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1 24 2 : ,2 1 2 Regression Analysis on Decay Curve of Contaminated Environment of Fukushima Nuclear Plant Accident Using Time Sequential Change of γ Ray Counting and Space Dose Rate Yukihiko SATO 1 and Koichi CHIDA 1,2 1 Course of Radiological Technology, Health Sciences, Tohoku University Graduate School of Medicine 2 Radiation Disaster Medicine, International Research Institute of Disaster Science, Tohoku University Key words : fallout, soil contamination, space dose rate, decay curve, Fukushima nuclear plant accident Mega quake occurred on March 11th, 2011 and the Tsunami with the height of 13 m had struck on Fukushima First Nuclear Power Plant. Three of six reactors melted down and huge amount of radioactivity were spread out around the peripheral zone. We had reported decay curve of contaminated soil before 1. In this paper, we analyzed this decay curve of radioactivity more precisely using well type NaI Tl scintillation gamma ray spectroscopy. And we also got decay curve of space dose rate by reading out from the home page of the Nuclear Regulation Office of Japan and other two official data, which also decreased following decay curve theory. We have gotten the following results. The decay curve of sampled soil data showed that the ratio of / at the explosion time was 0.5. This ratio indicates the used time of nuclear fuel. On the other hand, on space dose rate, the ratio was about at the explosion time. This difference of the ratio means that contribute to space dose rate more than. This may correlate to the quality of emitted radiation, for example, the energy of β ray and γ ray m

2 30 km 10 km km 131 I cps Bq/g μsv/h 20 km km : 1 g 20 mm 35 mm 55 mm NaI Tl 3 inch 3 inch 660 V Aloka γ 1 g 9.7 mm 104 mm AEG45SM 10 μg =21,600 η 1 =0.863 η 2 =0.559 η=η 1 η 2 =0.482 γ 20 1, cps 4.95 cps 0.10 cps γ 1 32 X km : μsv/h m γ NaI Tl : 131 I 2 : 3 : cps μsv/h : frt W= m10$e -m1t +m20$e -m2t +m30$e -m3t +b g 90

3 : grt W= m10$e -m1t +m20$e -m2t +m30$e -m3t +b g KaleidaGraph Ver4.1 λ t f t cps : count per second g t : μsv/hour Kaleida- Graph t f t g t m 10 m 20 m 30 λ 1 λ 2 λ 3 山形圏 : 山形市, 蔵王山, 米沢市 [ 北西へ, ~100km] 計数率 :Y1~Y5 仙台圏 : 仙台市, 丸森町, 角田市, 亘理町, 山元町 [ 北方へ,70~100km] 計数率 :S1~S10 線量率 :K7~K11 福島圏 : 福島市, 伊達市, 二本松市, 会津若松市, 南相馬市, 飯舘村 [ 北西へ,40~100km] 計数率 :F1,F4~F11 線量率 :K1~K6 福島圏 : 大熊町, 双葉町, 浪江町, 南相馬市 [ 北西へ,3~20km] 線量率 :N1~N8 福島第一 原子力発電所 福島圏 : 広野町 [ 南へ,~20km] 計数率 :F2~F3 東京圏 : さいたま市, 東京, 横浜市 [ 南南西へ,200~250km] 計数率 :T1~T

4 1: 131 I= : = : =30.07 m 1 m 2 m m 10 m 20 m 30 m 10 m 20 m 30 b g f t b g =5.05 cps g t b g =0.05 μsv/h γ ,563 RI I 土壌大学キャンパス内 ( 採取 ) 21 日目 ( ): 測定値 =7.123cps 土壌大学キャンパス内 38 日目 ( )=5.989cps 131 Cs 132 Cs 30 鉛 I K Cs 132 Cs I 364 土壌大学キャンパス内 49 日目 ( )=5.744cps バックグラウンド ( ガラス管のみ ) BG=5.154cps 131 Cs 132 Cs I 364 鉛 K X 131 I

5 草 ( スイバ ) 大学キャンパス内 26 日目 ( )=7.877cps 草 ( スイバ ): 大学キャンパス内 38 日目 ( )=6.741cps 131 Cs 132 Cs I Cs 132 Cs I 364 草 ( スイバ ): 大学キャンパス内 50 日目 ( )=6.300cps 草 ( スイバ ): 大学キャンパス内 57 日目 ( )=6.146cps 131 Cs 132 Cs 137 Cs I Cs 132 Cs I 364 バックグラウンド ( ガラス管のみ ) BG=5.165cps 鉛 X 131 I K 1461 X Cs 9.7 EC 100% 132 Cs 6.5 EC 97% 136 Cs 13 β - 91% β - 18% 5,6 93

6 30.07 X D ,500 空気フィルタ 147 日目 ( )=37.000cps 空気フィルタ 493 日目 ( )=30.768cps 32.2 後方散乱 ピーク K 空気フィルタ 895 日目 ( )=26.095cps 空気フィルタ 1223 日目 ( )=23.152cps 空気フィルタ 1563 日目 ( )=20.955cps バックグラウンド ( ガラス管のみ ) BG=5.19cps 137 Cs Cs 662 鉛 134 Cs K

7 I cps m 10 m 20 m 30 R 2 1 NaI Tl Bq/gm m 10 m 20 m 30 2 γ 4 X 30 count/12 h count/6 h I 2 K2 1, R R A I m 10 m 20 m I t=0 cps %

8 1. 1,000 cps 1,000 Bq/g R 2 / 131 I / Sendai S1 N 97 km 2011/3/ g S2 2011/4/ g S3 2011/3 2 ml S4 2011/ mm 0.5 g ,220 S5 2011/11/ g S6 2011/4/ g S7 2011/4/ g S8 2011/11/ g S9 2012/5/ g S /8/ g Yamagata Y1 NW 100 km 2011/12/ g Y2 NNW 110 km 2012/7/ g Y3 NNW 110 km 2011/11/ g Y4 1,500 m NNW 95 km 2011/6/5 2 ml Y5 1,500 m NNW 95 km 2011/6/5 2 ml Fukushima F1 W 100 km 2011/6/ g F2 S 20 km 2011/6/ g F3 S 20 km 2011/6/ g F4 NW 63 km 2011/11/ g F5 2011/11/ g F6 2011/11/ g F7 2011/6/ g F8 2011/7/ g ,544 F9 N 25 km 2011/7/ g ,134 F10 NW 63 km 2012/5/ g F /6/ g ,176 Tokyo T1 SSW 230 km 2012/8/ g T2 2012/8/ g T3 2012/8/ g T4 SSW 250 km 2013/4/ g T5 SSW 210 km 2013/4/ g

9 3. 97

10 3. 98

11 3. 99

12 3. B R 2 : : R 2 = R 2 1 R

13 4. X 30 β γ 2,7 C / 131 I/ / γ β % β %

14 佐 藤 行 彦 千 田 浩 一 図 5. 続き 各地の空間線量率の減衰曲線 102

15 5. 2 β m Ba 662 γ μsv/bq μsv/bq 7 1 cm Γ μsv m 2 / MBq h μsv m 2 / MBq h D 30 X 2 30 X 131 Cs 132 Cs EC : Electron Capture Xe X 29.8 Ba X Cs β ,048 γ 5,6 γ Cs 132 Cs 136 Cs

16 2. 1,000 μsv/h R 2 / 131 I / HP 20 km N1 Nuc. Reg. Office 3.0 km WSW 2.4 km N2 3.7 km SSW 3.7 km N3 9.1 km WNW 9.1 km N4 7.1 km WNW 9.1 km N5 11 km NNW 11 km N6 16 km NW 16 km N7 10 km WNW 10 km N8 19 km NW 19 km K1 K2 30 km HP K1 Kahoku WNW 7 km K2 NNW 5 km K3 30 NW 63 km K4 6 NW 65 km K5 6 WNW 57 km K6 5, km HP K7 NNW 60 km K8 1.5 km N 64 km K9 NW 66 km K10 N 72 km K N 97 km NaI Tl Xe Ba X 1 2 Ge 104

17 fallout 1 : γ km 22 2, 79-89, : : go.jp/ja/list/204/list - 1.html 4 : ac.jp/index.html 5 Lederer, C.M., Hollander, J.M., Perlman, I. : Table of Isotopes 6th Edition, John Wiley & Sons Inc, New York, Firestone, R.B., Baglin, C.M., Editor Shirley, V.S. : Table of Isotopes 8th Edition, John Wiley & Sons Inc, New York, : III

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