[15] 1970 Chiu [16, 17] [18-22] [20] Chiu [23] [24] [25] Chiu [16, 17] Chiu G 2

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1 Spray Combustion. Droplet Group Combustion 1. ml 20 µm 2.4 [1-12] [13] [14] 1

2 [15] 1970 Chiu [16, 17] [18-22] [20] Chiu [23] [24] [25] Chiu [16, 17] Chiu G 2

3 N: TOTAL NUMBER OF DROPLETS GROUP COMBUSTION OF LIQUID DROPLETS EXTERNAL SHEATH COMBUSTION EXTERNAL GROUP COMBUSTION INTER- NAL GROUP COMBUS- TION G= SINGLE DROPLET COMBUSTION G = 1. 5Le + 1 [32] 1 / 2 1 / 3 2 / 3 ( Re Sc ) n ( d / l) Le Re Sc n T D d l G 4 1 (a) G < -2 (b) -2 < G <1 (c) 1 < G 2 (d) 2 < G T S= ( d/r 1/2 1/3 l ) ( Re Pr ) 2 G [17] n T S G 2 Chiu [17]

4 f Burgoyne Cohen [26][23] [27] 3 [23] 40 µm m / ma Burgoyne & Cohen µm 3 [23] [28] [15] 4

5 4 [15] 4 3 (A) (B) (C) [29] Laser Doppler Velocimetry: LDV CO CO 2 Phase Doppler Particle Analyzer: PDPA [30] 5 Cessou PDPA OH Laser Induced Fluorescence: LIF [29, 30] 5 5

6 [31] 6 [32] [33] [19-22] 7 [22] (a) (b) 8 OH CH 5 [22] 6 [31] (a)(b) 1/15 sec 1/00 sec 7 [22] 8 5 [22] 6

7 9 OH Chiu (a) h = 35 mm (b) h = 70 mm [6] 11 [34] (c) h = 0 mm (d) h = 130 mm 9 [22] [22] [35] 7

8 [23, 27, 36-41] [23] [42] 12 L = mm L = mm L = 14 mm L = mm L = 20 mm L = 20 mm L = 20 mm L = 16 mm L = 30 mm L = 30 mm L = 30 mm L = 32 mm (A) Butanol (B) Large Butanol (C) Hexanol (D) Hexadecanol 11 [34] [24] 13 Williams [43] 12 ([24] 8

9 Williams 14 [23] (b) [42] (a) 13 [43] [44] 15 [45-52] (b) 14 [23] 9

10 16 PDPA Particle Tracking Velocimetry: PTV [53, 54] 2-3. [20] OH Chiu Chiu Geometrical Group Combustion Number, G 0, Gasification correction factor, C v G [55] G 0 G G [44] [53, 54] 16

11 Yeh Cummins[56] LDV 1970 [57] PDPA [58-60] PDPA 2 [61] [62] [63] Particle Image Velocimetry: PIV PTV PDPA LDV PIV PTV PTV [64] [65] EXCIPLEX 11

12 OH CH C 2 [18, 20-22] [66] [67] [68] [69, 70] OH Planar Laser Induced Fluorescence: PLIF C 2 H 2 Planar Multi-Photon Dissociation: PMPDOH [71-73] LIF PLIF 2. LIF Coherent Anti-Stokes Raman Scattering: CARS LIF [71-75] Allen Hanson 12

13 [1] 1 pp [2] 26 pp [3] pp [4] B pp [5] pp [6] B pp [7] 琚 B pp [8] B pp [9] B pp [] Williams, A., Combustion and Flame 21, pp. 1-31, [11] Annamalai, K. and Ryan, W., Prog. Energy Combust. Sci. 18, pp , [12] Faeth, G.M., Prog. Energy Combust. Sci. 3, pp , [13] 6 16 pp [14] McCreath, C.G. and Chigier, N.A., Proc. of the Combustion Institute, Vol. 14, pp , [15] Onuma, Y. and Ogasawara, M., Proc. of the Combustion Institute, Vol. 15, pp , [16] Chiu, H.H. and Liu, T.M., Combust. Sci. Tech., 17, pp , [17] Chiu, H.H., Kim, H.Y. and Croke, E.J., Proc. of the Combustion Institute, Vol. 19, pp , [18] Salah Hassan EL-EMAM B pp [19] B pp [20] B pp [21] B pp [22] B pp [23] 13

14 pp pp pp [24] Tsushima, S., Saitoh, H., Akamatsu, F. and Katsuki, M., Proc. of the Combustion Institute, Vol.27, pp , [25] Chigier, N., Combustion and Flame 51, pp , [26] Burgoyne, J. and Cohen, L., Proc. Roy. Soc. (London), A225, pp , [27] Hayashi, S. and Kumagai, S., Proc. of the Combustion Institute, Vol. 15, pp , [28] 29 7 pp [29] B pp [30] 37 pp [31] Cessou, A., Goix, P. and Stepowski, D., Atomization and Sprays 9, pp. 1-27, [32] 2 pp [33] pp [34] 36 pp [35] 33 pp [36] 69 4 pp [37] B pp [38] Cekalin, E.K., Proc. of the Combustion Institute, Vol. 8, pp , [39] Hayashi, S., Kumagai, S. and Sakai, T., Combust. Sci. Tech., 15, pp , [40] Brzustowski, T.A., Sobiesiak, A. and Wojcicki, S., Proc. of the Combustion Institute, Vol. 18, pp , [41] Myers, G.D. and Lefebvre, A.H., Combustion and Flame 66, pp , [42] Aggarwal, S.K. and Sirignano, W.A., Combustion and Flame 62, pp , [43] Williams, F.A., Combustion Theory 2nd Edition, Benjamin Cummings, [44] Vol. 5 pp [45] Li, S.C., Libby, P.A. and Williams, F.A., Proc. of the Combustion Institute, Vol. 24, pp , [46] Lacas, F., Darabiha, N., Versaevel, P., Rolon, J.C. and Candel, S., Proc. of the Combustion Institute, Vol. 24, pp , [47] Chen, G. and Gomez, A., Proc. of the Combustion Institute, Vol. 24, pp , [48] Gao, L.P., D'angelo, Y., Silverman, I., Gomez, A. and Smooke, M.D., Proc. of the Combustion Institute, Vol. 26, pp , [49] Continillo, G. and Sirignano, W.A., Combustion and Flame 81, pp , [50] Gutheil, E. and Sirignano, W.A., Combustion 14

15 and Flame 113, pp. 92-5, [51] Chen, Z.H., Lin, T.H. and Sohrab, S.H., Combust. Sci. Tech., 60, pp , [52] Li, S.C., Prog. Energy Combust. Sci. 23, pp , [53] 24 3 pp [54] Wakabayashi, T., Mizutani, Y., Katsuki, M. and Akamatsu, F., 36th Aerospace Sciences Meeting and Exhibit, AIAA , [55] Chiu, H.H., Proc. of 2nd ASPACC, pp , [56] Yeh, Y. and Cummins, H.Z., Applied Phisics Letters 4, pp. 176, [57] Durst, F., Melling, A. and Whitelaw, J.H., Principal and Practice of Laser Doppler Anemometry, Academic Press, [58] B pp [59] 33 pp [60] 116 pp [61] pp [62] 8 pp [63] 37 Vol. 3 pp [64] B pp [65] B pp pp [66] Kauranen, K., Andersson-Engels, S. and Svanberg, S., Appl. Phys. B53, pp , [67] B pp [68] 24 3 pp [69] B pp [70] B pp [71] Allen, M.G. and Hanson, R.K., Optical Engineering, Vol. 25, No. 12, [72] Allen, M.G., McManus, K.R. and Sonnenfroh, D.M., 33rd Aerospace Sciences Meeting and Exhibit, AIAA , [73] Allen, M.G. and Hanson, R.K., Proc. of the Combustion Institute, Vol. 21, pp , [74] Bazile, R. and Stepowski, D., Experiments in Fluids 20, pp. 1-9, [75] Cessou, A. and Stepowski, D., Combust. Sci. Tech., 118, pp ,

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