NSR-V28-N2-P7-14訂正
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1 (imai@ias.tokushima-u.ac.jp) Particulate matter in rime, fresh snow and winter rain fall and suspended particulate matter from the summit of Mt. Kajigamori, Shikoku Island, Japan Yosuke Sanagawa 1, Yuhya Kurumi 2, Yuhei Yamoto 3 and Shoji Imai 3 1 Department of Chemistry, Graduate School of Integrated Arts and Sciences, The University of Tokushima, 1-1 Minamijosanjima, Tokushima Japan, Department of Chemistry, Faculty of Integrated Arts and Sciences, The University of Tokushima, 1-1 Minamijosanjima, Tokushima Japan, Division of Chemistry, Institute of Socio-Arts and Sciences, The University of Tokushima, 1-1 Minamijosanjima, Tokushima Japan, Corresponding Author: Shoji Imai (imai@ias.tokushima-u.ac.jp) Abstract The wet-depositions of rime, fresh snow and winter rain fall were collected on the summit of Mt. Kajigamori (ALT. 1400m), where is the watershed protection forest of Riv. Yoshinogawa. The insoluble particulate matter included in the wet-deposition was obtained by filtration with 0.45µm pore-sized filter. Small spherical particles such as flyash were found in the residue by SEM-EDX analysis. The amount of residue was increasing in the order of rain< snow< rime, and was influenced by the back trajectory of air mass. The suspended particulate matter such as black belt was able to observe above Shikoku Island, Japan. Keywards: suspended particulate matter, rime, snow, winter rain, Shikoku SPM PAH s 600 AEROS 1) ) 3) SOx -7-
2 1399m.. ADVANTEC 0.45 m U3000 HORIBA X EMAX Evolusion TM3000 X SwiftED HP 4) HP 5) CGER-METEX 6) 1500m.. Mt. Kajigamori ALT. 1399m Fig. 3km km 11km 1300m 20km 1000m 26km 730m 100km 2 12km m Fig. 1 Location of sampling site ( ) -8-
3 90km 1260m 167km 202km 25km Fig. 2 20cm Fig. 2 (B) 4) -9-
4 .. Fig /1/ /1/15~23 Fig. 3 Filtration residue of rime, snow and rain and S.E.M. image -10-
5 佐名川洋右 来見祐哉 山本祐平 今井昭二 NASA EARTH OBSERVATORY によれば 2013/1/3 と同年 1/14 の衛星画像 Fig.4 を比較 すると北京周辺の大気汚染の程度がわかる 7) 1/23 採取の樹氷や降雪は この中国華北エリア 周辺地域から流入した気団 8)の影響を受けたと 考えられる 2013/1/23 に採取した樹氷の濾過物を走査電子 顕微鏡エネルギー分散 X 線分析装置において顕 微鏡観察と含有粒子の分析を行った Fig.3 の S.E.M.イメージ中に小球体粒子が多数存在する 小球体粒子の組成分析を E.D.X.分析によって実 施したところ Al-Si-Ca-Mg-K-Fe Al-Si-Fe-Zn 等の組成を持つ粒子であることが分かった SEM イメージから石炭フライアッシュには組成 およびサイズの異なる小球体粒子が混在するこ とが分かった Jan. 3, 2013 Jan. 14, 2013 Fig.4 Air pollution in Beijin, Tianjin of China7) (NASA7), EARTH OBSERVATORY Air Quality Suffering China, Jan. 15, 2013) -11-
6 四国の梶ヶ森山頂における樹氷 降雪 冬季降雨中の粒子状物質と黒色浮遊性物質 ３.４. 2013/2/19 か ら 4 日 間 の 樹 氷 Fig. 5(A)では 2/19 から 2/23 の樹氷の汚染度 を示すメンブレンフィルターの写真を示した Fig. 5(B)には その間の大気塊の流入経路をしめ す後方流跡線をまとめた 2013/2/19 は 800ｇの 樹氷を濾過したときのフィルターである 非水 溶性の大気汚染物質で少しフィルターは灰色に 変色した その 4 日後には 現地に残っていた 同じ樹氷 500g を濾過した時のフィルターである 顕著に黒変している 大気汚染物質が この 4 日間に樹氷に付着したことを示す 2/ から 120 時間遡る高度 1500m における後方流跡 線はモンゴルと中国の国境付近を基点として 2/14 と 2/15 にかけて北京上空から大連上空を通 過したのち朝鮮半島東海上の黄海上でループを 画いてから梶ヶ森へ到着したことが分かる (A) Filtration residue of rime (B) Back trajectory Fig. 5 Filtration residue of rime (A) and back trajectory 6) (B). -12-
7 .. Fig. 6 Fig.6(A, B, C) 1399m Mt. Kurotakiyama ALT. 1210m , Mt. Kunimiyama ALT. 1409m Mt. Yahazuyama ALT. 1670m Fig. 6(A) 1400m Fig. 6(B) Fig. 6(C) m Fig.6(C) Fig. 6(D) 1000m 1500m A Jan. 5, 2014 Mt. Kajigamori (B) March 9, 2013 Mt. Kajigamori (C) Feb. 5, 2013 Mt. Kajigamori (D) Feb. 5, 2013 Tachino, Higashimiyosshi Tw. Fig. 6 Observation of atmosphere -13-
8 1) (accessed ). 2) (2010). 3) 75, (2011). 4) <tenki.jp (accessed ) 5) HP < hibiten/> (accessed ) 6) CGER-METEX < (accessed ). 7) NASA EARTH OBSERVATORY Air Quality Suffering China, Jan. 15, php?id=80152&eocn=image&eoci=related_ image, (accessed ). 8) SEM-EDX In preparation (2014)
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