ,2 2,9 31 [1] 2/2 2/2 H , [3] 2/2 2/2 H [6.5] 1/1 1/1 H28 1, , [2.7] 2/2 2/2 H29 1,1 2,6 4, [1.3] 2/2 2/ pg/m pg/m HCB HCB [] H , 57.9 [.3] 12/12 34/34 H /35 35/ [.78] H /34 34/34 H [.37] H H [.34] H H [.7] H H /24 24/24.9 [.3] H /22 22/22 H /22 22/22.22 [.8] H /36 36/36 (pg/m 3 H /34 34/34 ).6 [.2] H /34 34/34 H [.7] H H /35 35/ [.75] H H /36 36/ [1.4] H /36 36/36 H /36 36/ [1.3] H /36 36/36 H [.5] 36/36 36/36 H [.2] 35/35 35/35 H [.3] H [.2] 265

27 [2] HCB (pg/l) [](pg/l) 14.6 [.2] 15 5 [2] 16 3 [8] [5] [5] 19 8 [3] 2 3 [1] 21.5 [.2] [4] 23 5 [2] [.7] 25 7 [2] 26.9 [.4] [.6] 28.9 [.3] [.8] HCB [2] HCB (pg/g-dry) [](pg/g-dry) 14.9 [.3] 15 4 [2] 16 7 [3] 17 3 [1] [1.] 19 5 [2] 2 2. [.8] [.7] 22 3 [1] 23 7 [3] 24 3 [1] [1.8] 26 6 [2] 27 3 [1] 28 3 [1] 29 3 [1] HCB 266

28 [2] HCB [] [.6] [7.5] [4.6] [3.8] 18 3 [1] 19 7 [3] 2 7 [3] 21 4[2] 22 5 [2] 23 4 [1] [2.8] [1] 26 1 [3] 27 2 [6.5] [2.7] [1.3] HCB [2] HCB pg/m HCB [] (pg/m 3 ) 14.9 [.3] [.78] [.37] [.34] [.7] 19.9 [.3] 2.22 [.8] 21.6 [.2] [.7] [.75] [1.4] [1.3] [.5] 27.5 [.2] 28.8 [.3] 29.5 [.2] 267

29 [3] POPs [] H nd.6 [.2] 93/114 37/38 H nd.6 [.2] 34/36 34/36 H16 tr(1.5) tr(1.8) 13 nd 2 [.4] 33/38 33/38 H17 tr(.6) tr(.7) 5.7 nd.9 [.3] 32/47 32/47 (pg/l) H18 nd nd 4.4 nd 1.7 [.6] 18/48 18/48 H19 tr(.6) tr(.6) 9.5 nd 1. [.3] 34/48 34/48 H2 tr(.8) tr(.7) 21 nd 1.4 [.6] 26/48 26/48 H nd.7 [.3] 32/49 32/ [] (pg/g-dry) H nd 6 [2] 149/189 56/63 H , nd 2 [.6] 178/186 6/62 H nd 2 [.6] 17/189 62/63 H nd 1.4 [.5] 173/189 62/63 H nd 1.9 [.6] 184/192 64/64 H nd 1.8 [.6] 172/192 6/64 H nd 3 [1] 153/192 56/64 H nd.5 [.2] 18/192 64/

30 14 26 [] H14 tr(1.6) nd 34 nd 4.2 [1.4] 12/38 4/8 H15 tr(1.7) tr(.85) 51 nd 2.5 [.84] 15/3 3/6 H16 tr(2.5) tr(1.6) 46 nd 4. [1.3] 16/31 4/7 H17 tr(1.8) nd 84 nd 3.5 [1.2] 11/31 3/7 H18 tr(2) nd 19 nd 4 [2] 11/31 3/7 H19 tr(2) nd 26 nd 5 [2] 5/31 2/7 H2 tr(2) nd 2 nd 5 [2] 5/31 3/7 H21 tr(1.6) tr(.8) 89 nd 2.1 [.8] 16/31 6/7 H26 nd nd nd nd 1.8 [.7] /3 /3 H14 nd nd tr(2.) nd 4.2 [1.4] 1/7 1/14 H15 nd nd tr(1.9) nd 2.5 [.84] 16/7 7/14 H16 nd nd tr(2.4) nd 4. [1.3] 5/7 2/14 H17 nd nd 6.4 nd 3.5 [1.2] 11/8 5/16 H18 nd nd tr(2) nd 4 [2] 2/8 2/16 H19 nd nd tr(2) nd 5 [2] 2/8 2/16 H2 nd nd tr(2) nd 5 [2] 1/85 1/17 H21 nd nd 3.1 nd 2.1 [.8] 22/9 7/18 H26 nd nd 2.4 nd 1.8 [.7] 4/19 4/19 H14 nd nd nd nd 4.2 [1.4] /1 /2 H15 nd nd nd nd 2.5 [.84] /1 /2 H16 nd nd nd nd 4. [1.3] /1 /2 H17 nd nd nd nd 3.5 [1.2] /1 /2 H18 nd nd nd nd 4 [2] /1 /2 H19 nd nd nd nd 5 [2] /1 /2 H2 nd nd nd nd 5 [2] /1 /2 H21 nd nd nd nd 2.1 [.8] /1 /2 H26 nd --- nd nd 1.8 [.7] /2 / [] H14 tr(.3) nd 3.2 nd.6 [.2] 41/12 19/34 H nd 34/35 34/35.23 [.77] H /34 34/34 H16 tr(.12) nd 14 nd 15/37 15/37.15 [.5] H16 tr(.8) nd 13 nd 14/37 14/37 H nd 29/37 29/37.8 [.3] H17 tr(.4) nd 1.8 nd 9/37 9/37 H nd 31/37 31/37 (pg/m 3.14 [.5] ) H18 tr(.5) nd 1.1 nd 16/37 16/37 H nd 35/36 35/36.5 [.2] H nd 34/36 34/36 H tr(.2) 25/25 25/25.4 [.2] H nd 22/25 22/25 H21.7 nd 1 nd 1/25 1/25.4 [.2] H21 tr(.3) nd 1.8 nd 8/24 8/24 H26 nd nd 17 nd 12 [4] 6/34 6/

31 [3] [](pg/l) 14.6 [.2] 15.6 [.2] 16 2 [.4] 17.9 [.3] [.6] [.3] [.6] 21.7 [.3] (pg/l) / [3] (pg/g-dry) [](pg/g-dry) 14 6 [2] 15 2 [.6] 16 2 [.6] [.5] [.6] [.6] 2 3 [1] 21.5 [.2]

32 [3] [](pg/gwet) [1.4] [.84] 16 4 [1.3] [1.2] 18 4 [2] 19 5 [2] 2 5 [2] [.8] [.7] / [3] 2.5 pg/m [] (pg/m 3 ) 14.6 [.2] [.77] [.5] 17.8 [.3] [.5] 19.5 [.2] 2.4 [.2] 21.4 [.2] [4] /

33 [4] POPs [] (pg/l) H [.6] 114/114 38/38 H [.3] 36/36 36/36 H [.5] 38/38 38/38 H [.34] 47/47 47/47 H [1] 48/48 48/48 H [.7] 48/48 48/48 H [.6] 48/48 48/48 H [.2] 49/49 49/49 H [.6] 49/49 49/49 H [.2] 48/48 48/ [] (pg/g-dry) H ,3 4 3 [1] 189/189 63/63 H ,1 nd 4 [2] 184/186 62/62 H ,7 tr(1.9) 3 [.9] 189/189 63/63 H ,2 tr(2) 3 [1] 189/189 63/63 H ,5 tr(1.7) 2.9 [1.] 192/192 64/64 H ,7 tr(1.2) 2.7 [.9] 192/192 64/64 H ,9 tr(.7) 1.2 [.5] 192/192 64/64 H , [.3] 192/192 64/64 H ,2 2 5 [2] 64/64 64/

34 14 26 [] H , tr(7) 12 [4] 38/38 8/8 H , [1.6] 3/3 6/6 H , [1] 31/31 7/7 H , [3.4] 31/31 7/7 H , 3 7 [3] 31/31 7/7 H , 37 9 [3] 31/31 7/7 H , 47 9 [3] 31/31 7/7 H , 48 7 [2] 31/31 7/7 H , [1] 4/4 4/4 H [1] 3/3 3/3 H , [4] 7/7 14/14 H , [1.6] 7/7 14/14 H ,8 tr(23) 31 [1] 7/7 14/14 H , [3.4] 8/8 16/16 H , [3] 8/8 16/16 H , [3] 8/8 16/16 H , [3] 85/85 17/17 H , [2] 9/9 18/18 H , [1] 18/18 18/18 H , 27 3 [1] 19/19 19/19 H14 1,1 1,1 1, [4] 1/1 2/2 H15 1,3 1,4 2, [1.6] 1/1 2/2 H [1] 1/1 2/2 H , [3.4] 1/1 2/2 H , [3] 1/1 2/2 H [3] 1/1 2/2 H , [3] 1/1 2/2 H [2] 1/1 2/2 H [1] 1/1 1/1 H [1] 2/2 2/ [] H [.2] 12/12 34/34 H /35 35/ [.7] H tr(.82) 34/34 34/34 H [.11] H H [.24] H H [.1] H (pg/m 3 ) H /36 36/36.18 [.7] H /36 36/36 H [.9] H H [.2] H H /35 35/35.42 [.14] H H [.11] 36/36 36/

35 [4] (pg/l) [](pg/l) [.6] 15.7 [.3] 16 2 [.5] [.34] 18 3 [1] [.7] [.6] 21.6 [.2] [.6] 26.5 [.2] [4] (pg/g-dry) [](pg/g-dry) 14 3 [1] 15 4 [2] 16 3 [.9] 17 3 [1] [1.] [.9] [.5] 21.8 [.3] 23 5 [2]

36 [4] [] [4] [1.6] [1] [3.4] 18 7 [3] 19 9 [3] 2 9 [3] 21 7[2] 23 3 [1] 26 3 [1] [4] 2 pg/m [] (pg/m 3 ) 14.6 [.2] [.7] [.11] [.24] 18.3 [.1] [.7] 2.24 [.9] 21.6 [.2] [.14] [.11]

37 [5] POPs [] (pg/l) H14 tr(4.8) tr(5.5) 31 nd 6. [2.] 11/114 36/38 H [.3] 36/36 36/36 H tr(.7) 2 [.5] 38/38 38/38 H nd 1.1 [.4] 45/47 45/47 H nd 1.3 [.4] 44/48 44/48 H nd 1.9 [.6] 46/48 46/48 H nd 3 [1] 45/48 45/48 H nd.7 [.3] 39/49 39/49 H nd 1.6 [.6] 47/49 47/49 H tr(.4).5 [.2] 48/48 48/ [] (pg/g-dry) H , nd 6 [2] 141/189 54/63 H , nd 5 [2] 15/186 53/62 H ,9 nd 3 [.9] 182/189 63/63 H , nd 2.6 [.9] 17/189 61/63 H , nd 4 [1] 178/192 63/64 H , nd 5 [2] 151/192 55/64 H , nd 1.9 [.7] 168/192 61/64 H , nd 1.6 [.6] 168/192 63/64 H ,1 nd 1.1 [.4] 59/64 59/

38 14 26 [] H , nd 18 [6] 35/38 7/8 H , [1.6] 3/3 6/6 H ,6 tr(5.7) 12 [4.2] 31/31 7/7 H ,1 nd 17 [5.5] 27/31 7/7 H ,1 tr(5) 11 [4] 31/31 7/7 H , tr(6) 9 [3] 31/31 7/7 H ,5 tr(6) 8 [3] 31/31 7/7 H ,4 tr(5) 7 [3] 31/31 7/7 H tr(3) 4 [2] 4/4 4/4 H [1] 3/3 3/3 H nd 18 [6] 54/7 13/14 H nd 4.8 [1.6] 67/7 14/14 H nd 12 [4.2] 57/7 13/14 H17 19 tr(16) 2,1 nd 17 [5.5] 58/8 12/16 H18 13 tr(1) 15 nd 11 [4] 66/8 16/16 H nd 9 [3] 69/8 15/16 H nd 8 [3] 63/85 14/17 H nd 7 [3] 86/9 18/18 H nd 4 [2] 16/18 16/18 H nd 3 [1] 18/19 18/19 H nd 18 [6] 7/1 2/2 H [1.6] 1/1 2/2 H16 tr(11) nd 12 [4.2] 5/1 1/2 H nd 17 [5.5] 7/1 2/2 H tr(4) 11 [4] 1/1 2/2 H nd 9 [3] 9/1 2/2 H nd 8 [3] 5/1 1/2 H tr(3) 7 [3] 1/1 2/2 H tr(3) tr(3) 4 [2] 1/1 1/1 H [1] 2/2 2/ [] H nd.9 [.3] 9/12 32/34 H /35 35/35.42 [.14] H /34 34/34 H tr(.54).14 [.48] H nd 36/37 36/37 H17 tr(.4) tr(.3) 2.9 nd 27/37 27/37.5 [.2] H17 nd nd.7 nd 8/37 8/37 H nd 32/37 32/37.3 [.1] H18 nd nd 5. nd 7/37 7/37 (pg/m 3 ) H tr(.6) 36/36 36/36.9 [.4] H nd 33/36 33/36 H tr(.6).1 [.4] H nd 35/37 35/37 H nd 36/37 36/37.9 [.4] H nd 36/37 36/37 H nd 34/35 34/35.9 [.4] H nd 33/37 33/37 H nd.2 [.7] 32/36 32/

39 [5] (pg/l) [](pg/l) [2.] 15.7 [.3] 16 2 [.5] [.4] [.4] [.6] 2 3 [1] 21.7 [.3] [.6] 26.5 [.2] [5] (pg/g-dry) [](pg/g-dry) 14 6 [2] 15 5 [2] 16 3 [.9] [.9] 18 4 [1] 19 5 [2] [.7] [.6] [.4]

40 [5] [] [6] [1.6] [4.2] [5.5] [4] 19 9 [3] 2 8 [3] 21 7[3] 23 4 [2] 26 3 [1] [5].8 pg/m [] (pg/m 3 ) 14.9 [.3] [.14] [.48] 17.5 [.2] 18.3 [.1] 19.9 [.4] 2.1 [.4] 21.9 [.4] 23.9 [.4] 26.2 [.7] /

41 [6] DDT DDT HCH p,p'-ddt POPs 16 DDT DDT p,p'-ddt o,p'-ddt DDT p,p'-dde o,p'-dde p,p'-ddd o,p'-ddd p,p'-ddt p,p'-dde p,p'-ddd o,p'-ddt o,p'-dde o,p'-ddd p,p'-ddt p,p'-dde p,p'-ddd o,p'-ddt o,p'-dde o,p'-ddd p,p'-ddt p,p'-dde p,p'-ddd p,p'-ddt p,p'-dde p,p'-ddd p,p'-ddt [] H [.2] 114/114 38/38 H tr(2.8) 3 [.9] 36/36 36/36 H nd 6 [2] 36/38 36/38 H [1] 47/47 47/47 H tr(1.6) 1.9 [.6] 48/48 48/48 (pg/l) H nd 1.7 [.6] 46/48 46/48 H ,2 nd 1.2 [.5] 47/48 47/48 H [.6] 49/49 49/49 H ,5 tr(1.) 2.4 [.8] 49/49 49/49 H nd.4 [.1] 47/48 47/48 28

42 p,p'-dde [] H [.2] 114/114 38/38 H [2] 36/36 36/36 H tr(6) 8 [3] 38/38 38/38 H [2] 47/47 47/47 H tr(4) 7 [2] 48/48 48/48 (pg/l) H tr(2) 4 [2] 48/48 48/48 H [.4] 48/48 48/48 H [.4] 49/49 49/49 H , [.8] 49/49 49/49 H [.2] 48/48 48/48 p,p'-ddd [] H [.8] 114/114 38/38 H [.5] 36/36 36/36 H tr(2.4) 3 [.8] 38/38 38/38 H tr(1.8) 1.9 [.64] 47/47 47/47 H [.5] 48/48 48/48 (pg/l) H tr(1.5) 1.7 [.6] 48/48 48/48 H [.2] 48/48 48/48 H [.2] 49/49 49/49 H [.8] 49/49 49/49 H [.4] 48/48 48/ p,p'-ddt p,p'-dde p,p'-ddd p,p'-ddt [] H , tr(5) 6 [2] 189/189 63/63 H , 3 2 [.4] 186/186 62/62 H , 7 2 [.5] 189/189 63/63 H ,7, [.34] 189/189 63/63 H , [.5] 192/192 64/64 (pg/g-dry) H , [.5] 192/192 64/64 H ,4, [.5] 192/192 64/64 H ,1, [.4] 192/192 64/64 H , [.9] 64/64 64/64 H , tr(.2).4 [.2] 63/63 63/63 p,p'-dde [] (pg/g-dry) p,p'-ddd (pg/g-dry) H , [.9] 189/189 63/63 H , [.3] 186/186 62/62 H , 8 3 [.8] 189/189 63/63 H , [.94] 189/189 63/63 H , [.3] 192/192 64/64 H , [.4] 192/192 64/64 H , [.7] 192/192 64/64 H , [.3] 192/192 64/64 H , 11 5 [2] 64/64 64/64 H , [.6] 63/63 63/63 [] H , tr(2.2) 2.4 [.8] 189/189 63/63 H , [.3] 186/186 62/62 H , 4 2 [.7] 189/189 63/63 H , [.64] 189/189 63/63 H , [.2] 192/192 64/64 H , [.4] 192/192 64/64 H , [.4] 192/192 64/64 H , [.2] 192/192 64/64 H , [.5] 64/64 64/64 H , [1.4] 63/63 63/

43 14 25 p,p'-ddt p,p'-dde p,p'-ddd p,p'-ddt [] H , [1.4] 38/38 8/8 H , [3.5] 3/3 6/6 H , [1.1] 31/31 7/7 H , [1.7] 31/31 7/7 H , [2] 31/31 7/7 H , [2] 31/31 7/7 H , [2] 31/31 7/7 H , [1] 31/31 7/7 H [1] 6/6 6/6 H [1.1] 5/5 5/5 p,p'-dde H , [1.4] 7/7 14/14 H ,9 tr(3.7) 11 [3.5] 7/7 14/14 H , [1.1] 7/7 14/14 H ,4 tr(3.8) 5.1 [1.7] 8/8 16/16 H , tr(5) 6 [2] 8/8 16/16 H ,8 9 5 [2] 8/8 16/16 H ,9 7 5 [2] 85/85 17/17 H , 4 3 [1] 9/9 18/18 H ,1 7 3 [1] 18/18 18/18 H , [1.1] 19/19 19/19 H , [1.4] 1/1 2/2 H , [3.5] 1/1 2/2 H [1.1] 1/1 2/2 H [1.7] 1/1 2/2 H , [2] 1/1 2/2 H , [2] 1/1 2/2 H [2] 1/1 2/2 H , [1] 1/1 2/2 H nd 3 [1] 1/2 1/2 H [1.1] 2/2 2/2 [] H14 1, 1,7 6, [.8] 38/38 8/8 H15 1,2 1, 6, [1.9] 3/3 6/6 H16 1,3 1,4 8, [2.7] 31/31 7/7 H17 1,2 1,6 6, [2.8] 31/31 7/7 H18 1, 1,2 6, [.7] 31/31 7/7 H19 1,1 1,2 5, [1] 31/31 7/7 H2 9 1,1 5, [1] 31/31 7/7 H ,1 6, [1] 31/31 7/7 H22 1,1 1,3 6, [1] 6/6 6/6 H ,6 3, [1.4] 5/5 5/5 H14 2,9 2,2 98, [.8] 7/7 14/14 H15 2, 2,2 12, [1.9] 7/7 14/14 H16 3, 2,1 52, [2.7] 7/7 14/14 H17 2,4 2,4 73, [2.8] 8/8 16/16 H18 2,2 2,6 28, [.7] 8/8 16/16 H19 2,2 2, 22, 16 3 [1] 8/8 16/16 H2 2,5 2, 53, 32 3 [1] 85/85 17/17 H21 2,3 2,1 2, 26 4 [1] 9/9 18/18 H22 2,3 2,1 13, 26 3 [1] 18/18 18/18 H25 2,9 2,8 16, [1.4] 19/19 19/19 H14 36, 6, 17, 8,1 2.4 [.8] 1/1 2/2 H15 66, 76, 24, 18, 5.7 [1.9] 1/1 2/2 H16 34, 65, 2, 6,8 8.2 [2.7] 1/1 2/2 H17 44, 86, 3, 7,1 8.5 [2.8] 1/1 2/2 H18 38, 57, 16, 5,9 1.9 [.7] 1/1 2/2 H19 4, 56, 32, 6,7 3 [1] 1/1 2/2 H2 51, 79, 16, 7,5 3 [1] 1/1 2/2 H21 3, 64, 22, 4,3 4 [1] 1/1 2/2 H22 32, , 6,3 3 [1] 2/2 2/2 H25 17, , 17, 4.3 [1.4] 2/2 2/2 282

44 p,p'-ddd [] H , [1.8] 38/38 8/8 H ,6 tr(7.5) 9.9 [3.3] 3/3 6/6 H , [.7] 31/31 7/7 H , [.97] 31/31 7/7 H , [.9] 31/31 7/7 H ,5 7 3 [1] 31/31 7/7 H ,3 6 3 [1] 31/31 7/7 H , [.9] 31/31 7/7 H [.5] 6/6 6/6 H , [.7] 5/5 5/5 H , [1.8] 7/7 14/14 H , [3.3] 7/7 14/14 H , [.7] 7/7 14/14 H , [.97] 8/8 16/16 H , [.9] 8/8 16/16 H , [1] 8/8 16/16 H , [1] 85/85 17/17 H , [.9] 9/9 18/18 H , [.5] 18/18 18/18 H , [.7] 19/19 19/19 H , [1.8] 1/1 2/2 H , [3.3] 1/1 2/2 H , [.7] 1/1 2/2 H , [.97] 1/1 2/2 H , [.9] 1/1 2/2 H ,3 7 3 [1] 1/1 2/2 H , [1] 1/1 2/2 H , [.9] 1/1 2/2 H , [.5] 2/2 2/2 H [.7] 2/2 2/ p,p'-ddt p,p'-dde p,p'-ddd [] p,p'-ddt H [.8] 12/12 34/34 H /35 35/35.14 [.46] H /34 34/34 H [.74] H H [.54] H H [.6] H H /36 36/36 (pg/m 3.7 [.3] ) H /36 36/36 H [.3] H H [.3] H H [.3] H H /36 36/36.11 [.4] H /36 36/36 H [.5] 35/35 35/35 283

45 [] p,p'-dde H [.3] 12/12 34/34 H /35 35/35.4 [.13] H /34 34/34 H [.39] H H [.34] H H [.3] H H /36 36/36 (pg/m 3.4 [.2] ) H /36 36/36 H [.2] H H [.3] H H tr(.41).62 [.21] H tr(.47) H /36 36/36.1 [.3] H /36 36/36 H [.4] 35/35 35/35 [] p,p'-ddd H nd.18 [.6] 11/12 34/34 H /35 35/35.54 [.18] H tr(.37) 34/34 34/34 H tr(.36).53 [.18] H tr(.25) H tr(.7).16 [.5] H17 tr(.6) tr(.7).29 nd 28/37 28/37 H nd 36/37 36/37.13 [.4] H18.14 tr(.12).99 nd 36/37 36/37 H /36 36/36 (pg/m 3.11 [.4] ) H /36 36/36 H [.9] H H [.1] H tr(.2) H [.1] H H /36 36/36.18 [.7] H tr(.15) 36/36 36/36 H27 nd nd tr(.31) nd.33 [.11] 17/35 17/ o,p'-ddt o,p'-dde o,p'-ddd o,p'-ddt o,p'-dde o,p'-ddd o,p'-ddt [] H [.4] 114/114 38/38 H tr(1.5) 3 [.7] 36/36 36/36 H16 tr(4.5) 5 85 nd 5 [2] 29/38 29/38 H nd 3 [1] 42/47 42/47 H [.8] 48/48 48/48 (pg/l) H19 tr(2.1) tr(2.2) 86 nd 2.5 [.8] 38/48 38/48 H nd 1.4 [.5] 44/48 44/48 H [.6] 49/49 49/49 H tr(1.2) 7 nd 1.5 [.5] 43/49 43/49 H nd.4 [.2] 42/48 42/48 284

46 o,p'-dde [] H nd.9 [.3] 113/114 38/38 H tr(.42).8 [.3] 36/36 36/36 H tr(.6) 2 [.5] 38/38 38/38 H [.4] 47/47 47/47 H18 tr(1.6) tr(1.4) 21 nd 2.6 [.9] 28/48 28/48 (pg/l) H19 tr(1.5) tr(1.1) 21 nd 2.3 [.8] 29/48 29/48 H nd.7 [.3] 39/48 39/48 H nd.22 [.9] 47/49 47/49 H tr(.13).24 [.9] 49/49 49/49 H nd.3 [.1] 36/48 36/48 o,p'-ddd [] H nd.6 [.2] 113/114 38/38 H [.3] 36/36 36/36 H tr(.7) 2 [.5] 38/38 38/38 H tr(.5) 1.2 [.4] 47/47 47/47 H nd.8 [.3] 4/48 4/48 (pg/l) H tr(.3).8 [.3] 48/48 48/48 H nd.8 [.3] 47/48 47/48 H [.9] 49/49 49/49 H tr(.5).6 [.2] 49/49 49/49 H [.8] 48/48 48/ o,p'-ddt o,p'-dde o,p'-ddd o,p'-ddt [] H , nd 6 [2] 183/189 62/63 H ,2 nd.8 [.3] 185/186 62/62 H , tr(1.1) 2 [.6] 189/189 63/63 H ,.8.8 [.3] 189/189 63/63 H , tr(.8) 1.2 [.4] 192/192 64/64 (pg/g-dry) H , nd 1.8 [.6] 186/192 63/64 H , tr(.7) 1.5 [.6] 192/192 64/64 H , nd 1.2 [.5] 19/192 64/64 H , [.4] 64/64 64/64 H ,4 nd.4 [.2] 62/63 62/63 o,p'-dde [] (pg/g-dry) o,p'-ddd (pg/g-dry) H , nd 3 [1] 188/189 63/63 H , tr(.5).6 [.2] 186/186 62/62 H , nd 3 [.8] 184/189 63/63 H , nd 2.6 [.9] 181/189 62/63 H , tr(.4) 1.1 [.4] 192/192 64/64 H , nd 1.2 [.4] 186/192 63/64 H , nd 1.4 [.6] 186/192 63/64 H , nd.6 [.2] 191/192 64/64 H , tr(.7) 1.2 [.5] 64/64 64/64 H , tr(.5).8 [.3] 63/63 63/63 [] H , nd 6 [2] 184/189 62/63 H ,8 tr(1.) 2 [.5] 186/186 62/62 H , tr(.7) 2 [.5] 189/189 63/63 H , tr(.8) 1. [.3] 189/189 63/63 H , tr(.3).5 [.2] 192/192 64/64 H , tr(.5) 1. [.4] 192/192 64/64 H ,.5.3 [.1] 192/192 64/64 H ,.5.5 [.2] 192/192 64/64 H ,9 tr(.8).9 [.4] 64/64 64/64 H ,2 tr(.7) 1.2 [.5] 63/63 63/

47 14 25 o,p'-ddt o,p'-dde o,p'-ddd o,p'-ddt [] H [4] 38/38 8/8 H [.97] 3/3 6/6 H [.61] 31/31 7/7 H [.86] 31/31 7/7 H [1] 31/31 7/7 H [1] 31/31 7/7 H [1] 31/31 7/7 H , [.8] 31/31 7/7 H [1] 6/6 6/6 H [1] 5/5 5/5 o,p'-dde H ,3 tr(6) 12 [4] 7/7 14/14 H [.97] 7/7 14/14 H , [.61] 7/7 14/14 H , [.86] 8/8 16/16 H [1] 8/8 16/16 H [1] 8/8 16/16 H [1] 85/85 17/17 H [.8] 9/9 18/18 H [1] 18/18 18/18 H [1] 19/19 19/19 H14 12 tr(1) 58 nd 12 [4] 8/1 2/2 H [.97] 1/1 2/2 H tr(.87) 1.8 [.61] 1/1 2/2 H [.86] 1/1 2/2 H [1] 1/1 2/2 H tr(2) 3 [1] 1/1 2/2 H nd 3 [1] 8/1 2/2 H tr(1.4) 2.2 [.8] 1/1 2/2 H22 nd --- nd nd 3 [1] /2 /2 H25 nd --- tr(1) nd 3 [1] 1/2 1/2 [] H , [1.2] 38/38 8/8 H [1.2] 3/3 6/6 H [.69] 31/31 7/7 H [1.1] 31/31 7/7 H [1] 31/31 7/7 H [.9] 31/31 7/7 H [1] 31/31 7/7 H [1] 31/31 7/7 H [.6] 6/6 6/6 H [1] 5/5 5/5 H , [1.2] 7/7 14/14 H ,5 nd 3.6 [1.2] 67/7 14/14 H ,8 tr(.89) 2.1 [.69] 7/7 14/14 H , tr(1.4) 3.4 [1.1] 8/8 16/16 H ,8 tr(1) 3 [1] 8/8 16/16 H ,4 nd 2.3 [.9] 79/8 16/16 H , tr(1) 3 [1] 85/85 17/17 H ,3 tr(1) 3 [1] 9/9 18/18 H ,8 tr(1.2) 1.5 [.6] 18/18 18/18 H , tr(1) 4 [1] 19/19 19/19 H [1.2] 1/1 2/2 H15 tr(2.3) tr(2.) 4.2 nd 3.6 [1.2] 9/1 2/2 H16 tr(1.) tr(1.1) 3.7 nd 2.1 [.69] 5/1 1/2 H17 tr(1.2) tr(1.9) tr(2.9) nd 3.4 [1.1] 7/1 2/2 H18 tr(1) tr(2) 3 tr(1) 3 [1] 1/1 2/2 H19 tr(1.) tr(1.4) 2.8 nd 2.3 [.9] 6/1 2/2 H2 tr(1) nd 3 nd 3 [1] 5/1 1/2 H21 nd tr(1) tr(2) nd 3 [1] 6/1 2/2 H22 tr(1.1) nd 1.5 [.6] 1/2 1/2 H25 nd --- tr(1) nd 4 [1] 1/2 1/2 286

48 o,p'-ddd [] H ,9 tr(9) 12 [4] 38/38 8/8 H , [2.] 3/3 6/6 H , [1.9] 31/31 7/7 H , [1.1] 31/31 7/7 H , 7 4 [1] 31/31 7/7 H ,2 6 3 [1] 31/31 7/7 H ,1 5 4 [2] 31/31 7/7 H , 5 3 [1] 31/31 7/7 H [.2] 6/6 6/6 H , [.7] 5/5 5/5 H ,1 nd 12 [4] 66/7 14/14 H nd 6. [2.] 66/7 14/14 H ,7 nd 5.7 [1.9] 68/7 14/14 H ,4 nd 3.3 [1.1] 79/8 16/16 H ,1 tr(1) 4 [1] 8/8 16/16 H ,3 nd 3 [1] 78/8 16/16 H , nd 4 [2] 8/85 16/17 H nd 3 [1] 87/9 18/18 H [.2] 18/18 18/18 H nd 1.8 [.7] 18/19 18/19 H tr(8) 12 [4] 1/1 2/2 H tr(5.) 6. [2.] 1/1 2/2 H nd 5.7 [1.9] 9/1 2/2 H [1.1] 1/1 2/2 H [1] 1/1 2/2 H [1] 1/1 2/2 H2 4 tr(3) 14 tr(2) 4 [2] 1/1 2/2 H [1] 1/1 2/2 H [.2] 2/2 2/2 H [.7] 2/2 2/ o,p'-ddt o,p'-dde o,p'-ddd [] o,p'-ddt H [.5] 12/12 34/34 H /35 35/35.12 [.4] H /34 34/34 H [.31] H H [.34] H H [.3] H H /36 36/36 (pg/m 3.3 [.1] ) H /36 36/36 H [.1] H H [.8] H H [.5] H H /36 36/36.54 [.18] H /36 36/36 H [.4] 35/35 35/35 287

49 [] o,p'-dde H [.1] 12/12 34/34 H /35 35/35.2 [.68] H /34 34/34 H [.12] H H [.24] H H nd 36/37 36/37.9 [.3] H H /36 36/36 (pg/m 3.17 [.7] ) H /36 36/36 H [.9] H H [.6] H H [.1] H H /36 36/36.23 [.9] H /36 36/36 H nd.18 [.6] 34/35 34/35 [] o,p'-ddd H nd.21 [.7] 97/12 33/34 H /35 35/35.42 [.14] H /34 34/34 H tr(.52).14 [.48] H16.14 tr(.13).86 nd 35/37 35/37 H tr(.7).1 [.3] H17 tr(.7) tr(.7).21 nd 35/37 35/37 H tr(.5).1 [.3] H nd 34/37 34/37 H /36 36/36 (pg/m 3.5 [.2] ) H tr(.3) 36/36 36/36 H [.1] H H [.1] H tr(.2) H [.1] H tr(.2) H tr(.3) 36/36 36/36.5 [.2] H nd 35/36 35/36 H27 tr(.9) tr(.1).37 nd.2 [.7] 25/35 25/

50 [6-1] p,p'-ddt (pg/l) [] (pg/l) 14.6 [.2] 15 3 [.9] 16 6 [2] 17 4 [1] [.6] [.6] [.5] [.6] [.8] 26.4 [.1] p,p'-ddt [6-1] p,p'-ddt (pg/g-dry) [](pg/g-dry) 14 6 [2] 15 2 [.4] 16 2 [.5] [.34] [.5] [.5] [.5] [.4] [.9] 26.4 [.2] p,p'-ddt 289

51 [6-1] p,p'-ddt [] [1.4] [3.5] [1.1] [1.7] 18 6 [2] 19 5 [2] 2 5 [2] 21 3[1] 22 3 [1] [1.1] p,p'-ddt [6-1] p,p'-ddt 6 pg/m [] (pg/m 3 ) [.8] [.46] [.74] [.54] [.6] 19.7 [.3] 2.7 [.3] 21.7 [.3] 22.1 [.3] [.4] [.5] p,p'-ddt 29

52 [6-2] p,p'-dde (pg/l) [](pg/l) 14.6 [.2] 15 4 [2] 16 8 [3] 17 6 [2] 18 7 [2] 19 4 [2] [.4] [.4] [.8] 26.5 [.2] p,p'-dde [6-2] p,p'-dde (pg/g-dry) 1, [](pg/g-dry) [.9] 15.9 [.3] 16 3 [.8] [.94] [.3] [.4] [.7] 21.8 [.3] 22 5 [2] [.6] p,p'-dde 291

53 [6-2] p,p'-dde 3,5 3, 2,5 2, 1,5 1, [] [1.4] [3.5] [1.1] [1.7] 18 6 [2] 19 5 [2] 2 5 [2] 21 3[1] 22 3 [1] [1.4] p,p'-dde [6-2] p,p'-dde 8 pg/m [] (pg/m 3 ) 14.9 [.3] 15.4 [.13] [.39] [.34] 18.1 [.3] 19.4 [.2] 2.4 [.2] 21.8 [.3] [.21] 25.1 [.3] [.4] p,p'-dde 292

54 [6-3] p,p'-ddd (pg/l) [](pg/l) [.8] 15 2 [.5] 16 3 [.8] [.64] [.5] [.6] 2.6 [.2] 21.4 [.2] 22.2 [.8] [.4] p,p'-ddd [6-3] p,p'-ddd (pg/g-dry) [](pg/g-dry) [.8] 15.9 [.3] 16 2 [.7] [.64] 18.7 [.2] [.4] 2 1. [.4] 21.4 [.2] [.5] [1.4] p,p'-ddd 293

55 [6-3] p,p'-ddd [] [1.8] [3.3] [.7] [.97] [.9] 19 3 [1] 2 3 [1] [.9] [.5] [.7] p,p'-ddd [6-3] p,p'-ddd pg/m [] (pg/m 3 ) [.6] [.18] [.18] [.5] [.4] [.4] 2.25 [.9] 21.3 [.1] 22.2 [.1] [.7] [.11] / p,p'-ddd 294

56 [6-4] o,p'-ddt (pg/l) [](pg/l) [.4] 15 3 [.7] 16 5 [2] 17 3 [1] [.8] [.8] [.5] [.6] [.5] 26.4 [.2] o,p'-ddt [6-4] o,p'-ddt (pg/g-dry) [](pg/g-dry) 14 6 [2] 15.8 [.3] 16 2 [.6] 17.8 [.3] [.4] [.6] [.6] [.5] [.4] 26.4 [.2] o,p'-ddt 295

57 [6-4] o,p'-ddt [] [4] [.97] [.61] [.86] 18 3 [1] 19 3 [1] 2 3 [1] [.8] 22 3 [1] 25 3 [1] o,p'-ddt [6-4] o,p'-ddt 8 pg/m [] (pg/m 3 ) [.5] [.4] [.31] 17.1 [.34] 18.9 [.3] 19.3 [.1] 2.3 [.1] [.8] [.5] [.18] [.4] o,p'-ddt 296

58 [6-5] o,p'-dde (pg/l) [](pg/l) 14.9 [.3] 15.8 [.3] 16 2 [.5] [.4] [.9] [.8] 2.7 [.3] [.9] [.9] 26.3 [.1] o,p'-dde [6-5] o,p'-dde (pg/g-dry) [](pg/g-dry) 14 3 [1] 15.6 [.2] 16 3 [.8] [.9] [.4] [.4] [.6] 21.6 [.2] [.5] 26.8 [.3] o,p'-ddt o,p'-dde 297

59 [6-5] o,p'-dde [] 13 [1,] [1.2] [1.2] [.69] [1.1] 18 3 [1] [.9] 2 3 [1] 21 3[1] [.6] 25 4 [1] o,p'-dde [6-5] o,p'-dde 2 pg/m [] (pg/m 3 ) 14.3 [.1] 15.2 [.68] [.12] [.24] 18.9 [.3] [.7] 2.25 [.9] [.6] 22.4 [.1] [.9] [.6] o,p'-dde 298

60 [6-6] o,p'-ddd (pg/l) [](pg/l) 14.6 [.2] 15.8 [.3] 16 2 [.5] [.4] 18.8 [.3] 19.8 [.3] 2.8 [.3] [.9] 22.6 [.2] 26.2 [.8] o,p'-ddd [6-6] o,p'-ddd (pg/g-dry) [](pg/g-dry) 14 6 [2] 15 2 [.5] 16 2 [.5] [.3] 18.5 [.2] [.4] 2.3 [.1] 21.5 [.2] 22.9 [.4] o,p'-ddt o,p'-ddd 299

61 [6-6] o,p'-ddd [](pg/gwet) [4] [2.] [1.9] [1.1] 18 4 [1] 19 3 [1] 2 4 [2] 21 3[1] 22.6 [.2] [.7] o,p'-ddd [6-6] o,p'-ddd.5 pg/m [] (pg/m 3 ) [.7] [.14] [.48] 17.1 [.3] 18.1 [.3] 19.5 [.2] 2.4 [.1] 21.3 [.1] 22.3 [.1] 25.5 [.2] 27.2 [.7] o,p'-ddd 3

62 [7] POPs 16 cis- trans- γ- cis-trans- cis- trans cis-trans-cis- trans cis-trans-cis- trans cis-trans- cis- trans cis- trans- cis-47 1 pg/l pg/l trans-47 1 pg/l 47 tr(2) 15 pg/l 31

63 14 29 cis- trans- cis- [] H [.3] 114/114 38/38 H [.9] 36/36 36/36 H ,9 1 6 [2] 38/38 38/38 H [1] 47/47 47/47 H [2] 48/48 48/48 H nd 4 [2] 47/48 47/48 (pg/l) H [.6] 48/48 48/48 H [.4] 49/49 49/49 H nd 11 [4] 47/49 47/49 H [.6] 49/49 49/49 H [.6] 48/48 48/48 H [.9] 48/48 48/48 H [1] 47/47 47/47 trans- [] (pg/l) H [.5] 114/114 38/38 H [2] 36/36 36/36 H ,2 5 5 [2] 38/38 38/38 H [1] 47/47 47/47 H tr(4) 7 [2] 48/48 48/48 H nd 2.4 [.8] 47/48 47/48 H [1] 48/48 48/48 H [.3] 49/49 49/49 H22 15 tr(11) 31 nd 13 [4] 44/49 44/49 H [.4] 49/49 49/49 H [.8] 48/48 48/48 H [1] 48/48 48/48 H tr(2) 3 [1] 47/47 47/ cis pg/g-dry ,8 pg/g-dry trans-62 1 pg/g-dry 62 tr(1) 3, pg/g-dry cis- trans- cis- [] H , [.3] 189/189 63/63 H , tr(3.6) 4 [2] 186/186 62/62 H , 4 4 [2] 189/189 63/63 H , [.64] 189/189 63/63 H , tr(.9) 2.4 [.8] 192/192 64/64 H ,5 nd 5 [2] 191/192 64/64 H , tr(2.3) 2.4 [.9] 192/192 64/64 (pg/g-dry) H , [.3] 192/192 64/64 H ,2 tr(4) 6 [2] 64/64 64/64 H , [.4] 64/64 64/64 H , tr(2.6) 2.9 [1.] 63/63 63/63 H ,4 tr(1.9) 2. [.8] 63/63 63/63 H ,8 nd 4.8 [1.6] 61/62 61/62 32

64 trans- [] H , [.6] 189/189 63/63 H , tr(2.4) 4 [2] 186/186 62/62 H , 3 3 [.9] 189/189 63/63 H , [.84] 189/189 63/63 H , [.4] 192/192 64/64 H ,5 nd 2.2 [.8] 191/192 64/64 H , [.8] 192/192 64/64 (pg/g-dry) H , [.7] 192/192 64/64 H , tr(4) 11 [4] 64/64 64/64 H , [.5] 64/64 64/64 H , tr(2.9) 4. [1.3] 63/63 63/63 H , [.7] 63/63 63/63 H , tr(1) 4 [1] 62/62 62/ cis- trans pg/l pg/l cis-47.6 pg/l 47 tr(.6) 36 pg/l trans-47 1 pg/l 47 tr(2) 12 pg/l cis- trans- [] H nd 1.2 [.4] 96/114 35/38 H tr(.6) 2 [.5] 36/36 36/36 H tr(.7) 2 [.5] 38/38 38/38 H nd 1.1 [.4] 46/47 46/47 H18 tr(2.5) tr(2.4) 18 nd 2.8 [.9] 43/48 43/48 H19 tr(2) nd 41 nd 6 [2] 25/48 25/48 H nd 1.9 [.7] 4/48 4/48 (pg/l) H nd 1.1 [.4] 45/49 45/49 H nd.7 [.3] 47/49 47/49 H nd 1.3 [.5] 44/49 44/49 H nd.9 [.4] 44/48 44/48 H nd.9 [.4] 41/48 41/48 H29 nd nd 12 nd 4 [2] 19/47 19/47 cis- [] (pg/l) H [.6] 114/114 38/38 H [.1] 36/36 36/36 H [.2] 38/38 38/38 H [.2] 47/47 47/47 H [.3] 48/48 48/48 H nd 2.4 [.8] 43/48 43/48 H [.3] 48/48 48/48 H [.1] 49/49 49/49 H tr(.9) 1.3 [.4] 49/49 49/49 H [.2] 49/49 49/49 H [.3] 48/48 48/48 H tr(.7).8 [.3] 48/48 48/48 H tr(.6) 1.5 [.6] 47/47 47/47 33

65 trans- [] H [.4] 114/114 38/38 H [.5] 36/36 36/36 H ,1 tr(3) 4 [2] 38/38 38/38 H [.84] 47/47 47/47 H [1.] 48/48 48/48 H tr(2) 5 [2] 48/48 48/48 H [.6] 48/48 48/48 (pg/l) H [.4] 49/49 49/49 H nd 8 [3] 45/49 45/49 H [.5] 49/49 49/49 H [.6] 48/48 48/48 H [.6] 48/48 48/48 H tr(2) 3 [1] 47/47 47/ pg/g-dry pg/g-dry cis-62.7 pg/g-dry ,5 pg/g-dry trans-62 2 pg/g-dry ,6 pg/g-dry cis- trans- [] H nd 1.5 [.5] 153/189 59/63 H nd 1 [.4] 158/186 57/62 H16 tr(2.1) tr(1.3) 14 nd 3 [.8] 129/189 54/63 H tr(1.9) 16 nd 2. [.7] 133/189 51/63 H18 tr(2.5) tr(1.7) 28 nd 2.9 [1.] 141/192 54/64 H19 tr(2.1) tr(1.5) 76 nd 2.5 [.9] 117/192 46/64 H2 tr(2) tr(1) 34 nd 3 [1] 11/192 48/64 (pg/g-dry) H21 2 tr(1) 15 nd 2 [1] 97/192 45/64 H nd 1. [.4] 56/64 56/64 H23 tr(1.6) tr(1.2) 83 nd 2.2 [.9] 36/64 36/64 H24 tr(1.4) tr(1.) 75 nd 1.7 [.7] 38/63 38/63 H nd 1.3 [.5] 5/63 5/63 H29 tr(1) tr(1) 78 nd 3 [1] 41/62 41/62 34

66 cis- [] H ,8 nd 2.1 [.7] 188/189 63/63 H ,5 nd 3 [.9] 184/186 62/62 H ,4 tr(.8) 2 [.6] 189/189 63/63 H ,9 tr(1.1) 1.9 [.64] 189/189 63/63 H ,8 tr(.6) 1.2 [.4] 192/192 64/64 H ,2 nd 1.6 [.6] 191/192 64/64 H , [.2] 192/192 64/64 (pg/g-dry) H , [.4] 192/192 64/64 H , [.3] 64/64 64/64 H ,9 nd 1.1 [.4] 63/64 63/64 H ,9 tr(1) 3 [1] 63/63 63/63 H ,1 tr(.6).7 [.3] 63/63 63/63 H ,5 nd 1.7 [.7] 61/62 61/62 trans- [] H , [.5] 189/189 63/63 H , 2 2 [.6] 186/186 62/62 H , 3 2 [.6] 189/189 63/63 H , [.54] 189/189 63/63 H , [.4] 192/192 64/64 H ,4 tr(1.6) 1.7 [.6] 192/192 64/64 H ,4 tr(1.6) 2.2 [.8] 192/192 64/64 (pg/g-dry) H , [.3] 192/192 64/64 H ,2 tr(3) 6 [2] 64/64 64/64 H , [.3] 64/64 64/64 H , [.8] 63/63 63/63 H , [.4] 63/63 63/63 H ,6 nd 6 [2] 61/62 61/

67 28 cis- trans cis- trans- cis- [] H ,2 26, [.8] 38/38 8/8 H15 1,1 1,4 14, [1.3] 3/3 6/6 H16 1,3 1,6 14, [5.8] 31/31 7/7 H17 1, 96 13, [3.9] 31/31 7/7 H ,1 18, 67 4 [1] 31/31 7/7 H , 59 5 [2] 31/31 7/7 H , 85 5 [2] 31/31 7/7 H21 1,2 1,1 16, 83 4 [2] 31/31 7/7 H22 1,6 2,3 15, 67 4 [2] 6/6 6/6 H , [1] 4/4 4/4 H , [2] 5/5 5/5 H , [4] 5/5 5/5 H [1] 3/3 3/3 H , [.8] 7/7 14/14 H , [1.3] 7/7 14/14 H , [5.8] 7/7 14/14 H , [3.9] 8/8 16/16 H , [1] 8/8 16/16 H ,2 3 5 [2] 8/8 16/16 H , [2] 85/85 17/17 H , [2] 9/9 18/18 H , [2] 18/18 18/18 H , [1] 18/18 18/18 H , [2] 19/19 19/19 H , [4] 19/19 19/19 H , [1] 19/19 19/19 H [.8] 1/1 2/2 H [1.3] 1/1 2/2 H tr(5.8) 18 [5.8] 1/1 2/2 H tr(5.8) 12 [3.9] 1/1 2/2 H [1] 1/1 2/2 H tr(4) 5 [2] 1/1 2/2 H tr(3) 5 [2] 1/1 2/2 H [2] 1/1 2/2 H [2] 2/2 2/2 H [1] 1/1 1/1 H [2] 2/2 2/2 H tr(1) 13 [4] 2/2 2/2 H [1] 2/2 2/2 36

68 trans- [] H , [.8] 38/38 8/8 H , [2.4] 3/3 6/6 H , [16] 31/31 7/7 H ,4 4 1 [3.5] 31/31 7/7 H , [2] 31/31 7/7 H , [2] 31/31 7/7 H , [3] 31/31 7/7 H , 48 4 [1] 31/31 7/7 H , [1] 6/6 6/6 H , [1] 4/4 4/4 H , [2] 5/5 5/5 H , [5.2] 5/5 5/5 H [2] 3/3 3/3 H , [.8] 7/7 14/14 H , [2.4] 7/7 14/14 H ,2 tr(17) 48 [16] 7/7 14/14 H ,1 tr(9.8) 1 [3.5] 76/8 16/16 H , 14 4 [2] 8/8 16/16 H ,1 8 6 [2] 8/8 16/16 H , [3] 85/85 17/17 H ,3 1 4 [1] 9/9 18/18 H ,1 9 3 [1] 18/18 18/18 H ,3 2 4 [1] 18/18 18/18 H , [2] 19/19 19/19 H ,7 tr(14) 16 [5.2] 19/19 19/19 H [2] 19/19 19/19 trans- [] H [.8] 1/1 2/2 H tr(5.9) 7.2 [2.4] 1/1 2/2 H16 nd nd tr(26) nd 48 [16] 5/1 1/2 H tr(4.5) 1 [3.5] 1/1 2/2 H tr(3) 4 [2] 1/1 2/2 H tr(3) 6 [2] 1/1 2/2 H2 tr(5) 9 27 nd 7 [3] 7/1 2/2 H tr(3) 4 [1] 1/1 2/2 H tr(2) 3 [1] 2/2 2/2 H [1] 1/1 1/1 H24 tr(6) tr(4) 7 [2] 2/2 2/2 H tr(1) 16 [5.2] 2/2 2/2 H [2] 2/2 2/

69 14 28 cis- trans- [] cis- H [.2] 12/12 34/34 H , /35 35/35.51 [.17] H /34 34/34 H , [.19] H H , [.54] H H [.4] H H , /36 36/36.1 [.4] H /36 36/36 H [.5] (pg/m 3 ) H H [.6] H H [.6] H H /35 35/ [.42] H tr(.88) H /36 36/ [.51] H nd 35/36 35/36 H /36 36/36.7 [.2] H tr(.5) 36/36 36/36 H [.3] [] trans- H [.2] 12/12 34/34 H , /35 35/35.86 [.29] H /34 34/34 H , [.23] H H , [.14] H H , [.6] H H , /36 36/36.12 [.5] H /36 36/36 H [.6] (pg/m 3 ) H H [.5] H H [.4] H tr(1.) H tr(1.4) 35/35 35/ [.53] H tr(.7) H /36 36/ [.7] H nd 35/36 35/36 H /36 36/36.8 [.3] H tr(.4) 36/36 36/36 H ,1 tr(.7) 1. [.3]

70 cis- trans cis- trans- [] H ,6 nd 3.6 [1.2] 37/38 8/8 H , [2.8] 3/3 6/6 H , [3.1] 31/31 7/7 H , [3.1] 31/31 7/7 H ,4 7 7 [3] 31/31 7/7 H ,2 8 6 [2] 31/31 7/7 H ,1 7 7 [2] 31/31 7/7 H [1] 31/31 7/7 H , [3] 6/6 6/6 H [1] 4/4 4/4 H [1] 5/5 5/5 H [1] 5/5 5/5 H [1] 3/3 3/3 cis- H , [1.2] 7/7 14/14 H [2.8] 7/7 14/14 H , [3.1] 7/7 14/14 H , [3.1] 8/8 16/16 H , 28 7 [3] 8/8 16/16 H , [2] 8/8 16/16 H , [2] 85/85 17/17 H , [1] 9/9 18/18 H , 33 8 [3] 18/18 18/18 H , [1] 18/18 18/18 H [1] 19/19 19/19 H [1] 19/19 19/19 H [1] 19/19 19/19 H [1.2] 1/1 2/2 H , [2.8] 1/1 2/2 H [3.1] 1/1 2/2 H [3.1] 1/1 2/2 H [3] 1/1 2/2 H [2] 1/1 2/2 H [2] 1/1 2/2 H [1] 1/1 2/2 H [3] 2/2 2/2 H [1] 1/1 1/1 H [1] 2/2 2/2 H25 2, ,4 1,9 3 [1] 2/2 2/2 H , [1] 2/2 2/2 [] H [.4] 38/38 8/8 H , [1.6] 3/3 6/6 H , [1.1] 31/31 7/7 H , [1.5] 31/31 7/7 H , [1] 31/31 7/7 H , 26 3 [1] 31/31 7/7 H [1] 31/31 7/7 H , 31 3 [1] 31/31 7/7 H , [1] 6/6 6/6 H , [.7] 4/4 4/4 H [1] 5/5 5/5 H [.7] 5/5 5/5 H [.6] 3/3 3/3 H , [.4] 7/7 14/14 H , [1.6] 7/7 14/14 H , [1.1] 7/7 14/14 H , [1.5] 8/8 16/16 H , [1] 8/8 16/16 H , [1] 8/8 16/16 H , [1] 85/85 17/17 H , [1] 9/9 18/18 H , [1] 18/18 18/18 H , [.7] 18/18 18/18 H , [1] 19/19 19/19 H , [.7] 19/19 19/19 H , [.6] 19/19 19/19 39

71 cis- trans- [] H [.4] 1/1 2/2 H [1.6] 1/1 2/2 H [1.1] 1/1 2/2 H [1.5] 1/1 2/2 H [1] 1/1 2/2 H [1] 1/1 2/2 H [1] 1/1 2/2 H [1] 1/1 2/2 H [1] 2/2 2/2 H [.7] 1/1 1/1 H [1] 2/2 2/2 H [.7] 2/2 2/2 H [.6] 2/2 2/2 [] H ,1 1, [.8] 38/38 8/8 H , [1.2] 3/3 6/6 H , [4.2] 31/31 7/7 H , [2.1] 31/31 7/7 H , [1] 31/31 7/7 H , [3] 31/31 7/7 H , 94 6 [2] 31/31 7/7 H , 79 3 [1] 31/31 7/7 H , 84 4 [2] 6/6 6/6 H , 2 3 [1] 4/4 4/4 H , [1] 5/5 5/5 H , 98 1 [3.4] 5/5 5/5 H [1] 3/3 3/3 H14 1, 9 8, [.8] 7/7 14/14 H , [1.2] 7/7 14/14 H16 1, , [4.2] 7/7 14/14 H , [2.1] 8/8 16/16 H , [1] 8/8 16/16 H , [3] 8/8 16/16 H , [2] 85/85 17/17 H , [1] 9/9 18/18 H22 8 1, 4, [2] 18/18 18/18 H23 1,1 1, 5, 19 3 [1] 18/18 18/18 H24 1,1 1,3 4, [1] 19/19 19/19 H25 1,1 1,1 7, [3.4] 19/19 19/19 H , [1] 19/19 19/19 H , [.8] 1/1 2/2 H15 1,1 1,4 3, [1.2] 1/1 2/2 H , [4.2] 1/1 2/2 H , [2.1] 1/1 2/2 H , [1] 1/1 2/2 H ,4 2 7 [3] 1/1 2/2 H , [2] 1/1 2/2 H [1] 1/1 2/2 H [2] 2/2 2/2 H [1] 1/1 1/1 H [1] 2/2 2/2 H [3.4] 2/2 2/2 H [1] 2/2 2/

72 14 28 cis- trans- [] H nd.24 [.8] 11/12 34/34 H /35 35/35.45 [.15] H /34 34/34 H [.42] H H [.54] H H [.8] H tr(.13) H /36 36/36.5 [.2] H /36 36/36 H [.1] (pg/m 3 ) H H [.2] H H [.1] H H /35 35/35.7 [.3] H H /36 36/36.8 [.3] H /36 36/36 H /36 36/36.3 [.1] H /36 36/36 H [.6] [] cis- H [.1] 12/12 34/34 H /35 35/35.26 [.88] H /34 34/34 H [.24] H H [.3] H H [.5] H tr(.14) H /36 36/36.3 [.1] H /36 36/36 H [.1] (pg/m 3 ) H H [.2] H H [.4] H tr(.6) H /35 35/35.15 [.51] H nd 36/37 36/37 H /36 36/36.12 [.5] H tr(.5) 36/36 36/36 H /36 36/36.7 [.2] H tr(.6) 36/36 36/36 H tr(.13).14 [.5] 311

73 [] trans- H [.1] 12/12 34/34 H , /35 35/35.35 [.12] H /34 34/34 H [.16] H H [.44] H H [.3] H H /36 36/36.9 [.3] H /36 36/36 H [.3] (pg/m 3 ) H H [.3] H H [.3] H tr(.7) H /35 35/ [.35] H tr(.7) H /36 36/ [.41] H tr(.5) 36/36 36/36 H /36 36/36.5 [.2] H /36 36/36 H [.2]

74 [7-1] cis- (pg/l) [](pg/l) 14.9 [.3] 15 3 [.9] 16 6 [2] 17 4 [1] 18 5 [2] 19 4 [2] [.6] [.4] [4] [.6] [.6] [.9] 29 2 [1] cis- [7-1] cis- (pg/g-dry) [](pg/g-dry) 14.9 [.3] 15 4 [2] 16 4 [2] [.64] [.8] 19 5 [2] [.9] 21.7 [.3] 22 6 [2] [.4] [1.] 25 2.[.8] [1.6] cis- 313

75 [7-2] trans- (pg/l) [](pg/l) [.5] 15 5 [2] 16 5 [2] 17 4 [1] 18 7 [2] [.8] 2 3 [1] 21.8 [.3] [4] [.4] [.8] 25 3 [1] 29 3 [1] trans- [7-2] trans- (pg/g-dry) [](pg/g-dry) [.6] 15 4 [2] 16 3 [.9] [.84] [.4] [.8] 2 2. [.8] [.7] [4] [.5] [1.3] [.7] 29 4 [1] trans- 314

76 [7-3] (pg/l) [](pg/l) [.4] 15 2 [.5] 16 2 [.5] [.4] [.9] 19 6 [2] [.7] [.4] 22.7 [.3] [.5] 24.9 [.4] 25.9 [.4] 29 4 [2] / [7-3] (pg/g-dry) [](pg/g-dry) [.5] 15 1 [.4] 16 3 [.8] [.7] [1.] [.9] 2 3 [1] 21 2 [1] [.4] [.9] [.7] [.5] 29 3 [1]

77 [7-4] cis- (pg/l) [](pg/l) [.6] 15.3 [.1] 16.6 [.2] 17.5 [.2] 18.8 [.3] [.8] 2.9 [.3] 21.3 [.1] [.4] 23.6 [.2] 24.8 [.3] 25.8 [.3] [.6] cis- 8 [7-4] cis- (pg/g-dry) [](pg/g-dry) [.7] 15 3 [.9] 16 2 [.6] [.64] [.4] [.6] 2.6 [.2] [.4] 22.9 [.3] [.4] 24 3 [1] 25.7 [.3] [.7] cis- 316

78 [7-5] trans- (pg/l) [](pg/l) [.4] 15 2 [.5] 16 4 [2] [.84] [1.] 19 5 [2] [.7] [.4] 22 8 [3] [.5] [.6] [.6] 29 3 [1] trans- [7-5] trans- (pg/g-dry) [](pg/g-dry) [.5] 15 2 [.6] 16 2 [.6] [.54] [.4] [.6] [.8] 21.9 [.3] 22 6 [2] 23.8 [.3] [.8] [.4] 29 6 [2] trans- 317

79 [7-1] cis- 2, 1,5 1, 5 [] [.8] [1.3] [5.8] [3.9] 18 4 [1] 19 5 [2] 2 5 [2] 21 4[2] 22 4 [2] 23 3 [1] 24 5 [2] [4] 28 3 [1] cis- [7-1] cis- 12 pg/m [] (pg/m 3 ) 14.6 [.2] [.17] [.19] [.54] [.4] 19.1 [.4] 2.14 [.5] [.6] 22.9 [.3] [.42] [.51] 25.7 [.2] 28.9 [.3] cis- 318

80 [7-2] trans trans- [7-2] trans- pg/m [] (pg/m 3 ) 14.6 [.2] [.29] [.23] [.14] [.6] [.5] 2.17 [.6] [.5] [.4] [.53] [.7] 25.8 [.3] [.3] trans- 319

81 [7-3] [] [1.2] [2.8] [3.1] [3.1] 18 7 [3] 19 6 [2] 2 7 [2] 21 4[1] 22 8 [3] 23 3 [1] 24 3 [1] 25 3 [1] 28 3 [1] [7-3] 3 pg/m [] (pg/m 3 ) [.8] [.15] [.42] [.54] [.8] 19.5 [.2] 2.4 [.1] 21.4 [.2] 22.3 [.1] 23.7 [.3] 24.8 [.3] 25.3 [.1] [.6]

82 [7-4] cis [] [.4] [1.6] [1.1] [1.5] 18 3 [1] 19 3 [1] 2 4 [1] 21 3[1] 22 3 [1] [.7] 24 2 [1] [.7] [.6] cis- [7-4] cis- pg/m [] (pg/m 3 ) 14.3 [.1] [.88] [.24] 17.8 [.3] [.5] 19.3 [.1] 2.3 [.1] 21.4 [.2] [.4] [.51] [.5] 25.7 [.2] [.5] cis- 321

83 [7-5] trans- 1,2 1, [] [.8] [1.2] [4.2] [2.1] 18 3 [1] 19 7 [3] 2 6 [2] 21 3[1] 22 4 [2] 23 3 [1] 24 4 [1] 25 1 [3.4] 28 3 [1] trans- [7-5] trans- 1 pg/m [] (pg/m 3 ) 14.3 [.1] [.12] [.16] [.44] 18.1 [.3] 19.9 [.3] 2.9 [.3] 21.7 [.3] 22.8 [.3] [.35] [.41] 25.5 [.2] 28.7 [.2] trans- 322

84 [8] POPs cis- trans pg/l pg/l cis-47.6 pg/l pg/l trans-47.9 pg/l cis- trans- [] H14 tr(1.2) tr(1.) 25 nd 1.5 [.5] 97/114 38/38 H15 tr(1.8) tr(1.6) 7 tr(1.) 2 [.5] 36/36 36/36 H16 nd nd 29 nd 5 [2] 9/38 9/38 H17 nd tr(1) 54 nd 3 [1] 25/47 25/47 H18 nd nd 6 nd 5 [2] 5/48 5/48 H19 nd nd 5.2 nd 2.4 [.8] 12/48 12/48 (pg/l) H2 nd nd 4.6 nd 2.1 [.8] 19/48 19/48 H21 tr(.5) nd 17 nd.8 [.3] 2/49 2/49 H22 nd nd 43 nd 2.2 [.7] 4/49 4/49 H23 nd nd 22 nd 1.3 [.5] 6/49 6/49 H26 tr(.2) tr(.2) 1.5 nd.5 [.2] 28/48 28/48 H29 nd nd 6 nd 3 [1] 2/47 2/47 323

85 cis- [] H [.2] 36/36 36/36 H [.4] 38/38 38/38 H [.2] 47/47 47/47 H [.7] 48/48 48/48 H tr(.9) 1.3 [.4] 48/48 48/48 H nd.6 [.2] 46/48 46/48 (pg/l) H [.2] 49/49 49/49 H [.2] 49/49 49/49 H [.3] 49/49 49/49 H [.2] 48/48 48/48 H nd 1.6 [.6] 46/47 46/47 trans- [] H15 nd nd 2 nd 2 [.4] 4/36 4/36 H16 nd nd nd nd.9 [.3] /38 /38 H17 nd nd nd nd.7 [.2] /47 /47 H18 nd nd nd nd 1.8 [.6] /48 /48 H19 nd nd tr(.9) nd 2. [.7] 2/48 2/48 H2 nd nd nd nd 1.9 [.7] /48 /48 (pg/l) H21 nd nd nd nd.7 [.3] /49 /49 H22 nd nd 8. nd 1.3 [.5] 2/49 2/49 H23 nd nd 2.8 nd.8 [.3] 3/49 3/49 H26 nd nd nd nd.8 [.3] /48 /48 H29 nd nd nd nd 2.3 [.9] /47 / pg/g-dry pg/g-dry cis-62.5 pg/g-dry pg/g-dry trans-62.8 pg/g-dry

86 14 29 cis- trans- [] H nd 1.8 [.6] 167/189 6/63 H15 tr(2.7) tr(2.2) 16 nd 3 [1.] 138/186 53/62 H16 tr(2.8) tr(2.3) 17 nd 3 [.9] 134/189 53/63 H nd 2.5 [.8] 12/189 48/63 H nd 1.9 [.6] 19/192 64/64 H19 tr(1.8) tr(1.5) 11 nd 3. [.7] 143/192 57/64 (pg/g-dry) H2 tr(1) nd 85 nd 4 [1] 59/192 27/64 H nd 1.1 [.4] 144/192 59/64 H tr(.8) 35 nd 1.1 [.4] 51/64 51/64 H23 tr(1.3) tr(1.2) 48 nd 1.8 [.7] 4/64 4/64 H26 tr(1.) tr(.9) 49 nd 1.5 [.5] 38/63 38/63 H nd.9 [.3] 53/62 53/62 cis- (pg/g-dry) trans- (pg/g-dry) [] H nd 3 [1] 153/186 55/62 H16 tr(5) tr(3) 23 nd 6 [2] 136/189 52/63 H17 tr(4) tr(3) 14 nd 7 [2] 119/189 49/63 H nd 3. [1.] 157/192 58/64 H19 3 tr(2) 27 nd 3 [1] 141/192 53/64 H nd 2 [1] 13/192 51/64 H nd.7 [.3] 176/192 63/64 H nd.8 [.3] 62/64 62/64 H nd.6 [.2] 63/64 63/64 H nd.5 [.2] 59/63 59/63 H nd 1.2 [.5] 51/62 51/62 [] H15 nd nd nd nd 9 [3] /186 /62 H16 nd nd tr(2.5) nd 4 [2] 1/189 1/63 H17 nd nd nd nd 5 [2] /189 /63 H18 nd nd 19 nd 7 [2] 2/192 2/64 H19 nd nd 31 nd 1 [4] 2/192 2/64 H2 nd nd nd nd 1.7 [.7] /192 /64 H21 nd nd nd nd 1.4 [.6] /192 /64 H22 nd nd 4 nd 3 [1] 1/64 1/64 H23 nd nd 2.4 nd 2.3 [.9] 2/64 2/64 H26 nd nd 3.6 nd.7 [.3] 1/63 1/63 H29 nd nd nd nd 2. [.8] /62 /

87 cis- trans- [] H14 tr(3.5) nd 4.2 [1.4] 28/38 6/8 H15 tr(2.8) tr(2.4) 14 nd 6.6 [2.2] 16/3 4/6 H16 tr(3.4) nd 4.1 [1.4] 23/31 6/7 H17 tr(2.9) tr(2.9) 24 nd 6.1 [2.] 18/31 6/7 H18 tr(4) tr(4) 2 nd 6 [2] 23/31 6/7 H19 tr(3) tr(3) 12 nd 6 [2] 2/31 6/7 H2 tr(2) nd 9 nd 6 [2] 13/31 5/7 H21 tr(4) nd 12 nd 5 [2] 14/31 4/7 H22 3 tr(2) 78 nd 3 [1] 5/6 5/6 H nd 3 [1] 3/4 3/4 H24 tr(3) tr(3) 13 nd 4 [1] 4/5 4/5 H25 3 tr(2) 19 nd 3 [1] 4/5 4/5 H27 nd nd tr(1.7) nd 3. [1.] 1/3 1/3 H28 nd nd tr(1.4) nd 2.4 [.9] 1/3 1/3 cis- H nd 4.2 [1.4] 57/7 12/14 H15 nd nd 11 nd 6.6 [2.2] 29/7 8/14 H16 tr(2.3) tr(2.1) 46 nd 4.1 [1.4] 5/7 11/14 H17 nd nd 7.6 nd 6.1 [2.] 32/8 8/16 H18 tr(2) nd 8 nd 6 [2] 36/8 8/16 H19 tr(2) nd 7 nd 6 [2] 28/8 6/16 H2 nd nd 9 nd 6 [2] 25/85 7/17 H21 tr(2) nd 8 nd 5 [2] 3/9 11/18 H22 tr(2) tr(2) 5 nd 3 [1] 12/18 12/18 H23 tr(1) tr(1) 7 nd 3 [1] 13/18 13/18 H24 nd tr(1) 5 nd 4 [1] 1/19 1/19 H25 nd nd 12 nd 3 [1] 9/19 9/19 H27 nd nd 9.2 nd 3. [1.] 9/19 9/19 H28 nd nd 5.5 nd 2.4 [.9] 8/19 8/19 H14 tr(1.7) tr(2.8) 5.2 nd 4.2 [1.4] 7/1 2/2 H15 nd nd nd nd 6.6 [2.2] /1 /2 H16 nd nd tr(1.5) nd 4.1 [1.4] 1/1 1/2 H17 nd nd nd nd 6.1 [2.] /1 /2 H18 nd nd nd nd 6 [2] /1 /2 H19 nd nd nd nd 6 [2] /1 /2 H2 nd nd nd nd 6 [2] /1 /2 H21 nd nd nd nd 5 [2] /1 /2 H22 nd --- tr(1) nd 3 [1] 1/2 1/2 H nd nd 3 [1] /1 /1 H24 nd --- nd nd 4 [1] /2 /2 H25 nd --- nd nd 3 [1] /2 /2 H nd nd 3. [1.] /1 /1 H28 nd --- nd nd 2.4 [.9] /2 /2 [] H [2.3] 3/3 6/6 H tr(9.8) 9.9 [3.3] 31/31 7/7 H [1.2] 31/31 7/7 H ,1 8 4 [1] 31/31 7/7 H ,1 8 4 [1] 31/31 7/7 H [2] 31/31 7/7 H [1] 31/31 7/7 H , [.9] 6/6 6/6 H [.8] 4/4 4/4 H [.6] 5/5 5/5 H [.8] 5/5 5/5 H [.8] 3/3 3/3 H [.7] 3/3 3/3 326

88 cis- [] H [2.3] 7/7 14/14 H tr(3.3) 9.9 [3.3] 7/7 14/14 H [1.2] 8/8 16/16 H [1] 8/8 16/16 H [1] 8/8 16/16 H tr(3) 5 [2] 85/85 17/17 H [1] 9/9 18/18 H [.9] 18/18 18/18 H [.8] 18/18 18/18 H [.6] 19/19 19/19 H [.8] 19/19 19/19 H [.8] 19/19 19/19 H [.7] 19/19 19/19 H [2.3] 1/1 2/2 H [3.3] 1/1 2/2 H [1.2] 1/1 2/2 H [1] 1/1 2/2 H [1] 1/1 2/2 H [2] 1/1 2/2 H [1] 1/1 2/2 H [.9] 2/2 2/2 H [.8] 1/1 1/1 H [.6] 2/2 2/2 H [.8] 2/2 2/2 H [.8] 1/1 1/1 H [.7] 2/2 2/2 trans- [] H15 nd nd 48 nd 13 [4.4] 5/3 1/6 H16 nd nd 55 nd 12 [4.] 9/31 2/7 H17 nd nd 37 nd 23 [7.5] 5/31 1/7 H18 nd nd 45 nd 13 [5] 5/31 1/7 H19 nd nd 61 nd 13 [5] 5/31 1/7 H2 nd nd 33 nd 1 [4] 5/31 1/7 H21 tr(3) nd 24 nd 8 [3] 13/31 3/7 H22 3 tr(2) 24 nd 3 [1] 3/6 3/6 H23 nd nd tr(6) nd 7 [3] 1/4 1/4 H24 nd nd tr(4) nd 8 [3] 1/5 1/5 H25 nd nd nd nd 7 [3] /5 /5 H27 nd nd nd nd 7 [3] /3 /3 H28 nd nd nd nd 9 [3] /3 /3 H15 nd nd nd nd 13 [4.4] /7 /14 H16 nd nd tr(1) nd 12 [4.] 2/7 2/14 H17 nd nd nd nd 23 [7.5] /8 /16 H18 nd nd nd nd 13 [5] /8 /16 H19 nd nd nd nd 13 [5] /8 /16 H2 nd nd nd nd 1 [4] /85 /17 H21 nd nd nd nd 8 [3] /9 /18 H22 nd nd nd nd 3 [1] /18 /18 H23 nd nd nd nd 7 [3] /18 /18 H24 nd nd nd nd 8 [3] /19 /19 H25 nd nd nd nd 7 [3] /19 /19 H27 nd nd 1 nd 7 [3] 5/19 5/19 H28 nd nd nd nd 9 [3] /19 /19 H15 nd nd nd nd 13 [4.4] /1 /2 H16 nd nd nd nd 12 [4.] /1 /2 H17 nd nd nd nd 23 [7.5] /1 /2 H18 nd nd nd nd 13 [5] /1 /2 H19 nd nd nd nd 13 [5] /1 /2 H2 nd nd nd nd 1 [4] /1 /2 H21 nd nd nd nd 8 [3] /1 /2 H22 nd --- nd nd 3 [1] /2 /2 H nd nd 7 [3] /1 /1 H24 nd --- nd nd 8 [3] /2 /2 H25 nd --- tr(5) nd 7 [3] 1/2 1/2 H nd nd 7 [3] /1 /1 H28 nd --- nd nd 9 [3] /2 /

89 14 28 cis- trans- [] H [.4] 12/12 34/34 H /35 35/35.25 [.85] H /34 34/34 H [.78] H H [.54] H H [.4] H H /36 36/36.7 [.3] H /36 36/36 H [.2] H (pg/m 3 ) H [.1] H H [.4] H H /35 35/35.3 [.99] H tr(.13) H /36 36/36.41 [.14] H nd 35/36 35/36 H /36 36/36.16 [.5] H tr(.1) 36/36 36/36 H [.6] 35/35 35/35 H tr(.18).22 [.8] cis- [] H /35 35/35.15 [.48] H /34 34/34 H [.17] H H tr(.1).12 [.44] H H [.4] H nd 36/37 36/37 H /36 36/36.3 [.1] H /36 36/36 H [.8] H (pg/m 3 H ).3 [.1] H H [.1] H H /35 35/35.4 [.1] H H /36 36/36.5 [.2] H /36 36/36 H /36 36/36.3 [.1] H /36 36/36 H tr(.4).5 [.2] 35/35 35/35 H [.5]

90 trans- [] H15 tr(.36) tr(.38).3 nd 18/35 18/35.99 [.33] H15 nd nd tr(.94) nd 3/34 3/34 H16 nd nd tr(.38) nd 4/37 4/37.6 [.2] H16 nd nd nd nd /37 /37 H17 tr(.1) tr(.12) 1.2 nd 27/37 27/37.16 [.5] H17 nd nd.32 nd 3/37 3/37 H18 nd nd.7 nd 2/37 2/37.3 [.1] H18 nd nd tr(.1) nd 1/37 1/37 H19 nd nd.16 nd 8/36 8/36.14 [.6] H19 nd nd tr(.6) nd 1/36 1/36 H2 nd nd.17 nd 6/37 6/37.16 [.6] H2 nd nd nd nd /37 /37 (pg/m 3 H21 nd nd.18 nd 1/37 1/37 ).14 [.5] H21 nd nd tr(.6) nd 1/37 1/37 H22 nd nd.16 nd 6/37 6/37.16 [.6] H22 nd nd nd nd /37 /37 H23 nd nd.14 nd 5/35 5/35.13 [.5] H23 nd nd nd nd /37 /37 H24 nd nd tr(.8) nd 8/36 8/36.12 [.5] H24 nd nd nd nd /36 /36 H25 nd nd tr(.11) nd 7/36 7/36.12 [.5] H25 nd nd nd nd /36 /36 H27 nd nd nd nd.3 [.1] /35 /35 H28 nd nd tr(.2) nd.3 [.1] 1/37 1/

91 [8-1] (pg/g-dry) [](pg/g-dry) [.6] 15 3 [1.] 16 3 [.9] [.8] [.6] [.7] 2 4 [1] [.4] [.4] [.7] [.5] [.5] [8-2] cis- (pg/l) [](pg/l) 15.7 [.2] 16 2 [.4] 17.7 [.2] [.7] [.4] 2.6 [.2] 21.5 [.2] 22.4 [.2] 23.7 [.3] 26.5 [.2] [.6] cis- 33

92 [8-2] cis- (pg/g-dry) [](pg/g-dry) 15 3 [1] 16 6 [2] 17 7 [2] [1.] 19 3 [1] 2 2 [1] 21.7 [.3] 22.8 [.3] 23.6 [.2] 26.5 [.2] [.5] cis- [8-3] trans- (pg/g-dry) [](pg/g-dry) 15 9 [3] 16 4 [2] 17 5 [2] 18 7 [2] 19 1 [4] [.7] [.6] 22 3 [1] [.9] 26.7 [.3] [.8] trans- 331

93 [8-1] [] [1.4] [2.2] [1.4] [2.] 18 6 [2] 19 6 [2] 2 6 [2] 21 5[2] 22 3 [1] 23 3 [1] 24 4 [1] 25 3 [1] [1.] [.9] / [8-1] 3 pg/m [] (pg/m 3 ) [.4] [.85] [.78] [.54] [.4] 19.7 [.3] 2.6 [.2] 21.4 [.1] [.4] 23.3 [.99] [.14] [.5] [.6] [.8]

94 [8-2] cis [] [2.3] [3.3] [1.2] 18 4 [1] 19 4 [1] 2 5 [2] 21 3[1] [.9] [.8] [.6] [.8] [.8] [.7] cis- [8-2] cis- 4 pg/m [] (pg/m 3 ) [.48] [.17] [.44] [.4] 19.3 [.1] 2.22 [.8] 21.3 [.1] 22.2 [.1] 23.4 [.1] 24.5 [.2] 25.3 [.1] 27.5 [.2] [.5] cis- 333

95 [9] 14 9 POPs endo,3-exo,5-endo,6-exo,8,8,1,1- Parlar-262-endo,3-exo,5-endo,6-exo,8,8,9,1,1- Parlar-5 2,2,5,5,8,9,9,1,1- Parlar Parlar-26 Parlar-5 Parlar-62 Parlar-26 [] H15 nd nd nd nd 4 [2] /36 /36 H16 nd nd nd nd 9 [3] /38 /38 H17 nd nd nd nd 1 [4] /47 /47 H18 nd nd nd nd 16 [5] /48 /48 (pg/l) H19 nd nd nd nd 2 [5] /48 /48 H2 nd nd nd nd 8 [3] /48 /48 H21 nd nd nd nd 5 [2] /49 /49 Parlar-5 [] (pg/l) Parlar-62 (pg/l) H15 nd nd nd nd 7 [3] /36 /36 H16 nd nd nd nd 2 [7] /38 /38 H17 nd nd nd nd 2 [5] /47 /47 H18 nd nd nd nd 16 [5] /48 /48 H19 nd nd nd nd 9 [3] /48 /48 H2 nd nd nd nd 7 [3] /48 /48 H21 nd nd nd nd 7 [3] /49 /49 [] H15 nd nd nd nd 3 [9] /36 /36 H16 nd nd nd nd 9 [3] /38 /38 H17 nd nd nd nd 7[3] /47 /47 H18 nd nd nd nd 6 [2] /48 /48 H19 nd nd nd nd 7 [3] /48 /48 H2 nd nd nd nd 4 [2] /48 /48 H21 nd nd nd nd 4 [2] /49 /49 334

96 15 21 Parlar-26 Parlar-5 Parlar-62 Parlar-26 [] H15 nd nd nd nd 9 [3] /186 /62 H16 nd nd nd nd 6 [2] /189 /63 H17 nd nd nd nd 6 [3] /189 /63 H18 nd nd nd nd 12 [4] /192 /64 (pg/g-dry) H19 nd nd nd nd 7 [3] /192 /64 H2 nd nd nd nd 12 [5] /192 /64 H21 nd nd nd nd 1 [4] /192 /64 Parlar-5 [] (pg/g-dry) Parlar-62 (pg/g-dry) H15 nd nd nd nd 2 [5] /186 /62 H16 nd nd nd nd 6 [2] /189 /63 H17 nd nd nd nd 9 [4] /189 /63 H18 nd nd nd nd 24 [7] /192 /64 H19 nd nd nd nd 3 [1] /192 /64 H2 nd nd nd nd 17 [6] /192 /64 H21 nd nd nd nd 12 [5] /192 /64 [] H15 nd nd nd nd 4, [2,] /186 /62 H16 nd nd nd nd 2, [4] /189 /63 H17 nd nd nd nd 2, [7] /189 /63 H18 nd nd nd nd 21 [6] /192 /64 H19 nd nd nd nd 3 [7] /192 /64 H2 nd nd nd nd 9 [4] /192 /64 H21 nd nd nd nd 8 [3] /192 / Parlar-26 Parlar-5 Parlar- 62 Parlar-26 [] H15 nd nd tr(39) nd 45 [15] 11/3 3/6 H16 nd nd tr(32) nd 42 [14] 15/31 3/7 H17 nd nd tr(28) nd 47 [16] 7/31 4/7 H18 tr(9) tr(12) 25 nd 18 [7] 21/31 5/7 H19 tr(7) tr(8) 2 nd 1 [4] 26/31 6/7 H2 tr(7) tr(8) 22 nd 9 [3] 27/31 7/7 H nd 7 [3] 27/31 7/7 H27 tr(1) tr(15) tr(17) nd 23 [9] 2/3 2/3 H15 tr(28) tr(24) 81 nd 45 [15] 44/7 11/14 H16 43 tr(41) 1, nd 42 [14] 54/7 13/14 H17 tr(42) 53 9 nd 47 [16] 5/75 13/16 H nd 18 [7] 7/8 15/16 H nd 1 [4] 64/8 14/16 H nd 9 [3] 79/85 17/17 H nd 7 [3] 82/9 18/18 H nd 23 [9] 13/19 13/19 H ,5 nd 45 [15] 5/1 1/2 H nd 42 [14] 5/1 1/2 H ,2 nd 47 [16] 5/1 1/2 H nd 18 [7] 5/1 1/2 H nd 1 [4] 5/1 1/2 H ,2 nd 9 [3] 6/1 2/2 H nd 7 [3] 6/1 2/2 H tr(1) tr(1) 23 [9] 1/1 1/1 335

97 Parlar-5 [] H15 tr(12) tr(12) 58 nd 33 [11] 17/3 4/6 H16 tr(15) nd tr(45) nd 46 [15] 15/31 3/7 H17 nd nd tr(38) nd 54 [18] 9/31 4/7 H18 tr(1) nd 14 [5] 24/31 6/7 H nd 9 [3] 27/31 7/7 H2 tr(7) tr(6) 23 nd 1 [4] 23/31 6/7 H nd 8 [3] 27/31 7/7 H27 tr(11) tr(15) tr(16) nd 3 [1] 2/3 2/3 H ,1 nd 33 [11] 55/7 14/14 H ,3 nd 46 [15] 59/7 14/14 H17 tr(52) 66 1,4 nd 54 [18] 55/8 13/16 H ,3 nd 14 [5] 79/8 16/16 H ,1 nd 9 [3] 77/8 16/16 H , nd 1 [4] 77/85 17/17 H nd 8 [3] 85/9 18/18 H27 tr(25) tr(13) 64 nd 3 [1] 13/19 13/19 H , nd 33 [11] 5/1 1/2 H , nd 46 [15] 5/1 1/2 H ,5 nd 54 [18] 5/1 1/2 H , nd 14 [5] 5/1 1/2 H nd 9 [3] 5/1 1/2 H ,6 nd 1 [4] 5/1 1/2 H nd 8 [3] 5/1 1/2 H nd nd 3 [1] /1 /1 Parlar-62 [] H15 nd nd nd nd 12 [4] /3 /6 H16 nd nd nd nd 98 [33] /31 /7 H17 nd nd nd nd 1 [34] /31 /7 H18 nd nd nd nd 7 [3] /31 /7 H19 nd nd nd nd 7 [3] /31 /7 H2 nd nd nd nd 8 [3] /31 /7 H21 nd nd nd nd 7 [2] /31 /7 H27 nd nd nd nd 15 [6] /3 /3 H15 nd nd 58 nd 12 [4] 9/7 3/14 H16 nd nd 87 nd 98 [33] 24/7 7/14 H17 nd nd 83 nd 1 [34] 23/8 8/16 H18 tr(3) nd 87 nd 7 [3] 28/8 1/16 H19 tr(3) nd 53 nd 7 [3] 22/8 7/16 H2 tr(3) nd 59 nd 8 [3] 31/85 8/17 H21 tr(2) nd 66 nd 7 [2] 24/9 8/18 H27 nd nd 32 nd 15 [6] 2/19 2/19 H15 tr(96) 2 53 nd 12 [4] 5/1 1/2 H16 tr(64) nd 98 [33] 5/1 1/2 H17 tr(78) nd 1 [34] 5/1 1/2 H nd 7 [3] 5/1 1/2 H19 tr(6) 1 3 nd 7 [3] 5/1 1/2 H2 tr(7) nd 8 [3] 5/1 1/2 H21 tr(4) 8 21 nd 7 [2] 5/1 1/2 H nd nd 15 [6] /1 /

98 15 21 Parlar-26 Parlar-5 Parlar-62 [] Parlar-26 H tr(.17) 35/35 35/35.2 [.66] H15 tr(.17) tr(.17).27 tr(.91) 34/34 34/34 H tr(.17).2 [.66] H16 tr(.15) tr(.15).5 tr(.94) H17 nd nd nd nd /37 /37.3 [.1] H17 nd nd nd nd /37 /37 H18 nd nd nd nd /37 /37 (pg/m [.6] ) H18 nd nd nd nd /37 /37 H19 nd nd tr(.3) nd 18/36 18/36.6 [.2] H19 nd nd nd nd /36 /36 H2 tr(.21) tr(.12).22 [.8] H2 tr(.11) tr(.12) tr(.2) nd 36/37 36/37 H21 tr(.18) tr(.19).26 tr(.11).23 [.9] H21 tr(.12) tr(.13).27 nd 33/37 33/37 [] Parlar-5 H15 nd nd tr(.37) nd 2/35 2/35.81 [.27] H15 nd nd nd nd /34 /34 H16 nd nd nd nd /37 / [.4] H16 nd nd nd nd /37 /37 H17 nd nd nd nd /37 /37.6 [.2] H17 nd nd nd nd /37 /37 H18 nd nd nd nd /37 /37 (pg/m [.5] ) H18 nd nd nd nd /37 /37 H19 nd tr(.1) tr(.2) nd 29/36 29/36.3 [.1] H19 nd nd nd nd /36 /36 H2 nd nd tr(.19) nd 15/37 15/37.25 [.9] H2 nd nd nd nd /37 /37 H21 nd nd tr(.1) nd 11/37 11/37.3 [.1] H21 nd nd tr(.1) nd 1/37 1/37 [] Parlar-62 H15 nd nd nd nd /35 / [.52] H15 nd nd nd nd /34 /34 H16 nd nd nd nd /37 / [.81] H16 nd nd nd nd /37 /37 H17 nd nd nd nd /37 / [.4] H17 nd nd nd nd /37 /37 H18 nd nd nd nd /37 /37 (pg/m 3 8 [3] ) H18 nd nd nd nd /37 /37 H19 nd nd nd nd /36 / [.6] H19 nd nd nd nd /36 /36 H2 nd nd nd nd /37 / [.6] H2 nd nd nd nd /37 /37 H21 nd nd nd nd /37 / [.6] H21 nd nd nd nd /37 /37 337

99 [9-1] Parlar [] [15] [14] [16] [7] 19 1 [4] 2 9 [3] 21 7[3] 27 23[9] / Parlar-26 [9-1] Parlar-26 pg/m [] (pg/m 3 ) 15.2 [.66] 16.2 [.66] 17.3 [.1] [.6] 19.6 [.2] 2.22 [.8] [.9] / Parlar

100 [9-2] Parlar [] [11] [15] [18] [5] 19 9 [3] 2 1 [4] 21 8[3] 27 3 [1] Parlar-5 339

101 [1] 14 9 POPs [] (pg/l) 22 H15 tr(.13) tr(.12).8 nd.3 [.9] 25/36 25/36 H16 nd nd 1.1 nd.4 [.2] 18/38 18/38 H17 nd nd 1. nd.4 [.1] 14/47 14/47 H18 nd nd.7 nd 1.6 [.5] 1/48 1/48 H19 nd nd tr(.5) nd 1.1 [.4] 2/48 2/48 H2 nd nd.7 nd.6 [.2] 4/48 4/48 H21 nd nd.5 nd.4 [.2] 8/49 8/49 H23 nd nd.8 nd.5 [.2] 3/49 3/ [] (pg/g-dry) H15 2 tr(1.6) 1,5 nd 2 [.4] 137/186 51/62 H16 2 tr(1.6) 22 nd 2 [.5] 153/189 55/63 H ,3 nd.9 [.3] 134/189 48/63 H nd.6 [.2] 156/192 57/64 H nd.9 [.3] 147/192 55/64 H nd.7 [.3] 117/192 48/64 H nd 1. [.4] 126/192 49/64 H ,9 nd.9 [.4] 42/64 42/

102 15 23 [] H tr(1.6) 2.4 [.81] 3/3 6/6 H tr(1.1) 2.5 [.82] 31/31 7/7 H tr(1.9) 3. [.99] 31/31 7/7 H tr(2) 3 [1] 31/31 7/7 H tr(2) 3 [1] 31/31 7/7 H2 4 tr(3) 18 tr(2) 4 [1] 31/31 7/7 H tr(1.7) 2.1 [.8] 31/31 7/7 H [.8] 4/4 4/4 H tr(1.7) 2.4 [.81] 7/7 14/14 H [.82] 7/7 14/14 H tr(1.) 3. [.99] 8/8 16/16 H tr(2) 3 [1] 8/8 16/16 H tr(1) 3 [1] 8/8 16/16 H tr(1) 4 [1] 85/85 17/17 H tr(.9) 2.1 [.8] 9/9 18/18 H tr(1.3) 1.9 [.8] 18/18 18/18 H [.81] 1/1 2/2 H [.82] 1/1 2/2 H [.99] 1/1 2/2 H [1] 1/1 2/2 H [1] 1/1 2/2 H [1] 1/1 2/2 H [.8] 1/1 2/2 H [.8] 1/1 1/ [] H /35 35/35 H [.28] 34/34 34/34 H tr(.42).5 [.17] H16 tr(.46) tr(.47).23 tr(.19) H17 tr(.9) tr(.9).24 tr(.5).1 [.3] H17 tr(.4) tr(.4) tr(.8) nd 29/37 29/37 H18 tr(.7) tr(.1).22 nd 29/37 29/37.13 [.4] H18 tr(.7) tr(.7) 2.1 nd 27/37 27/37 (pg/m 3 ) H /36 36/36.3 [.1] H tr(.2) 36/36 36/36 H [.1] H H [.6] H H /35 35/35.4 [.1] H tr(.3)

103 [1] (pg/g-dry) [](pg/g-dry) 15 2 [.4] 16 2 [.5] 17.9 [.3] 18.6 [.2] 19.9 [.3] 2.7 [.3] [.4] 23.9 [.4] [1] [] [.81] [.82] [.99] 18 3 [1] 19 3 [1] 2 4 [1] [.8] [.8]

104 [1].16 pg/m [] (pg/m 3 ) [.28] 16.5 [.17] 17.1 [.3] [.4] 19.3 [.1] 2.3 [.1] [.6] 23.4 [.1]

105 [11] HCH HCH POPs 4 COP4HCH α-hch β-hch γ-hch 22 4 HCH α-β-γ- δ α- β γ- 9 δ α- β- 14 α- β- γ- δ α-hch47.4 pg/l pg/l β-hch47.7 pg/l pg/l γ-hch47.5 pg/l pg/l δ-hch47.4 pg/l 47 tr(.4) 69 pg/l 344

106 14 29 α-hch β-hch γ-hch δ-hch α-hch [] H , [.3] 114/114 38/38 H [.9] 36/36 36/36 H , [2] 38/38 38/38 H [1] 47/47 47/47 H , [1] 48/48 48/48 H [.6] 48/48 48/48 H ,1 9 4 [2] 48/48 48/48 H [.4] 49/49 49/49 (pg/l) H , [1] 49/49 49/49 H , 11 7 [3] 49/49 49/49 H , [.5] 48/48 48/48 H ,9 9 7 [2] 48/48 48/48 H [1.5] 48/48 48/48 H [.4] 48/48 48/48 H [.4] 48/48 48/48 H [.4] 47/47 47/47 β-hch [] (pg/l) γ-hch (pg/l) H , [.3] 114/114 38/38 H , [.7] 36/36 36/36 H , [2] 38/38 38/38 H , [.9] 47/47 47/47 H , [.6] 48/48 48/48 H , [.9] 48/48 48/48 H , [.4] 48/48 48/48 H , [.2] 49/49 49/49 H , [.7] 49/49 49/49 H [.8] 49/49 49/49 H [.5] 48/48 48/48 H ,1 2 7 [2] 48/48 48/48 H , [.4] 48/48 48/48 H , [.4] 48/48 48/48 H , [.4] 48/48 48/48 H [.7] 47/47 47/47 [] H [2] 36/36 36/36 H , [7] 38/38 38/38 H tr(8) 14 [5] 47/47 47/47 H tr(9) 18 [6] 48/48 48/48 H [.7] 48/48 48/48 H [1] 48/48 48/48 H [.2] 49/49 49/49 H tr(5) 6 [2] 49/49 49/49 H [1] 49/49 49/49 H [.4] 48/48 48/48 H [.8] 48/48 48/48 H [.4] 48/48 48/48 H [.3] 48/48 48/48 H [.3] 48/48 48/48 H [.5] 47/47 47/47 δ-hch [] H tr(1.1) 2 [.5] 36/36 36/36 H tr(1.4) 2 [.7] 38/38 38/38 H nd 62 nd 1.5 [.5] 23/47 23/47 H , [.8] 48/48 48/48 H tr(.7) 1.2 [.4] 48/48 48/48 H ,9 tr(1.1) 2.3 [.9] 48/48 48/48 H tr(.7).9 [.4] 49/49 49/49 (pg/l) H [.3] 49/49 49/49 H [.2] 49/49 49/49 H tr(.5) 1.1 [.4] 48/48 48/48 H tr(.6) 1.1 [.4] 48/48 48/48 H [.2] 48/48 48/48 H [.1] 48/48 48/48 H tr(.5).8 [.3] 48/48 48/48 H tr(.4) 1. [.4] 47/47 47/

107 α-hch62.2 pg/g-dry ,9 pg/g-dry β-hch62.6 pg/g-dry ,4 pg/g-dry γ-hch62.4 pg/g-dry 62 tr(.4) 1,9 pg/g-dry δ-hch62.2 pg/g-dry 62 tr(.2) 1,7 pg/g-dry α-hch β-hch γ-hch δ-hch α-hch [] H , [.4] 189/189 63/63 H ,5 2 2 [.5] 186/186 62/62 H ,7 tr(1.5) 2 [.6] 189/189 63/63 H , [.6] 189/189 63/63 H ,3 tr(2) 5 [2] 192/192 64/64 H , tr(1.3) 1.8 [.6] 192/192 64/64 H ,2 nd 1.6 [.6] 191/192 64/64 H ,3 nd 1.1 [.4] 191/192 64/64 (pg/g-dry) H , [.8] 64/64 64/64 H , [.6] 64/64 64/64 H ,9 tr(1.1) 1.6 [.5] 63/63 63/63 H ,2 tr(.6) 1.5 [.5] 63/63 63/63 H ,3 nd 2.4 [.8] 62/63 62/63 H , [.3] 62/62 62/62 H , [.3] 62/62 62/62 H , [.2] 62/62 62/62 β-hch [] (pg/g-dry) H , [.3] 189/189 63/63 H , 5 2 [.7] 186/186 62/62 H , 4 3 [.8] 189/189 63/63 H , [.9] 189/189 63/63 H , [.4] 192/192 64/64 H , [.3] 192/192 64/64 H , [.3] 192/192 64/64 H , [.5] 192/192 64/64 H , [.8] 64/64 64/64 H , 3 3 [1] 64/64 64/64 H , [.6] 63/63 63/63 H , [.1] 63/63 63/63 H , [.3] 63/63 63/63 H , [.3] 62/62 62/62 H , [.3] 62/62 62/62 H , [.6] 62/62 62/62 346

108 γ-hch (pg/g-dry) δ-hch (pg/g-dry) [] H , tr(1.4) 2 [.4] 186/186 62/62 H ,1 tr(.8) 2 [.5] 189/189 63/63 H ,4 tr(1.8) 2. [.7] 189/189 63/63 H ,5 tr(1.4) 2.1 [.7] 192/192 64/64 H ,2 tr(.6) 1.2 [.4] 192/192 64/64 H ,2 tr(.7).9 [.4] 192/192 64/64 H ,8 nd.6 [.2] 191/192 64/64 H ,3 tr(1.5) 2. [.7] 64/64 64/64 H ,5 nd 3 [1] 62/64 62/64 H ,5 nd 1.3 [.4] 61/63 61/63 H ,1.9.6 [.2] 63/63 63/63 H ,6 nd 2.7 [.9] 61/63 61/63 H ,8 tr(.3).5 [.2] 62/62 62/62 H ,1 tr(.7).8 [.3] 62/62 62/62 H ,9 tr(.4) 1. [.4] 62/62 62/62 [] H ,4 nd 2 [.7] 18/186 61/62 H ,5 tr(.5) 2 [.5] 189/189 63/63 H ,2 nd 1. [.3] 188/189 63/63 H , nd 1.7 [.6] 189/192 64/64 H ,4 nd 5 [2] 165/192 6/64 H ,3 nd 2 [1] 186/192 64/64 H , nd 1.2 [.5] 19/192 64/64 H , [.5] 64/64 64/64 H , nd 1.4 [.5] 63/64 63/64 H ,1 nd.8 [.3] 62/63 62/63 H ,5.4.3 [.1] 63/63 63/63 H ,9.4.4 [.1] 63/63 63/63 H ,9 tr(.4).5 [.2] 62/62 62/62 H ,1 nd.5 [.2] 6/62 6/62 H ,7 tr(.2).6 [.2] 62/62 62/ α-hch3 1 pg/g-wet pg/g-wet 19 1 pg/g-wet pg/g-wet 2 1 pg/g-wet pg/g-wet β-hch3 1 pg/g-wet pg/g-wet 19 1 pg/gwet pg/g-wet 2 1 pg/g-wet 2 3 3,5pg/g-wet γ-hch3 1 pg/g-wet 3 tr(2) 11pg/g-wet 19 1 pg/g-wet pg/g-wet 2 1 pg/g-wet 2 tr(1) 2pg/g-wet

109 5 5 δ-hch3.9 pg/g-wet 3 tr(1) 3pg/g-wet 19.9 pg/g-wet pg/g-wet 2.9 pg/g-wet 2 1 tr(1)pg/gwet α-hch β-hch γ-hch δ-hch α-hch [] H , [1.4] 38/38 8/8 H [.61] 3/3 6/6 H ,8 tr(12) 13 [4.3] 31/31 7/7 H ,1 tr(7.1) 11 [3.6] 31/31 7/7 H [1] 31/31 7/7 H ,4 8 7 [2] 31/31 7/7 H [2] 31/31 7/7 H ,2 9 5 [2] 31/31 7/7 H [1] 6/6 6/6 H , [1] 4/4 4/4 H [1.2] 5/5 5/5 H [1] 5/5 5/5 H [1] 3/3 3/3 H [1.] 3/3 3/3 H [1] 3/3 3/3 H [1] 3/3 3/3 H tr(1.9) 4.2 [1.4] 7/7 14/14 H [.61] 7/7 14/14 H ,9 nd 13 [4.3] 63/7 14/14 H , nd 11 [3.6] 75/8 16/16 H tr(2) 3 [1] 8/8 16/16 H tr(2) 7 [2] 8/8 16/16 H nd 6 [2] 84/85 17/17 H tr(2) 5 [2] 9/9 18/18 H tr(1) 3 [1] 18/18 18/18 H tr(2) 3 [1] 18/18 18/18 H nd 3.7 [1.2] 18/19 18/19 H tr(2) 3 [1] 19/19 19/19 H nd 3 [1] 18/19 18/19 H tr(1.3) 3. [1.] 19/19 19/19 H nd 3 [1] 18/19 18/19 H nd 3 [1] 18/19 18/19 H [1.4] 1/1 2/2 H [.61] 1/1 2/2 H , [4.3] 1/1 2/2 H [3.6] 1/1 2/2 H [1] 1/1 2/2 H [2] 1/1 2/2 H [2] 1/1 2/2 H [2] 1/1 2/2 H [1] 2/2 2/2 H [1] 1/1 1/1 H [1.2] 2/2 2/2 H [1] 2/2 2/2 H [1] 2/2 2/2 H [1.] 1/1 1/1 H [1] 2/2 2/2 H [1] 2/2 2/2 348

110 14 29 α-hch β-hch γ-hch δ-hch β-hch [] H , [4] 38/38 8/8 H , [3.3] 3/3 6/6 H , [2.] 31/31 7/7 H , [.75] 31/31 7/7 H [1] 31/31 7/7 H , [3] 31/31 7/7 H , [2] 31/31 7/7 H , [2] 31/31 7/7 H , [1] 6/6 6/6 H , 39 3 [1] 4/4 4/4 H [.8] 5/5 5/5 H [.8] 5/5 5/5 H [.9] 3/3 3/3 H [1.] 3/3 3/3 H [1] 3/3 3/3 H [1] 3/3 3/3 γ-hch H ,8 tr(5) 12 [4] 7/7 14/14 H ,1 tr(3.5) 9.9 [3.3] 7/7 14/14 H ,1 tr(3.9) 6.1 [2.] 7/7 14/14 H , [.75] 8/8 16/16 H ,1 4 3 [1] 8/8 16/16 H [3] 8/8 16/16 H tr(4) 6 [2] 85/85 17/17 H tr(5) 6 [2] 9/9 18/18 H [1] 18/18 18/18 H [1] 18/18 18/18 H [.8] 19/19 19/19 H [.8] 19/19 19/19 H [.9] 19/19 19/19 H [1.] 19/19 19/19 H [1] 19/19 19/19 H [1] 19/19 19/19 H14 3, 3, 7,3 1,6 12 [4] 1/1 2/2 H15 3,4 3,9 5,9 1,8 9.9 [3.3] 1/1 2/2 H16 2,3 2,1 4,8 1,1 6.1 [2.] 1/1 2/2 H17 2,5 2,8 6, [.75] 1/1 2/2 H18 2,1 2,4 4,2 1,1 3 [1] 1/1 2/2 H19 2, 1,9 3,2 1,4 7 [3] 1/1 2/2 H2 2,4 2, 5,6 1,3 6 [2] 1/1 2/2 H21 1,6 1,4 4, [2] 1/1 2/2 H22 1, , [1] 2/2 2/2 H ,5 4,5 3 [1] 1/1 1/1 H24 1, , [.8] 2/2 2/2 H25 1, , [.8] 2/2 2/2 H , [.9] 2/2 2/2 H [1.] 1/1 1/1 H28 1, , [1] 2/2 2/2 H29 1, --- 3,5 3 3 [1] 2/2 2/2 [] H [1.1] 3/3 6/6 H16 tr(24) tr(16) 23 nd 31 [1] 28/31 7/7 H tr(5.7) 8.4 [2.8] 31/31 7/7 H [2] 31/31 7/7 H tr(4) 9 [3] 31/31 7/7 H tr(3) 9 [3] 31/31 7/7 H tr(3) 7 [3] 31/31 7/7 H [1] 6/6 6/6 H [1] 4/4 4/4 H [.9] 5/5 5/5 H tr(2.1) 2.4 [.9] 5/5 5/5 H [.8] 3/3 3/3 H tr(3.6) 4.8 [1.6] 3/3 3/3 H [1] 3/3 3/3 H tr(2) 3 [1] 3/3 3/3 349

111 γ-hch δ-hch [] H tr(1.7) 3.3 [1.1] 7/7 14/14 H16 tr(28) tr(24) 66 nd 31 [1] 55/7 11/14 H nd 8.4 [2.8] 78/8 16/16 H tr(2) 4 [2] 8/8 16/16 H nd 9 [3] 71/8 15/16 H nd 9 [3] 7/85 15/17 H nd 7 [3] 81/9 17/18 H tr(1) 3 [1] 18/18 18/18 H tr(1) 3 [1] 18/18 18/18 H nd 2.3 [.9] 18/19 18/19 H nd 2.4 [.9] 17/19 17/19 H nd 2.2 [.8] 16/19 16/19 H nd 4.8 [1.6] 14/19 14/19 H nd 3 [1] 18/19 18/19 H nd 3 [1] 16/19 16/19 H [1.1] 1/1 2/2 H16 64 tr(21) 1,2 tr(11) 31 [1] 1/1 2/2 H [2.8] 1/1 2/2 H [2] 1/1 2/2 H tr(8) 9 [3] 1/1 2/2 H tr(5) 9 [3] 1/1 2/2 H tr(6) 7 [3] 1/1 2/2 H [1] 2/2 2/2 H [1] 1/1 1/1 H [.9] 2/2 2/2 H tr(1.5) 2.4 [.9] 2/2 2/2 H [.8] 2/2 2/2 H nd nd 4.8 [1.6] /1 /1 H tr(2) 3 [1] 2/2 2/2 H tr(1) 3 [1] 2/2 2/2 [] H tr(2.6) 1,3 nd 3.9 [1.3] 29/3 6/6 H tr(2.1) 1,5 nd 4.6 [1.5] 25/31 6/7 H tr(2.1) 1,6 nd 5.1 [1.7] 23/31 6/7 H18 6 tr(2) 89 tr(1) 3 [1] 31/31 7/7 H19 4 nd 75 nd 4 [2] 12/31 4/7 H2 tr(3) nd 61 nd 6 [2] 7/31 3/7 H21 tr(4) nd 7 nd 5 [2] 14/31 4/7 H22 4 tr(2) 87 nd 3 [1] 5/6 5/6 H23 9 tr(2) 1,4 tr(1) 3 [1] 4/4 4/4 H24 3 tr(1) 58 nd 3 [1] 3/5 3/5 H25 3 tr(1) 23 nd 3 [1] 3/5 3/5 H26 tr(1) tr(2) 3 nd 3 [1] 2/3 2/3 H27 nd nd tr(1.5) nd 2.1 [.8] 1/3 1/3 H28 tr(1) tr(1) tr(2) tr(1) 3 [1] 3/3 3/3 H29 tr(1.7) tr(1.6) 3 tr(1) 2.3 [.9] 3/3 3/3 H15 tr(3.6) nd 3.9 [1.3] 59/7 13/14 H16 tr(4.2) tr(3.5) 27 nd 4.6 [1.5] 54/7 11/14 H17 tr(3.2) tr(3.1) 32 nd 5.1 [1.7] 55/8 12/16 H nd 3 [1] 72/8 16/16 H19 tr(3) tr(2) 31 nd 4 [2] 42/8 1/16 H2 tr(4) tr(3) 77 nd 6 [2] 54/85 12/17 H21 tr(3) tr(3) 18 nd 5 [2] 57/9 13/18 H22 tr(2) tr(2) 36 nd 3 [1] 13/18 13/18 H nd 3 [1] 14/18 14/18 H24 tr(2) tr(2) 12 nd 3 [1] 14/19 14/19 H25 3 tr(2) 4 nd 3 [1] 14/19 14/19 H26 tr(2) tr(2) 23 nd 3 [1] 14/19 14/19 H27 tr(1.7) tr(1.8) 17 nd 2.1 [.8] 12/19 12/19 H28 tr(2) tr(2) 1 nd 3 [1] 17/19 17/19 H nd 2.3 [.9] 15/19 15/19 35

112 δ-hch [] H [1.3] 1/1 2/2 H [1.5] 1/1 2/2 H [1.7] 1/1 2/2 H [1] 1/1 2/2 H [2] 1/1 2/2 H tr(3) 6 [2] 1/1 2/2 H tr(3) 5 [2] 1/1 2/2 H [1] 2/2 2/2 H [1] 1/1 1/1 H tr(2) 3 [1] 2/2 2/2 H tr(2) 3 [1] 2/2 2/2 H26 tr(2) tr(1) 3 [1] 2/2 2/2 H nd nd 2.1 [.8] /1 /1 H28 tr(1) --- tr(2) tr(1) 3 [1] 2/2 2/2 H29 nd --- tr(1) nd 2.3 [.9] 1/2 1/ α-hch37.3 pg/m pg/m 3 β-hch37.4 pg/m pg/m γ-hch37.4 pg/m pg/m δ-hch37.3 pg/m pg/m 3 HCH 15 2 HCH HCH 遡 α-hch β-hch γ-hch δ-hch α-hch [] H [.5] H H [.47] H H /35 35/ [.83] H H /36 36/36 (pg/m [.7] ) H /36 36/36 H /36 36/ [1.7] H tr(3.9) 36/36 36/36 H [.6] 36/36 36/36 H [.6] 35/35 35/35 H [.7] H [.3] 351

113 β-hch (pg/m 3 ) γ-hch (pg/m 3 ) δ-hch (pg/m 3 ) [] H [.3] H H [.9] H tr(.26) H /35 35/35.39 [.13] H tr(.31) H /36 36/36.36 [.12] H tr(.26) 36/36 36/36 H /36 36/36.21 [.7] H tr(.17) 36/36 36/36 H [.8] 36/36 36/36 H [.8] 35/35 35/35 H [.1] H [.4] [] H [.2] H H [.12] H H /35 35/ [.52] H tr(1.1) H /36 36/36.95 [.32] H tr(.63) 36/36 36/36 H tr(2.) 36/36 36/ [.7] H nd 34/36 34/36 H [.6] 36/36 36/36 H [.6] 35/35 35/35 H [.7] H [.4] [] H [.2] H H [.2] H H /35 35/35.63 [.21] H tr(.5) H tr(.6) 36/36 36/36.7 [.3] H nd 35/36 35/36 H tr(.5) 36/36 36/36.8 [.3] H nd 34/36 34/36 H tr(.7).19 [.6] 36/36 36/36 H nd.15 [.5] 32/35 32/35 H nd.2 [.8] 35/37 35/37 H nd.8 [.3] 36/37 36/37 352

114 [11-1] α-hch (pg/l) [](pg/l) 14.9 [.3] 15 3 [.9] 16 6 [2] 17 4 [1] 18 3 [1] [.6] 2 4[2] [.4] 22 4 [1] 23 7 [3] [.5] 25 7 [2] [1.5] [.4] [.4] 29.9 [.4] α-hch [11-1] α-hch (pg/g-dry) [](pg/g-dry) [.4] 15 2 [.5] 16 2 [.6] [.6] 18 5 [2] [.6] [.6] [.4] [.8] [.6] [.5] [.5] [.8] 27.7 [.3] 28.9 [.3] 29.5 [.2] α-hch 353

115 [11-1] α-hch [] [1.4] [.61] [4.3] [3.6] 18 3 [1] 19 7 [2] 2 6 [2] 21 5[2] 22 3 [1] 23 3 [1] [1.2] 25 3 [1] 26 3 [1] [1.] 28 3[1] 29 3[1] α-hch [11-1] α-hch pg/m [] (pg/m 3 ) [.5] [.47] [.83] [.7] [1.7] [.16] [.6] [.7] 29.8 [.3] α-hch 354

116 [11-2] β-hch (pg/l) [](pg/l) 14.9 [.3] 15 3 [.7] 16 4 [2] [.9] [.6] [.9] 2 1. [.4] 21.6 [.2] [.7] [.8] [.5] 25 7 [2] [.4] [.4] [.4] [.7] β-hch [11-2] β-hch (pg/g-dry) [](pg/g-dry) 14.9 [.3] 15 2 [.7] 16 3 [.8] [.9] [.4] 19.9 [.3] 2.8 [.3] [.5] [.8] 23 3 [1] [.6] 25.4 [.1] 26.9 [.3] 27.8 [.3] 28.9 [.3] [.6] β-hch 355

117 [11-2] β-hch β-hch [] [4] [3.3] [2.] [.75] 18 3 [1] 19 7 [3] 2 6 [2] 21 6[2] 22 3 [1] 23 3 [1] 24 2 [.8] [.8] [.9] [1.] 28 3 [1] 29 3 [1] [11-2] β-hch 6 pg/m [] (pg/m 3 ) 21.9 [.3] [.9] [.13] [.12] [.7] [.8] [.8] 28.3 [.1] [.4] β-hch 356

118 [11-3] γ-hch (pg/l) [](pg/l) 15 7 [2] 16 2 [7] [5] [6] [.7] 2 3 [1] 21.6 [.2] 22 6 [2] 23 3 [1] [.4] [.8] [.4] 27.9 [.3] 28.8 [.3] [.5] γ-hch [11-3] γ-hch (pg/g-dry) [](pg/g-dry) 15 2 [.4] 16 2 [.5] [.7] [.7] [.4] 2.9 [.4] 21.6 [.2] [.7] 23 3 [1] [.4] 25.6 [.2] [.9] 27.5 [.2] 28.8 [.3] [.4] γ-hch γ-hch 357

119 [11-3] γ-hch [] [1.1] [1] [2.8] 18 4 [2] 19 9 [3] 2 9 [3] 21 7[3] 22 3 [1] 23 3 [1] [.9] [.9] [.8] [1.6] 28 3 [1] 29 3 [1] γ-hch [11-3] γ-hch 2 pg/m [] (pg/m 3 ) 21.6 [.2] [.12] [.52] [.32] [.7] [.6] [.6] [.7] 29.1 [.4] γ-hch 358

120 [11-4] δ-hch (pg/l) [](pg/l) 15 2 [.5] 16 2 [.7] [.5] [.8] [.4] [.9] 21.9 [.4] 22.8 [.3] 23.4 [.2] [.4] [.4] 26.4 [.2] 27.3 [.1] 28.8 [.3] [.4] δ-hch [11-4] δ-hch (pg/g-dry) [](pg/g-dry) 15 2 [.7] 16 2 [.5] [.3] [.6] 19 5 [2] 2 2 [1] [.5] [.5] [.5] 24.8 [.3] 25.3 [.1] 26.4 [.1] 27.5 [.2] 28.5 [.2] 29.6 [.2] δ-hch δ-hch 359

121 [11-4] δ-hch [] [1.3] [1.5] [1.7] 18 3 [1] 19 4 [2] 2 6 [2] 21 5[2] 22 3 [1] 23 3 [1] 24 3 [1] 25 3 [1] 26 3 [1] [.8] 28 3 [1] [.9] / δ-hch [11-4] δ-hch 1.6 pg/m [] (pg/m 3 ) 21.4 [.2] 21.5 [.2] [.21] 24.7 [.3] 25.8 [.3] [.6] [.5] 28.2 [.8] 29.8 [.3] δ-hch 36

122 [12] 21 5 POPs 4 COP [] (pg/l) 21 H2 nd nd.76 nd.14 [.5] 13/46 13/46 H22 tr(.4) nd 1.6 nd.9 [.4] 13/49 13/49 H23 nd nd.7 nd.2 [.5] 15/49 15/ [] (pg/g-dry) H2 nd nd 5.8 nd.42 [.16] 23/129 1/49 H22 nd nd 2.8 nd.4 [.2] 9/64 9/64 H23 nd nd 1.5 nd.4 [.2] 9/64 9/ [] H2 nd nd nd nd 5.6 [2.2] /31 /7 H22 nd nd nd nd 5.9 [2.3] /6 /6 H23 nd nd nd nd.5 [.2] /4 /4 H2 nd nd nd nd 5.6 [2.2] /85 /17 H22 nd nd nd nd 5.9 [2.3] /18 /18 H23 nd nd nd nd.5 [.2] /18 /18 H2 nd nd nd nd 5.6 [2.2] /1 /2 H22 nd --- nd nd 5.9 [2.3] /2 /2 H nd nd.5 [.2] /1 /

123 22 23 [] H22 nd nd nd nd /37 /37.4 [.2] H22 nd nd nd nd /37 /37 (pg/m 3 ) H23 nd nd nd nd /35 /35.4 [.2] H23 nd nd nd nd /37 /37 362

124 [13] 21 5 POPs 4 COP [] H21 nd nd nd nd 5.7 [2.2] /49 /49 H22 nd nd nd nd 3 [1] /49 /49 (pg/l) H23 nd nd nd nd 2.2 [.9] /49 / [][] [] H21 nd nd 12 nd 1.1 [.4] 45/19 21/64 H22 nd nd 18 nd 1.5 [.6] 1/64 1/64 (pg/g-dry) H23 nd nd 6.3 nd 3.6 [1.4] 8/64 8/64 H27 nd nd 15 nd.8 [.3] 9/62 9/ [][] [] H21 nd nd tr(.53) nd 1.3 [.43] 1/31 1/7 H22 nd nd nd nd 24 [1] /6 /6 H23 nd nd nd nd 3 [1] /4 /4 H27 nd nd nd nd 14 [5] /3 /3 H21 tr(.49) tr(.43) 6. nd 1.3 [.43] 46/9 12/18 H22 nd nd nd nd 24 [1] /18 /18 H23 nd nd 3 nd 3 [1] 5/18 5/18 H27 nd nd nd nd 14 [5] /19 /19 363

125 [] H tr(1.2) 1.3 [.43] 1/1 2/2 H22 nd --- nd nd 24 [1] /2 /2 H [1] 1/1 1/1 H nd nd 14 [5] /1 / [][] [] H22 nd nd nd nd /37 /37.3 [.1] H22 nd nd nd nd /37 /37 (pg/m 3 H23 nd nd nd nd /35 /35 ).3 [.1] H23 nd nd nd nd /37 /37 H27 nd nd 1.1 nd.6 [.2] 2/35 2/

126 [14] POPs 4 COP POPs 8 COP pg/l pg/l 47 1 pg/l pg/l pg/l 47 1 tr(6)pg/l 47 5 pg/l pg/l 47 1 pg/l pg/l 47 3 pg/l

127 37 46 pg/l 47 8 pg/l ,1 pg/l [] H nd 8 [3] 44/49 44/49 H22 nd nd 39 nd 9 [3] 17/49 17/49 H nd 4 [2] 48/49 48/49 H24 tr(3) tr(3) 22 nd 4 [1] 47/48 47/48 (pg/l) H26 tr(6) tr(6) 51 tr(4) 8 [3] 48/48 48/48 H tr(1.2) 3.6 [1.2] 48/48 48/48 H28 5 tr(5) 47 tr(3) 5 [2] 48/48 48/48 H29 tr(4) tr(4) 12 nd 9 [3] 44/47 44/47 (pg/l) (pg/l) (pg/l) (pg/l) (pg/l) [] H nd 11 [4] 43/49 43/49 H22 tr(1) tr(1) 13 nd 3 [1] 25/49 25/49 H nd 3 [1] 48/49 48/49 H24 tr(1) tr(1) 2 nd 2 [1] 32/48 32/48 H26 nd nd 39 nd 4 [2] 19/48 19/48 H27 tr(3.) tr(3.2) 31 nd 6.3 [2.1] 34/48 34/48 H28 tr(1.5) tr(1.3) 36 nd 2.4 [.9] 39/48 39/48 H29 nd tr(1) 8 nd 3 [1] 24/47 24/47 [] H21 tr(.9) tr(.7) 18 nd 1.4 [.6] 26/49 26/49 H22 nd nd 51 nd 4 [2] 16/49 16/49 H23 tr(1) nd 39 nd 3 [1] 21/49 21/49 H24 nd nd 7 nd 3 [1] 6/48 6/48 H26 nd nd 8 nd 4 [1] 1/48 1/48 H27 nd nd 12 nd 1.5 [.6] 5/48 5/48 H28 nd nd 9.1 nd 2.1 [.8] 9/48 9/48 H29 nd nd tr(6) nd 7 [3] 1/47 1/47 [] H21 nd nd 4 nd 4 [2] 9/49 9/49 H22 nd nd 14 nd 3 [1] 17/49 17/49 H23 nd nd 14 nd 6 [2] 14/49 14/49 H24 nd nd 1 nd 4 [1] 9/48 9/48 H26 nd nd 8 nd 8 [3] 3/48 3/48 H27 nd nd 28 nd 2. [.8] 9/48 9/48 H28 nd nd 11 nd 7 [3] 1/48 1/48 H29 nd nd 3 nd 14 [5] 1/47 1/47 [] H nd 1.4 [.6] 37/49 37/49 H22 tr(2) tr(2) 69 nd 3 [1] 4/49 4/49 H nd 2 [1] 44/49 44/49 H24 tr(2) nd 35 nd 4 [2] 16/48 16/48 H nd 1.6 [.6] 33/48 33/48 H nd 1.5 [.6] 31/48 31/48 H nd.8 [.3] 44/48 44/48 H29 tr(2) nd 33 nd 2 [1] 22/47 22/47 [] H21 tr(46) tr(38) 5 nd 91 [3] 32/49 32/49 H22 tr(17) tr(13) 62 nd 21 [7] 39/49 39/49 H nd 1 [4] 47/49 47/49 H24 tr(21) tr(19) 32 nd 4 [13] 3/48 3/48 H nd 6 [2] 47/48 47/48 H nd 6 [2] 47/48 47/48 H ,9 tr(2) 4 [1] 48/48 48/48 H nd 7 [3] 37/47 37/47 366

128 [] H21 tr(31) tr(22) 3,4 nd 6 [2] 26/49 26/49 H22 tr(25) tr(2) 13, nd 3 [1] 31/49 31/49 H , nd 6 [2] 45/49 45/49 H24 tr(4) tr(32) 12, nd 66 [22] 31/48 31/48 (pg/l) H ,6 tr(14) 22 [9] 48/48 48/48 H , [7] 48/48 48/48 H , tr(12) 14 [6] 48/48 48/48 H ,1 nd 24 [8] 46/47 46/ pg/g-dry pg/g-dry pg/g-dry pg/g-dry 62 2 pg/g-dry pg/g-dry pg/g-dry pg/g-dry 62 2 pg/g-dry ,9 pg/g-dry pg/g-dry , pg/g-dry pg/g-dry 62 tr(27) 58,pg/g-dry [] H21 tr(6) tr(44) 1,4 nd 69 [23] 131/192 51/64 H nd 6 [2] 57/64 57/64 H ,6 nd 3 [1] 47/64 47/64 H ,5 nd 2 [1] 6/63 6/63 (pg/g-dry) H26 tr(24) tr(19) 55 nd 27 [9] 44/63 44/63 H ,4 nd 21 [7] 44/62 44/62 H28 tr(21) tr(16) 39 nd 33 [11] 35/62 35/62 H nd 9 [4] 44/62 44/62 367

129 [] H ,7 nd 24 [8] 146/192 57/64 H nd 5 [2] 58/64 58/64 H ,7 nd 5 [2] 62/64 62/64 H ,9 nd 2.4 [.9] 62/63 62/63 (pg/g-dry) H nd 6 [2] 53/63 53/63 H ,3 nd 18 [6] 44/62 44/62 H28 13 tr(1) 4 nd 12 [4] 46/62 46/62 H29 1 tr(5.5) 56 nd 9 [4] 37/62 37/62 [] H ,6 nd 5 [2] 139/192 53/64 H nd 4 [2] 57/64 57/64 H , nd 9 [3] 52/64 52/64 H ,7 nd 3 [1] 48/63 48/63 (pg/g-dry) H nd 5 [2] 5/63 5/63 H nd 3 [1] 42/62 42/62 H nd 8 [3] 4/62 4/62 H nd 6 [2] 44/62 44/62 [] H , nd 9 [4] 125/192 51/64 H nd 4 [2] 58/64 58/64 H ,4 nd 7 [3] 55/64 55/64 H ,4 nd 4 [2] 48/63 48/63 (pg/g-dry) H26 19 tr(14) 68 nd 16 [6] 41/63 41/63 H ,8 nd 3 [1] 44/62 44/62 H ,1 nd 6 [2] 44/62 44/62 H nd 15 [6] 36/62 36/62 [] H , nd 1.2 [.5] 182/192 63/64 H ,8 nd 1 [4] 6/64 6/64 H , nd 1 [4] 55/64 55/64 H , nd 19 [6] 47/63 47/63 (pg/g-dry) H , nd 12 [4] 55/63 55/63 H27 58 tr(44) 1,4 nd 48 [16] 41/62 41/62 H ,4 nd 6 [2] 55/62 55/62 H ,9 nd 5 [2] 48/62 48/62 [] H21 1, , nd 9 [4] 181/192 64/64 H , nd 24 [9] 6/64 6/64 H , nd 23 [9] 62/64 62/64 H , nd 34 [11] 52/63 52/63 (pg/g-dry) H , nd 6 [2] 6/63 6/63 H , nd 24 [8] 55/62 55/62 H , nd 27 [9] 6/62 6/62 H , nd 15 [5] 61/62 61/62 [] H21 6, 4,8 88, tr(3) 6 [2] 192/192 64/64 H22 5,1 4,2 7, nd 22 [8] 6/64 6/64 H23 4,2 4,7 7, nd 4 [2] 62/64 62/64 H24 5,7 6,3 76, nd 27 [89] 6/63 6/63 (pg/g-dry) H26 5,6 5, 98, nd 24 [8] 61/63 61/63 H27 6,6 7,2 49, 4 4 [2] 62/62 62/62 H28 4,7 5,1 94, nd 12 [41] 61/62 61/62 H29 4,6 5,7 58, tr(27) 3 [1] 62/62 62/ pg/gwet pg/g-wet 19 6 pg/g-wet 19 tr(7) 36pg/g-wet 2 6 pg/g-wet pg/g-wet

130 3 5 pg/gwet 3 tr(6) 62pg/g-wet 19 5 pg/g-wet pg/g-wet 2 5 pg/g-wet pg/g-wet 3 7 pg/gwet pg/g-wet 19 7 pg/g-wet pg/g-wet 2 7 pg/g-wet ,pg/g-wet 3 8 pg/gwet 3 1 tr(9)pg/g-wet 19 8 pg/g-wet pg/g-wet 2 8 pg/g-wet 2 tr(18) 44pg/g-wet 3 8 pg/gwet 3 1 tr(9)pg/g-wet 19 8 pg/g-wet pg/g-wet 2 8 pg/g-wet pg/g-wet 3 2 pg/g-wet pg/g-wet pg/g-wet 2 2 pg/g-wet pg/g-wet 3 1 tr(18)pg/g-wet 19 8 pg/g-wet ,1pg/g-wet 2 8 pg/g-wet [] H [2.2] 31/31 7/7 H nd 43 [16] 5/6 5/6 H [6] 4/4 4/4 H [7] 5/5 5/5 H [6] 3/3 3/3 H [6] 3/3 3/3 H [5] 3/3 3/3 H [6] 3/3 3/3 369

131 [] H , [2.2] 85/85 17/17 H tr(16) 43 [16] 18/18 18/18 H tr(9) 16 [6] 18/18 18/18 H tr(1) 19 [7] 19/19 19/19 H , [6] 19/19 19/19 H tr(14) 15 [6] 19/19 19/19 H tr(1) 13 [5] 19/19 19/19 H tr(7) 16 [6] 19/19 19/19 H , [2.2] 1/1 2/2 H [16] 2/2 2/2 H [6] 1/1 1/1 H [7] 2/2 2/2 H [6] 2/2 2/2 H [6] 1/1 1/1 H [5] 2/2 2/2 H [6] 2/2 2/2 [] H tr(11) 16 [5.9] 31/31 7/7 H tr(9) 14 [6] 6/6 6/6 H tr(12) 15 [6] 4/4 4/4 H tr(8) 18 [6] 5/5 5/5 H [5] 3/3 3/3 H [5] 3/3 3/3 H tr(8) 9 [4] 3/3 3/3 H tr(6) 12 [5] 3/3 3/3 H nd 16 [5.9] 72/85 16/17 H nd 14 [6] 16/18 16/18 H nd 15 [6] 17/18 17/18 H nd 18 [6] 17/19 17/19 H nd 12 [5] 18/19 18/19 H nd 13 [5] 18/19 18/19 H tr(4) 9 [4] 19/19 19/19 H nd 12 [5] 18/19 18/19 H [5.9] 1/1 2/2 H [6] 2/2 2/2 H [6] 1/1 1/1 H [6] 2/2 2/2 H [5] 2/2 2/2 H [5] 1/1 1/1 H [4] 2/2 2/2 H [5] 2/2 2/2 [] H tr(5.3) 14 [5.] 31/31 7/7 H nd 8 [3] 4/6 4/6 H [4] 4/4 4/4 H tr(6) 1 [4] 5/5 5/5 H [4] 3/3 3/3 H27 tr(9) tr(6) 41 nd 12 [5] 2/3 2/3 H28 tr(13) tr(13) 4 nd 21 [8] 2/3 2/3 H29 tr(14) 2 36 nd 17 [7] 2/3 2/3 H nd 14 [5.] 83/85 17/17 H nd 8 [3] 16/18 16/18 H nd 1 [4] 17/18 17/18 H nd 1 [4] 18/19 18/19 H ,1 nd 1 [4] 18/19 18/19 H nd 12 [5] 18/19 18/19 H nd 21 [8] 18/19 18/19 H nd 17 [7] 18/19 18/19 H [5.] 1/1 2/2 H [3] 2/2 2/2 H [4] 1/1 1/1 H [4] 2/2 2/2 H [4] 2/2 2/2 H [5] 1/1 1/1 H [8] 2/2 2/2 H , [7] 2/2 2/2 37

132 [] H2 tr(8.5) tr(7.6) 35 nd 18 [6.7] 2/31 7/7 H22 nd nd tr(1) nd 3 [1] 1/6 1/6 H nd 11 [4] 3/4 3/4 H24 tr(8) tr(6) 59 nd 12 [5] 3/5 3/5 H26 nd nd 13 nd 12 [5] 1/3 1/3 H27 nd nd tr(11) nd 12 [5] 1/3 1/3 H28 nd nd tr(8) nd 13 [5] 1/3 1/3 H29 nd nd tr(9) nd 22 [8] 1/3 1/3 H2 tr(11) tr(8.1) 77 nd 18 [6.7] 44/85 1/17 H22 nd nd 4 nd 3 [1] 4/18 4/18 H nd 11 [4] 13/18 13/18 H24 tr(11) nd 12 [5] 11/19 11/19 H26 tr(1) nd 12 [5] 1/19 1/19 H27 nd nd 44 nd 12 [5] 4/19 4/19 H28 tr(9) tr(7) 85 nd 13 [5] 11/19 11/19 H29 tr(11) tr(12) 55 nd 22 [8] 1/19 1/19 H [6.7] 1/1 2/2 H22 tr(19) nd 3 [1] 1/2 1/2 H [4] 1/1 1/1 H [5] 2/2 2/2 H nd 12 [5] 1/2 1/2 H tr(11) tr(11) 12 [5] 1/1 1/1 H [5] 2/2 2/2 H tr(18) 22 [8] 2/2 2/2 [] H2 nd nd 1 nd 9.6 [3.6] 15/31 6/7 H22 nd nd tr(1) nd 11 [4] 2/6 2/6 H nd 7 [3] 3/4 3/4 H24 8 tr(7) 25 nd 8 [3] 4/5 4/5 H26 tr(9.2) tr(5) 11 [4] 3/3 3/3 H27 nd nd nd nd 14 [5] /3 /3 H28 nd nd nd nd 16 [6] /3 /3 H29 nd nd tr(9) nd 2 [8] 1/3 1/3 H2 tr(5.7) nd 73 nd 9.6 [3.6] 35/85 7/17 H22 tr(6) nd 1 nd 11 [4] 8/18 8/18 H23 tr(6) tr(7) 15 nd 7 [3] 1/18 1/18 H24 tr(7) 8 16 nd 8 [3] 12/19 12/19 H nd 11 [4] 15/19 15/19 H27 tr(7) nd 6 nd 14 [5] 9/19 9/19 H28 tr(8) nd 86 nd 16 [6] 9/19 9/19 H29 tr(9.7) nd 88 nd 2 [8] 9/19 9/19 H [3.6] 1/1 2/2 H [4] 2/2 2/2 H [3] 1/1 1/1 H [3] 2/2 2/2 H nd 11 [4] 1/2 1/2 H tr(5) tr(5) 14 [5] 1/1 1/1 H [6] 2/2 2/2 H [8] 2/2 2/2 [] H2 nd nd tr(23) nd 35 [13] 5/31 1/7 H22 tr(16) tr(15) 6 nd 3 [1] 5/6 5/6 H23 tr(12) tr(11) 4 nd 22 [9] 3/4 3/4 H24 tr(15) nd 24 [9] 3/5 3/5 H26 4 tr(2) 11 tr(2) 3 [1] 3/3 3/3 H27 nd nd tr(11) nd 23 [9] 1/3 1/3 H28 nd nd nd nd 36 [14] /3 /3 H29 nd nd nd nd 5 [2] /3 /3 H2 nd nd tr(15) nd 35 [13] 2/85 2/17 H22 nd nd 4 nd 3 [1] 3/18 3/18 H23 nd nd tr(15) nd 22 [9] 5/18 5/18 H24 nd nd 54 nd 24 [9] 9/19 9/19 H26 tr(1) tr(2) 4 nd 3 [1] 16/19 16/19 H27 nd nd 35 nd 23 [9] 6/19 6/19 H28 nd nd tr(22) nd 36 [14] 3/19 3/19 H29 nd nd 68 nd 5 [2] 1/19 1/19 371

133 [] H2 tr(21) tr(2) tr(33) nd 35 [13] 9/1 2/2 H tr(2) 3 [1] 2/2 2/2 H [9] 1/1 1/1 H [9] 2/2 2/2 H26 tr(1) --- tr(2) tr(1) 3 [1] 2/2 2/2 H tr(12) tr(12) 23 [9] 1/1 1/1 H28 nd --- tr(21) nd 36 [14] 1/2 1/2 H29 nd --- nd nd 5 [2] /2 /2 [] H2 nd nd tr(17) nd 22 [74] 8/31 3/7 H22 nd nd tr(19) nd 27 [97] 2/6 2/6 H23 nd nd 24 nd 23 [8] 1/4 1/4 H nd 12 [5] 4/5 4/5 H26 22 tr(15) 57 tr(12) 17 [6] 3/3 3/3 H27 nd nd tr(7) nd 17 [7] 1/3 1/3 H28 nd nd tr(11) nd 3 [1] 1/3 1/3 H29 nd nd tr(18) nd 21 [8] 1/3 1/3 H2 nd nd 23 nd 22 [74] 5/76 4/16 H22 nd nd tr(15) nd 27 [97] 2/18 2/18 H23 nd nd tr(9) nd 23 [8] 2/18 2/18 H24 tr(59) tr(6) 38 nd 12 [5] 11/19 11/19 H26 tr(75) tr(7) 3 nd 17 [6] 13/19 13/19 H27 nd nd 38 nd 17 [7] 5/19 5/19 H28 nd nd tr(19) nd 3 [1] 7/19 7/19 H29 nd nd 2,1 nd 21 [8] 1/19 1/19 H2 nd nd tr(11) nd 22 [74] 4/1 1/2 H22 nd --- nd nd 27 [97] /2 /2 H tr(17) tr(17) 23 [8] 1/1 1/1 H [5] 2/2 2/2 H26 tr(65) --- tr(14) nd 17 [6] 1/2 1/2 H tr(9) tr(9) 17 [7] 1/1 1/1 H28 nd --- nd nd 3 [1] /2 /2 H29 nd --- nd nd 21 [8 ] /2 / pg/m pg/m pg/m pg/m pg/m pg/m pg/m pg/m pg/m pg/m pg/m pg/m pg/m pg/m 3 372

134 [] H [.4] H tr(.4) H [.5] H tr(.9) H tr(.11) 35/35 35/35.18 [.7] H nd 35/37 35/37 (pg/m 3 ) H nd 35/36 35/36.3 [.1] H24 tr(.2) tr(.2) 1.7 nd 25/36 25/36 H tr(.9).28 [.9] 36/36 36/36 H27 tr(.3) tr(.3) 2.7 nd.4 [.1] 3/35 3/35 H nd.4 [.2] 3/37 3/37 H tr(.6).15 [.5] [] H nd 33/37 33/37.16 [.6] H nd 29/37 29/37 H nd 35/37 35/37.12 [.5] H nd 34/37 34/37 H nd 31/35 31/35.16 [.6] H23.16 tr(.14) 2.6 nd 31/37 31/37 (pg/m 3 ) H24 tr(.13) tr(.12) 2.4 nd 3/36 3/36.14 [.6] H24 tr(.9) tr(.9).77 nd 26/36 26/36 H26 tr(.13) tr(.14).8 nd.28 [.9] 25/36 25/36 H27 nd nd.9 nd.6 [.2] 6/35 6/35 H28 nd nd 28 nd.4 [.2] 6/37 6/37 H nd.1 [.4] 33/37 33/37 [] H21 tr(.11) tr(.11) 2. nd 19/37 19/37.22 [.9] H21 tr(.2) nd 24/37 24/37 H22 tr(.14) tr(.13) 4.9 nd 29/37 29/37.16 [.6] H nd 31/37 31/37 H23 tr(.11) tr(.1) 1.2 nd 28/35 28/35.14 [.5] H nd 3/37 3/37 (pg/m 3 ) H24 nd nd 3.1 nd 9/36 9/36.3 [.1] H24 tr(.1) tr(.1).5 nd 22/36 22/36 H26 nd nd.4 nd.4 [.1] 5/36 5/36 H27 nd nd 2. nd 1.1 [.4] 3/35 3/35 H28 nd nd 2.7 nd.6 [.2] 3/37 3/37 H29 nd nd 2.1 nd.3 [.1] 11/37 11/37 [] H21 tr(.1) nd 1.7 nd 17/37 17/37.3 [.1] H21 tr(.2).3 2 nd 25/37 25/37 H22 tr(.2) tr(.1) 1.4 nd 24/37 24/37.3 [.1] H nd 28/37 28/37 H23 tr(.1) tr(.1) 1.1 nd 2/35 2/35.3 [.1] H23 tr(.2) tr(.2) 2.3 nd 25/37 25/37 (pg/m 3 ) H24 nd nd 1.8 nd 6/36 6/36.5 [.2] H24 nd nd.7 nd 8/36 8/36 H26 nd nd tr(.4) nd.7 [.2] 2/36 2/36 H27 nd nd tr(.6) nd 1.3 [.4] 2/35 2/35 H28 nd nd 1.3 nd 1.1 [.4] 1/37 1/37 H29 nd nd 3.2 nd.4 [.2] 1/37 1/37 [] H21 tr(.2) nd 23/37 23/37.3 [.1] H nd 26/37 26/37 H nd 3/37 3/37.15 [.6] H nd 32/37 32/37 H nd 27/35 27/35.2 [.8] H nd 3/37 3/37 (pg/m 3 ) H24 tr(.2) tr(.2) 1.2 nd 29/36 29/36.3 [.1] H nd 3/36 3/36 H26 tr(.1) tr(.1).7 nd.4 [.1] 22/36 22/36 H27 nd nd 3.8 nd 1.1 [.4] 9/35 9/35 H28 nd nd 1.6 nd.6 [.2] 18/37 18/37 H29 tr(.19) nd.21 [.7] 28/37 28/

135 (pg/m 3 ) [] H21 tr(.7) tr(.7) 3. nd 22/37 22/ [.6] H21 tr(1.) tr(.8) 3.9 nd 27/37 27/37 H22 nd nd 24 nd 12/37 12/ [1.2] H22 tr(1.2) tr(1.3) 7.1 nd 22/37 22/37 H23 tr(.8) nd 29/35 29/35.9 [.4] H nd 3/37 3/37 H24 tr(.5) tr(.5) 5.1 nd 24/36 24/ [.4] H24 tr(.9) tr(1.1) 4.7 nd 3/36 3/36 H26 nd nd tr(3) nd 4 [1] 7/36 7/36 H27 nd nd 12 nd 3.2 [1.1] 14/35 14/35 H28 tr(.9) tr(.9) 11 nd 1.4 [.5] 28/37 28/37 H nd.6 [.2] 31/37 31/37 [] H21 tr(7) tr(9) 31 nd 28/37 28/37 16 [5] H21 tr(1) tr(11) 45 nd 29/37 29/37 H22 nd nd 29 nd 1/37 1/37 27 [9.1] H22 tr(11) tr(12) 88 nd 21/37 21/37 H23 tr(8.2) tr(9.) 3 nd 31/35 31/35 12 [4.] H23 tr(8.4) tr(9.) 44 nd 29/37 29/37 (pg/m 3 ) H24 nd nd 31 nd 17/36 17/36 16 [5] H24 tr(1) tr(12) 73 nd 28/36 28/36 H26 tr(4.7) tr(5.) 64 nd 9 [3] 24/36 24/36 H nd 2.2 [.7] 3/35 3/35 H nd 3 [1] 35/37 35/37 H nd 2.4 [.8] 34/37 34/

136 [14-1] 2 15 [](pg/l) 21 8[3] 22 9[3] 23 4 [2] 24 4 [1] 26 8 [3] [1.2] 28 5 [2] (pg/l) / [14-1] (pg/g-dry) [](pg/g-dry) [23] 22 6[2] 23 3 [1] 24 2 [1] [9] [7] [11] 29 9 [4]

137 [14-1] [] [2.2] [16] [6] [7] [6] [6] [5] [6] [14-1] 1 pg/m [] (pg/m 3 ) [.4] [.5] [.7] 24.3 [.1] [.9] 27.4 [.1] 28.4 [.2] [.5]

138 [14-2] [](pg/l) [4] 22 3[1] 23 3 [1] 24 2 [1] 26 4 [2] [2.1] [.9] 29 3 [1] (pg/l) / [14-2] (pg/g-dry) [](pg/g-dry) [8] 22 5[2] 23 5 [2] [.9] 26 6 [2] [6] [4] 29 9 [4]

139 [14-2] [] 2 16 [5.9] [6] [6] [6] [5] [5] 28 9 [4] [5] [14-2].25 pg/m [] (pg/m 3 ) [.6] [.5] [.6] [.6] [.9] 27.6 [.2] 28.4 [.2] [.5] /

140 [14-3] (pg/g-dry) [](pg/g-dry) 21 5 [2] 22 4[2] 23 9 [3] 24 3 [1] 26 5 [2] 27 3 [1] 28 8 [3] 29 6 [2] [14-3] [] 2 14 [5.] 22 8[3] 23 1 [4] 24 1 [4] 26 1 [4] [5] [8] [7]

141 [14-4] (pg/g-dry) [](pg/g-dry) 21 9 [4] 22 4[2] 23 7 [3] 24 4 [2] [6] 27 3 [1] 28 6 [2] [6] [14-5] [](pg/l) [.6] 22 3[1] 23 2 [1] 24 4 [2] [.6] [.6] 28.8 [.3] 29 2 [1] (pg/l)

142 [14-5] (pg/g-dry) [](pg/g-dry) [.5] 22 1 [4] 23 1 [4] [6] [4] [16] 28 6 [2] 29 5 [2] [14-5] [] [3.6] [4] 23 7 [3] 24 8 [3] [4] [5] [6] 29 2 [8]

143 [14-5].5 pg/m [] (pg/m 3 ) 21.3 [.1] [.6] 23.2 [.8] 24.3 [.1] 26.4 [.1] [.4] 28.6 [.2] [.7] / [14-6] [](pg/l) [3] [7] 23 1 [4] 24 4 [13] 26 6 [2] 27 6 [2] 28 4 [1] 29 7 [3] (pg/l)

144 [14-6] (pg/g-dry) 1,2 1, 8 6 [](pg/g-dry) 21 9 [4] [9] [9] [11] 26 6 [2] [8] [9] [5] [14-6] 1.4 pg/m [] (pg/m 3 ) [.6] [1.2] 23.9 [.4] [.4] 26 4 [1] [1.1] [.5] 29.6 [.2] /

145 [14-7] 8 6 [](pg/l) 21 6 [2] 22 3 [1] 23 6 [2] [22] [9] [7] [6] [8] (pg/l) [14-7] (pg/g-dry) 8, 6, 4, [](pg/g-dry) 21 6 [2] [8] 23 4 [2] [89] [8] 27 4 [2] [41] 29 3 [1] 2,

146 [14-7] pg/m [] (pg/m 3 ) [5] [9.1] [4.] [5] 26 9 [3] [.7] 28 3 [1] [.8] /

147 [15] PFOS PFOS 21 5 POPs 4 COP ( -1-) ( -1-) ( -1- ) pg/g-wet pg/g-wet 19 4 pg/gwet 19 tr(4) 11,pg/g-wet 2 4 pg/g-wet 2 3, 32,pg/g-wet PFOS [] PFOS H nd 19 [7.4] 17/31 5/7 H nd 25 [9.6] 5/6 5/6 H [4] 4/4 4/4 H tr(4) 7 [3] 5/5 5/5 H nd 5 [2] 2/3 2/3 H27 7 tr(2) 21 nd 4 [2] 2/3 2/3 H28 11 tr(6) 16 nd 9 [3] 2/3 2/3 H nd 12 [4] 2/3 2/3 H , nd 19 [7.4] 83/9 17/18 H , nd 25 [9.6] 17/18 17/18 H ,2 nd 1 [4] 16/18 16/18 H ,3 tr(5) 7 [3] 19/19 19/19 H ,6 nd 5 [2] 18/19 18/19 H ,5 nd 4 [2] 18/19 18/19 H ,2 nd 9 [3] 18/19 18/19 H , tr(4) 12 [4] 19/19 19/19 386

148 PFOS [] H [7.4] 1/1 2/2 H22 1, , [9.6] 2/2 2/2 H [4] 1/1 1/1 H [3] 2/2 2/2 H26 4, , 19 5 [2] 2/2 2/2 H [2] 1/1 1/1 H28 3, ,1 1,4 9 [3] 2/2 2/2 H29 9, , 3, 12 [4] 2/2 2/ pg/m pg/m PFOS [] PFOS H [.1] H H /35 35/35.5 [.2] H H /36 36/36 (pg/m 3 ) H [.2] 36/36 36/36 H /36 36/36.3 [.1] H /36 36/36 H [.6] 36/36 36/36 H [.6] 35/35 35/35 H [.2] H [.1] 387

149 PFOS [] PFOS (pg/l) 25 H , tr(26) 37 [14] 49/49 49/49 H , tr(37) 5 [2] 49/49 49/49 H , tr(2) 5 [2] 49/49 49/49 H , [12] 48/48 48/48 H ,5 nd 5 [2] 47/48 47/48 H , [11] 48/48 48/48 H , tr(23) 5 [2] 48/48 48/ PFOS [] PFOS (pg/g-dry) H ,9 nd 9.6 [3.7] 18/19 64/64 H ,7 tr(3) 5 [2] 64/64 64/64 H ,1 nd 5 [2] 63/64 63/64 H ,2 tr(7) 9 [4] 63/63 63/63 H nd 5 [2] 62/63 62/63 H ,2 7 3 [1] 62/62 62/62 H [2] 62/62 62/

150 [15] PFOS [] [7.4] [9.6] 23 1 [4] 24 7 [3] 26 5 [2] 27 4 [2] 28 9 [3] [4] PFOS [15] PFOS pg/m [] (pg/m 3 ) 22.4 [.1] 23.5 [.2] 24.5 [.2] 25.3 [.1] [.6] [.6] 28.6 [.2] 29.3 [.1] PFOS 389

151 [15] PFOS (pg/l) [](pg/l) [14] 22 5 [2] 23 5 [2] [12] 26 5 [2] [11] 28 5 [2] PFOS [15] PFOS (pg/g-dry) [](pg/g-dry) [3.7] 22 5[2] 23 5 [2] 24 9 [4] 26 5 [2] 27 3 [1] 28 5 [2] PFOS 39

152 [16] PFOA PFOA PFOS POPs POPs pg/g-wet pg/g-wet 19 4 pg/gwet pg/g-wet 2 4 pg/g-wet pg/g-wet PFOA PFOA [] H21 tr(2) tr(21) 94 nd 25 [9.9] 27/31 7/7 H nd 26 [9.9] 5/6 5/6 H23 tr(19) tr(22) tr(4) nd 41 [14] 3/4 3/4 H24 tr(21) tr(23) 46 nd 38 [13] 4/5 4/5 H26 tr(4) tr(6) 1 nd 1 [3] 2/3 2/3 H27 tr(6.5) tr(6.3) 26 nd 1 [3.4] 2/3 2/3 H nd 4 [2] 2/3 2/3 H29 tr(6.3) tr(7) 18 nd 12 [4] 2/3 2/3 H21 tr(23) tr(19) 49 nd 25 [9.9] 74/9 17/18 H22 tr(13) tr(11) 95 nd 26 [9.9] 13/18 13/18 H23 nd nd 51 nd 41 [14] 7/18 7/18 H24 tr(35) tr(32) 86 nd 38 [13] 18/19 18/19 H26 tr(6) tr(4) 85 nd 1 [3] 11/19 11/19 H27 tr(5.7) tr(5.3) 99 nd 1 [3.4] 11/19 11/19 H28 4 tr(3) 2 tr(2) 4 [2] 19/19 19/19 H29 tr(6.4) tr(4) 79 nd 12 [4] 12/19 12/19 391

153 PFOA [] H tr(16) 25 [9.9] 1/1 2/2 H [9.9] 2/2 2/2 H nd nd 41 [14] /1 /1 H24 tr(27) --- tr(28) tr(26) 38 [13] 2/2 2/2 H ,6 nd 1 [3] 1/2 1/2 H [3.4] 1/1 1/1 H [2] 2/2 2/2 H [4] 2/2 2/ pg/m pg/m PFOA PFOA [] H [.2] H H tr(3.5) 35/35 35/ [1.8] H nd 36/37 36/37 H /36 36/36.7 [.2] H /36 36/36 (pg/m 3 ) H /36 36/ [.6] H /36 36/36 H [.1] 36/36 36/36 H tr(3.7) 4.2 [1.4] 35/35 35/35 H [.4] H tr(2.) 3.3 [1.1] PFOA PFOA [] H21 1,6 1,3 31, [23] 49/49 49/49 H22 2,7 2,4 23, 19 6 [2] 49/49 49/49 H23 2, 1,7 5, 38 5 [2] 49/49 49/49 H24 1,4 1,1 26, [55] 48/48 48/48 (pg/l) H26 1,4 1,4 26, 14 5 [2] 48/48 48/48 H27 1,4 1,2 17, [22] 48/48 48/48 H28 1,3 1,2 21, 26 5 [2] 48/48 48/ PFOA PFOA (pg/g-dry) [] H nd 8.3 [3.3] 182/19 64/64 H nd 12 [5] 62/64 62/64 H , [2] 64/64 64/64 H [2] 63/63 63/63 H tr(6) 11 [5] 63/63 63/63 H [1] 62/62 62/62 H nd 9 [4] 61/62 61/

154 [16] PFOA [] [9.9] [9.9] [14] [13] 26 1 [3] 27 1 [3.4] 28 4 [2] [4] / PFOA [16] PFOA pg/m [] (pg/m 3 ) 22.5 [.2] [1.8] 24.7 [.2] [.6] 26.4 [.1] [1.4] [.4] [1.1] PFOA 393

155 [16] PFOA 3, 2,5 2, [](pg/l) [23] 22 6 [2] 23 5 [2] [55] 26 5 [2] [22] 28 5 [2] (pg/l) 1,5 1, PFOA [16] PFOA [](pg/g-dry) [3.3] [5] 23 5 [2] 24 4 [2] [5] 27 3 [1] 28 9 [4] (pg/g-dry) PFOA 394

156 [17] 21 5 POPs 4 COP pg/l pg/l [] H19 nd nd nd nd 3,3 [1,3] /48 /48 H tr(1) 4 [1] 49/49 49/49 H [.9] 49/49 49/49 H [1] 48/48 48/48 (pg/l) H tr(3) 4 [1] 48/48 48/48 H [.3] 48/48 48/48 H [.5] 48/48 48/48 H [.6] 47/47 47/ pg/g-dry ,8 pg/g-dry [] H19 tr(46) nd 2,4 nd 86 [33] 79/192 35/64 H , [.3] 64/64 64/64 H ,5 3 5 [2] 64/64 64/64 H ,1 nd 2.5 [.8] 62/63 62/63 H , [.7] 63/63 63/63 (pg/g-dry) H ,6 tr(1.2) 2.4 [.8] 63/63 63/63 H , [.5] 62/62 62/62 H ,7 tr(1.1) 1.8 [.6] 62/62 62/62 H , [.5] 62/62 62/

157 3 1 pg/g-wet pg/g-wet 19 1 pg/g-wet pg/g-wet 2 1 pg/g-wet pg/g-wet [] H19 nd nd tr(15) nd 18 [61] 1/31 1/7 H [.7] 6/6 6/6 H [1] 4/4 4/4 H tr(5.8) 8.1 [2.7] 5/5 5/5 H25 nd nd 87 nd 78 [26] 1/5 1/5 H [3.1] 3/3 3/3 H27 tr(11) tr(9.7) 18 tr(7.4) 12 [4.] 3/3 3/3 H28 tr(13) tr(12) 15 tr(11) 15 [5.1] 3/3 3/3 H [1] 3/3 3/3 H19 nd nd 48 nd 18 [61] 36/8 1/16 H [.7] 18/18 18/18 H [1] 18/18 18/18 H tr(5.) 8.1 [2.7] 19/19 19/19 H25 tr(35) tr(4) 16 nd 78 [26] 11/19 11/19 H nd 9.3 [3.1] 18/19 18/19 H nd 12 [4.] 18/19 18/19 H nd 15 [5.1] 16/19 16/19 H [1] 19/19 19/19 H19 tr(14) tr(14) 21 tr(89) 18 [61] 1/1 2/2 H [.7] 2/2 2/2 H [1] 1/1 1/1 H [2.7] 2/2 2/2 H [26] 2/2 2/2 H tr(5.6) 9.3 [3.1] 2/2 2/2 H [4.] 1/1 1/1 H [5.1] 2/2 2/2 H [1] 2/2 2/

158 37.1 pg/m pg/m [] H /78 26/26 12 [4.8] H /75 25/25 H /111 37/ [2.5] H tr(5.) 111/111 37/37 H [.5] H H /35 35/ [.7] H (pg/m 3 ) H /36 36/ [.6] H /36 36/36 H /36 36/ [.6] H /36 36/36 H [.3] 36/36 36/36 H [.2] 35/35 35/35 H [.2] H [.1] 2 397

159 [17] [](pg/l) 19 3,3 [1,3] 22 4[1] [.9] 24 3 [1] 25 4 [1] 26.8 [.3] [.5] [.6] (pg/l) [17] (pg/g-dry) [](pg/g-dry) [33] 22.9 [.3] 23 5 [2] [.8] [.7] [.8] [.5] [.6] [.5]

160 [17] [] [61] [.7] 23 4 [1] [2.7] [26] [3.1] [4.] [5.1] 29 4 [1] / [17] 1 pg/m [] (pg/m 3 ) [4.8] [2.5] [.5] [.7] [.6] [.6] 26.9 [.3] 27.6 [.2] 28.5 [.2] 29.3 [.1]

161 [18] 23 4 POPs 5 COP α- β- α- [] H23 nd nd 18 nd 12 [5] 2/49 2/49 (pg/l) H24 nd nd 3 nd 27 [1] 3/48 3/48 β- [] H23 nd nd 27 nd 22 [9] 8/49 8/49 (pg/l) H24 nd nd tr(12) nd 24 [9] 1/48 1/ α- β- α- [] H23 tr(13) tr(11) 48 nd 3 [1] 35/64 35/64 (pg/g-dry) H24 nd nd 48 nd 13 [5] 19/63 19/63 β- [] H23 tr(5) tr(4) 24 nd 9 [4] 38/64 38/64 (pg/g-dry) H24 nd nd 25 nd 13 [5] 8/63 8/ α- β- α- [] H nd 5 [2] 3/4 3/4 H24 tr(54) tr(61) 2 nd 71 [24] 4/5 4/5 H26 tr(2) nd 13 nd 6 [2] 1/3 1/3 H27 nd nd 13 nd 12 [38] 1/3 1/3 H23 tr(2) tr(2) 14 nd 5 [2] 1/18 1/18 H24 nd nd tr(54) nd 71 [24] 6/19 6/19 H26 nd nd tr(3) nd 6 [2] 1/19 1/19 H27 nd nd tr(49) nd 12 [38] 1/19 1/19 H nd nd 5 [2] /1 /1 H24 nd --- nd nd 71 [24] /2 /2 H26 nd --- nd nd 6 [2] /2 /2 H nd nd 12 [38] /1 /1 4

162 β- [] H [4] 4/4 4/4 H nd 14 [5] 4/5 4/5 H26 nd nd 23 nd 19 [6] 1/3 1/3 H27 nd nd tr(22) nd 32 [11] 1/3 1/3 H23 nd nd 37 nd 11 [4] 9/18 9/18 H24 nd nd 15 nd 14 [5] 6/19 6/19 H26 nd nd tr(8) nd 19 [6] 3/19 3/19 H27 nd nd tr(11) nd 32 [11] 1/19 1/19 H nd nd 11 [4] /1 /1 H24 nd --- tr(7) nd 14 [5] 1/2 1/2 H26 nd --- tr(8) nd 19 [6] 1/2 1/2 H nd nd 32 [11] /1 / α- β- α- [] H tr(7.8) 35/35 35/35 12 [4.] H23 tr(9.6) tr(9.8) 45 nd 35/37 35/37 H tr(6.) 36/36 36/36 16 [5.3] (pg/m 3 H24 nd nd 19 nd 15/36 15/36 ) H [.3] 36/36 36/36 H [.3] 35/35 35/35 H [.3] β- [] H nd 34/35 34/ [.39] H23 tr(.8) tr(.9) 8.3 nd 31/37 31/37 H nd 33/36 33/ [.4] (pg/m 3 H24 nd nd 1.7 nd 17/36 17/36 ) H nd 1.2 [.4] 33/36 33/36 H nd.5 [.2] 33/35 33/35 H28.8 tr(.7) 3.3 nd.8 [.3] 34/37 34/

163 [18-1] α- 4 pg/m [] (pg/m 3 ) [4.] [5.3] 26.8 [.3] [.4] 28.8 [.3] / α- [18-2] β- pg/m [] (pg/m 3 ) [.39] [.4] [.4] 27.5 [.2] 28.8 [.3] / β- 42

164 [19] 1,2,5,6,9,1-1,2,5,6,9, POPs 6 COP6 α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9, α-1,2,5,6,9,1-β-1,2,5,6,9,1- γ-1,2,5,6,9,1- δ-1,2,5,6,9,1- ε-1,2,5,6,9, α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9,1-29 α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1-3 9 pg/g-wet pg/g-wet 19 9 pg/g-wet 19 tr(9) 7,8pg/g-wet 2 9 pg/g-wet 2 5 2,2pg/g-wet β-1,2,5,6,9,1-3 9 pg/g-wet pg/g-wet 19 9 pg/g-wet 19 2 tr(12)pg/g-wet 2 9 pg/g-wet 2 γ-1,2,5,6,9,1-3 9 pg/g-wet 3 tr(2) 2pg/g-wet 19 9 pg/g-wet pg/g- 43

165 wet 2 9 pg/g-wet 2 1 tr(18)pg/g-wet α-1,2,5,6,9,1- β-1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1- [] H23 1,1 1,2 13, tr(86) 17 [7] 1/1 4/4 H , [2] 5/5 5/5 H [1] 3/3 3/3 H [1] 3/3 3/3 H [9] 3/3 3/3 H [9] 3/3 3/3 H , nd 17 [7] 41/51 16/17 H ,7 nd 5 [2] 18/19 18/19 H , nd 3 [1] 18/19 18/19 H , nd 3 [1] 18/19 18/19 H ,1 tr(12) 22 [9] 19/19 19/19 H ,8 tr(9) 24 [9 ] 19/19 19/19 H23 2 nd 53 nd 17 [7] 1/3 1/1 H ,4 nd 5 [2] 1/2 1/2 H , [1] 2/2 2/2 H [1] 1/1 1/1 H , [9] 2/2 2/2 H , [9 ] 2/2 2/2 β-1,2,5,6,9,1- [] H23 tr(7) tr(85) 24 nd 98 [4] 7/1 3/4 H24 tr(25) 4 9 nd 4 [1] 4/5 4/5 H26 tr(1) tr(1) tr(2) tr(1) 3 [1] 3/3 3/3 H27 tr(1) tr(1) 3 nd 3 [1] 2/3 2/3 H28 nd tr(8) tr(9) nd 21 [8] 2/3 2/3 H29 tr(9) nd 36 nd 23 [9] 1/3 1/3 H23 nd nd 76 nd 98 [4] 11/51 5/17 H24 nd nd 4 nd 4 [1] 8/19 8/19 H26 nd nd 3 nd 3 [1] 5/19 5/19 H27 nd nd tr(2) nd 3 [1] 2/19 2/19 H28 nd nd tr(12) nd 21 [8] 3/19 3/19 H29 nd nd tr(12) nd 23 [9] 2/19 2/19 H23 nd nd nd nd 98 [4] /3 /1 H24 nd --- nd nd 4 [1] /2 /2 H26 nd --- nd nd 3 [1] /2 /2 H nd nd 3 [1] /1 /1 H28 nd --- nd nd 21 [8] /2 /2 H29 nd nd nd nd 23 [9] /2 /2 γ-1,2,5,6,9,1- [] H ,3 nd 21 [8] 8/1 4/4 H [1] 5/5 5/5 H [1] 3/3 3/3 H tr(2) 3 [1] 3/3 3/3 H tr(21) 24 [9] 3/3 3/3 H tr(2) 24 [9] 3/3 3/3 H23 21 tr(9) 5, nd 21 [8] 26/51 1/17 H ,6 nd 3 [1] 16/19 16/19 H26 3 tr(2) 2,8 nd 3 [1] 12/19 12/19 H27 tr(2) tr(1) 23 nd 3 [1] 1/19 1/19 H28 tr(16) tr(13) 16 nd 24 [9] 11/19 11/19 H29 tr(16) tr(18) 12 nd 24 [9] 12/19 12/19 H23 tr(18) nd 46 nd 21 [8] 1/3 1/1 H nd 3 [1] 1/2 1/2 H26 tr(1) --- tr(1) tr(1) 3 [1] 2/2 2/2 H tr(1) tr(1) 3 [1] 1/1 1/1 H28 tr(1) --- tr(2) nd 24 [9] 1/2 1/2 H29 tr(9) --- tr(18) nd 24 [9] 1/2 1/

166 23 27 δ-1,2,5,6,9,1- ε-1,2,5,6,9,1- δ-1,2,5,6,9,1- [] H23 nd nd nd nd 14 [6] /1 /4 H24 nd nd nd nd 5 [2] /5 /5 H26 nd nd nd nd 3 [1] /3 /3 H27 nd nd nd nd 3 [1] /3 /3 ε-1,2,5,6,9,1- H23 nd nd nd nd 14 [6] /51 /17 H24 nd nd nd nd 5 [2] /19 /19 H26 nd nd nd nd 3 [1] /19 /19 H27 nd nd tr(2) nd 3 [1] 1/19 1/19 H23 nd nd nd nd 14 [6] /3 /1 H24 nd --- nd nd 5 [2] /2 /2 H26 nd --- nd nd 3 [1] /2 /2 H nd nd 3 [1] /1 /1 [] H23 nd nd nd nd 14 [6] /1 /4 H24 nd nd tr(3) nd 4 [2] 1/5 1/5 H26 nd nd tr(2) nd 3 [1] 1/3 1/3 H27 nd nd tr(1) nd 3 [1] 1/3 1/3 H23 nd nd nd nd 14 [6] /51 /17 H24 nd nd tr(3) nd 4 [2] 3/19 3/19 H26 nd nd 8 nd 3 [1] 3/19 3/19 H27 nd nd tr(1) nd 3 [1] 1/19 1/19 H23 nd nd nd nd 14 [6] /3 /1 H24 nd --- nd nd 4 [2] /2 /2 H26 nd --- nd nd 3 [1] /2 /2 H nd nd 3 [1] /1 / α-1,2,5,6,9, pg/m pg/m 3 β-1,2,5,6,9, pg/m pg/m 3 γ-1,2,5,6,9, pg/m pg/m α-1,2,5,6,9,1-β- 1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1- [] H nd 31/36 31/36.6 [.2] H nd 35/36 35/36 H26 tr(.6) tr(.7) 3.1 nd 1.2 [.4] 25/36 25/36 (pg/m 3 ) H27 tr(.6) tr(.7) 3 nd.9 [.3] 26/35 26/35 H tr(.1).3 [.1] H nd.3 [.1] 36/37 36/37 β-1,2,5,6,9,1- (pg/m 3 ) [] H nd 3/36 3/36.3 [.1] H nd 35/36 35/36 H26 nd nd tr(.8) nd 1. [.3] 8/36 8/36 H27 nd nd 3.9 nd.8 [.3] 7/35 7/35 H28 tr(.1) tr(.1).7 nd.3 [.1] 21/37 21/37 H29 tr(.2) tr(.1 ).8 nd.3 [.1] 33/37 33/37 45

167 γ-1,2,5,6,9,1- (pg/m 3 ) [] H nd 31/36 31/36.3 [.1] H nd 35/36 35/36 H26 nd nd tr(1.2) nd 1.3 [.4] 4/36 4/36 H27 nd nd 4.4 nd.8 [.3] 11/35 11/35 H28 tr(.1) nd 1.4 nd.3 [.1] 16/37 16/37 H29 tr(.1) tr(.1).8 nd.3 [.1] 2/37 2/ δ-1,2,5,6,9,1- ε- 1,2,5,6,9,1- δ-1,2,5,6,9,1- [] H24 nd nd.8 nd 1/36 1/36.4 [.2] H24 nd nd 1.1 nd 1/36 1/36 (pg/m 3 ) H26 nd nd nd nd 1.8 [.6] /36 /36 H27 nd nd 1.9 nd 1.9 [.6] 1/35 1/35 ε-1,2,5,6,9,1- (pg/m 3 ) [] H24 nd nd nd nd /36 /36.6 [.2] H24 nd nd tr(.5) nd 1/36 1/36 H26 nd nd nd nd.9 [.3] /36 /36 H27 nd nd nd nd.9 [.3] /35 /

168 ,2,5,6,9,1- α-1,2,5,6,9,1- [] H23 nd nd 6,3 nd 1,5 [6] 4/47 4/47 (pg/l) H26 nd nd 1,6 nd 1,5 [6] 1/48 1/48 β-1,2,5,6,9,1- [] H23 nd nd 1,3 nd 1,3 [5] 4/47 4/47 (pg/l) H26 nd nd tr(3) nd 5 [2] 1/48 1/48 γ-1,2,5,6,9,1- [] H23 nd nd 65, nd 1,2 [5] 5/47 5/47 (pg/l) H26 nd nd nd nd 7 [3] /48 /48 δ-1,2,5,6,9,1- [] H23 nd nd nd nd 79 [3] /47 /47 (pg/l) H26 nd nd nd nd 6 [2] /48 /48 ε-1,2,5,6,9,1- [] H23 nd nd nd nd 74 [3] /47 /47 (pg/l) H26 nd nd nd nd 4 [2] /48 / α-1,2,5,6,9,1-β- 1,2,5,6,9,1- γ-1,2,5,6,9,1- α-1,2,5,6,9,1- [] H23 43 nd 24, nd 42 [28] 78/186 35/62 H , nd 18 [7] 47/63 47/63 (pg/g-dry) H , nd 15 [6] 47/62 47/62 H , nd 13 [6] 43/62 43/62 β-1,2,5,6,9,1- (pg/g-dry) γ-1,2,5,6,9,1- (pg/g-dry) δ-1,2,5,6,9,1- (pg/g-dry) ε-1,2,5,6,9,1- (pg/g-dry) [] H23 nd nd 14, nd 25 [17] 48/186 21/62 H24 tr(93) nd 8,9 nd 15 [6] 29/63 29/63 H ,6 nd 15 [6] 33/62 33/62 H28 tr(87) nd 7,4 nd 13 [5] 31/62 31/62 [] H23 67 nd 57, nd 4 [26] 89/186 36/62 H , nd 16 [6] 52/63 52/63 H , nd 11 [42] 48/62 48/62 H , nd 15 [6] 42/62 42/62 [] H23 nd nd 8 nd 35 [25] 11/186 6/62 H24 nd nd 68 nd 3 [1] 5/63 5/63 H27 nd nd nd nd 18 [7] /62 /62 [] H23 nd nd tr(26) nd 28 [21] 2/186 1/62 H24 nd nd 31 nd 15 [6] 7/63 7/63 H27 nd nd nd nd 13 [51] /62 /

169 [19-1] α-1,2,5,6,9,1-1,2 1, 8 6 [] [7] 24 5 [2] 26 3 [1] 27 3 [1] [9] [9] α-1,2,5,6,9,1- [19-1] α-1,2,5,6,9,1- pg/m [] (pg/m 3 ) 24.6 [.2] [.4] 27.9 [.3] 28.3 [.1] 29.3 [.1] α-1,2,5,6,9,1-48

170 [19-2] β-1,2,5,6,9, [] [4] 24 4 [1] 26 3 [1] 27 3 [1] [8] [9] / β-1,2,5,6,9,1- [19-2] β-1,2,5,6,9,1-1 pg/m [] (pg/m 3 ) 24.3 [.1] [.3] 27.8 [.3] 28.3 [.1] 29.3 [.1] / β-1,2,5,6,9,1-49

171 [19-3] γ-1,2,5,6,9, [] [8] 24 3 [1] 26 3 [1] 27 3 [1] [9] [9] γ-1,2,5,6,9,1- [19-3] γ-1,2,5,6,9,1-2.5 pg/m [] (pg/m 3 ) 24.3 [.1] [.4] 27.8 [.3] 28.3 [.1] 29.3 [.1] / γ-1,2,5,6,9,1-41

172 [19-1] α-1,2,5,6,9,1-5 4 [](pg/g-dry) [28] [7] [6] [6] (pg/g-dry) α-1,2,5,6,9,1- [19-2] β-1,2,5,6,9, [](pg/g-dry) [17] [6] [6] [5] 1 (pg/g-dry) / β-1,2,5,6,9,1-411

173 [19-3] γ-1,2,5,6,9, [](pg/g-dry) 23 4 [26] [6] [42] [6] (pg/g-dry) γ-1,2,5,6,9,1-412

174 [2] POPs COP pg/g-dry 62 tr(16) 32, pg/g-dry 2 29 [] H , nd 84 [3] 166/189 58/63 H , nd 59 [2] 59/62 59/62 (pg/g-dry) H , tr(16) 27 [9.1] 62/62 62/ [] [] pg/g-wet 3 2 1,4pg/g-wet 19 12pg/g-wet pg/g-wet 2 12pg/g-wet 2 tr(18) 46pg/g-wet [] H tr(19) 27 [11] 31/31 7/7 H ,3 tr(11) 26 [1] 31/31 7/7 H nd 54 [18] 2/3 2/3 H28 72 tr(49) 79 nd 57 [19] 2/3 2/3 H ,4 nd 33 [12] 2/3 2/3 413

175 [] H ,7 nd 27 [11] 78/8 16/16 H ,2 nd 26 [1] 79/85 17/17 H27 tr(5) nd 54 [18] 13/19 13/19 H28 tr(44) tr(48) 34 nd 57 [19] 13/19 13/19 H nd 33 [12] 17/19 17/19 H18 tr(17) tr(18) 27 tr(11) 27 [11] 1/1 2/2 H2 tr(1) nd tr(22) nd 26 [1] 5/1 1/2 H tr(2) tr(2) 54 [18] 1/1 1/1 H tr(49) 57 [19] 2/2 2/2 H tr(18) 33 [12] 2/2 2/ [] [] pg/m pg/m [] H /22 22/22 4. [1.3] H2 tr(9.6) tr(9.8) 45 nd 36/36 36/36 (pg/m 3 H , [1.] 36/36 36/36 ) H [.28] H [.24] 1[] [] [] H2 nd nd 18 nd 85[3] 9/48 9/48 (pg/l) [] [] 414

176 [2] 8 [](pg/g-dry) 2 84 [3] [2] [9.1] 6 (pg/g-dry) [2] [] [11] 2 26 [1] [18] [19] [12]

177 [2] 25 pg/m [] (pg/m 3 ) 2 4. [1.3] [1.] [.28] [.24]

178 [21] -1,3- -1, POPs COP pg/m ,1 23,pg/m ,3- - [] 1,3- H27 1,1 1,2 3, [11] 12/12 34/34 (pg/m 3 H , [2] 111/111 37/37 ) H29 4,2 4, 23, 1,1 6 [2] ,3- - [] 1,3- H19 nd nd nd nd 87 [34] /48 /48 (pg/l) H25 nd nd tr(43) nd 94 [37] 1/48 1/ ,3- - [] 1,3- H19 nd nd 1,3 nd 22 [8.5] 22/192 1/64 (pg/g-dry) H25 nd nd 1,6 nd 9.9 [3.8] 4/189 2/

179 ,3- - [] 1,3- H19 nd nd nd nd 36 [12] /31 /7 H25 nd nd tr(7.1) nd 9.4 [3.7] 3/13 1/5 H19 nd nd nd nd 36 [12] /8 /16 H25 nd nd 59 nd 9.4 [3.7] 7/57 4/19 H19 nd nd nd nd 36 [12] /1 /2 H25 nd nd nd nd 9.4 [3.7] /6 /

180 [22] 27 5 POPs 7 COP pg/l ,5 pg/l 47 5 pg/l , pg/l [] H27 tr(13) tr(9) 26, nd 26 [85] 25/48 25/48 (pg/l) H ,5 nd 3 [1] 43/47 43/47 [] (pg/l) H29 tr(1) tr(8) 1, nd 14 [5] 32/47 32/ pg/g-dry ,4 pg/g-dry 62 2 pg/g-dry pg/g-dry 419

181 29 [] H ,4 8 4 [2] 62/62 62/62 (pg/g) [] H nd 5 [2] 61/62 61/62 (pg/g) 3 12 pg/g-wet 3 1 tr(35)pg/g-wet pg/g-wet pg/g-wet 2 12 pg/g-wet ,pg/g-wet 3 1 pg/g-wet 3 tr(2) 36pg/g-wet 19 1 pg/g-wet 19 tr(1) 12pg/g-wet 2 1 pg/g-wet pg/g-wet [] H28 tr(45) tr(46) 65 tr(3) 63 [21] 3/3 3/3 H29 nd nd tr(35) nd 36 [12] 1/3 1/3 H nd 63 [21] 18/19 18/19 H29 tr(15) tr(15) 11 nd 36 [12] 14/19 14/19 H28 1, , [21] 2/2 2/2 H29 1, , 3 36 [12] 2/2 2/2 [] H [1] 3/3 3/3 H29 6 tr(3) 36 tr(2) 4 [1] 3/3 3/3 H tr(1) 3 [1] 19/19 19/19 H tr(1) 4 [1] 19/19 19/19 H [1] 2/2 2/2 H [1] 2/2 2/2 42

182 37.2 pg/m pg/m pg/m pg/m [] H [.2] (pg/m 3 ) H [.2] [] H [.4] (pg/m 3 ) H [.5] 421

183 [23] POPs 8 COP ,1 pg/l 47 1 tr(1,6)pg/l 47 5 pg/l ,1 pg/l 47 1,1 pg/l , pg/l 47 1,2 pg/l , pg/l 29 (pg/l) [] H29 nd nd tr(1,6) nd 3,3 [1,1] 1/47 1/47 [] H29 (pg/l) nd nd 3,1 nd 1,5 [5] 13/47 13/47 (pg/l) [] H29 nd nd 1, nd 3,3 [1,1] 4/47 4/47 [] H29 (pg/l) nd nd 1, nd 3,6 [1,2] 7/47 7/ , pg/g-dry

184 17, pg/g-dry 62 4, pg/g-dry , pg/g-dry 62 4, pg/g-dry , pg/g-dry 62 5, pg/g-dry , pg/g-dry 29 (pg/g-dry) [] H29 nd nd 17, nd 1, [4,] 12/62 12/62 [] H29 (pg/g-dry) nd nd 37, nd 1, [4,] 19/62 19/62 (pg/g-dry) [] H29 nd nd 44, nd 11, [4,] 19/62 19/62 [] H29 (pg/g-dry) nd nd 94, nd 12, [5,] 18/62 18/ pg/g-wet 3 2 1,8pg/g-wet 19 2 pg/g-wet ,1pg/g-wet 2 2 pg/g-wet 2 1 1,6pg/g-wet 3 3 pg/g-wet 3 tr(3) 11,pg/g-wet 19 3 pg/g-wet ,pg/g-wet 2 3 pg/g-wet ,pg/g-wet 3 3 pg/g-wet 3 1,3 4,7pg/g-wet 19 3 pg/g-wet ,pg/g-wet 2 3 pg/g-wet 2 1,2 25,pg/g-wet 3 2 pg/g-wet 3 tr(3) 3,1pg/g-wet 19 2 pg/g-wet ,1pg/g-wet 423

185 2 2 pg/g-wet 2 1 8,1pg/g-wet [] H28 tr(7) tr(7) 2,2 nd 1,3 [5] 2/3 2/3 H ,7 1,8 nd 5 [2 ] 2/3 2/3 H28 tr(6) tr(7) 2,8 nd 1,3 [5] 13/19 13/19 H29 tr(41) tr(4) 2,1 nd 5 [2 ] 16/19 16/19 H28 tr(1,) --- 1,3 tr(8) 1,3 [5] 2/2 2/2 H29 tr(4) --- 1,6 nd 5 [2 ] 1/2 1/2 [] H28 tr(2,9) tr(2,) 6, tr(2,) 3, [1,] 3/3 3/3 H29 2,2 3,4 11, tr(3) 8 [3 ] 3/3 3/3 H28 tr(2,9) tr(2,) 15, nd 3, [1,] 18/19 18/19 H29 1,9 1,1 24, nd 8 [3 ] 16/19 16/19 H28 4, , 3, 3, [1,] 2/2 2/2 H29 5, , 8 8 [3 ] 2/2 2/2 [] H28 tr(1,4) tr(1,5) tr(1,8) tr(1,1) 2,1 [7] 3/3 3/3 H29 2, 1,4 4,7 1,3 9 [3 ] 3/3 3/3 H28 tr(1,8) tr(1,8) 8,7 nd 2,1 [7] 17/19 17/19 H29 2,1 2,1 19, nd 9 [3 ] 18/19 18/19 H28 3, ,6 2,2 2,1 [7] 2/2 2/2 H29 5, , 1,2 9 [3 ] 2/2 2/2 [] H28 tr(7) tr(7) tr(9) tr(5) 1,1 [4] 3/3 3/3 H ,1 tr(3) 5 [2 ] 3/3 3/3 H28 tr(8) tr(8) 4,9 nd 1,1 [4] 17/19 17/19 H29 tr(29) nd 4,1 nd 5 [2 ] 8/19 8/19 H28 1, ,5 1,4 1,1 [4] 2/2 2/2 H ,1 nd 5 [2 ] 1/2 1/ pg/m ,5pg/m pg/m ,3pg/m pg/m pg/m pg/m ,6pg/m [] H28 tr(17) tr(2) 94 nd 29 [11] 24/37 24/37 (pg/m 3 ) H ,5 tr(7) 14 [5] 424

186 [] H28 tr(35) tr(32) 3,2 nd 61 [24] 2/37 2/37 (pg/m 3 ) H ,3 tr(9) 19 [6] [] H28 nd nd 74 nd 43 [17] 7/37 7/37 (pg/m 3 ) H tr(3) 1 [3] [] H28 nd nd 51 nd 32 [12] 13/37 13/37 (pg/m 3 ) H ,6 nd 12 [4] 35/37 35/

187 [24] POPs POPs (pg/l) [] H2 nd nd 76 nd 25 [1] 13/48 13/48 2 [] H2 nd nd 46 nd 16 [63] 13/63 3/186 (pg/g-dry) 18 2 [] H18 tr(58) tr(7) 24 nd 92 [36] 22/31 5/7 H2 tr(11) nd 12 [48] 28/31 7/7 H18 nd nd 29 nd 92 [36] 5/8 1/16 H2 tr(62) tr(77) 27 nd 12 [48] 55/85 14/17 H18 nd nd nd nd 92 [36] /1 /2 H2 nd nd 3 nd 12 [48] 1/1 1/2 28 (pg/m 3 ) H28 [] nd nd 1. nd.5 [.2] 1/37 1/37 426

188 i) ( ii) ( iii) ( iv) ( 427